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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
NASA NTRS1973

Solubilities of noble gases in magnetite - Implications for planetary gases in meteorites.

Solubilities of noble gases in magnetite were determined by growing magnetite in a noble-gas atmosphere between 450 and 700 K. Henry's law is obeyed at pressures up to .01 atm for He, Ne, Ar and up to .00001 atm for Kr, Xe, with the following distribution coefficients at 500 K: He 0.042, Ne 0.016, Ar 3.6, Kr 1.3, Xe 0.88, some 100 to 100,000 times higher than previous determinations on silicate and fluoride melts. Apparent heats of solution are in sharp contrast with earlier determinations on melts which were small and positive, but are comparable to the values for clathrates. Presumably the gases are held in anion vacancies.

Lancet, M. S.↗
NASA NTRS1974

Electron avalanche in liquid xenon

Measurements in liquid Xe are reported of the characteristic function that describes the avalanche, the first Townsend coefficient. An electron avalanche occurs when the drifting electrons attain sufficient kinetic energy from the electric field to cause additional ionization. Data on the avalanche were obtained by studying the pulses in a liquid-filled proportional chamber as a function of applied voltage and anode diameter. The results of the investigation show that the avalanche of free electrons in purified liquid Xe is adequately described by the same formalism used for the avalanche of electrons in gases.

Derenzo, S. E.↗
NASA NTRS1974

Some interesting aspects of physisorption stay-time measurements obtained using molecular-beam techniques

Stay-time distributions have been obtained for Xe physisorbing on polycrystalline nickel as a function of the target temperature using a pulsed molecular-beam technique. Some interesting effects due to ion bombardment of the surface using He, Ar, and Xe ions are presented. Measured detector signal shapes are found to deviate from those predicted for first-order desorption with velocities corresponding to Maxwellian effusion at the surface temperature. Evidence is found for interaction between beam pulse adsorption and steady-state adsorption of beam species background atoms.

Wilmoth, R. G.↗
NASA NTRS1974

Primordial noble gases in separated meteoritic minerals. II

A stepwise heating technique was used to analyze eight silicate samples from the Orgueil carbonaceous chondrite for He, Ne, Ar, and Xe. Six samples, of which two were etched with NaOH, were density fractions. The other two samples were grain-size fractions separated according to their ability to form a colloid at pH 11.5. Results showed the LiCl separation procedure to be gentler than the NaOH procedure. All fractions were found to be deficient in cosmogenic neon. Above 950 C the fractions gave low 20Ne/22Ne ratios particularly in the low-density and noncolloidal fraction. Compared to the other fractions the fraction from 2.35 to 2.45 g/cu cm contained less Xe and released it more rapidly at low temperatures.

Herzog, G. F.↗
NASA NTRS1976

A target for production of radioxenons

A liquid cesium target has been developed which allows the production and separate identification of the neutron deficient isotopes of xenon. The present report describes irradiations utilizing 34 to 41 MeV protons to produce millicurie quantities of Xe-127 and Xe-129m. At higher energies, however, the target could be used without modification to produce xenon isotopes as light as 119.

Blue, J. W.↗
NASA NTRS1976

Production of I-123

Bombarding a cesium heat pipe with high energy particles causes a spallation reaction which produces vapors of Xe-123 and contaminants. The contaminants are removed in a dry ice cold trap while the Xe-123 condenses in a liquid nitrogen trap where it decays.

Blue, J. W.↗
NASA NTRS1976

Spectrum of carbonaceous-chondrite fission xenon

Estimations of the fission spectrum in xenon isotopes from the progenitor of the strange carbonaceous-chondrite xenon must take account of p-process nucleosynthesis if the latter is the source of anomalous Xe-124, 126. Sample calculations of the p-process yields illustrate the magnitude of the effect, which can greatly increase the estimated Xe-132 fission yield.

Clayton, D. D.↗
NASA NTRS1976

Evaluation of nuclear-reactor-produced iodine-123

Iodine-123 has such great potential for nuclear medicine that all possible production methods should be considered. In this report, an experimental study related to I-123 production at a high-intensity fast-flux reactor using the reaction Xe-124(n,2n)Xe-123 is considered. The conclusion is that I-123 could be made in small quantities and the cost would be higher than the cyclotron methods presently used.

