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At least 253 records · Page 14

AGR-5/6/7 Experiment Monitoring and Simulation Progress

Advanced Gas Reactor (AGR)--5/6/7 is the last of a series of AGR experiments conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) in support of development and qualification of tri-structural isotropic (TRISO) low-enriched fuel for use in high temperature gas-cooled reactors. The test train contains five separate capsules that are independently controlled and monitored. Each capsule contains multiple 12.51 mm long compacts filled with low-enriched uranium carbide/oxide (UCO) TRISO fuel particles. The objectives of the AGR-5/6/7 experiment are to: 1. Irradiate reference-design fuel particles to support fuel qualification. 2. Establish operating margins for the fuel beyond normal operating conditions. 3. Provide irradiated fuel performance data and irradiated fuel samples for post-irradiation examination (PIE) and safety testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Neutron irradiation effects on the corrosion of Zircaloy-4 in a pressurized water reactor environment - 2016-0085

Long-time Advanced Test Reactor (ATR) corrosion weight-gain data from non-fueled α-processed Zircaloy-4 cladding coupons are presented herein. The data were generated in pressurized loops that simulated pressurized water reactor (PWR) chemistry, temperature, and neutron flux conditions. High neutron flux and high-fluence post-transition corrosion rates were accelerated over out-of-flux post-transition corrosion rates by more than 40 times at 270 deg. C and more than 30 times at 310 deg. C We conclude in large part that the acceleration was caused by irradiation-induced changes to the base metal. The effect that irradiation has on the base metal and its effect on corrosion has been shown in the past to be carried over into post-irradiation tests in autoclave environments, but its impact was shown in this study to be accentuated in the in-reactor environment, in which sustained corrosion accelerations were much greater than observed in the postirradiation tests (in non-irradiation environments). This suggests some aspect of the radiation environment potentially acts synergistically with the corrosion film formed from the irradiation-damaged base metal to further accelerate in-reactor corrosion rates. We also present results from detailed microstructural examinations of thick (more than 25 μm) oxide films formed on α-processed Zircaloy-4 grown in a 360 deg. C autoclave and in the reactor. The examinations consisted of optical microscopy, field emission gun scanning electron microscopy, focused ion beam microscopy, analytical electron microscopy, and X-ray diffraction, with a focus on the evolution of the microstructure of the intermetallic precipitates in the oxide films during exposure to autoclave water or to the corroding environment under neutron irradiation. The film microstructure suggests that the water environment was closer to the oxide-metal interface in the films grown in the reactor than in the autoclave-grown corrosion films examined, but it was not obvious from the microstructural examinations how the radiation environment facilitated that effect. (authors)

36 MATERIALS SCIENCE↗

High-temperature irradiation-resistant thermocouple instability model for in-pile reactor use

This article presents an instability model for the high-temperature irradiation-resistant thermocouple (HTIR-TC). Here the term instability defines the superposition of both drift and inhomogeneity of TC thermoelements occurring simultaneously. The HTIR-TC is an advanced thermocouple (TC) that uses the refractory metals niobium and molybdenum as sensing thermoelements for generating electromotive force (EMF) in a field of neutrons and at temperatures upward of 1,600°C. In the Advanced Gas Reactor (AGR) 5/6/7 tests conducted at Idaho National Laboratory’s Advanced Test Reactor (ATR), the HTIR-TCs showed low to moderate instability throughout the life of the test. The instability model reveals that HTIR-TCs can, when the operating temperature of the reactor fuel is normal, maintain performance throughout an 18-month refueling cycle typical of nuclear power plants, reflecting an instability of less than ±1%. The HTIR-TC is also qualified for incorporation into a test fixture during the testing of new fuels.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Determination of the Quantity of I-135 Released from the AGR Experiment Series

