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DOE OSTI2022

Quantifying vertical wind shear effects in shallow cumulus clouds over Amazonia

Abstract. This study analyses and quantifies the effects of vertical wind shear (VWS) on the properties of shallow cumulus cloud fields over Central Amazonia. We perform idealised simulations with high resolution (50 m horizontally and 20 m vertically) using the Dutch Atmospheric Large-Eddy Simulation (DALES) model, changing the initial conditions and large-scale forcing of VWS. The resulting cloud field is analysed by applying a cloud tracking algorithm to generate Lagrangian datasets of the life cycle of individual clouds as well as their time-varying core and margin dimensions. The reference run has no wind speed or directional shear and represents a typical day in the local dry season. Numerical experiments with moderate and high wind speed shear are simulated by adding linear increases in the wind speed of 1.2 and 2.4 m s−1 km−1, respectively. Three additional runs are made by adding 90∘ of wind rotation between the surface and the top of the domain (5 km) on top of the three wind speed shear conditions. We find that clouds developing in a sheared environment have horizontal equivalent diameter increased by up to 100 m on average, but the cloud depth is reduced. Our quantification shows that VWS tends to increase the size of the cloud cores but reduces their relative area, volume, and mass fractions compared to the overall cloud dimensions. The addition of 2.4 m s−1 km−1 of VWS decreases the relative core area by about 0.03 (about 10 % of the overall average) and its volume and mass ratios by about 0.05 (10 %–25 % in relative terms). Relevant for the cloud transport properties is that the updraught speed and the liquid water content are lower within the cores, and consequently so is the upward mass flux. All quantifications of mean cloud properties point to the inhibition of convective strength by VWS, therefore hampering the shallow-to-deep transition. However, open questions still remain given that the individually deepest clouds were simulated under high environmental shear, even though they occur in small numbers. This could indicate other indirect effects of VWS that have opposite effects on cloud development if found to be significant in the future.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1980

A numerical determination of the evolution of cloud drop spectra due to condensation on natural aerosol particles

The time variation in size of aerosol particles growing by condensation is studied numerically by means of an air parcel model which allows entrainment of air and aerosol particles. Particles of four types of aerosols typically occurring in atmospheric air masses were considered. The present model circumvents any assumption about the size distribution and chemical composition of the aerosol particles by basing the aerosol particle growth on actually observed size distributions and on observed amounts of water taken up under equilibrium by a deposit of the aerosol particles. Characteristic differences in the drop size distribution, liquid water content and supersaturation were found for the clouds which evolved from the four aerosol types considered.

Lee, I. Y.↗

DOE OSTI2020

A Climatology of Marine Boundary Layer Cloud and Drizzle Properties derived from Ground-based Observations over the Azores

In this study, more than four years of ground-based observations and retrievals were collected and analyzed to investigate the seasonal and diurnal variations of single-layered MBL (with three subsets: non-drizzling, virga and rain) cloud and drizzle properties, as well as their vertical and horizontal variations. The annual mean drizzle frequency was ~55%, with ~70% in winter and ~45% in summer. The cloud-top (-base) height for rain clouds was the highest (lowest), resulted in the deepest cloud layer (0.8 km), which is four (two) times of non-drizzling (virga) clouds. The retrieved cloud-droplet effective radii (rc) were the largest (smallest) for rain (non-drizzling) clouds, and the nighttime values were greater than the daytime values. Drizzle number concentration (Nd) and liquid water content (LWCd) were three and one order(s) lower than their cloud counterparts. The rc and LWCc increased from the cloud base to ???? = ~0.75 by condensational growth, while drizzle median radii (rd) increased from the cloud top downwards the cloud base by collision-coalescence. The adiabaticity values monotonically increased from the cloud top to the cloud base with maxima of ~0.7 (0.3) for non-drizzling (rain) clouds. The drizzling process decreases the adiabaticity by 0.25 to 0.4, and the cloud-top entrainment mixing impacts as deep as upper 40% of the cloud layers. Cloud and drizzle homogeneities decreased with increased horizontal sampling lengths. Cloud homogeneity increases with increasing cloud fraction. These results can serve as baselines for studying MBL cloud-to-rain conversion and growth processes over the Azores.

