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At least 235 records · Page 13

Cloud–Aerosol–Turbulence Interactions: Science Priorities and Concepts for a Large-Scale Laboratory Facility

The purpose of this meeting summary, therefore, is to outline the range of scientific questions, and the facility concepts that were explored.We began the workshop with a series of overview talks to highlight scientific questions that could be investigated in a large-scale aerosol-cloud-turbulence laboratory facility. Topics included warm and mixed-phase cloud microphysics, aerosol and cloud chemistry, atmospheric turbulence, radiative transfer, cloud/aerosol instrumentation, and remote sensing. There was ample time for questions and discussion following each overview presentation. We also broke into groups for several hours at various points to enable more active discussion among all participants.

54 ENVIRONMENTAL SCIENCES↗

A Public-Private-Acadmic Partnership to Advance Solar Power Forecasting

The National Center for Atmospheric Research (NCAR) is pleased to have led a partnership to advance the state-of-the-science of solar power forecasting by designing, developing, building, deploying, testing, and assessing the SunCast™ Solar Power Forecasting System. The project has included cutting edge research, testing in several geographically- and climatologically-diverse high penetration solar utilities and Independent System Operators (ISOs), and wide dissemination of the research results to raise the bar on solar power forecasting technology. The partners include three other national laboratories, six universities, and industry partners. This public-private-academic team has worked in concert to perform use-inspired research to advance solar power forecasting through cutting-edge research to advance both the necessary forecasting technologies and the metrics for evaluating them. The project has culminated in a year-long, full-scale demonstration of provide irradiance and power forecasts to utilities and ISOs to use in their operations. The project focused on providing elements of a value chain, beginning with the weather that causes a deviation from clear sky irradiance and progresses through monitoring and observations, modeling, forecasting, dissemination and communication of the forecasts, interpretation of the forecast, and through decision-making, which produces outcomes that have an economic value. The system has been evaluated using metrics developed specifically for this project, which has provided rich information on model and system performance. Research was accomplished on the very short range (0-6 hours) Nowcasting system as well as on the longer term (6-72 hour) forecasting system. The shortest range forecasts are based on observations in the field. The shortest range system, built by Brookhaven National Laboratory (BNL) and based on Total Sky Imagers (TSIs) is TSICast, which operates on the shortest time scale with a latency of only a few minutes and forecasts that currently go out to about 15 min. This project has facilitated research in improving the hardware and software so that the new high definition cameras deployed at multiple nearby locations allow discernment of the clouds at varying levels and advection according to the winds observed at those levels. Improvements over “smart persistence” are about 29% for even these very short forecasts. StatCast is based on pyranometer data measured at the site as well as concurrent meteorological observations and forecasts. StatCast is based on regime-dependent artificial intelligence forecasting techniques and has been shown to improve on “smart persistence” forecasts by 15-50%. A second category of short-range forecasting systems employ satellite imagery and use that information to discern clouds and their motion, allowing them to project the clouds, and the resulting blockage of irradiance, in time. CIRACast (the system produced by the Cooperative Institute for Atmospheric Research [CIRA] at Colorado State University) was already one of the more advanced cloud motion systems, which is the reason that team was brought to this project. During the project timeframe, the CIRA team was able to advance cloud shadowing, parallax removal, and implementation of better advecting winds at different altitudes. CIRACast shows generally a 25-40% improvement over Smart Persistence between sunrise and approximately 1600 UTC (Coordinated Universal Time) . A second satellite-based system, MADCast (Multi-sensor Advective