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At least 235 records · Page 13

Compilation of a Global Emission Inventory from 1980 to 2000 for Global Model Simulations of the Long-term Trend of Tropospheric Aerosols

The approach to create a comprehensive emission inventory for the time period 1980 to 2000 is described in this paper. We have recently compiled an emission database, which we will use for a 21 year simulation of tropospheric aerosols with the GOCART model. Particular attention was paid to the time-dependent SO2, black carbon and organic carbon aerosol emissions. For the emission of SO2 from sporadically erupting volcanoes, we assembled emission data from the Global Volcanism Program of the Smithsonian Institution, using the VEI to derive the volcanic cloud height and the SO2 amount, and amended this dataset by the SO2 emission data from the TOMS instrument when available. 3-dimensional aircraft emission data was obtained for a number of years from the AEAP project, converted from burned fuel to SO2 and interpolated to each year, taking the sparsity of the flight patterns into account. Other anthopogenic SO2 emissions are based on gridded emissions from the EDGAR 2000 database (excluding sources from aircraft, biomass burning and international ship traffic), which were scaled to individual years with country/regional based emission inventories. Gridded SO2 emissions from international ship traffic for 2000 and the scaling factors for other years are from [Eyring et al., 2005]. We used gridded anthropogenic black and organic carbon emissions for 1996 [Bond et al., 2005], again excluding aircraft, biomass burning and ship sources. These emissions were scaled with regional based emission inventories from 1980 to 2000 to derive gridded emissions for each year. The biomass burning emissions are based on a climatology, which is scaled with regional scaling factors derived from the TOMS aerosol index and the AVHRR/ATSR fire counts to each year [Duncan et al., 2003]. Details on the integration of the information from the various sources will be provided and the distribution patterns and total emissions in the final product will be discussed.

Diehl, T. L.↗

Physics-Based GOES Product for Use in NREL's National Solar Radiation Database: Preprint

The Global Solar Insolation Project (GSIP) is an operational physical model from the National Oceanic and Atmospheric Administration (NOAA) that computes global horizontal radiation (GHI) using the visible and infrared channel measurements from geostationary operational environmental satellites (GOES). GSIP uses a two-stage scheme that retrieves cloud properties and uses those properties in the Satellite Algorithm for Surface Radiation Budget (SASRAB) model to calculate surface radiation. The National Renewable Energy Laboratory, University of Wisconsin, and NOAA have recently collaborated to adapt GSIP to create a high-temporal and spatial resolution data set. The data sets are currently being incorporated into the widely used National Solar Radiation Data Base.

14 SOLAR ENERGY↗

High-resolution oscillator strength measurements of the v' = 0,1 bands of the B-X, C-X, and E-X systems in five isotopologues of carbon monoxide

We report oscillator strengths for six strong vibrational bands between 105.0 and 115.2 nm, associated with transitions from the v = 0 level of the X {sup 1}Σ{sup +} ground state to the v = 0 and 1 levels of the B {sup 1}Σ{sup +}, C {sup 1}Σ{sup +}, and E {sup 1}Π states, in {sup 12}C{sup 16}O, {sup 12}C{sup 17}O, {sup 12}C{sup 18}O, {sup 13}C{sup 16}O, and {sup 13}C{sup 18}O. These measurements extend the development of a comprehensive database of line positions, oscillator strengths, and linewidths of photodissociating transitions for all astrophysically relevant CO isotopologues. The E-X bands, in particular, play central roles in CO photodissociation and fractionation models of interstellar clouds and circumstellar disks including the early solar nebula. The resolving powers of the room-temperature measurements, R = 300,000-400,000, allow for the analysis of individual line strengths within bands; the measurements reveal J-dependences in the branch intensities of the C(v = 0,1)-X(0) and E(v = 0,1)-X(0) bands in all isotopologues. Minimal or no isotopologue dependence was found in the f-values of the C(v = 0,1)-X(0) and E(v = 0,1)-X(0) bands at a ∼5% uncertainty level. Revised dissociation branching ratios for the C(v = 0,1) and E(v = 0,1) levels are computed based on these f-values. The weak isotopologue dependence of the f-values presented here eliminates this mechanism as an explanation for the large {sup 17}O enrichments seen in recent laboratory photolysis experiments on CO at wavelengths from 105 to 108 nm.