A series of three Advanced Gas Reactor (AGR) experiments have been conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). From 2006 through 2014, these experiments supported the development and qualification of the new U.S. tri structural isotropic (TRISO) particle fuel for Very High Temperature Reactors (VHTR). Each AGR experiment consisted of multiple fueled capsules, each plumbed for independent temperature control using a mix of helium and neon gases. The gas leaving a capsule was routed to individual Fission Product Monitor (FPM) detectors. For intact fuel particles, the TRISO particle coatings provide a substantial barrier to fission product release. However, particles with failed coatings, whether because of a minute percentage of initially defective particles, those which fail during irradiation, or those designed to fail (DTF) particles, can release fission products to the flowing gas stream. Because reactive fission product elements like iodine and cesium quickly deposit on cooler capsule components and piping structures as the effluent gas leaves the reactor core, only the noble fission gas isotopes of Kr and Xe tend to reach FPM detectors. The FPM system utilizes High Purity Germanium (HPGe) detectors coupled with a thallium activated sodium iodide NaI(Tl) scintillator. The germanium detector provides individual isotopic information, while the NaI(Tl) scintillator is used as a gross count rate meter. During irradiation, the 135mXe concentration reaching the FPM detectors is from both direct fission and by decay of the accumulated 135I. About ~2.5 hours after irradiation (ten 15.3 minute 135mXe half lives) the directly produced 135mXe has decayed and only the longer lived 135I remains as a source. Decay systematics dictate that 135mXe will be in secular equilibrium with its 135I parent, such that it’s production rate very nearly equals the decay rate of the parent, and its concentration in the flowing gas stream will appear to decay with the parent half life. This equilibrium condition enables the determination of the amount of 135I released from the fuel particles by measurement of the 135mXe at the FPM following reactor shutdown. In this paper, the 135I released will be reported and compared to similar releases for noble gases as well as the unexpected finding of 131I deposition from intentional impure gas injection into capsule 11 of experiment AGR 3/4.

AGR↗

Status Report on Efforts to Enhance Instrumentation to Support Advanced Test Reactor Irradiations

The Department of Energy (DOE) designated the Advanced Test Reactor (ATR) as a National Scientific User Facility (NSUF) in April 2007 to support the growth of nuclear science and technology in the United States (US). By attracting new research users - universities, laboratories, and industry - the ATR NSUF facilitates basic and applied nuclear research and development, further advancing the nation's energy security needs. A key component of the ATR NSUF effort at the Idaho National Laboratory (INL) is to design, develop, and deploy new in-pile instrumentation techniques that are capable of providing real-time measurements of key parameters during irradiation. To address this need, an assessment of instrumentation available and under-development at other test reactors was completed. Based on this initial review, recommendations were made with respect to what instrumentation is needed at the ATR, and a strategy was developed for obtaining these sensors. In 2009, a report was issued documenting this program’s strategy and initial progress toward accomplishing program objectives. Since 2009, annual reports have been issued to provide updates on the program strategy and the progress made on implementing the strategy. This report provides an update reflecting progress as of January 2014.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Validation of the Fast and Thermal Neutron Flux Profiles in the Advanced Test Reactor for the AGR-3/4 Experiment

The AGR-3/4 experiment was designed to irradiate TRISO particle fuel in the Advanced Test Reactor (ATR) at the Idaho National Laboratory. Temperature control of the test capsules containing the TRISO particles was important since the goal was to measure diffusion rates of fission product elements through graphite as a function of temperature. During the experiment, differences were observed between temperatures measured by the thermocouples and temperatures calculated with the thermal analysis model. To rule out the possibility that the used ATR driver fuel elements were the root cause of these temperature differences, an experiment was devised to measure the axial fast and thermal neutron flux profiles in the northeast flux trap containing the AGR-3/4 experiment. An important input parameter to the thermal analysis model was the calculated compact heat rates from the MCNP physics model. To verify these calculated heat rates were consistent with the ATR driver fuel element loading and operating lobe power, axial flux wires were inserted into ATR northeast flux trap. The measured fast and thermal neutron axial flux profiles derived from the flux wire activation showed excellent agreement with the calculated flux profiles. This agreement dispelled any concerns that the used ATR fuel elements in the northeast lobe might have introduced unusual axial flux variation. In addition, the agreement provided a validation basis for the physics calculation, specifically, (1) MCNP physics model, (2) Monte Carlo depletion methodology, (3) method used to load the ATR driver fuel, and (4) ATR measured lobe power data used in the calculation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Non-destructive analysis of swelling in the EMPIrE fuel test