Diffusive foreCast system), assimilates data from multiple satellite imagers and profilers to assimilate a fully three-dimensional picture of the cloud into the dynamic core of WRF. During 2015, MADCast (provided at least 70% improvement over Smart Persistence, with most of that skill being derived during partly cloudy conditions. That allows advection of the clouds via the Weather Research and Forecasting (WRF) model dynamics directly. After WRF-Solar™ showed initial success, it was also deployed in nowcasting mode with coarser runs out to 6 hours made hourly. It provided improvements on the order of 50-60% over Smart Persistence for forecasts up to 1600 UTC. The advantages of WRF-Solar-Nowcasting and MADCast were then blended to develop the new MAD-WRF model that incorporates the most important features of each of those models, both assimilating satellite cloud fields and using WRF-So far physics to develop and dissipate clouds. MAE improvements for MAD-WRF for forecasts from 3-6 hours are improved over WRF-Solar-Now by 20%. While all the Nowcasting system components by themselves provide improvement over Smart Persistence, the largest benefit is derived when they are smartly blended together by the Nowcasting Integrator to produce an integrated forecast. The development of WRF-Solar™ under this project has provided the first numerical weather prediction (NWP) model specifically designed to meet the needs of irradiance forecasting. The first augmentation improved the solar tracking algorithm to account for deviations associated with the eccentricity of the Earth’s orbit and the obliquity of the Earth. Second, WRF-Solar™ added the direct normal irradiance (DNI) and diffuse (DIF) components from the radiation parameterization to the model output. Third, efficient parameterizations were implemented to either interpolate the irradiance in between calls to the expensive radiative transfer parameterization, or to use a fast radiative transfer code that avoids computing three-dimensional heating rates but provides the surface irradiance. Fourth, a new parameterization was developed to improve the representation of absorption and scattering of radiation by aerosols (aerosol direct effect). A fifth advance is that the aerosols now interact with the cloud microphysics, altering the cloud evolution and radiative properties, an effect that has been traditionally only implemented in atmospheric computationally costly chemistry models. A sixth development accounts for the feedbacks that sub-grid scale clouds produce in shortwave irradiance as implemented in a shallow cumulus parameterization Finally, WRF-Solar™ also allows assimilation of infrared irradiances from satellites to determine the three dimensional cloud field, allowing for an improved initialization of the cloud field that increases the performance of short-range forecasts. We find that WRF-Solar™ can improve clear sky irradiance prediction by 15-80% over a standard version of WRF, depending on location and cloud conditions. In a formal comparison to the NAM baseline, WRF-Solar™ showed improvements in the Day-Ahead forecast of 22-42%. The SunCast™ system requires substantial software engineering to blend all of the new model components as well as existing publically available NWP model runs. To do this we use an expert system for the Nowcasting blender and the Dynamic Integrated foreCast (DICast®) system for the NWP models. These two systems are then blended, we use an empirical power conversion method to convert the irradiance predictions to power, then apply an analog ensemble (AnEn) approach to further tune the forecast as well as to estimate its uncertainty. The AnEn module decreased RMSE (root mean squared error) by 17% over the blended SunCast™ power forecasts and provided skill in the probabilistic forecast with a Brier Skill Score of 0.55. In addition, we have also developed a Gridded Atmospheric Forecast System (GRAFS) in parallel, leveraging cost share funds. An economic evaluation based on Production Cost Modeling in the Public Service Company of Colorado showed that the observed 50% improvement in forecast accuracy will save their customers $819,200 with the projected MW deployment for 2024. Using econometrics, NCAR has scaled this savings to a national level and shown that an annual expected savings for this 50% forecast error reduction ranges from $11M in 2015 to $43M expected in 2040 with increased solar deployment. This amounts to a $455M discounted savings over the 26 year period of analysis.