74 ATOMIC AND MOLECULAR PHYSICS↗

Comparison of GFED3, QFED2 and FEER1 Biomass Burning Emissions Datasets in a Global Model

Biomass burning contributes about 40% of the global loading of carbonaceous aerosols, significantly affecting air quality and the climate system by modulating solar radiation and cloud properties. However, fire emissions are poorly constrained in models on global and regional levels. In this study, we investigate 3 global biomass burning emission datasets in NASA GEOS5, namely: (1) GFEDv3.1 (Global Fire Emissions Database version 3.1); (2) QFEDv2.4 (Quick Fire Emissions Dataset version 2.4); (3) FEERv1 (Fire Energetics and Emissions Research version 1.0). The simulated aerosol optical depth (AOD), absorption AOD (AAOD), angstrom exponent and surface concentrations of aerosol plumes dominated by fire emissions are evaluated and compared to MODIS, OMI, AERONET, and IMPROVE data over different regions. In general, the spatial patterns of biomass burning emissions from these inventories are similar, although the strength of the emissions can be noticeably different. The emissions estimates from QFED are generally larger than those of FEER, which are in turn larger than those of GFED. AOD simulated with all these 3 databases are lower than the corresponding observations in Southern Africa and South America, two of the major biomass burning regions in the world.

biomass burning↗

The Influence of SLD Drop Size Distributions on Ice Accretion in the NASA Icing Research Tunnel

An ice shape database has been created to document ice accretions on a 21-inch chord NACA0012 model and a 72-inch chord NACA 23012 airfoil model resulting from an exposure to a Supercooled Large Drop (SLD) icing cloud with a bimodal drop size distribution. The ice shapes created were documented with photographs, laser scanned surface measurements over a section of the model span, and measurement of the ice mass over the same section of each accretion. The icing conditions used in the test matrix were based upon previously used conditions on the same models but with an alternate approach to evaluation of drop distribution effects. Ice shapes resulting from the bimodal distribution as well as from equivalent monomodal drop size distributions were obtained and compared. Results indicate that the ice shapes resulting from the monomodal and bimodal drop size distributions had similar shapes, but the bimodal distributions had greater mass and volume measurements and icing limits that extended further back on the chord of the model.

Potapczuk, Mark G.↗

The National Climate Data Base (NCDB): A Bias-Corrected High-Resolution Climate Dataset

Assessing renewable energy resources under future climate scenarios has been highlighted in recent years to analyze and understand potential impacts of future change in renewable generation on the power sector. Solar energy is well-known as the most plentiful among various renewable resources and usually converted to electricity using photovoltaics (PV) technologies, and the global deployment of PV technology has increased rapidly in recent decades. In this study, we develop a statistical technique to downscale the future projection of solar irradiance for PV energy-related applications. A set of Regional Climate Model (RCM)-based projections obtained from the North American Coordinated Regional Climate Downscaling Experiment (NA-CORDEX) are used as inputs to statistical methods to generate high-resolution global horizontal irradiance (GHI) over the contiguous United States (CONUS). The main steps of the statistical downscaling method include (1) regridding RCM output (0.22 degree and daily resolutions) to handle the modeled-observed data sets on a common grid, (2) correcting bias of RCM GHI using satellite-derived observation, and (3) implementing temporal and spatial downscaling to generate GHI at 8-km and hourly resolution. Basically, complex physical processes and interactions between solar radiation and various atmospheric constituents lead solar irradiance to be highly variable and uncertain. Underrepresentation of clouds from the RCM parameterizations is the main source of error and uncertainty in modeling solar irradiance. Thus, we adapt and use the high-quality satellite-derived data from the National Solar Radiation Database (NSRDB) to analyze the bias and error of RCM GHI as well as estimate the statistical parameters for spatial and temporal downscaling. This presentation will summarize the comprehensive analysis conducted to produce and assess the results under two climate scenarios (RCP4.5 and RCP8.5). We will also present a detailed validation demonstrating the strengths of the proposed downscaling method and future extension of this research.

