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DOE OSTI2023

Hard x-ray – optical four-wave mixing using a split-and-delay line

New, hard x-ray free electron lasers (FEL) produce intense femtosecond-to-attosecond pulses at angstrom wavelengths, giving access to the fundamental spatial and temporal scales of matter. These revolutionary light sources open the door to applying the suite of nonlinear, optical spectroscopy methods at hard x-ray photon energies. Nonlinear spectroscopy with hard x-rays can allow for measuring the coherence properties of short wavelength excitations with atomic specificity and for understanding how high energy excitations couple to other degrees of freedom in atomic, molecular or condensed-phase systems. As a step in this direction, here we present hard x-ray, optical four-wave mixing (4WM) measurements done at 9.8 keV at the split-and-delay line at the x-ray correlation spectroscopy (XCS) hutch of the Linac Coherent Light Source (LCLS). In this work, we create an x-ray transient grating (TG) from a pair of crossing x-ray beams and diffract optical laser pulses at 400 nm from the TG. The key technical advance here is being able to independently vary the delays of the x-ray pulses. Measurements were made in 3 different solid samples: bismuth germinate (BGO), zinc oxide (ZnO) and yttrium aluminum garnet (YAG). The resulting phase-matched, 4WM signal is measured in two different ways: by varying the x-ray, x-ray pulse delay which can reveal both material and light source coherence properties and also by varying the optical laser delay with respect to the x-ray TG to study how the x-ray excitation couples to the optical properties. Although no coherent 4WM signal was seen in these measurements, the absence of this signal gives important information on experimental requirements for detecting this in future work. Also, our laser-delay scans, although not a new measurement, were applied to different materials than in past work and reveal new examples x-ray induced lattice dynamics in solids. This work represents a key step towards extending nonlinear optics and time-resolved spectroscopy into the hard x-ray regime.

47 OTHER INSTRUMENTATION↗

DOE OSTI2016

Study of hard double-parton scattering in four-jet events in p p collisions at s = 7 TeV with the ATLAS experiment

Inclusive four-jet events produced in proton--proton collisions at a centre-of-mass energy of sqrt{s} = 7 TeV are analysed for the presence of hard double-parton scattering using data corresponding to an integrated luminosity of 37.3 pb^-1, collected with the ATLAS detector at the LHC. The contribution of hard double-parton scattering to the production of four-jet events is extracted using an artificial neural network, assuming that hard double-parton scattering can be approximated by an uncorrelated overlaying of dijet events. For events containing at least four jets with transverse momentum p_T > 20 GeV and pseudorapidity eta < 4.4, and at least one having p_T > 42.5 GeV, the contribution of hard double-parton scattering is estimated to be f_{DPS} = 0.092 ^{+0.005}_{-0.011} (stat.) ^{+0.033}_{-0.037} (syst.). After combining this measurement with those of the inclusive dijet and four-jet cross-sections in the appropriate phase space regions, the effective cross-section, sigma_{eff}, was determined to be sigma_{eff} = 14.9 ^{+1.2}_{-1.0} (stat.) ^{+5.1}_{-3.8} (syst.) mb. This result is consistent within the quoted uncertainties with previous measurements of sigma_{eff}, performed at centre-of-mass energies between 63 GeV and 8 TeV using various final states, and it corresponds to 21^{+7}_{-6}% of the total inelastic cross-section measured at sqrt{s} = 7 TeV. The distributions of the observables sensitive to the contribution of hard double-parton scattering, corrected for detector effects, are also provided

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Hardness Prediction by Incorporating Heat Transfer and Molten Pool Fluid Flow in a Multi-pass, Multi-layer Weld for Onsite Repair of Grade 91 steel

