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At least 235 records · Page 13

Alternative low cost electrodes for hybrid flow batteries

A redox flow battery may include: a membrane interposed between a first electrode positioned at a first side of the membrane and a second electrode positioned at a second side of the membrane opposite to the first side; a first flow field plate comprising a plurality of positive flow field ribs, each of the plurality of positive flow field ribs contacting the first electrode at first supporting regions on the first side; and the second electrode, including an electrode spacer positioned between the membrane and a second flow field plate, the electrode spacer comprising a plurality of main ribs, each of the plurality of main ribs contacting the second flow field plate at second supporting regions on the second side, each of the second supporting regions aligned opposite to one of the plurality of first supporting regions. As such, a current density distribution at a plating surface may be reduced.

Evans, Craig E.↗

Improvement of Quantification in Non-Destructive Characterization of Radioactive Waste Packages -Introduction to the Ideas of a Currently Started Project - 20197

For the characterization of radioactive waste packages (e.g. 200-L drums) with inhomogeneous activity and density distributions preferably non-destructive methods like segmented gamma scanning and transmission measurements are applied. While the first is used for identification of the radioactive inventory, both are necessary for a reliable activity quantification. Although at nuclear facilities, segmented gamma scanner are state-of-the-art and are mostly equipped with a vertically moveable transmission source the combining of this data and further a-priori information improving accuracy in data estimation giving realistic, reliable and traceable uncertainty estimations are improvable. This challenge is tackled by a R and D project funded by the German Federal Ministry of Education and Research (BMBF). The boundary conditions for this project are (i) taking into account the typical instrumentation available at nuclear facilities, (ii) minimize the overall measurement time and (iii) combining data from emission and transmission measurements by Bayesian methods. For the R and D project, being still in its initial stage, the basic ideas, the data used for evaluation and the result of a preliminary investigation demonstrating the proof of principle are presented. Additionally, some first aspects on spatial resolution in emission and transmission measurements are addressed. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Mergers Matter: Gravothermal Collapse in Dwarf Halos with Self-Interacting Dark Matter

Self-Interacting Dark Matter (SIDM) models with large cross sections at relative velocities below $\sim100\,{\rm km \, s}^{-1}$ can be tested with dwarf galaxy observations. We analyze six dark-matter-only zoom-in $\sim10^{10}\,{\rm M}_\odot$ halos with diverse assembly histories, adopting a cross section over mass of $σ/m = 70\,cm^2 \, g^{-1}$. We find that mergers inject orbital kinetic energy into the halo, altering the heat transport and the gravothermal evolution of the core. Three of the six halos -- those with the most quiescent merger histories -- show clear signs of core collapse in these simulations. Halos with sustained mergers do not collapse. Furthermore, merger-induced heat transport drives two non-collapsing halos to central densities well below the predictions of the gravothermal fluid model. These findings suggest a novel mechanism for producing dark-matter-deficient galaxies and expanding the diversity of rotation curves beyond what halo concentration alone predicts. Merger histories are thus essential for understanding central density distributions of dwarf galaxy halos in SIDM.

Silverman, Maya [UC, Irvine; Bohr Inst.] (ORCID:00↗

Densities and momentum distributions in A ≤ 12 nuclei from chiral effective field theory interactions

Current and future electron and neutrino scattering experiments will be greatly aided by a better understanding of the role played by short-range correlations in nuclei. Two-body physics, including nucleon-nucleon correlations and two-body electroweak currents, is required to explain the body of experimental data for both static and dynamical nuclear properties. In this work, we focus on examining nucleon-nucleon correlations from a chiral effective field theory perspective and provide a comprehensive set of new variational Monte Carlo calculations of one- and two-body densities and momentum distributions based on the Norfolk many-body nuclear Hamiltonians for A ≤ 12 systems. Here, online access to detailed tables and figures is available.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Chandra measurements of gas homogeneity and turbulence at intermediate radii in the Perseus Cluster

