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NASA NTRS1992

The contribution of electron collisions to rotational excitations of cometary water

The e-H2O collisional rate for exciting rotational transitions in cometary water is evaluated for conditions found in comet Halley during the Giotto spacecraft encounter. In the case of the O(sub 00) yields 1(sub 11) rotational transition, the e-H2O collisional rate exceeds that for excitation by neutral-neutral collisions at distances exceeding 3000 km from the cometary nucleus. Thus, the rotational temperature of the water molecule in the intermediate coma may be controlled by collisions with electrons rather than with neutral collisions, and the rotational temperature retrieved from high resolution infrared spectra of water in comet Halley may reflect electron temperatures rather than neutral gas temperature in the intermediate coma.

Xie, Xingfa↗

NASA NTRS1991

Infrared spectroscopy of cometary parent molecules

The wealth of information on cometary physics provided by high-resolution spectroscopy of the IR water transitions is discussed. Specifically, the absolute line intensities and spatial brightness profiles are used to determine water production rates and lifetimes; the relative line intensities and spatial brightness profiles are used to determine water production rates and lifetimes; the relative line intensities probe the kinetic temperature profile in the coma; the line widths and line positions shed light on the coma outflow dynamics; and the temporal variability in the lines provides information on the structure of the nucleus. These observations also make it possible to determine the water ortho-to-para ratio, which may elucidate the origin and/or evolution of cometary nuclei. Recent advances in IR instrumentation promise to extend sensitivities for parent molecule searches to relative abundances well below 1 percent, especially if cooled, earth-orbiting facilities are available.

Weaver, H. A.↗

NASA NTRS1991

Irradiation effects on comets and cometary debris

Experimental results obtained over the past 10 years on the chemical and physical changes induced by ion and electron irradiation of materials relevant to comets are reviewed, and their physical interpretation and their relevance for cometary astrophysics are addressed. Four phases of the irradiation history are considered: the precometary phase, the accretion phase, the cometary phase, and the postcometary phase. The relevant applications of laboratory results are reviewed. The ability of ion irradiation of simple carbon-containing ices to produce complex refractory organic materials is discussed. In the Oort cloud, this process can occur several meters into the surface, so that the buildup of a stable organic crust may occur. Ion irradiation at various stages is compared with other models for the production of organics.

Strazzulla, G.↗

NASA NTRS1991

Optical properties of cometary dust

The application of measured optical constants to the interaction of electromagnetic radiation with small cometary dust particles is discussed, with emphasis on the interpretation of cometary observations. It is found that in some spectral regions optical constants vary greatly with wavelength. The optical constants may be incorrect. Because of errors in measurement, or the application of the Kramers-Kronig relationship over too small a spectral region, or an improperly prepared sample, the derived optical constants may be in error. It is suggested that a full Kramers-Kronig analysis and application of the more important sum rules should be performed on any set of optical constants whose accuracy is important. Optical constants derived from the measurement of inhomogeneous materials, where the inhomogeneities are of comparable size to that of the beam of radiation used in the experiment, should not be used to predict the optical properties of small particles.

Lien, David J.↗

NASA NTRS1992

Cometary origin of carbon, nitrogen, and water on the earth

In this paper, two assumptions on the origin of the earth are substantiated: (1) that the earth accreted from fine hot degassed dust particles containing no volatiles; and (2) that, after the accretion was finished, all the volatiles of the biosphere, including the atmosphere and the oceans, were brought to the earth by cometary bombardment. A temperature of more than 1000 K is deduced at the time when the dust that was going to form the earth was separated from the gas phase. This implies grains of anhydrous silicates and of reduced iron, without either water, carbon, or any labile elements, which remained in gas phase; thus, the minor bodies could not produce atmosphere or oceans. The second assumption is based on the evidence that cometary nuclei are formed in the outer space, by accumulation of frosty particles containing large amounts of ice and volatile molecules. It is shown that the icy bodies which hit the earth are more than enough to explain the whole biosphere.