14 SOLAR ENERGY↗

Multiscale ACI Satellite Database

The SATELLITE_EAGLES_PNNL NetCDF dataset contains a suite of satellite- and reanalysis-derived atmospheric and surface parameters on a regular latitude–longitude grid. The dataset includes core geophysical fields such as land fraction, aerosol optical depth at multiple wavelengths (465, 550, 667, and 865 nm), sea surface temperature, estimated inversion strength, and various thermodynamic and dynamic quantities (e.g., relative humidity, vertical velocity, boundary-layer height, and surface fluxes) from both MERRA and ERA reanalysis products, provided as daily-mean and instantaneous values. A major component of the dataset consists of MODIS-retrieved cloud microphysical properties, including cloud droplet number concentration, cloud effective radius, optical thickness, and liquid water path, provided for three compositing regimes (“All,” “Q06,” and “G18”). Corresponding cloud-top parameters—temperature, height, and pressure—along with total and domain-mean cloud fraction fields are also included. The file further integrates additional satellite data from AMSR-E (for cloud water, rain water, and surface precipitation retrievals) and CERES (for top-of-atmosphere radiative fluxes, cloud fractions, and albedo). This dataset is designed to evaluate aerosol–cloud interactions in warm clouds, emphasizing the use of MODIS for deriving cloud droplet number concentration and liquid water path statistics. The complementary satellite and reanalysis fields are co-located and time-matched to the same instantaneous MODIS observations, enabling consistent comparisons between cloud properties, aerosol loading, and large-scale meteorological conditions. The dataset is recently featured in Christensen et al. (2025), Machine Learning Reveals Strong Grid-Scale Dependence in the Satellite Nd–LWP Relationship, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2025-3850, 2025.

Christensen, Matthew [Pacific Northwest National L↗

Multiscale ACI Satellite Database

The SATELLITE_EAGLES_PNNL NetCDF dataset contains a suite of satellite- and reanalysis-derived atmospheric and surface parameters on a regular latitude–longitude grid. The dataset includes core geophysical fields such as land fraction, aerosol optical depth at multiple wavelengths (465, 550, 667, and 865 nm), sea surface temperature, estimated inversion strength, and various thermodynamic and dynamic quantities (e.g., relative humidity, vertical velocity, boundary-layer height, and surface fluxes) from both MERRA and ERA reanalysis products, provided as daily-mean and instantaneous values. A major component of the dataset consists of MODIS-retrieved cloud microphysical properties, including cloud droplet number concentration, cloud effective radius, optical thickness, and liquid water path, provided for three compositing regimes (“All,” “Q06,” and “G18”). Corresponding cloud-top parameters—temperature, height, and pressure—along with total and domain-mean cloud fraction fields are also included. The file further integrates additional satellite data from AMSR-E (for cloud water, rain water, and surface precipitation retrievals) and CERES (for top-of-atmosphere radiative fluxes, cloud fractions, and albedo). This dataset is designed to evaluate aerosol–cloud interactions in warm clouds, emphasizing the use of MODIS for deriving cloud droplet number concentration and liquid water path statistics. The complementary satellite and reanalysis fields are co-located and time-matched to the same instantaneous MODIS observations, enabling consistent comparisons between cloud properties, aerosol loading, and large-scale meteorological conditions. The dataset is recently featured in Christensen et al. (2025), Machine Learning Reveals Strong Grid-Scale Dependence in the Satellite Nd–LWP Relationship, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2025-3850, 2025.

54 ENVIRONMENTAL SCIENCES↗

Observational and Modeling Studies of Clouds and the Hydrological Cycle

Our approach involved validating parameterizations directly against measurements from field programs, and using this validation to tune existing parameterizations and to guide the development of new ones. We have used a single-column model (SCM) to make the link between observations and parameterizations of clouds, including explicit cloud microphysics (e.g., prognostic cloud liquid water used to determine cloud radiative properties). Surface and satellite radiation measurements were used to provide an initial evaluation of the performance of the different parameterizations. The results of this evaluation will then used to develop improved cloud and cloud-radiation schemes, which were tested in GCM experiments.