The European Mini-Plate Irradiation Experiment (EMPIrE) was designed to support the development and testing of a coated uranium-molybdenum (U-Mo) dispersion fuel for the conversion of select high-performance research reactors (HPRRs) to utilize low-enriched uranium (LEU). To aid in the development of the coated fuel form, the EMPIrE test included several plate designs and irradiated them in the Idaho National Laboratory (INL) Advanced Test Reactor (ATR) at a high meat power density (~21 kW/cm 3 ) and to high fuel particle fission densities (~6.4 × 10 21 fissions/cm 3 ). These conditions mimic the bounding conditions of the BR-2 reactor in Belgium, where a concurrent irradiation experiment was performed, and exceed those previously explored in dispersion U-Mo fuel plates. A local fuel swelling analysis, as determined through high-fidelity, post-irradiation mini-plate profilometry, was used along with statistical methods to non-destructively evaluate the overall performance and separate the effects of convoluted fabrication variables. While some effects observed with this non-destructive analysis were subtle, others had more significant, and possibly competing, effects on the fuel swelling behavior. In closing, these observations will be examined further with destructive examinations to more fully assess them as the fuel design is developed and qualified.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NEW AS-RUN NEUTRONICS ANALYSIS FOR RERTR-12 FUEL FOIL EXPERIMENTS

The Reduced Enrichment Research and Test Reactor (RERTR)-12 experiments were designed and carried out in support of what was known as Global Threat Reduction Initiative (GTRI) but has been more recently renamed as Materials Management and Minimization for the Fuel Development (FD) program. From February 2010 through May 2012, the RERTR-12 experimental capsules were inserted into the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) for five irradiation cycles. The purpose of these experiments was to “provide comprehensive information on the performance of uranium-molybdenum (U-Mo) based monolithic fuels for research reactor applications.” As-run neutronics, in-cluding depletion, analyses of the experiments have been performed within the Experiment Design and Analysis group at the Idaho National Laboratory. This paper summarizes the results from a new, in-depth as-run analysis that has been recently completed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Computer Network Connection for the Advanced Test Reactor Critical (ATR-C) Facility

The proposed activity would install a computer network connection in the Advanced Test Reactor Critical (ATR-C) Facility by running conduit from the west side office area near the entry into ATR-C and pulling in four category 5E (Cat5E) cables. The proposed activity would include running the Cat5E cables and associated conduit approximately 70 ft through the corridor from the office area and through the block wall into the southwest corner of ATR-C.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Design and Laboratory Evaluation of Future Elongation and Diameter Measurements at the Advanced Test Reactor

New materials are being considered for fuel, cladding, and structures in next generation and existing nuclear reactors. Such materials can undergo significant dimensional and physical changes during high temperature irradiations. In order to accurately predict these changes, real-time data must be obtained under prototypic irradiation conditions for model development and validation. To provide such data, researchers at the Idaho National Laboratory (INL) High Temperature Test Laboratory (HTTL) are developing several instrumented test rigs to obtain data real-time from specimens irradiated in well-controlled pressurized water reactor (PWR) coolant conditions in the Advanced Test Reactor (ATR). This paper reports the status of INL efforts to develop and evaluate prototype test rigs that rely on Linear Variable Differential Transformers (LVDTs) in laboratory settings. Although similar LVDT-based test rigs have been deployed in lower flux Materials Testing Reactors (MTRs), this effort is unique because it relies on robust LVDTs that can withstand higher temperatures and higher fluxes than often found in other MTR irradiations. Specifically, the test rigs are designed for detecting changes in length and diameter of specimens irradiated in ATR PWR loops. Once implemented, these test rigs will provide ATR users with unique capabilities that are sorely needed to obtain measurements such as elongation caused by thermal expansion and/or creep loading and diameter changes associated with fuel and cladding swelling, pellet-clad interaction, and crud buildup.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Thermal Predictions of the AGR-3/4 Experiment With Time-Varying Gas Gaps