Delsemme, A. H.↗

NASA NTRS1993

Identification of cometary and asteroidal particles in stratospheric IDP collections

He release temperature curves were determined for a specially processed set of 5 microns to 15 microns stratospheric IDP's whose masses, densities, and compositions were accurately measured. The He release temperature in combination with atmospheric entry calculations yields a most probable entry velocity for each particle and association with either an asteroidal (low velocity) or cometary (high velocity) origin. It was found that over half of the 5-15 microns IDP's have entry velocities consistent with asteroidal origin and that at least 20 percent have cometary origins. A few of the asteroidal particles are porous aggregates and it appears that there may be close material similarities among some primitive asteroids and comets. In the processing of individual 5 microns IDP's and determination of entry velocities, a few dozen microtome slices that can be used for a variety of detailed TEM, IR, and ion probe studies were preserved. These procedures provide laboratory samples that can be generically associated with asteroids and comets and are in a sense a limited sample return mission from these primitive bodies.

Brownlee, D. E.↗

NASA NTRS1993

Geochemical evidences for two chondritic-like cometary or asteroidal impacts before and at the K/T boundary

A number of geological and palaeontological evidences support multiple impacts of cometary showers within a short time (approximately 1-3 Ma) and their connection with mass extinctions. Observations include clustered crater ages, stratigraphic horizons of impact ejecta closely spaced in time, and evidence for stepwise mass extinctions spanning intervals of 1-3 Ma. For the K/T boundary, three candidates, Popigai, Manson, and Yucatan, have been proposed as impact craters. Two distinct strata at the K/T boundary in western North America have been interpreted as evidence for two sequential impacts. If multiple impacts occurred within a time span of about 1 Ma then multiple Ir enrichments should be observed. DSDP Hole 577B on the Shatsky Plateau in the northern Pacific at K/T time is the first site. Samples contain approximately greater than 97 percent CaCO3, which exhibit clear chemical signals associated with asteroidal/cometary impact. Ir, Fe, and Cr data are presented. From the Th-normalized data, two satellite peaks below the major peak at 78 cm and 81 cm of 577B-1-4 are clearly shown. The major Ir peak (K/T boundary) is at 72 cm. Fe and Cr, from C1-like impactor ejecta fallout, also show two peaks at the same positions. For hole 738C on the southern Kerguelen Plateau, Ir values reach a peak concentration of 18 ppb in the clay layer at 96.0-96.2 cm in section 20R-5, and gradually tail off. In the sample 115 cm above the boundary, Ir concentrations have still not reached background levels. From the Ir peak downward to the lowermost sample analyzed at 102 cm, the Ir concentration is still as high as 1.7 ppb. From the Th-normalized data, we observe a small Ir/Th peak at 100-101 cm. Though this peak is within the error margin, the trend is clear. Fe and Cr exhibit the same pattern. The third case is Hole 690C on the Queen Maud Ridge. Again, the Ir/Th plot indicates the strong possibility of satellite peaks at approximately 52 cm. The main peak is at 39-40 cm. For the Stevns Klint K/T boundary layers, the stratification of trace elements appears threefold with peak concentrations in sublayers A1, A3, and B2 for different element groups, including Ir. C1 ratios for many siderophile elements found in combined layers III and IV, corresponding to layers A, B, C, and D, strongly support the impact hypothesis. Also, multiple Ir anomalies in the K/T section at Lattengebirge, Bavarian Alps are reported. Recent works on Ni-rich spinels and Ir at the K/T boundaries clearly establish cometary/asteroidal impacts at the K/T boundary. Lastly, cometary showers can explain the enhanced Ir contents over approximately a 1 Ma interval in Gubbio shales.