Introduction: In the current fleet of fossil-fired power plants, creep strength enhanced ferritic steels (CSEF) are used to sustain the harsh service conditions. Enhanced properties of Grade 91 steel result from tempered martensite with a fine distribution of MX and M23C6 carbides. Grade 91 steel is subjected to onsite welding repair to remedy their degradation due to extreme service condition. Knowledge of weld repairability of these steels, such as as-welded hardness distribution, is essential to establishing sound repair procedures. Experimental trial and error tests can consume a lot of time as many welding variables need to be studied. For numerical modelling, most of the multi-pass multi-layer models are based on finite element method, which are limited to solve the heat conduction equation and ignore convective heat transfer due to melt flow. Moreover, the mesh has to be pre-built based on a known or assumed weld cross-section geometry. These finite element based models thus have limited predictive capability as defects are not considered and nugget size are pre-assumed. This research aims at developing a thermal and microstructure evolution model incorporating molten pool dynamics in a multi-pass multi-layer material deposition to predict the as-welded hardness distribution. Technical Approach: All the thermal, physical, and metallurgical properties of Grade 91 as a function of temperature are collected from the literature and inputted into the thermo-fluid model based on Flow-3D, a computational fluid dynamics software. A multi-pass, multi-layer material deposition is simulated where the melting of filler wire into the molten pool is directly considered based on the volume of fluid (VOF) method. The flow behaviour of the molten pool is used to understand the formation of deposition geometry and defects. The temperature profiles during the multi-pass, multi-layer welding are calculated. The results computed using the new model are compared against the experimental data of fusion zone geometry and thermal cycles. Hardness prediction in the heat-affected zone (HAZ) are made using Johnson-Mehl-Avrami (JMA) equation for solid-state phase transformation kinetics. The JMA parameters are extracted from the experimental data available in the literature. For comparison, a standard finite element heat conduction model is also developed to predict the thermal cycles and hardness distribution in the multi-pass, multi-layer weld. Expected Result: Results obtained using the molten pool dynamic simulation versus the finite element heat conduction model are compared. Specifically, the effects of convective heat transfer on the accuracy of the calculated thermal history, bead shape and size, and HAZ hardness distribution are examined.

Modeling, Grade 91 steel, Multi-pass multi-layer d↗

DOE OSTI2020

Hard X-Ray Excess from the Magnificent Seven Neutron Stars

We report significant hard X-ray excesses in the energy range 2–8 keV for two nearby isolated neutron stars: RX J1856.6-3754 and RX J0420.0-5022. These neutron stars have previously been observed in soft X-rays to have nearly thermal spectra at temperatures ~100 eV, which are thought to arise from the warm neutron star surfaces. We find nontrivial hard X-ray spectra well above the thermal surface predictions with archival data from the XMM-Newton and Chandra X-ray telescopes. We analyze possible systematic effects that could generate such spurious signals, such as nearby X-ray point sources and pileup of soft X-rays, but we find that the hard X-ray excesses are robust to these systematics to the extent that is possible to test. We also investigate possible sources of hard X-ray emission from the neutron stars and find no satisfactory explanation with known mechanisms, suggesting that a novel source of X-ray emission is at play. Here, we do not find high-significance hard X-ray excesses from the other five Magnificent Seven isolated neutron stars.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1981

A comparison of the height distributions of solar flare hard X-rays in thick target and thermal models

Using recent observations of solar hard X-ray bursts having a spatial resolution of a few arcsec, a computation is made of the theoretically predicted spatial variation of hard X-ray flux versus height in both thick target nonthermal and thermal models of solar hard X-ray bursts. The work on the thick target model revises previous results in this area by adopting a more realistic model for the flaring atmospheric structure and also by taking into account energy loss and scattering processes in the evolution of the nonthermal electron beam which have previously been neglected. It is noted that in the so-called 'thermal' model currently in vogue there is a substantial nonthermal bremsstrahlung component at all photon energies; it is further demonstrated that this nonthermal component results in a hard X-ray flux versus height distribution whose maximum brightness per unit length is, similarly to the thick target model, located in the chromosphere and not in the thermal source itself. The characteristics of the hard X-ray height distributions in both thick target and thermal models are summarized and compared.

Emslie, A. G.↗

NASA NTRS1985

Temporal and spectral characteristics of solar flare hard X-ray emission

Solar Maximum Mission observations of three flares that impose stringent constraints on physical models of the hard X-ray production during the impulsive phase are presented. Hard X-ray imaging observations of the flares on 1980 November 5 at 22:33 UT show two patches in the 16 to 30 keV images that are separated by 70,000 km and that brighten simultaneously to within 5 s. Observations to O V from one of the footprints show simultaneity of the brightening in this transition zone line and in the total hard X-ray flux to within a second or two. These results suggest but do not require the existence of electron beams in this flare. The rapid fluctuations of the hard X-ray flux within some flares on the time scales of 1 s also provide evidence for electron beams and limits on the time scale of the energy release mechanism. Observations of a flare on 1980 June 6 at 22:34 UT show variations in the 28 keV X-ray counting rate from one 20 ms interval to the next over a period of 10 s. The hard X-ray spectral variations measured with 128 ms time resolution for one 0.5 s spike during this flare are consistent with the predictions of thick-target non-thermal beam model.