Wu, Peng↗

DOE OSTI2025

Profiles of Radiative Fluxes at ENA

Profiles of radiative fluxes observed at the Atmospheric Radiation Measurement (ARM)’s Eastern North Atlantic (ENA) observatory along with the ancillary measurements are reported. The below-cloud drizzle properties were derived by combining the data from the ceilometer and Ka-band ARM Zenith Radar (KAZR) following the technique explained by Ghate et al. (2021 JAMC). The cloud and drizzle water path values were derived from the brightness temperatures reported by the microwave radiometer following the technique of Cadeddu et al. (2020 AMT). The cloud water path was then scaled to the KAZR-reported radar reflectivity to calculate profiles of liquid water content (LWC). Following the analysis from Ghate et al. (2023 JGR), cloud droplet effective radius was calculated using the number concentration value of 100 cm-3. The cloud properties, along with the thermodynamic properties, served as an input to the Rapid Radiative Transfer Model (RRTM) to yield profiles of radiative fluxes at a 1-minute temporal and 50-m vertical resolution. The fluxes were then averaged to hourly temporal resolution for analysis. In Mitra et al. (2025 JClim), the calculated profiles were compared against those derived from the satellite measurements (SYN1deg). Flux profiles from the SYN1deg and the thermodynamic and cloud properties used for deriving them are also reported here. Both all-sky and clear-sky radiative flux profiles were calculated. Due to the large data volume, the surface and top-of-atmosphere (TOA) radiative fluxes for the six-year period, and the hourly profiles of the radiative fluxes for January 2018, are submitted here. Full profiles of radiative fluxes calculated from the thermodynamic and cloud properties measured at the ENA site at 1-minute temporal and 50-m vertical resolution for a six-year period are available from the authors. Six files here correspond to the following data: 1_ENARAD_CERES_with_cld_amount_timeseries.nc: Time-series of hourly values of RRTM-simulated values of upwelling and downwelling fluxes at the surface and TOA, observed boundary-layer cloud fractions, and upwelling and downwelling fluxes from the SYN1deg from July 2015 to January 2022. 2_CERES_2018_at_CERES_levels.nc: SYN1deg radiative fluxes at six levels for the year 2018. 3_ENARad_2018_at_CERES_levels.nc: RRTM calculated fluxes at the SYN1deg vertical levels for the year 2018. 4_ENARad_rrtminputs_hourly_201801.nc: Thermodynamic and cloud properties used as an input to the RRTM for January 2018. 5_CERES_inputs_hourly_201801.nc: Thermodynamic and cloud properties utilized by SYN1deg algorithm for January 2018. 6_ENARAD_hourly_201801.nc: Full profiles of hourly averaged radiative fluxes from the RRTM simulations for January 2018.

Atmosphere↗

NASA NTRS2016

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300% over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were approx. 40- 60% smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq)/ and various biomass burning tracers (BBt/ across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACIs, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be approx. 0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/cu m and very high aerosol concentrations (2000- 3000/ cu cm in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 W/sq m or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic.We lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.

cloud microphysics↗

NASA NTRS1986

T-28 data acquisition during COHMEX 1986

As part of the 1986 Cooperative Huntsville Meteorological Experiment (COHMEX) a cloud physics instrumented T-28 aircraft was used in conjunction with multiple ground based Doppler radars to characterize hydrometeors and updraft structure within developing summertime cumulus and cumulonimbus cloud systems near Huntsville, Alabama. Instrumentation aboard the aircraft included a Particle Measuring Systems (PMS) Forward Scattering Spectrometer Probe (FSSP), a PMS 2D Cloud Probe and a PMS 2D Precipitation Probe, as well as a hail spectrometer and a foil impactor. Hydrometeor spectra were obtained in the interior of mature thunderstorms over the size range from cloud droplets through hailstones. In addition, vertical wind speed, temperature, Johnson-Williams (JW) liquid water content and electric field measurements were made. Significant microphysical differences exist between these clouds and summertime cumulonimbus clouds which develop over the Central Plains. One notable difference in clouds displaying similar radar reflectivities is that COHMEX hydrometeors are typically smaller and more numerous than those observed in the Central Plains. The COHMEX cloud microphysical measurements represent ground truth values for the remote sensing instrumentation which was flown over the cloud tops at altitudes between 60,000 and 70,000 ft aboard NASA U-2 and ER-2 aircraft. They are also being used jointly with a numerical cloud model to assist in understanding the development of summertime subtropical clouds.