Liu, Y.-G.↗

NASA NTRS1995

Organic Compounds Produced by Photolysis of Realistic Interstellar and Cometary Ice Analogs Containing Methanol

The InfraRed (IR) spectra of UltraViolet (UV) and thermally processed, methanol-containing interstellar / cometary ice analogs at temperatures from 12 to 300 K are presented. Infrared spectroscopy, H-1 and C-13 Nuclear Magnetic Resonance (NMR) spectroscopy, and gas chromatography-mass spectrometry indicate that CO (carbon monoxide), CO2 (carbon dioxide), CH4 (methane), HCO (the formyl radical), H2CO (formaldehyde), CH3CH2OH (ethanol), HC([double bond]O)NH2 (formamide), CH3C([double bond]O)NH2 (acetamide), and R[single bond]C[triple bond]N (nitriles) are formed. In addition, the organic materials remaining after photolyzed ice analogs have been warmed to room temperature contain (in rough order of decreasing abundance), (1) hexamethylenetetramine (HMT, C6H12N4), (2) ethers, alcohols, and compounds related to PolyOxyMethylene (POM, ([single bond]CH2O[single bond](sub n)), and (3) ketones (R[single bond]C([double bond]O)[single bond]R') and amides (H2NC([double bond]O)[single bond]R). Most of the carbon in these residues is thought to come from the methanol in the original ice. Deuterium and C-13 isotopic labeling demonstrates that methanol is definitely the source of carbon in HMT. High concentrations of HMT in interstellar and cometary ices could have important astrophysical consequences. The ultraviolet photolysis of HMT frozen in H2O ice readily produces the 'XCN' band observed in the spectra of protostellar objects and laboratory ices, as well as other nitriles. Thus, HMT may be a precursor of XCN and a source of CN in comets and the interstellar medium. Also, HMT is known to hydrolyze under acidic conditions to yield ammonia, formaldehyde, and amino acids. Thus, HMT may be a significant source of prebiogenic compounds on asteroidal parent bodies. A potential mechanism for the radiative formation of HMT in cosmic ices is outlined.

Bernstein, Max P.↗

NASA NTRS2001

Responses of the Jovian Atmosphere to Cometary Particles and Photon Impacts

Detailed calculations were performed of the deposition of energetic oxygen ions into the atmosphere of Jupiter. A Monte Carlo simulation was used. Similar processes occur in other astrophysical environments to which our methods can be applied. In particular Cravens has suggested that the X-ray emissions seen from comets are due to transitions from excited states following capture of electrons by solar wind ions colliding with the atmosphere of the comet. Alternative proposals have been advanced for the source of the cometary X-rays. We have carried out a study of the spectra and have shown that with the spectral resolution of about 20 eV the different excitation mechanisms can be distinguished. The response of the two components of the solar wind predict a spectrum that is consistent with the cometary observations. X-rays from the comets arise from the slow solar wind.

Dalgarno, Alex↗

NASA NTRS2004

Modeling of Cometary Atmospheres

The NASA supported project 'Modeling of Cometary Atmospheres' has been quite successful in broadening our understanding of the cometary environment. We list peer reviewed publications and conference presentation that have been made as a result of studies performed under this project. Following the list we present details of a selection of the results.

Gombosi, Tamas↗

NASA NTRS2006

Implications of Cometary Water: Deep Impact, Stardust and Hayabusa

Three recent in situ spacecraft missions have explored comets or asteroids, producing data in conflict with the standard comet paradigm, the Whipple Dirty Snowball Model (DSM). We have developed an alternative Wet Comet Model (WCM) which proposes that comets undergo an irreversible phase change to a wet comet when they enter within Mars orbit. The WCM may explain some of the observational discrepancies seen by Deep Impact, Stardust and Hayabusa. In particular, it accurately predicted Deep Impact observation of organics, biominerals, and meltwater temperatures. Predictions concerning Stardust s returned cometary dust particles have yet to be falsified, but if comets are largely composed of the silicates seen by Stardust, there may be a cometary explanation for Itokawa s low density rubble-pile observed by Hayabusa.