In this paper, a thermal analysis was performed for the Advanced Gas Reactor test experiment (AGR-3/4) with time-varying gas gaps. The experiment was irradiated at the Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL). Several fuel irradiation experiments are planned for the AGR Fuel Development and Qualification Program that supports the development of the Very-High-Temperature Gas-Cooled Reactor (VHTR) under the Next-Generation Nuclear Plant (NGNP) project. AGR-3/4 combines two tests in a series of planned AGR experiments to test tristructural-isotropic (TRISO)-coated, low-enriched uranium oxy-carbide fuel. Forty-eight TRISO-fueled compacts were inserted into 12 separate capsules for the experiment (four compacts per capsule). The purpose of this analysis was to calculate the temperatures of each compact and graphite layer to obtain daily average temperatures using time (fast neutron fluence)-varying gas gaps and to compare with experimentally measured thermocouple data. A finite-element heat transfer model was created for each capsule using the commercial code ABAQUS. Finally, model results are compared to thermocouple data taken during the experiment.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

As-Run Thermal Analysis for the AGC-4 Experiment Irradiated in the ATR

The Advanced Graphite Capsule (AGC) irradiation experiment will provide irradiation creep rate data for the new graphite proposed for the Next Generation Nuclear Plant (NGNP) program. The fourth experiment in the series (AGC-4) was designed to irradiate various types of graphite specimens at a temperature of 900 ºC and targeted displacements per atom (DPA) of 6. This experiment has been irradiated in the east flux trap of the Advanced Test Reactor (ATR) during the cycles of 157D, 158A, 162A, 162B, 164A, 164B, 166A, and 166B. Temperatures were monitored using twelve thermocouples (TC) located at various elevations in the reactor core, and variable helium-argon gas mixtures were used for gas gap temperature control of the specimens. The purpose of this Engineering Calculation and Analysis Report (ECAR) is to calculate the specimen temperature after the model is calibrated by the measured TC data with the as-run heating rates of the components, DPA of the graphite, and the gas mixture compositions during the experiment. As-run specimen mean temperature and the tolerance will be obtained.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Thermal Model for Horizontal In-Water and In-Air Mini-Plate Experiments in the Advanced Test Reactor

Mini-Plate (MP) irradiation tests are a fueled experiment designed for irradiation in multiple test locations in the Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL). MP experiments are considered a non-instrumented drop-in test where small aluminum-clad fuel plate samples are cooled directly by the ATR Primary Coolant System (PCS) water. These fueled experiments contain aluminum-clad fuel mini plates consisting of monolithic U-10Mo. Previous thermal analyses have been documented concerning oxide growth[1] and thermal safety margin[2] for the MP-2 experiment. A thermal analysis has been performed on the MP-2 experiment using a new technique for calculating the necessary time after the experiment has been irradiated and reactor shutdown necessary to not exceed the 95% lower bound blister threshold temperature for the fuel in a horizontal in air configuration. A horizontal in water model has also been analyzed and will be discussed. After the experiment is irradiated in the ATR, it is necessary to calculate the fuel meat temperatures at 12 hours after shutdown. This is done to assure that at the 12 hour mark, if this experiment is removed from the reactor and accidentally dropped onto the working tray and is in the most severe geometrical configuration of horizontal (minimum heat transfer) that fission products will not be released. The blister threshold temperature is considered this safety limit. The horizontal in air analysis is also performed considering that the experiment is horizontal in a drained canal and filled with air and natural convection heat transfer with air on the outside. The initial mini-plate testing campaign known as MP-1 [3] has been irradiated and its purpose was to form the base fuel specimens fabricated by various processes so that a single process can be down-selected for qualification. MP-2 will then serve to populate a comprehensive fuel performance data set for the down-selected fabrication process. The MP-2 experiment will be irradiated in several locations of the ATR as shown in Figure 1. The fuel plate thickness and geometry is identical to the MP-1 experiment [3], with the only variable being the fuel meat thickness. This model of the B-12 position is treated as encompassing the I-21, I-24, and B-9 positions since it has more fuel and higher total heat than the other positions. Since the blister threshold temperature is a function of fission density, a series of fission densities is calculated for the B-12 position to cover the other three positions. The B 12 position specifically uses fuel meat that is 0.016 in thick by 3.25 in long and 0.75 in tall. The total plate thickness is 0.050 in. Aluminum cladding forms the barrier between the PCS and the fuel meat. The purpose of this paper is to demonstrate this new technique developed to calculate the necessary decay time after shutdown for a series of fission densities using the ABAQUS [4] finite element and heat transfer code.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TEM Characterization of Nanostructured Grade 91 Neutron Irradiated to 6 DPA at 300 °C and 500 °C