Somerville, Richard C. J.↗

The Role of Clouds: An Introduction and Rapporteur Report

This paper presents an overview of discussions during the Cloud s Role session at the Observing and Modelling Earth s Energy Flows Workshop. N. Loeb and B. Soden convened this session including 10 presentations by B. Stevens, B. Wielicki, G. Stephens, A. Clement, K. Sassen, D. Hartmann, T. Andrews, A. Del Genio, H. Barker, and M. Sugi addressing critical aspects of the role of clouds in modulating Earth energy flows. Presentation topics covered a diverse range of areas from cloud microphysics and dynamics, cloud radiative transfer, and the role of clouds in large-scale atmospheric circulations patterns in both observations and atmospheric models. The presentations and discussions, summarized below, are organized around several key questions raised during the session. (1) What is the best way to evaluate clouds in climate models? (2) How well do models need to represent clouds to be acceptable for making climate predictions? (3) What are the largest uncertainties in clouds? (4) How can these uncertainties be reduced? (5) What new observations are needed to address these problems? Answers to these critical questions are the topics of ongoing research and will guide the future direction of this area of research.

Taylor, Patrick C.↗

Toward Understanding the Simulated Phase Partitioning of Arctic Single-Layer Mixed-Phase Clouds in E3SM

21 Mixed-phase clouds are widespread in the Arctic and have substantial impacts on the 22 surface energy budget, sea ice extent, and regional climate. Significant changes are found in the 23 modeled phase partitioning of Arctic mixed-phase clouds in the newly developed U.S. 24 Department of Energy (DOE) Energy Exascale Earth System Model (E3SM) Atmosphere Model 25 version 1 (EAMv1) compared to its predecessor (CAM5/EAMv0). The mixed-phase clouds 26 simulated by EAMv1 is overly dominated by super-cool liquid which is often underestimated by 27 CAM5. Compared to CAM5, EAMv1 has made several important changes in its cloud physical 28 parameterizations, including using CLUBB to unify shallow convection, PBL turbulence, and 29 cloud macrophysics, as well as updating the MG two-moment cloud microphysics scheme and 30 using the CNT heterogeneous ice nucleation scheme to replace the Meyers scheme for mixed- 31 phase clouds. To understand which of the newly-implemented physical parameterizations is 32 responsible for the change of modeled mixed-phase cloud phase partitioning in EAMv1, 33 sensitivity tests are conducted by utilizing the short-term hindcast approach and results are 34 compared to the observations from the ARM Mixed-Phase Arctic Cloud Experiment (M-PACE) 35 field campaign. 36 It is found that although each scheme contributes to the decrease of cloud ice water 37 content (IWC) and increase of cloud liquid water content (LWC), only the combined effect of 38 CLUBB and CNT can explain the significant underestimation of IWC. By examining the budgets 39 of cloud microphysical processes, CLUBB is found to play a dominant role due to the fact that 40 CLUBB does not diagnoses cloud ice phase water in its assumed joint PDF method and thus may 41 not provide sufficient cloud ice to initialize ice phase microphysical processes such as the growth 42 of ice crystals through vapor deposition. Although a more effective heterogeneous ice nucleation 43 may alleviate the underestimation of IWC, the ice phase process in CLUBB requires urgent 44 attention in the future model development.

Zhang, Meng↗

High-resolution lidar observations of sedimentation-induced size sorting of droplets near a laboratory cloud top

Cloud optical properties and precipitation, which are crucial to weather and climate, are strongly influenced by cloud microphysical properties that are still poorly understood. Here, we develop a high-resolution time-correlated single-photon-counting lidar and apply it to observe cloud microphysical properties at one-centimeter range resolution in a convection chamber under well-controlled conditions. Together with concurrent in-situ measurements and theoretical analysis, our lidar observations indicate that although turbulent mixing tends to homogenize the cloud in the bulk region, entrainment and sedimentation cause inhomogeneities in droplet concentrations near the cloud top. Specifically, the topmost region is directly affected by entrainment, and lidar profiles show clear evidence of entrained air and detrained cloud filament. The transition region below exhibits vertical size sorting of cloud droplets caused by sedimentation. Our results suggest that using a single sedimentation velocity for all cloud droplets, as is done in many atmospheric models, overlooks key physics relevant to the microphysical structure near the cloud top. In conclusion, our conceptual model used to describe these measurements can serve as a step toward improving the current modeling of processes in the cloud top region.