climate data↗

Objective method for analysis and tracking of convective cells as seen by radar

A special method has been developed for the study of cells that are embedded in convective rain systems. This method consists of a package of computer programs that use pattern recognition techniques on three-dimensional digital radar data to identify the rain cells, track them with time, and calculate their properties. The product of the computations is a comprehensive database of physically meaningful properties of rain cells, which can be used to infer the internal structure and the dynamics of convective rain systems. The cell-tracking method has been applied to the summer convective clouds of south Florida for the following purposes: (1) derivation of the relationship between the echo top height and the precipitation characteristics (e.g., area, water yield, rain intensity and duration of the rain cells); (2) study of the microphysical behaviorof cumulus clouds in relation to their cell properties; (3) evaluation of the effect of seeding on cumulus clouds on the cell scale; and (4) examination of cloud-to-ground lightning discharges in relation to convective cell intensity. The cell-tracking method is also currently being used in rain enhancement projects in Texas, Israel, and South Africa. The cell-tracking method, its products and their use in meteorological research are described in this paper.

Rosenfeld, Daniel↗

Bimodal SLD Ice Accretion on Swept NACA 0012 Airfoil Models

An ice shape database has been created to document ice accretions on a swept 15-inch chord NACA0012 model and a swept 36-inch chord NACA0012 airfoil model resulting from an exposure to a Supercooled Large Drop (SLD) icing cloud with a bimodal drop size distribution. The ice shapes created were documented with photographs, laser scanned surface measurements over a section of the model span, and measurement of the ice mass over the same section of each accretion. The icing conditions were based on a series of reference conditions that were previously used to generate ice shapes on these models. Drop distribution effects were evaluated by using the same IRT icing conditions except with either monomodal or bimodal drop distributions. Ice shapes resulting from the bimodal distribution as well as from equivalent monomodal drop size distributions were obtained and compared. Results indicate that the ice shapes and mass values from the monomodal and bimodal drop size distributions were the same within the range of repeatability for the conditions tested in this campaign.

Icing↗

Towards an Improved High Resolution Global Long-Term Solar Resource Database

This paper presents an overview of an ongoing project to develop and deliver a solar mapping processing system to the National Renewable Energy Laboratory (NREL) using the data sets that are planned for production at the National Climatic Data Center (NCDC). NCDC will be producing a long-term radiance and cloud property data set covering the globe every three hours at an approximate resolution of 10 x 10 km. NASA, the originators of the Surface meteorology and Solar Energy web portal are collaborating with SUNY-Albany to develop the production system and solar algorithms. The initial result will be a global long-term solar resource data set spanning over 25 years. The ultimate goal of the project is to also deliver this data set and production system to NREL for continual production. The project will also assess the impact of providing these new data to several NREL solar decision support tools.

Stackhouse, Paul W.↗

Flight Planning in the Cloud

This new interface will enable Principal Investigators (PIs), as well as UAVSAR (Uninhabited Aerial Vehicle Synthetic Aperture Radar) members to do their own flight planning and time estimation without having to request flight lines through the science coordinator. It uses an all-in-one Google Maps interface, a JPL hosted database, and PI flight requirements to design an airborne flight plan. The application will enable users to see their own flight plan being constructed interactively through a map interface, and then the flight planning software will generate all the files necessary for the flight. Afterward, the UAVSAR team can then complete the flight request, including calendaring and supplying requisite flight request files in the expected format for processing by NASA s airborne science program. Some of the main features of the interface include drawing flight lines on the map, nudging them, adding them to the current flight plan, and reordering them. The user can also search and select takeoff, landing, and intermediate airports. As the flight plan is constructed, all of its components are constantly being saved to the database, and the estimated flight times are updated. Another feature is the ability to import flight lines from previously saved flight plans. One of the main motivations was to make this Web application as simple and intuitive as possible, while also being dynamic and robust. This Web application can easily be extended to support other airborne instruments.