Previously, samples of coarse grained (CG, grain diameter > 1 µm), ultra-fine grained (UFG, 1 µm> grain diameter> 100 nm), and nanocrystalline (NC, 100 nm> grain diameter) grade 91 steel were neutron irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). Grade 91 is a ferritic/martensitic steel alloy with a nominal composition of Fe-9%Cr-1%Mo by weight, and it is being studied for applications in advanced nuclear reactor designs including as a fuel cladding material in gas cooled reactors. To assess the viability of this alloy for nuclear applications, the role of grain boundary size has not been sufficiently explored as a mechanism for developing radiation-tolerant materials. To achieve an UFG microstructure the material was processed using equal channel angular pressing (ECAP), and the NC microstructure was achieved through high pressure torsion (HPT). Such samples of various geometries for different types of characterization were irradiated to a dose of 6 displacements per atom (DPA) at separate temperature conditions of 300 °C and 500 °C. Thus, there were a total of 6 experimental conditions, three grain sizes (CG, UFG, and NC), each irradiated at two different temperature conditions (300 °C and 500 °C).

36 - MATERIALS SCIENCE↗

Monitoring Methods for Early Detection of Inadvertent Fission Product Release at the Advanced Test Reactor

Isotope effluent data obtained during three instances of experiment failures at the Advanced Test Reactor (ATR) are analyzed to provide an overview of the methods used to detect initial signs of unintended fission product release. The data is contextualized with the operational experience, including means of identification and subsequent mitigation strategies, gained during these events. General trends as well as variations in isotopic behavior between the three failures are explored. Background on the Real Time Monitor, a High Purity Germanium detector, and other fission product monitoring systems utilized at the Advanced Test Reactor is also provided. The presented analysis was used to establish administrative action levels which are currently utilized by ATR for early detection of experiment fission product release. Early identification provides time to make programmatic decisions before approaching safety and environmental limits.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

GAIN Fuel Safety Research Workshop

The Gateway for Accelerated Innovation in Nuclear (GAIN) Fuel Safety Research Workshop was held in Idaho Falls, Idaho, at the Idaho National Laboratory (INL) meeting center in the Energy Innovation Laboratory (EIL). The purpose of the workshop was to gather fuel safety research needs from the broad range of industrial nuclear technology users and developers. The needs will be analyzed relative to the national laboratory capabilities to help inform program planning and funding. The workshop provided a forum to learn about transient testing from a research and regulatory perspective and tour participation of the Transient Reactor Test Facility (TREAT), Advanced Test Reactor (ATR), and Materials and Fuels Complex (MFC).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Release-to-Birth Ratios for AGR-2 Operating Cycles 147A through 154B

This Engineering Calculations and Analysis Report (ECAR) documents the release-to-birth (R/B) ratios of the Advanced Gas Reactor (AGR) experiment, AGR-2, irradiated in the Advanced Test Reactor (ATR) B-12 position during Cycle 147A (AGR-2 irradiation interval #1) through Cycle 154B (AGR-2 irradiation interval #11).

22 GENERAL STUDIES OF NUCLEAR REACTORS↗