54 ENVIRONMENTAL SCIENCES↗

High Latitude Climate Modeling: ARM Takes Us Beyond Case Studies (Final Report)

The main thrust of this project was to devise a method by which the majority of North Slope of Alaska (NSA) meteorological and radiometric data, collected on a daily basis, could be used to evaluate and improve global climate model (GCM) simulations and their parameterizations, particularly for cloud microphysics. Although the standard ARM Program sensors for a less complete suite of instruments for cloud and aerosol studies than the instruments on an intensive field program such as the 2008 Indirect and Semi-Direct Aerosol Campaign (ISDAC), the advantage they offer lies in the long time base and large volume of data that covers a wide range of meteorological and climatological conditions. The challenge has been devising a method to interpret the NSA data in a practical way, so that a wide variety of meteorological conditions in all seasons can be examined with climate models. If successful, climate modelers would have a robust alternative to the usual “case study” approach (i.e., from intensive field programs only) for testing and evaluating their parameterizations’ performance. Understanding climate change on regional scales requires a broad scientific consideration of anthropogenic influences that goes beyond greenhouse gas emissions to also include aerosol-induced changes in cloud properties. For instance, it is now clear that on small scales, human-induced aerosol plumes can exert microclimatic radiative and hydrologic forcing that rivals that of greenhouse gas–forced warming. This project has made significant scientific progress by investigating what causes successive versions of climate models continue to exhibit errors in cloud amount, cloud microphysical and radiative properties, precipitation, and radiation balance, as compared with observations and, in particular, in Arctic regions. To find out what is going wrong, we have tested the models' cloud representation over the full range of meteorological conditions found in the Arctic using the ARM North Slope of Alaska (NSA) data.

54 ENVIRONMENTAL SCIENCES↗

Precipitation over Land and the Southern Ocean (PLATO) Field Campaign Report

In order to complement the precipitation data collected as part of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Measurements of Aerosols, Radiation, and Clouds over the Southern Ocean (MARCUS) campaign deployment aboard our Australian Antarctic Division (AAD) icebreaker Aurora Australis during summer 2017/18, we installed a Metek Micro Rain Radar (MRR-PRO model) and an Eigenbrodt OceanRAIN disdrometer on the monkey island. Biases in absorbed shortwave radiation over the Southern Ocean in numerical models compared to observations are most likely associated with biases in the representation of cloud microphysical properties such as liquid cloud droplet concentration and liquid water path that can be assessed by understanding precipitation together with cloud phase. The addition of these two AAD instruments will, together with MARCUS, enable studies relating precipitation and cloud properties (drop size distribution, number concentration, and modal diameter) to aerosol properties over the Southern Ocean. We deployed the disdrometer for all four voyages of Aurora Australis during summer 2017/18. The MRR was installed on Voyage 1 (Davis Base resupply) and again on Voyage 4 (Macquarie Island resupply), but was removed for the other two voyages due to commitments elsewhere. Instead of using up one ship’s expeditioner berth for our own technician to monitor these instruments, we asked the ARM technicians, through the ARM field campaign office, to monitor data collection of the MRR and disdrometer and notify me of any issues. The MRR performed well on the voyages and collected data nearly continuously. However, the disdrometer’s performance was very disappointing, with very little data collected at all. This seems due to instrumental faults; indeed we thank the ARM technicians who performed as much technical diagnostics as were possible while aboard.