ABSTRACT We present a Chandra study of surface brightness fluctuations in the diffuse intracluster medium of the Perseus Cluster. Our study utilizes deep, archival imaging of the cluster core as well as a new mosaic of 29 short $\, 5\,$-ks observations extending in eight different directions out to radii of $r_{500} \sim 2.2\, r_{2500}$. Under the assumption that the distribution of densities at a given radius is log-normally distributed, two important quantities can be derived from the width of the log-normal density distribution on a given spatial scale: the density bias, that is equal to the square root of the clumping factor C; and the one-component turbulent velocity, vk,1D. We forward-model all contributions to the measured surface brightness, including astrophysical and particle background components, and account for the Poisson nature of the measured signal. Measuring the distribution of surface brightness fluctuations in 1 arcmin2 regions, spanning the radial range $0.3\rm {-}2.2\, r_{2500}$ ($7.8\rm {-}57.3\,$ arcmin), we find a small to moderate average density bias of around $3{{\ \rm per\ cent}}$ at radii below $1.6\, r_{2500}$. We also infer an average turbulent velocity at these radii of V1D < 400 km s−1. Direct confirmation of our results on turbulent velocities inferred from surface brightness fluctuations should be possible using the X-ray calorimeter spectrometers to be flown aboard the XRISM and Athena observatories.

79 ASTRONOMY AND ASTROPHYSICS↗

Mapping valence electron distributions with multipole density formalism using 4D-STEM

Recent advancement in aberration correction and detector technology opened a door to various applications using 4D-STEM, which yields a diffraction pattern for each scanning position within a crystal unit-cell in scanning transmission electron microscopy (STEM) and generates incredible amounts of data in momentum space. Currently 4D-STEM analysis relies on the center-of-mass of the diffraction patterns in electric field and charge density mapping. It only derives the total projected charge density and is limited to phase objects, e.g. extremely thin samples. Here, we propose a new analytical method to accurately map aspherical valence electron distributions with atom-centered multipolar functions formalism using the whole 4D-STEM dataset. We demonstrate that, with the full dynamical calculations for various sample thicknesses, the method is sensitive not only to the miniscule charge transfer, but also to the atomic site symmetry and aspherical electron orbitals. The process of the refinement is much more robust and reliable than quantitative convergent beam electron diffraction.

4D-STEM↗

Surface Water Mass Transformation in the Southern Ocean: The Role of Eddies Revisited

The water mass transformation (WMT) framework describes how water of one class, such as a discrete interval of density, is converted into another class via air–sea fluxes or interior mixing processes. Here, this paper investigates how this process is modified at the surface when mesoscale ocean eddies are present, using a state-of-the-art high-resolution climate model with reasonable fidelity in the Southern Ocean. The method employed is to coarse-grain the high-resolution model fields to remove eddy signatures, and compare the results with those from the full model fields. This method shows that eddies reduced the WMT by 2–4 Sv (10%–20%; 1 Sv ≡ 10 6 m 3 s −1 ) over a wide range of densities, from typical values of 20 Sv in the smoothed case. The corresponding water mass formation was reduced by 40% at one particular density increment, namely, between 1026.4 and 1026.5 kg m −3 , which corresponds to the lighter end of the range of Indian Ocean Mode Water in the model. The effect of eddies on surface WMT is decomposed into three terms: direct modulation of the density outcrops, then indirectly, by modifying the air–sea density flux, and the combined effect of the two, akin to a covariance. It is found that the first and third terms dominate, i.e., smoothing the outcrops alone has a significant effect, as does the combination of smoothing both outcrops and density flux distributions, but smoothing density flux fields alone has little effect. Results from the coarse-graining method are compared to an alternative approach of temporally averaging the data. Implications for climate model resolution are also discussed.

54 ENVIRONMENTAL SCIENCES↗

Laser power density dependence on charge state distribution of Ta ion laser plasma

Laser power density per pulse, which is commonly expressed with the unit of “W/cm2,” is an important parameter to characterize ablation plasma. To match a design charge state of heavy ion beam induced by a laser ion source, a laser power density must be carefully chosen. Above around 108 W/cm2 of laser power density, laser ablation plasma is emitted from the surface of solid material. Then, up to 109 W/cm2, the most abundant charge state is 1+. Because the ionization energy increases with higher charge states, increasing the laser intensity leads to the charge state distribution shifting higher. Increasing the density to increase charge states also results in lower time of flight due to higher velocities. The maximum laser power density is obtained by the smallest available laser spot size on the target material which is determined by the quality of the laser beam. For many accelerator applications, higher charge state beams are preferred. In particular cases, singly charge ion beams are demanded. Therefore, production of intermediate charge state beams has not been investigated well. In this study, we selected Ta4+ as an example demanded beam and tried to clarify how the transition of charge state distribution depends on laser power density. Conclusively, the possible specification of a laser ion source for Ta4+ delivery was elucidated.