Flores, Sarah L.↗

Simulated sulfur K-edge X-ray absorption spectroscopy database of lithium thiophosphate solid electrolytes

X-ray absorption spectroscopy (XAS) is a premier technique for materials characterization, providing key information about the local chemical environment of the absorber atom. In this work, we develop a database of sulfur K-edge XAS spectra of crystalline and amorphous lithium thiophosphate materials based on the atomic structures reported in Chem. Mater., 34, 6702 (2022). The XAS database is based on simulations using the excited electron and core-hole pseudopotential approach implemented in the Vienna Ab initio Simulation Package. Our database contains 2681 S K-edge XAS spectra for 66 crystalline and glassy structure models, making it the largest collection of first-principles computational XAS spectra for glass/ceramic lithium thiophosphates to date. This database can be used to correlate S spectral features with distinct S species based on their local coordination and short-range ordering in sulfide-based solid electrolytes. The data is openly distributed via the Materials Cloud, allowing researchers to access it for free and use it for further analysis, such as spectral fingerprinting, matching with experiments, and developing machine learning models.

36 MATERIALS SCIENCE↗

Bimodal SLD Ice Accretion on a CRM Midspan Wing Section Model

An ice shape database has been created to document ice accretions on a 65 per cent scale version of the mid-span section of the Common Research Model resulting from an exposure to a Supercooled Large Drop (SLD) icing cloud with a bimodal drop size distribution. The ice shapes created were documented with photographs, laser scanned surface measurements over a section of the model span, and measurement of the ice mass over the same section of each accretion. Drop distribution effects were evaluated by using the same IRT icing conditions except with either monomodal or bimodal drop distributions. Ice shapes resulting from the bimodal distribution as well as from equivalent monomodal drop size distributions were obtained and compared. Results indicate that the ice shapes resulting from the monomodal and bimodal drop size distributions had equivalent mass and volume, as expected with this approach. Note: No audio portion for this record, additionally slide 9 has a playable video but must be downed in order to view.

Icing↗

Scalability Testing Approach for Internet of Things for Manufacturing SQL and NoSQL Database Latency and Throughput

The proliferation of low-cost sensors and industrial data solutions has continued to push the frontier of manufacturing technology. Machine learning and other advanced statistical techniques stand to provide tremendous advantages in production capabilities, optimization, monitoring, and efficiency. The tremendous volume of data gathered continues to grow, and the methods for storing the data are critical underpinnings for advancing manufacturing technology. This work aims to investigate the ramifications and design tradeoffs within a decoupled architecture of two prominent database management systems (DBMS): sql and NoSQL. A representative comparison is carried out with Amazon Web Services (AWS) DynamoDB and AWS Aurora MySQL. The technologies and accompanying design constraints are investigated, and a side-by-side comparison is carried out through high-fidelity industrial data simulated load tests using metrics from a major US manufacturer. The results support the use of simulated client load testing for comparing the latency of database management systems as a system scales up from the prototype stage into production. As a result of complex query support, MySQL is favored for higher-order insights, while NoSQL can reduce system latency for known access patterns at the expense of integrated query flexibility. Here, by reviewing this work, a manufacturer can observe that the use of high-fidelity load testing can reveal tradeoffs in IoTfM write/ingestion performance in terms of latency that are not observable through prototype-scale testing of commercially available cloud DB solutions.

AWS↗

Long-term changes in reflectivity and large scale motions in the atmosphere of Jupiter and Saturn

A systematic photographic program, utilizing broad-band UV, blue, green, red and near IR pass-bands were carried out at the 60 cm. Tortugas Mountain Telescope. This is part of an ongoing program that spans two Jovian years (25 yrs). The purpose of this program is to provide an ongoing database to characterize high resolution data from spacecraft and earth-orbiting observatories. The standard observing program was maintained and support was given to other investigators who are carrying out complementary observing programs. The general aspect of the cloud decks were monitored, and reveal an interval that shows little variation in the general aspect of the clouddeck of Jupiter since 1981, when the North Temperature Belt darkened. A charge coupled device (CCD) camera was adapted for low cost operation, utilizing an IBM-AT clone for data acquisition. An RCA frame grabber was modified for encoding the archival images.