MARCUS campaign, Southern Ocean, cloud microphysic↗

Investigation of Turbulent Entrainment-Mixing Processes With a New Particle-Resolved Direct Numerical Simulation Model

Here, a new particle-resolved three dimensional direct numerical simulation (DNS) model is developed that combines Lagrangian droplet tracking with the Eulerian field representation of turbulence near the Kolmogorov microscale. Six numerical experiments are performed to investigate the processes of entrainment of clear air and subsequent mixing with cloudy air and their interactions with cloud microphysics. The experiments are designed to represent different combinations of three configurations of initial cloudy area and two turbulence modes (decaying and forced turbulence). Five existing measures of microphysical homogeneous mixing degree are examined, modified, and compared in terms of their ability as a unifying measure to represent the effect of various entrainment-mixing mechanisms on cloud microphysics. Also examined and compared are the conventional Damköhler number and transition scale number as a dynamical measure of different mixing mechanisms. Relationships between the various microphysical measures and dynamical measures are investigated in search for a unified parameterization of entrainment-mixing processes. The results show that even with the same cloud water fraction, the thermodynamic and microphysical properties are different, especially for the decaying cases. Further analysis confirms that despite the detailed differences in cloud properties among the six simulation scenarios, the variety of turbulent entrainment-mixing mechanisms can be reasonably represented with power-law relationships between the microphysical homogeneous mixing degrees and the dynamical measures.

54 ENVIRONMENTAL SCIENCES↗

Cloud Remote Sensing with EPIC/DSCOVR Observations: A Sensitivity Study with Radiative Transfer Simulations

The Earth Polychromatic Imaging Camera (EPIC) onboard the Deep Space Climate Observatory (DSCOVR) views nearly the whole sunlit face of the Earth with 10 spectral bands ranging from the UV to the near-infrared, including two oxygen absorbing bands centered at 764 nm (A-band) and 687.75 nm (B-band). Clouds are among the primary remote sensing targets using EPIC images because of their important impacts on the Earth’s radiation budget. In order to facilitate the EPIC cloud data product development, we have built a radiative transfer simulator featuring flexible cloud microphysical parameters, gas absorptions, and the instrument line shape functions for each EPIC band. The radiative transfer simulator is used to explore the sensitivity of EPIC observations on liquid-phase cloud microphysical parameters, including optical depth, geometric thickness, and cloud top height. We found that the ratios of the reflectances in the oxygen A and B bands to their respective continuum measurements can be used to increase the confidence level of cloud masking over scenes with sun-glint. In addition, the 388 nm band can be used to differentiate low and high clouds with the uncertainty of roughly 2–3 km. Combining this information with the oxygen absorption bands, the cloud geometric thickness can be obtained with the rough uncertainty of 3–4 km.

atmospheric and ocean optics↗

Cloud Phase Simulation at High Latitudes in EAMv2: Evaluation using CALIPSO Observations and Comparison with EAMv1

This study performs a comprehensive evaluation of the simulated cloud phase in the U.S. Department of Energy (DOE) Energy Exascale Earth System Model (E3SM) atmosphere model version 2 (EAMv2) and version 1 (EAMv1). Enabled by the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) simulator, EAMv2 and EAMv1 predicted cloud phase is compared against the GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) at high latitudes where mixed-phase clouds are prevalent. Our results indicate that the underestimation of cloud ice in simulated high-latitude mixed-phase clouds in EAMv1 has been significantly reduced in EAMv2. The increased ice clouds in the Arctic mainly result from the modification on the WBF (Wegner-Bergeron-Findeisen) process in EAMv2. The impact of the modified WBF process is moderately compensated by the low limit of cloud droplet number concentration (CDNC) in cloud microphysics and the new dCAPE_ULL trigger used in deep convection in EAMv2. Moreover, it is found that the new trigger largely contributes to the better cloud phase simulation over the Norwegian Sea and Barents Sea in the Arctic and the Southern Ocean where large errors are found in EAMv1. However, errors in simulated cloud phase in EAMv1, such as the overestimation of supercooled liquid clouds near the surface in both hemispheres and the underestimation of ice clouds over Antarctica, persist in EAMv2. In conclusion, this study highlights the impact of deep convection parameterizations, which has received little attention, on high-latitude mixed-phase clouds, and the importance of continuous improvement of cloud microphysics in climate models for accurately representing mixed-phase clouds.