Okamura, Masahiro (ORCID:0000000255521706)↗

Two-component axionic dark matter halos

We consider a two-component dark matter halo (DMH) of a galaxy containing ultra-light axions (ULA) of different mass. The DMH is described as a Bose–Einstein condensate (BEC) in its ground state. In the mean-field (MF) limit, we have derived the integro-differential equations for the spherically symmetrical wave functions of the two DMH components. We studied, numerically, the radial distribution of the mass density of ULA and constructed the parameters which could be used to distinguish between the two- and one-component DMH. Here, we also discuss an interesting connection between the BEC ground state of a one-component DMH and Black Hole temperature and entropy, and Unruh temperature.

97 MATHEMATICS AND COMPUTING↗

Fast Faraday cup for measuring the longitudinal distribution of particle charge density in non-relativistic beams

A Fast Faraday cup includes a group of electrodes including a ground electrode having a through hole and a collector electrode configured with a blind hole that functions a collector hole. The electrodes are configured to allow a beam (e.g., a non-relativistic beam) to fall onto the ground electrode so that the through hole cuts a beamlet that flies into the collector hole and facilitates measurement of the longitudinal distribution of particle charge density in the beam. The diameters, depths, spacing and alignment of the collector hole and the through hole are controllable to enable the Fast Faraday day cup to operate with a fast response time (e.g., fine time resolution) and capture secondary particles.

Sun, Ding↗

Fast faraday cup for measuring the longitudinal distribution of particle charge density in non-relativistic beams

A Fast Faraday Cup includes a group of electrodes including a grounded electrode having a through hole and a collector electrode configured with a blind hole that functions a collector hole. The electrodes are configured to allow a beam (e.g., a non-relativistic beam) to fall onto the grounded electrode so that the through hole cuts a beamlet that flies into the collector hole and facilitates measurement of the longitudinal distribution of particle charge density in the beam. The diameters, depths, spacing and alignment of the collector hole and the through hole are controllable to enable the Fast Faraday day cup to operate with a fast response time (e.g., fine time resolution) and capture secondary particles.

Sun, Ding↗

Scaling of pulsed nanosecond capillary plasmas at different specific energy deposition

Nano-second, capillary discharges (nCDs) are unique plasma sources in their ability to sustain high specific energy deposition ω dep approaching 10 eV/molecule in molecular gases. This high energy loading on short timescales produces both high plasma densities and high densities of molecular exited states. These high densities of electrons and excited states interact with each other during the early afterglow through electron collision quenching and associative ionization. In this paper we discuss results from a two-dimensional computational investigation of a nCD sustained in air at a pressure of 28.5 mbar and with a voltage amplitude 20 kV. Discharges were investigated for two circuit configurations—a floating low voltage electrode and with the low voltage electrode connected to ground through a ballast resistor. The first configuration produced a single ionization wave from the high to low voltage electrode. The second produced converging ionization waves beginning at both electrodes. With a decrease of the tube radius, the velocity of the ionization fronts decreased while the shape of the ionization wave changed from the electron density being distributed smoothly in the radial direction, to being hollow shaped where there is a higher electron density near the tube wall. For sufficiently small tubes, the near-wall maxima merge to have the higher density on the axis of the capillary tube. In the early afterglow, the temporal and radial behavior of the N 2 (C 3 Π u ) density is a sensitive function of ω dep due to electron collision quenching. Finally, these trends indicate that starting from ω dep $\geqslant$ 0.3 eV/molecule, it is necessary to take into account interactions of electrons with electronically excited species during the discharge and early afterglow.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Signatures of self-interacting dark matter on cluster density profile and subhalo distributions

Non-gravitational interactions between dark matter particles with strong scattering, but relatively small annihilation and dissipation, has been proposed to match various observables on cluster and group scales. In this paper, we present the results from large cosmological simulations which include the effects of different self-interaction scenarios. In particular we explore a model with the differential cross section that can depend on both the relative velocity of the interacting particles and the angle of scattering. We focus on how quantities, such as the stacked density profiles, subhalo counts and the splashback radius change as a function of different forms of self-interaction. We find that self-interactions not only affect the central region of the cluster, the effect well known from previous studies, but also significantly alter the distribution of subhalos and the density of particles out to the splashback radius. Therefore, our results suggest that current weak lensing data can already put constraints on the self-interaction cross-section that are only slightly weaker than the Bullet Cluster constraints (σ/m ≲ 2 cm 2 /g), and future lensing surveys should be able to tighten them even further making halo profiles on cluster scales a competitive probe for DM physics.