Musil, Dennis J.↗

DOE OSTI2020

Analytical Investigation of the Role of Lateral Mixing in the Evolution of Nonprecipitating Cumulus. Part II: Dissolving Stage

A minimalistic analytical model allowing analysis of the dissolving stage of nonprecipitating convective clouds is proposed. The model takes into account two mechanisms: turbulent mixing with a dry environment and cloud volume settling. The temporal changes in the spatial structure of a cloud and in its immediate environment in the course of cloud dissolving are analyzed. The comparison of the effects of a temperature increase in the course of cloud descent and mixing with dry surrounding air shows that the descent is a dominating factor determining a decrease in the liquid water content (LWC), while mixing has a stronger effect on the cloud shape. Narrowing/broadening of clouds due to lateral mixing with dry air during cloud dissolving is determined by the potential evaporation parameter proportional to the ratio of the saturation deficit in the cloud environment to LWC. An equation for cloud dissolving time is obtained. After a cloud totally dissolves, it leaves behind an area with humidity exceeding that of the environment. The main parameter determining the dissolving time is the downdraft velocity. It should exceed 50 cm s -1 in order to provide reasonable dissolving time. The turbulent intensity, LWC, and humidity of the environment air also have an impact on dissolving time: the lower the LWC and the humidity of environment air, the faster cloud dissolving is. The simple solution presented in this paper can be useful for evaluation of cloud characteristics at the dissolving stage and can be included in procedures of parameterization of cloud cover formed by nonprecipitating or slightly precipitating cumulus clouds (Cu). Values of the environment humidity and temperature, LWC at cloud top, cloud width, vertical velocity of downdraft, and the turbulent coefficient should be parameters of this parameterization.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2016

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300 over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were 50 smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq))/ and various biomass burning tracers (BBt/ across the multi-campaign dataset, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACI, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be 0.12 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/ cu m) and very high aerosol concentrations (2000-3000 cu m) in the most polluted clouds, the estimated ACI value was only 0.06. In this case, competition for water vapor by the high concentration of CCN strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease shortwave radiative flux by 2 and 4 W/sq or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic. We lastly show evidence to suggest that numerous northern latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei. However, the influence of background particles on smoke-driven indirect effects is currently unclear.

Arctic↗

NASA NTRS2000

Analysis of the Meteorology Associated with the 1997 NASA Glenn Twin Otter Icing Events

This part of the document contains an analysis of the meteorology associated with the premier icing encounters from the January-March 1997 NASA Twin Otter dataset. The purpose of this analysis is to provide a meteorological context for the aircraft data collected during these flights. For each case, the following data elements are presented: (1) A detailed discussion of the Twin Otter encounter, including locations, liquid water contents, temperatures and microphysical makeup of the clouds and precipitation aloft, (2) Upper-air charts, providing hand-analyzed locations of lows, troughs, ridges, saturated/unsaturated air, temperatures, warm/cold advection, and jet streams, (3) Balloon-borne soundings, providing vertical profiles of temperature, moisture and winds, (4) Infrared satellite data, providing cloud locations and cloud top temperature, (5) 3-hourly surface charts, providing hand-analyzed locations of lows, highs, fronts, precipitation (including type) and cloud cover, (6) Hourly plots of icing pilot reports, providing the icing intensity, icing type, icing altitudes and aircraft type, (7) Hourly, regional radar mosaics, providing fine resolution of the locations of precipitation (including intensity and type), pilot reports of icing (including intensity and type), surface observations of precipitation type and Twin Otter tracks for a one hour window centered on the time of the radar data, and (8) Plots of data from individual NEXRAD radars at times and elevation angles that have been matched to Twin Otter flight locations. Outages occurred in nearly every dataset at some point. All relevant data that was available is presented here. All times are in UTC and all heights are in feet above mean sea level (MSL).

Bernstein, Ben C.↗

NASA NTRS2000

Analysis of the Meteorology Associated with the 1998 NASA Glenn Twin Otter Icing Flights