Dennis, B. R.↗

NASA NTRS1986

Beta Backscatter Measures the Hardness of Rubber

Nondestructive testing method determines hardness, on Shore scale, of room-temperature-vulcanizing silicone rubber. Measures backscattered beta particles; backscattered radiation count directly proportional to Shore hardness. Test set calibrated with specimen, Shore hardness known from mechanical durometer test. Specimen of unknown hardness tested, and radiation count recorded. Count compared with known sample to find Shore hardness of unknown.

Morrissey, E. T.↗

NASA NTRS1987

High spectral resolution measurements of a solar flare hard X-ray burst

Observations are reported of an intense solar flare hard X-ray burst on June 27, 1980, made with a balloon-borne array of liquid nitrogen-cooled Ge detector which provided unprecedented spectral resolution (no more than 1 keV FWHM). The hard X-ray spectra throughout the impulsive phase burst fitted well to a double power-law form, and emission from an isothermal 0.1-1 billion K plasma can be specifically excluded. The temporal variations of the spectrum indicate that the hard X-ray burst is made up of two superposed components: individual spikes lasting about 3-15 sec, which have a hard spectrum and a break energy of 30-65 keV; and a slowly varying component characterized by a soft spectrum with a constant low-energy slope and a break energy which increases from 25 kev to at least 100 keV through the event. The double power-law shape indicates that DC electric field acceleration, similar to that occurring in the earth's auroral zone, may be the source of the energetic electrons which produce the hard X-ray emission.

Lin, R. P.↗

NASA NTRS1988

Energetic electrons in impulsive and extended solar flares as deduced from flux correlations between hard X-rays and microwaves

The peak flux relationship between hard X-rays and microwaves from solar flares is studied using about 400 events simultaneously recorded with the hard X-ray burst spectrometer on the SMM satellite and the Nobeyama 17 GHz radiometer. The data indicate that the hard X-ray and microwave peak fluxes correlate best for X-ray energies of less than about 80 keV for impulsive flares and greater than about 360 keV for extended flares. By postulating that electrons responsible for microwave emission at 17 GHz are those emitting hard X-rays at these photon energies, it is concluded that: (1) in impulsive flares, microwaves at about 20 GHz are emitted mainly by electrons of less than about 200 keV from a layer through which the electrons stream down into the thick-target hard X-ray source; and (2) in extended flares, microwaves are emitted mainly by MeV electrons trapped in a coronal loop or loops.

Kosugi, Takeo↗

NASA NTRS1990

Statistical study of the correlation of hard X-ray and type III radio bursts in solar flares

A large number of hard X-ray events which occurred during the maximum of solar cycle 21 have been analyzed in order to study their correlation with type III bursts. It is found that the distribution of occurrences of hard X-ray bursts correlated with type III radio bursts is significantly different from the distribution of all hard X-ray bursts. This result is consistent with the assumption that the hard X-ray and type III intensities are somewhat correlated. A bivariate distribution function of the burst intensities is fitted to the data and is used to determine that the typical ratio of X-ray intensity to type II intensity is about 10 and that the ratio of the number of X-ray producing-electrons to type III-producing electrons is about 1000. Three models which have been proposed to explain the relation between the accelerated hard X-ray and type III-producing electrons are examined in the context of these observations.

Hamilton, Russell J.↗

NASA NTRS1991

The association of solar millisecond radio spikes with hard X-ray emission

Conventional observational data regarding solar millisecond spikes are compared with data gathered simultaneously in the hard X-ray band by means of a statistical analysis. The analysis considers the association rate, correlation degree, and relative time delays between hard X-ray emissions (in the 25-438 keV range) and radio-spike events. About 95 percent of the radio-spike bursts occur during impulsive hard X-ray bursts, and approximately 43 percent of the compared events are characterized by hard X-ray time profiles that mimic the concentration of simultaneous radio spikes. The delay of the radio emission with respect to the hard X-ray bursts puts some constraints on the acceleration and propagation of particles. The time delays and the quantization into discrete radio events are theorized to be caused by the operation of the accelerator.