79 ASTRONOMY AND ASTROPHYSICS↗

Position-dependent Voronoi probability distribution functions for matter and halos

Here, we measure the Voronoi density probability distribution function (PDF) for both dark matter and halos in N-body simulations. For the dark matter, Voronoi densities represent the matter density field smoothed on a uniform mass scale, which approximates the Lagrangian density field. For halos, the Voronoi densities contain information about the local environment of each halo. We measure the halo virial masses, the total amount of dark matter within each halo Voronoi cell, and the halo Voronoi cell volumes, and we show how halo abundances depend on these three quantities. We then study the position-dependent Voronoi density PDF, measured within finite subregions of the Universe, using separate universe simulations. We demonstrate that the spatial variation of the position-dependent PDF is due to large-scale density fluctuations, indicating that the position-dependent PDF is a biased tracer of large-scale structure. We measure this bias for the dark matter, and interpret it as the bias of regions of the Lagrangian density field that are selected based on density. For the halos, this bias can be interpreted as a form of assembly bias. We present the mapping from late-time to early-time Voronoi density for each simulation dark matter particle, which is highly stochastic. We compare the median of this stochastic map with spherical collapse calculations and discuss challenges involved in modeling the evolution of the density field on these scales.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

From noise to information: The transfer function formalism for uncertainty quantification in reconstructing the nuclear density

The neutron distribution of neutron-rich nuclei provides critical information on the structure of finite nuclei and neutron stars. Parity violating experiments—such as PREX and CREX—provide a clean and largely model-independent determination of neutron densities. Such experiments, however, are challenging and expensive, which is why sound statistical arguments are required to maximize the information gained. We introduce a new framework, the “transfer function formalism,” aimed at uncertainty quantification, model selection, and experimental design in the context of neutron densities. The transfer functions (TFs) are built analytically by expressing the linear response of the objective function (e.g., χ2) to small perturbations of the data. Using the TF formalism, we are able to analyze the expected overall uncertainty—quantified in terms of bias and variance—of the mean square radius and interior density of 48 Ca and 208 Pb. Using relativistic mean field models as a proxy for the weak-charge density—and assuming that a total of five measurements could be performed on the weak form factor of 48 Ca and 208 Pb—we identify the optimal models and experimental locations that minimize the uncertainty in the extraction of the radius and interior density. We also explore the use of the TF formalism to understand the influence of prior distributions for the model parameters, as well as the optimization of model hyperparameters not constrained by the data. Here,we establish how the choice of experimental locations and the model that is used can have a significant impact on the final uncertainties of the extracted quantities of interest. For challenging experiments such as CREX and PREX, a proper quantification of such uncertainties is critical. We have demonstrated how the TF formalism provides several advantages for this type of analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Survey on stochastic distribution systems: A full probability density function control theory with potential applications

Complex systems seen either in general engineering practice or economics are subjected to ever increased uncertainties that are mostly represented as random variables or parameters, and the characteristics of random variables are represented by their probability density functions (PDFs). Controlling their PDFs means to shape their stochastic distributions and in general it would provide a full treatment for system analysis and operational control and optimization. This leads to the development of stochastic distribution control (SDC) systems theory in the past decades, where the original aim of the controller design is to realize a shape control of the distributions of certain random variables in their PDFs sense for some engineering processes. Indeed, once the PDFs of these random variables or parameters are used to describe their distribution characters, the control task is to obtain control signals so that the output PDFs of stochastic systems are made to follow their target PDFs. The subject of SDC was initially originated for non-Gaussian stochastic control systems design but has found a wide spectrum of applications in general systems in terms of data-driven modeling, analysis, signal processing (filtering), data mining via multivariable statistics, decision-making (optimization) for systems subjected to uncertainties and even in economics. In this context, SDC constitutes an effective primer tool for complex system analysis, control and operational optimizations. In this review paper, a detailed survey of the developments on the research of SDC systems will be made together with their wide spectrum applications and future perspectives.

42 ENGINEERING↗