This document contains a basic analysis of the meteorology associated with the NASA Glenn Twin Otter icing encounters between December 1997 and March 1998. The purpose of this analysis is to provide a meteorological context for the aircraft data collected during these flights. For each case, the following data elements are presented: (1) A brief overview of the Twin Otter encounter, including locations, liquid water contents, temperatures and microphysical makeup of the clouds and precipitation aloft, (2) Upper-air charts, providing hand-analyzed locations of lows, troughs, ridges, saturated/unsaturated air, temperatures, warm/cold advection, and jet streams, (3) Balloon-borne soundings, providing vertical profiles of temperature, moisture and winds, (4) Infrared and visible satellite data, providing cloud locations and cloud top temperature, (5) 3-hourly surface charts, providing hand-analyzed locations of lows, highs, fronts, precipitation (including type) and cloud cover, (6) Hourly, regional radar mosaics, providing fine resolution of the locations of precipitation (including intensity and type), pilot reports of icing (including intensity and type), surface observations of precipitation type and Twin Otter tracks for a one hour window centered on the time of the radar data, and (7) Hourly plots of icing pilot reports, providing the icing intensity, icing type, icing altitudes and aircraft type. Outages occurred in nearly every dataset at some point. All relevant data that was available is presented here. All times are in UTC and all heights are in feet above mean sea level (MSL).

Bernstein, Ben C.↗

NASA NTRSDate not supplied

A Preliminary Study of Inter-Facility LWC Differences in Appendix C and Supercooled Large Drop Conditions due to Calibration Instruments

The simulation of clouds containing Supercooled Large Droplets has received increasing attention due to the introduction of Appendix O and future associated requirements for means of compliance. Supercooled Large Droplet conditions can cover four orders of magnitude in drop sizes, imposing a larger instrument measurement challenge than for Appendix C conditions. Wind tunnel facilities have adopted different instrumentation for liquid water content measurement, with fundamentally different principles of operation. In order to explore the comparability of the different instruments used for Appendix C and SLD measurement, and its impact on confidence in measurements used for means of compliance, a project was established to conduct a series of dedicated tests at three wind tunnel facilities. To date, liquid water content measurements have been completed using a Multi-Element sensor as the common instrument at two of the facilities. The data have provided preliminary information suggesting that substantial inter-facility differences likely exist in liquid water content estimates in Supercooled Large Droplet conditions that appear to be largely attributable to the choice of calibration instruments. These results are dependent on the assumption that the Multi-Element probe would produce equivalent measurements at the two facilities if the liquid water content were the same, regardless of other environmental differences that may exist between the two facilities. Planned further testing with other liquid water content measurement techniques may provide further information to confirm or refute the results of this study.

aircraft icing↗

DOE OSTI2024

Designing a Convection‐Cloud Chamber for Collision‐Coalescence Using Large‐Eddy Simulation With Bin Microphysics

Abstract Collisional growth of cloud droplets is an essential yet uncertain process for drizzle and precipitation formation. To improve the quantitative understanding of this key component of cloud‐aerosol‐turbulence interactions, observational studies of collision‐coalescence in a controlled laboratory environment are needed. In an existing convection‐cloud chamber (the Pi Chamber), collisional growth is limited by low liquid water content and short droplet residence times. In this work, we use numerical simulations to explore various configurations of a convection‐cloud chamber that may intensify collision‐coalescence. We employ a large‐eddy simulation (LES) model with a size‐resolved (bin) cloud microphysics scheme to explore how cloud properties and the intensity of collision‐coalescence are affected by the chamber size and aspect ratio, surface roughness, side‐wall wetness, side‐wall temperature arrangement, and aerosol injection rate. Simulations without condensation and evaporation within the domain are first performed to explore the turbulence dynamics and wall fluxes. The LES wall fluxes are used to modify the Scalar Flux‐budget Model, which is then applied to demonstrate the need for non‐uniform side‐wall temperature (two side walls as warm as the bottom and the two others as cold as the top) to maintain high supersaturation in a tall chamber. The results of LES with full cloud microphysics reveal that collision‐coalescence is greatly enhanced by employing a taller chamber with saturated side walls, non‐uniform side‐wall temperature, and rough surfaces. For the conditions explored, although lowering the aerosol injection rate broadens the droplet size distribution, favoring collision‐coalescence, the reduced droplet number concentration decreases the frequency of collisions.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1984

A model for the estimation of the surface fluxes of momentum, heat and moisture of the cloud topped marine atmospheric boundary layer from satellite measurable parameters

A model is developed for the estimation of the surface fluxes of momentum, heat, and moisture of the cloud topped marine atmospheric boundary layer by use of satellite remotely sensed parameters. The parameters chosen for the problem are the integrated liquid water content, q sub li, the integrated water vapor content, q sub vi, the cloud top temperature, and either a measure of the 10 meter neutral wind speed or the friction velocity at the surface. Under the assumption of a horizontally homogeneous, well-mixed boundary layer, the model calculates the equivalent potential temperature and total water profiles of the boundary layer along with the boundary layer height from inputs of q sub li, q sub vi, and cloud top temperature. These values, along with the 10m neutral wind speed or friction velocity and the sea surface temperature are then used to estimate the surface fluxes. The development of a scheme to parameterize the integrated water vapor outside of the boundary layer for the cases of cold air outbreak and California coastal stratus is presented.