Guedel, M.↗

NASA NTRS1992

Stereoscopic observations of a solar flare hard X-ray source in the high corona

The vertical structure of the impulsive and gradual hard X-ray sources in high coronae and the characteristics of the impulsive soft X-ray emission are investigated on the basis of PVE, ICE, and GOES observations of the energetic flare on February 16, 1984. The average photon spectra observed by these instruments during the impulsive and gradual hard X-ray bursts are summarized. A comparison of these unocculted and partially occulted spectra shows that the sources of the impulsive hard X-ray (greater than about 25 keV) and impulsive soft X-ray (2-5 keV) emissions in this flare extended to coronal altitudes greater than about 200,000 km above the photosphere. At about 100 keV, the ratio of the coronal source brightness to the total source brightness was 0.001 during the impulsive phase and less than about 0.01 during the gradual hard X-ray burst. The sources of the gradual hard X-ray burst and gradual soft X-ray burst were almost completely occulted, indicating that these sources were located at heights less than 200,000 km above the photosphere.

Kane, S. R.↗

NASA NTRS1992

Imaging solar flares in hard X-rays using Fourier telescopes

The sun emits hard X-rays (above 10 keV) during solar flares. Imaging hard X-ray sources on the sun with spatial resolutions on the order of 1-5 arcsec and integration times of 1 sec will provide greater insight into the energy release processes during a solar flare. In these events, tremendous amounts of energy stored in the solar magnetic field are rapidly released leading to emission across the electromagnetic spectrum. Two Fourier telescope designs, a spatial modulation collimator and a rotating modulation collimator, were developed to image the full sun in hard X-rays (10-100 keV) in an end-to-end simulation. Emission profiles were derived for two hard X-ray solar flare models taken from the current solar theoretical literature and used as brightness distributions for the telescope simulations. Both our telescope models, tailored to image solar sources, were found to perform equally well, thus offering the designer significant flexibility in developing systems for space-based platforms. Given sufficient sensitive areas, Fourier telescopes are promising concepts for imaging solar hard X-rays.

Campbell, Jonathan W.↗

NASA NTRS1994

The correlation of solar flare hard X-ray bursts with Doppler blueshifted soft X-ray flare emission

We have investigated the temporal correlation between hard X-ray bursts and the intensity of Doppler blueshifted soft X-ray spectral line emission. We find a strong correlation for many events that have intense blueshifted spectral signatures and some correlation in events with modest blueshifts. The onset of hard X-rays frequently coincides to within a few seconds with the onset of blueshifted emission. The peak intensity of blueshifted emission is frequently close in time to the peak of the hard X-ray emission. Decay rates of the blueshifted and hard X-ray emission are similar, with the decay of the blueshifted emission tending to lag behind the hard X-ray emission in some cases. There are, however, exceptions to these conclusions, and, therefore, the results should not be generalized to all flares. Most of the data for this work were obtained from instruments flown on the Japanese Yohkoh solar spacecraft.

Bentley, R. D.↗

NASA NTRS1998

Discovery of Correlated Behavior Between the Hard X-Ray and the Radio Bands in Cygnus X-3

Using CGRO/BATSE hard X-ray data and GHz radio monitoring data from the Green Bank Interferometer (GBI), we have performed a long term study (approximately 1800 days) of the unusual X-ray binary Cygnus X-3 resulting in the discovery of a remarkable relationship between the two wavelength bands. We find that quiescent radio states are strongly anticorrelated with the intensity of the hard X-ray emission. With the onset of a flaring state the relationship switches to a correlation. This is most easily seen in the larger (> or = 1 Jy) flares where the preflare quenched radio emission is accompanied by a very low hard X-ray intensity, and recovery of the hard X-ray flux during the radio flare. The injection of plasma into the radio jets, associated with Cyg X-3, can be directly related to changes in the hard X-ray emission, and suggests the possibility of accretion-related and jet-related components of the high energy emission.

McCollough, M. L.↗

NASA NTRS2002

Hard X-Ray Emission of X-Ray Bursters

The primary goal of this proposal was to increase our understanding of the accretion dynamics and emission mechanisms in neutron-star low-mass x-ray binaries via accurate measurements of their broad-band x-ray spectrum with particular emphasis on the hard x-ray emission. We obtained an extensive set of Rossi X-Ray Timing Explorer (RXTE) observations of a bright hard x-ray outburst from the source 4U1728-34 including data obtained under this proposal and previously scheduled observations for another observer. We have constructed x-ray light curves in several energy bands, including hard energy bands, from these data. We also completed spectral analysis of several observations which show strong hard x-ray emission. We are currently performing timing analysis to search for possible correlations between the spectral and timing evolution of 4U1728-34. Due to the one-year delay in obtaining the observations made for the other observer (which are the ones containing the peak of the hard X-ray emission), the analysis for this project is not yet complete. Because 4U1728-34 shows interesting high-frequency timing behavior, we plan to complete the analysis as part of our on-going investigation of high-frequency timing of X-ray binaries.