Sheldon, Robert B.↗

NASA NTRS2006

TOF-SIMS Analysis of Crater Residues from Wild 2 Cometary on Stardust Aluminum Foil

Impact residues of cometary particles on aluminum foils from the Stardust mission were investigated with TOF-SIMS for their elemental and organic composition. The residual matter from comet 81P/Wild 2 shows a wide compositional range, from nearly monomineralic grains to polymict aggregates. Despite the comparably small analyzed sample volume, the average element composition of the investigated residues is similar to bulk CI chondritic values. Analysis of organic components in impact residues is complicated, due to fragmentation and alteration of the compounds during the impact process and by the presence of contaminants on the aluminum foils. Nevertheless, polycyclic aromatic hydrocarbons (PAHs) that are unambiguously associated with the impact residues were observed, and thus are most likely of cometary origin.

Leutner, Jan↗

NASA NTRS2007

Stardust in STARDUST - the C, N, and O Isotopic Compositions of Wild 2 Cometary Matter in Al foil Impacts

In January 2006, the STARDUST mission successfully returned dust samples from the tail of comet 81P/Wild 2 in two principal collection media, low density silica aerogel and Al foil. While hypervelocity impacts at 6.1 km/s, the encounter velocity of STARDUST, into Al foils are generally highly disruptive for natural, silicate-dominated impactors, previous studies have shown that many craters retain sufficient residue to allow a determination of the elemental and isotopic compositions of the original projectile. We have used the NanoSIMS to perform C, N, and O isotope imaging measurements on four large (59-370 microns diameter) and on 47 small (0.32-1.9 microns diameter) Al foil impact craters as part of the STARDUST Preliminary Examination. Most analyzed residues in and around these craters are isotopically normal (solar) in their C, N, and O isotopic compositions. However, the debris in one large crater shows an average 15N enrichment of approx. 450 %, which is similar to the bulk composition of some isotopically primitive interplanetary dust particles. A 250 nm grain in another large crater has an O-17 enrichment with approx. 2.65 times the solar O-17/O-16 ratio. Such an O isotopic composition is typical for circumstellar oxide or silicate grains from red giant or asymptotic giant branch stars. The discovery of this circumstellar grain clearly establishes that there is authentic stardust in the cometary samples returned by the STARDUST mission. However, the low apparent abundance of circumstellar grains in Wild 2 samples and the preponderance of isotopically normal material indicates that the cometary matter is a diverse assemblage of presolar and solar system materials.

Stadermann, Frank J.↗

NASA NTRS2007

Non-Random Spatial Distribution of Impacts in the Stardust Cometary Collector

In January 2004, the Stardust spacecraft flew through the coma of comet P81/Wild2 at a relative speed of 6.1 km/sec. Cometary dust was collected at in a 0.1 sq m collector consisting of aerogel tiles and aluminum foils. Two years later, the samples successfully returned to earth and were recovered. We report the discovery that impacts in the Stardust cometary collector are not distributed randomly in the collecting media, but appear to be clustered on scales smaller than approx.10 cm. We also report the discovery of at least two populations of oblique tracks. We evaluated several hypotheses that could explain the observations. No hypothesis was consistent with all the observations, but the preponderance of evidence points toward at least one impact on the central Whipple shield of the spacecraft as the origin of both clustering and low-angle oblique tracks. High-angle oblique tracks unambiguously originate from a noncometary impact on the spacecraft bus just forward of the collector. Here we summarize the observations, and review the evidence for and against three scenarios that we have considered for explaining the impact clustering found on the Stardust aerogel and foil collectors.

Westphal, Andrew J.↗

NASA NTRS2007

Discovery of Non-random Spatial Distribution of Impacts in the Stardust Cometary Collector

We report the discovery that impacts in the Stardust cometary collector are not distributed randomly in the collecting media, but appear to be clustered on scales smaller than 10 cm. We also report the discovery of at least two populations of oblique tracks. We evaluated several hypotheses that could explain the observations. No hypothesis was consistent with all the observations, but the preponderance of evidence points toward at least one impact on the central Whipple shield of the spacecraft as the origin of both clustering and low-angle oblique tracks. High-angle oblique tracks unambiguously originate from a non-cometary impact on the spacecraft bus just forward of the collector.