Beebe, Reta↗

Quantifying Global Uncertainties in a Simple Microwave Rainfall Algorithm

While a large number of methods exist in the literature for retrieving rainfall from passive microwave brightness temperatures, little has been written about the quantitative assessment of the expected uncertainties in these rainfall products at various time and space scales. The latter is the result of two factors: sparse validation sites over most of the world's oceans, and algorithm sensitivities to rainfall regimes that cause inconsistencies against validation data collected at different locations. To make progress in this area, a simple probabilistic algorithm is developed. The algorithm uses an a priori database constructed from the Tropical Rainfall Measuring Mission (TRMM) radar data coupled with radiative transfer computations. Unlike efforts designed to improve rainfall products, this algorithm takes a step backward in order to focus on uncertainties. In addition to inversion uncertainties, the construction of the algorithm allows errors resulting from incorrect databases, incomplete databases, and time- and space-varying databases to be examined. These are quantified. Results show that the simple algorithm reduces errors introduced by imperfect knowledge of precipitation radar (PR) rain by a factor of 4 relative to an algorithm that is tuned to the PR rainfall. Database completeness does not introduce any additional uncertainty at the global scale, while climatologically distinct space/time domains add approximately 25% uncertainty that cannot be detected by a radiometer alone. Of this value, 20% is attributed to changes in cloud morphology and microphysics, while 5% is a result of changes in the rain/no-rain thresholds. All but 2%-3% of this variability can be accounted for by considering the implicit assumptions in the algorithm. Additional uncertainties introduced by the details of the algorithm formulation are not quantified in this study because of the need for independent measurements that are beyond the scope of this paper. A validation strategy for these errors is outlined.

Kummerow, Christian↗

Remote Sensing of Crystal Shapes in Ice Clouds

Ice crystals in clouds exist in a virtually limitless variation of geometries. The most basic shapes of ice crystals are columnar or plate-like hexagonal prisms with aspect ratios determined by relative humidity and temperature. However, crystals in ice clouds generally display more complex structures owing to aggregation, riming and growth histories through varying temperature and humidity regimes. Crystal shape is relevant for cloud evolution as it affects microphysical properties such as fall speeds and aggregation efficiency. Furthermore, the scattering properties of ice crystals are affected by their general shape, as well as by microscopic features such as surface roughness, impurities and internal structure. To improve the representation of ice clouds in climate models, increased understanding of the global variation of crystal shape and how it relates to, e.g., location, cloud temperature and atmospheric state is crucial. Here, the remote sensing of ice crystal macroscale and microscale structure from airborne and space-based lidar depolarization observations and multi-directional measurements of total and polarized reflectances is reviewed. In addition, a brief overview is given of in situ and laboratory observations of ice crystal shape as well as the optical properties of ice crystals that serve as foundations for the remote sensing approaches. Lidar depolarization is generally found to increase with increasing cloud height and to vary with latitude. Although this variation is generally linked to the variation of ice crystal shape, the interpretation of the depolarization remains largely qualitative and more research is needed before quantitative conclusions about ice shape can be deduced. The angular variation of total and polarized reflectances of ice clouds has been analyzed by numerous studies in order to infer information about ice crystal shapes from them. From these studies it is apparent that pristine crystals with smooth surfaces are generally inconsistent with the data and thus crystal impurity, distortion or surface roughness is prevalent. However, conclusions about the dominating ice shapes are often inconclusive and contradictory and are highly dependent on the limited selection of shapes included in the investigations. Since ice crystal optical properties are mostly determined by the aspect ratios of the crystal components and their microscale structure, it is advised that remote sensing applications focus on the variation of these ice shape characteristics, rather than on the macroscale shape or habit. Recent studies use databases with nearly continuous ranges of crystal component aspect ratio and-or roughness levels to infer the variation of ice crystal shape from satellite and airborne remote sensing measurements. Here, the rationale and results of varying strategies for the remote sensing of ice crystal shape are reviewed. Observed systematic variations of ice crystal geometry with location, cloud height and atmospheric state suggested by the data are discussed. Finally, a prospective is given on the future of the remote sensing of ice cloud particle shapes.

clouds↗

Department of Energy’s Atmospheric System Research (ASR) Program’s Workshop on the Future of Atmospheric Large Eddy Simulation (LES): Workshop Report