Kaaret, P.↗

NASA NTRS2003

Non-Thermal Hard X-Ray Emission in Galaxy Clusters Observed with the BeppoSAX PDS

We study the X-ray emission in a Sample of galaxy clusters using the BeppoSAX PDS instrument in the 20 - 80 keV energy band. We estimate the non-thermal hard X-ray cluster emission (HXR) by modeling the thermal contribution from the cluster gas and the non-thermal contamination from the unobscured AGN in the clusters. We also evaluate the systematic uncertainties due to the background fluctuations. Assuming negligible contamination from the obscured AGN, the resulting non-thermal component is detected at a 2 sigma level in approx. 50% of the non-significantly AGN-contaminated clusters: A2142, A2199, A2256, A3376, Coma, Ophiuchus and Virgo. The data are consistent with a scenario whereby relaxed clusters have no hard X-ray component of non-thermal origin, whereas merger clusters do. The co-added spectrum of the above clusters indicates a power-law spectrum for the HXR with a photon index of 2.8+0.3-0.4 in the 12 - 115 keV band, and we find indication that it has extended distribution. These indications argue against significant contamination from obscured AGN, which have harder spectra and centrally concentrated distribution. These results are supportive of the assumption of the merger shock acceleration of electrons in clusters, which has been proposed as a possible origin of the non-thermal hard X-ray emission models. Assuming that the Cosmic Microwave Background photons experience Inverse Compton scattering from the merger-accelerated relativistic electrons, and thus produce the observed HXR, the measured hard X-ray slope corresponds to a differential momentum spectra of the relativistic electrons with a slope of mu = 3.8 - 5.0. In presence of cluster magnetic fields this relativistic electron population produces synchrotron emission with a spectral index of 1.4 - 2.1, consistent with radio halo observations of merger clusters. Thus both hard X-ray and radio observations of merger clusters are consistent with the Inverse Compton model. The observed slope of HXR is also consistent with that predicted by the non-thermal bremsstrahlung, which chus cannot be ruled by the fit to the current data, even though this model requires an extreme, untenable cluster energetics. Assuming centrally concentrated distribution of HXR, the data requires a harder slope for the HXR spectrum, which is consistent with secondary electron models, but this model yields a worse fit to the PDS data and thus seems to be disfavored over the primary electron Inverse Compton model.

Nevalainen, J.↗

NASA NTRS2004

Non-Thermal Hard X-Ray Emission in Galaxy Clusters Observed with the BeppoSAX PDS

We study the X-ray emission in a sample of galaxy clusters using the BeppoSAX PDS instrument in the 20-80 keV energy band. We estimate the nonthermal hard X-ray (HXR) cluster emission by modeling the thermal contribution from the cluster gas and the nonthermal contamination from the unobscured active galactic nuclei (AGNs) in the clusters. We also evaluate the systematic uncertainties due to the background fluctuations. Assuming negligible contamination from the obscured AGNs, the resulting nonthermal component is detected at a 2 sigma level in approx. 50% of the nonsignificantly AGN-contaminated clusters: A2142, A2199, A2256, A3376, Coma, Ophiuchus, and Virgo. The data are consistent with a scenario whereby relaxed clusters have no hard X-ray component of nonthermal origin, whereas merger clusters do, with a 20-80 keV luminosity of approx. 10(exp 43)-10(exp 44) h(sup -2 sub 50) ergs/s. The co-added spectrum of the above clusters indicates a power-law spectrum for the HXR emission with a photon index of 2.8(sup +0.3 sub -0.4) in the 12-115 keV band, and we find indication that it has extended distribution. These indications argue against significant contamination from obscured AGNs, which have harder spectra and a centrally concentrated distribution. These results are supportive of the assumption of the merger shock acceleration of electrons in clusters, which has been proposed as a possible origin of the nonthermal hard X-ray emission models. Assuming that the cosmic microwave background photons experience inverse Compton scattering from the merger-accelerated relativistic electrons and thus produce the observed HXR, the measured hard X-ray slope corresponds to a differential momentum spectra of the relativistic electrons with a slope of mu = 3.8-5.0. In presence of cluster magnetic fields this relativistic electron population produces synchrotron emission with a spectral index of 1.4-2.1, consistent with radio halo observations of merger clusters. Thus both hard X-ray and radio observations of merger clusters are consistent with the inverse Compton model.

Nevalainen, J.↗