Horz, Friedrich↗

NASA NTRS2007

Stardust in STARDUST - the C, N, and O Isotopic Compositions of Wild 2 Cometary Matter in Al Foil Impacts

In January 2006, the Stardust mission successfully returned dust samples from the tail of comet 81P/Wild 2 in two principal collection media, low density silica aerogel and Al foil. While hypervelocity impacts at the Stardust encounter velocity of 6.1 kilometers per second into Al foils are generally highly disruptive for natural, silicate-dominated impactors, previous studies have shown that many craters retain sufficient residue to allow a determination of the elemental and isotopic compositions of the original projectile. We have used two NanoSIMS ion microprobes to perform C, N, and O isotope imaging measurements on four large (59-295 micrometer diameter) and on 47 small (0.32-1.9 micrometer diameter) Al foil impact craters as part of the Stardust Preliminary Examination. Most analyzed residues in and around these craters are isotopically normal (solar) in their C, N, and O isotopic compositions. However, the debris in one large crater shows an average N-15 enrichment of approx. 450%o, which is similar to the bulk composition of some isotopically primitive interplanetary dust particles and to components of some primitive meteorites. A 250 nm grain in another large crater has an O-17 enrichment with approx. 2.65 times the solar O-17/O-16 ratio. Such an O isotopic composition is typical for circumstellar oxide or silicate grains from red giant or asymptotic giant branch stars. The discovery of this circumstellar grain clearly establishes that there is authentic stardust in the cometary samples returned by the Stardust mission. However, the low apparent abundance of circumstellar grains in Wild 2 samples and the preponderance of isotopically normal material indicates that the cometary matter is a diverse assemblage of presolar and solar system materials.

Stadermann, Frank J.↗

NASA NTRS2008

Collisional Processing of Olivine and Pyroxene in Cometary Dust

According to the nebular theory of solar-system formation, collisions between bodies occurred frequently early in the solar system s history and continue at a lower rate even today. Collisions have reworked the surface compositions and structures of cometary nuclei, though to an unknown degree. The majority of the collisional history of a typical Jupiter-family comet takes place while it resides in the Kuiper Belt. Impacts occur on the surfaces of small bodies over a large range of velocities by impactors of all sizes, but typical encounter speeds within the Kuiper Belt are 1.5 to 2.0 km/s[1]. Durda and Stern suggest that the interiors of most cometary nuclei with diameters <5 km have been heavily damaged by collisions [2]. They estimate that over a period of 3.5 Gy, a nucleus with a diameter of 2 km and an orbit between 35-45 AU will experience 90-300 collisions with objects greater than 8 m in diameter. In this same time interval, collisions between a typical Trans-Neptunian Object (TNO) 200 km in diameter and objects with d > 8 m would rework up to one-third of that TNO s surface. In fact, it has been proposed that most short-period comets from the Kuiper Belt (90%) are collisional fragments from larger TNOs - not primordial objects themselves [3] - and that most short-period comets from the Kuiper Belt will be collisionally processed both on their surfaces as well as in their interiors.

Lederer, S. M.↗

NASA NTRS2009

Cometary Glycine Detected in Samples Returned by Stardust

Our previous analysis of cometary samples returned to Earth by NASA's Stardust spacecraft showed several amines and amino acids, but the or igin of these compounds could not be firmly established. Here, we pre sent the stable carbon isotopic ratios of glycine and E-amino-n-caproic acid (EACA), the two most abundant amino acids identified in Stardu st-returned foil samples measured by gas chromatography-mass spectrom etry coupled with isotope ratio mass spectrometry. The Delta C-13 value for glycine of +29 +/- ? 6%: strongly suggests an extraterrestrial origin For glycine, while the Delta C-13 value for EACA of -25 +/-2 % indicates terrestrial contamination by Nylon-6 during curation. This represents the first detection of a cometary amino acid.

Elsila, Jamie E.↗