54 ENVIRONMENTAL SCIENCES↗

Stability of the Early Mars Atmosphere to Collapse into Permanent Polarcaps

The presence of a permanent CO2 polar ice cap on Mars has important consequences for the planet's climate system. The heat balance of such a cap, which is determined mainly by atmospheric heat transport, and the downward solar in infrared radiative fluxes, determines its surface temperature, which through the vapor pressure relation sets the mean annual surface pressure. On Mars today, for example, the south residual CO2 cap is present year-round with a mean annual temperature of approximately 145 K which corresponds to a mean annual CO2 vapor pressure of approximately 600 Pa. On early Mars, permanent polar caps are also possible especially since the sun was less luminous 3.5-4.0 Gya. Thus, the existence of permanent polar caps on early Mars is central to understanding the nature of the planets climate system in those ancient times and whether or not the atmosphere might have been capable of sustaining conditions suitable for liquid water flowing over the surface as is indicated in the geological record. Forget et al [1] showed that for present orbital properties atmospheric collapse into permanent polar caps could only be prevented for surface pressures roughly between 500 - 3000 hPa. Though follow-on studies confirm and extend the Forget et al. results [2], the full sensitivity of this "window" of stability has not been explored. There are many factors to consider such the albedo of the caps, dust content of the atmosphere, and the presence of water ice clouds. However, we begin our exploration of the stability of the early Martian atmosphere by focusing on the role of CO2 ice clouds. In some preliminary simulations with the Ames Mars General Circulation Model (GCM) we found that atmospheric collapse depends on assumptions regarding the fate of CO2 ice clouds. If, for example, we assume the clouds immediately fall to the surface, then in some cases collapse is favored. On the other hand if the clouds are allowed to fall and evaporate, collapse can be averted. This implies that CO2 ice cloud microphysics is important to the overall stability of the atmosphere. Though the Ames GCM has a sophisticated CO2 cloud microphysics package that includes nucleation, growth, and sedimentation (see accompanying poster by Kahre et al. [3]), we have implemented a simpler scheme based on the Forget et al. [1] approach to CO2 ice clouds. Our goal is to reproduce and expand their study. The key parameter in this approach is the concentration and vertical distribution of cloud condensation nuclei (CCN), i.e., dust particles. Fewer CCN lead to larger particles which fall faster, while higher CCN concentrations lead to smaller particles and thicker clouds that remain suspended for longer periods of time. We plan to explore the stability of the atmosphere to CCN concentrations and distributions and then assess the capability of thick early atmospheres to loft and distribute dust particles (CCN) around the planet. Thus, our work will shed light on the nature of the coupling between the dust and CO2 cycles and the implications it has for the early Mars climate system.

ice cap↗

Remote sensing of cloud radiation and microphysical parameters

Multispectral cloud radiometer (MCR) data, retrieved from a radiometer installed in a nadir viewing position on a high-altitude aircraft flying at 200 m/s and at an altitude of 60,000 ft above the mean sea level, are analyzed. The data discussed were obtained in the 0.754, 0.7609, 0.7634, 1.626, 2.125, and 11.38-micron channels, and are compared to lidar-derived profiles. Among the cloud parameters under consideration are the cloud scaled optical thickness, cloudtop altitude, scaled volume scattering coefficient, particle thermodynamic phase, mean particle size, and cloudtop temperature.

Wu, M.-L. C.↗

Investigation of Aerosol Indirect Effects using a Cumulus Microphysics Parameterization in a Regional Climate Model