Allison, D. E.↗

DOE OSTI2022

ShupeTurner cloud microphysics

This product is the ShupeTurner cloud microphysics product derived for the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in the central Arctic. The product includes time-height derivations of the cloud type (phase type) and the condensed water content and characteristic effective particle size for liquid and ice hydrometeor populations. Additionally, it includes the vertical integral of the condensed water content for liquid and ice, i.e., the liquid water path and ice water path. These are derived using a combination of sensors, including: cloud radar, depolarization lidar, microwave radiometer, ceilometer, and radiosondes. During MOSAiC, these sensors were installed and operated onboard the Polarstern icebreaker while within the Arctic sea ice. Most data were obtained while Polarstern was moored to the MOSAiC sea ice floe, passively drifting through the Arctic. However, the data from 16 May 2020 - 17 June 2020 and 31 July 2020 - 21 August 2020 were obtained while Polarstern was underway transiting through the sea ice during relocations of the expedition. General details of the retrieval algorithm, its application, and uncertainties are provided in Shupe et al. (2015), with the cloud classification being described in more detail in Shupe (2007). General details about the MOSAiC expedition including instruments, locations, and meteorological context is provided in Shupe et al. (2022).

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Analytical advances to study the air – water interfacial chemistry in the atmosphere

Formation of aqueous secondary organic aerosol (aqSOA) at the air – liquid interface recently has attracted a lot of attention in atmospheric chemistry. The discrepancies in mass distributions, aerosol oxidative capacity, liquid water content, hygroscopic growth of aerosols, and formation of clouds and fogs suggest that interfacial chemistry play a more important role than previously deemed. However, detailed mechanisms at the air–water interface remain unclear owing to the lack of comprehensive understanding that underpins complicated interfacial phenomena, which are not easily measurable from field campaigns, laboratory measurements, or computational simulations. Here, this review highlights relevant and recent technical advancement employed to study aqSOA encompassing spectroscopy and mass spectrometry. The current knowledge on the aqSOA processes is digested with an emphasis on recent research of interfacial aqSOA formation including laboratory studies and model simulations. Finally, future directions of the interfacial chemistry are recommended for field and laboratory studies as well as theoretical efforts to resolve interfacial challenges in atmospheric chemistry.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1984

Comparison of icing cloud instruments for 1982-1983 icing season flight program

A number of modern and old style liquid water content (LWC) and droplet sizing instruments were mounted on a DeHavilland DHC-6 Twin Otter and operated in natural icing clouds in order to determine their comparative operating characteristics and their limitations over a broad range of conditions. The evaluation period occurred during the 1982-1983 icing season from January to March 1983. Time histories of all instrument outputs were plotted and analyzed to assess instrument repeatability and reliability. Scatter plots were also generated for comparison of instruments. The measured LWC from four instruments differed by as much as 20 percent. The measured droplet size from two instruments differed by an average of three microns. The overall effort demonstrated the need for additional data, and for some means of calibrating these instruments to known standards.

Ide, R. F.↗

NASA NTRS1984

Comparison of icing cloud instruments for 1982-1983 icing season flight program

Ide, R. F.↗

NASA NTRS1984

Comments on 'Inference of cloud temperature and thickness by microwave radiometry from space'

The method proposed by Pandey et al. (1983) for estimating the temperature differential and thickness of clouds from microwave data obtained with the scanning multichannel microwave radiometers of the Seasat and Nimbus-7 satellites is examined critically. It is pointed out that both the thicknesses and the temperature differentials derived from them may not be meaningful unless accurate measurements of cloud-top height (from IR radiometry) and reliable data on liquid-water content are available. It is suggested that the good fits obtained in generating regression coefficients for the proposed method may be artifacts of the fixed or limited-range liquid-water densities of the cloud models used. With respect to cloud-top height, the need to quantify and account for differences in the fields of view and spatial resolutions of the IR and microwave radiometers, as undertaken for the case of precipitating clouds by Yeh and Liou (1983), is stressed.

Yeh, H.-Y. M.↗