Large-eddy simulation (LES) is used as a tool to understand physical processes such as turbulence, aerosols, clouds, precipitation, radiation, the interactions among all these, and their interactions with the underlying surface. Over the next 10 years, LES will drive fundamental progress in open scientific questions in these areas as LES is increasingly used to gain understanding of complex interacting physical processes involving atmospheric turbulence. This growth will be driven both by scientific demand and the expansion of computational resources needed to conduct LES, and the form that the growth takes will largely be determined by how computational resources are leveraged for scientific gain. In particular, we suggest that computational resources are likely to be leveraged in two separate but not necessarily distinct ways. On one hand, growth in computational resources will allow LES to be made more routine, that is, performed more frequently, while on the other hand, the computational expense (measured in total floating point operations) afforded to individual LES will expand dramatically, allowing simulations to increase in both domain size and resolution as well as physical detail. Current U.S. Department of Energy (DOE) projects such as LES ARM Symbiotic Simulation and Observation Activity (LASSO) are leading the way in conducting routine LES, building large, public databases that are accessible for data science, sensitivity studies, and training for machine learning. LES will also become more routine as it becomes more accessible for individual researchers to address their scientific questions of interest. Scientific questions addressed by LES over the next 10 years are likely to include cloud organization and aggregation; aerosol cloud interactions and atmospheric chemistry (including geo-engineering); urban-scale LES; atmospheric extreme events, ranging from small-scale severe weather to wildfires; and ocean-wave-atmosphere interactions. Further LES-related research will likely grow significantly in areas related to societal impact studies of air quality and extreme weather events, applications to renewable energy forecasting and resource assessment, and aid in decision-making processes. The growth in the use of LES in atmospheric science research will drive the need for better physical process representations (e.g., cloud aerosol microphysics, radiation, and atmospheric chemistry) at the scales resolved by LES. To date, many of the process representations used by LES have been taken directly from coarser-resolution models. Promising methods for LES process representations include superdroplet and quadrature methods for microphysics, 3D approaches for radiation, and better representation of chemistry and aerosol processes. At LES resolution, land-atmosphere interactions for complex terrains, land cover/types, biogeochemistry, and plant canopy models are needed as an improvement beyond traditional and widely used Monin-Obuhkov similarity theory.

54 ENVIRONMENTAL SCIENCES↗

Department of Energy’s Atmospheric System Research (ASR) Program’s Workshop on the Future of Atmospheric Large Eddy Simulation (LES) (Workshop Report)

Large-eddy simulation (LES) is used as a tool to understand physical processes such as turbulence, aerosols, clouds, precipitation, radiation, the interactions among all these, and their interactions with the underlying surface. Over the next 10 years, LES will drive fundamental progress in open scientific questions in these areas as LES is increasingly used to gain understanding of complex interacting physical processes involving atmospheric turbulence. This growth will be driven both by scientific demand and the expansion of computational resources needed to conduct LES, and the form that the growth takes will largely be determined by how computational resources are leveraged for scientific gain. In particular, we suggest that computational resources are likely to be leveraged in two separate but not necessarily distinct ways. On one hand, growth in computational resources will allow LES to be made more routine, that is, performed more frequently, while on the other hand, the computational expense (measured in total floating point operations) afforded to individual LES will expand dramatically, allowing simulations to increase in both domain size and resolution as well as physical detail. Current U.S. Department of Energy (DOE) projects such as LES ARM Symbiotic Simulation and Observation Activity (LASSO) are leading the way in conducting routine LES, building large, public databases that are accessible for data science, sensitivity studies, and training for machine learning. LES will also become more routine as it becomes more accessible for individual researchers to address their scientific questions of interest. Scientific questions addressed by LES over the next 10 years are likely to include cloud organization and aggregation; aerosol cloud interactions and atmospheric chemistry (including geo-engineering); urban-scale LES; atmospheric extreme events, ranging from small-scale severe weather to wildfires; and ocean-wave-atmosphere interactions. Further LES-related research will likely grow significantly in areas related to societal impact studies of air quality and extreme weather events, applications to renewable energy forecasting and resource assessment, and aid in decision-making processes.

54 ENVIRONMENTAL SCIENCES↗