A new Zhang and McFarlane (ZM) cumulus scheme includes a two-moment cloud microphysics parameterization for convective clouds. This allows aerosol effects to be investigated more comprehensively by linking aerosols with microphysical processes in both stratiform clouds that are explicitly resolved and convective clouds that are parameterized in climate models. This new scheme is implemented in the Weather Research and Forecasting (WRF) model, which is coupled with the physics and aerosol packages from the Community Atmospheric Model version 5 (CAM5). A test case of July 2008 during the East Asian summer monsoon is selected to evaluate the performance of the new ZM scheme and to investigate aerosol effects on monsoon precipitation. The precipitation and radiative fluxes simulated by the new ZM scheme show a better agreement with observations compared to simulations with the original ZM scheme that does not include convective cloud microphysics and aerosol convective cloud interactions. Detailed analysis suggests that an increase in detrained cloud water and ice mass by the new ZM scheme is responsible for this improvement. To investigate precipitation response to increased anthropogenic aerosols, a sensitivity experiment is performed that mimics a clean environment by reducing the primary aerosols and anthropogenic emissions to 30% of that used in the control simulation of a polluted environment. The simulated surface precipitation is reduced by 9.8% from clean to polluted environment and the reduction is less significant when microphysics processes are excluded from the cumulus clouds. Ensemble experiments with ten members under each condition (i.e., clean and polluted) indicate similar response of the monsoon precipitation to increasing aerosols.

aerosol indirect effects↗

A new WRF-Chem treatment for studying regional-scale impacts of cloud processes on aerosol and trace gases in parameterized cumuli

A new treatment of cloud effects on aerosol and trace gases within parameterized shallow and deep convection, and aerosol effects on cloud droplet number, has been implemented in the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) version 3.2.1 that can be used to better understand the aerosol life cycle over regional to synoptic scales. The modifications to the model include treatment of the cloud droplet number mixing ratio; key cloud microphysical and macrophysical parameters (including the updraft fractional area, updraft and downdraft mass fluxes, and entrainment) averaged over the population of shallow clouds, or a single deep convective cloud; and vertical transport, activation/resuspension, aqueous chemistry, and wet removal of aerosol and trace gases in warm clouds. These changes have been implemented in both the WRF-Chem chemistry packages as well as the Kain–Fritsch (KF) cumulus parameterization that has been modified to better represent shallow convective clouds. Testing of the modified WRF-Chem has been completed using observations from the Cumulus Humilis Aerosol Processing Study (CHAPS). The simulation results are used to investigate the impact of cloud–aerosol interactions on regional-scale transport of black carbon (BC), organic aerosol (OA), and sulfate aerosol. Based on the simulations presented here, changes in the column-integrated BC can be as large as –50% when cloud–aerosol interactions are considered (due largely to wet removal), or as large as +40% for sulfate under non-precipitating conditions due to sulfate production in the parameterized clouds. The modifications to WRF-Chem are found to account for changes in the cloud droplet number concentration (CDNC) and changes in the chemical composition of cloud droplet residuals in a way that is consistent with observations collected during CHAPS. Efforts are currently underway to port the changes described here to the latest version of WRF-Chem, and it is anticipated that they will be included in a future public release of WRF-Chem.

54 ENVIRONMENTAL SCIENCES↗

Effects of Aerosols on Autumn Precipitation over Mid-Eastern China

Long-term observational data indicated a decreasing trend for the amount of autumn precipitation (i.e. 54.3 mm per decade) over Mid-Eastern China, especially after 1980s (~ 5.6% per decade). To examine the cause of the decreasing trend, the mechanisms associated with the change of autumn precipitation were investigated from the perspective of water vapor transportation, atmospheric stability and cloud microphysics. Results show that the decrease of convective available potential energy (i.e. 12.81 J kg-1/ decade) and change of cloud microphysics, which were closely related to the increase of aerosol loading during the past twenty years, were the two primary factors responsible for the decrease of autumn precipitation. Ours results showed that increased aerosol could enhance the atmospheric stability thus weaken the convection. Meanwhile, more aerosols also led to a significant decline of raindrop concentration and to a delay of raindrop formation because of smaller size of cloud droplets. Thus, increased aerosols produced by air pollution could be one of the major reasons for the decrease of autumn precipitation. Furthermore, we found that the aerosol effects on precipitation in autumn was more significant than in other seasons, partly due to the relatively more stable synoptic system in autumn. The impact of large-scale circulation dominated in autumn and the dynamic influence on precipitation was more important than the thermodynamic activity.

AEROSOLS↗