Blue, J. W.↗
NASA NTRS1977

Mass-dependent channel electron multiplier operation

The absolute counting efficiency and pulse height distributions of a continuous-channel electron multiplier used in the detection of hydrogen, argon and xenon ions are assessed. The assessment technique, which involves the post-acceleration of 8-eV ion beams to energies from 100 to 4000 eV, provides information on counting efficiency versus post-acceleration voltage characteristics over a wide range of ion mass. The charge pulse height distributions for H2 (+), A (+) and Xe (+) were measured by operating the experimental apparatus in a marginally gain-saturated mode. It was found that gain saturation occurs at lower channel multiplier operating voltages for light ions such as H2 (+) than for the heavier ions A (+) and Xe (+), suggesting that the technique may be used to discriminate between these two classes of ions in electrostatic analyzers.

Fields, S. A.↗
NASA NTRS1976

Measurement techniques for analysis of fission fragment excited gases

Spectroscopic analysis of fission fragment excited He, Ar, Xe, N2, Ne, Ar-N2, and Ne-N2 have been conducted. Boltzmann plot analysis of He, Ar and Xe have indicated a nonequilibrium, recombining plasma, and population inversions have been found in these gases. The observed radiating species in helium have been adequately described by a simple kinetic model. A more extensive model for argon, nitrogen and Ar-N2 mixtures was developed which adequately describes the energy flow in the system and compares favorably with experimental measurements. The kinetic processes involved in these systems are discussed.

Schneider, R. T.↗
NASA NTRS1977

The composition of the atmosphere at the surface of Mars

The current status is summarized of investigations of the composition of the Martian atmosphere, in which use was made of the mass spectrometers that function as the analytical component of the molecular analysis experiments on the two Viking landers. The following points seem well established: N2, Ar-40, Ne, Kr, Xe, and the primordial isotope of Ar are present. The present atmosphere of Mars represents only a small fraction of the total amount of volatiles outgassed by the planet, so that high surface pressure and abundant water may have been present. The noble gases in the Martian atmosphere exhibit a relative abundance pattern similar to that in the earth's atmosphere and (except for Xe) to that in the primordial component of meteorites. The existence of a 'planetary component' is thus proven, supporting the arguments of those who favor a fractionation of noble gases prior to the formation of the planets. In spite of these similarities, the isotopic ratios of nitrogen, argon, and xenon indicate that the histories of the Martian and the earth's atmospheres have been very different.

Owen, T.↗
NASA NTRS1978

Mars - Regolith adsorption and the relative concentrations of atmospheric rare gases

Laboratory measurements of Kr and Xe adsorption on samples of ground montmorillonite, limonite and basalt at -77 C have been performed. Results suggest that (1) most degassed martian Xe could be adsorbed on a regolith with a large effective surface area, and (2) if this is the case the elemental composition of martian nonradiogenic rare gas (counting that in the regolith) may be virtually identical to that of ordinary chondrites.

Fanale, F. P.↗
NASA NTRS1977

The regolith history of 14307

Noble gas and trace element analyses of matrix and a clast from breccia 14307 are reported. This sample was exposed to a large neutron fluence, as seen by an elevated Sm-150/Sm-149 ratio and by noble gases, particularly Xe-136 from neutron fission of U-235. Strong constraints on the exposure history result from combined consideration of Sm-150, Xe-136, and spallation noble gases. Both clast and matrix were irradiated for about 1 AE under substantial shielding beginning at least 2 AE ago, probably more than 3 AE ago. The manifestations of soil exposure seen in the matrix - solar wind gases, glass formation, etc. - thus must have been acquired in an ancient epoch. The matrix has had a longer exposure to cosmic rays than the clast, presumably during its prebrecciation history as a soil. Brecciation probably occurred more than 1 AE ago, perhaps more than 3 AE ago, but at least 0.4 AE after the formation of the matrix constituents.

Bernatowicz, T.↗
NASA NTRS1977

Exposure histories of lunar rocks 71135 and 71569

Rare-gas isotopic analyses have been performed on lunar rocks 71135 and 71569. The conventional (Kr-81)-Kr cosmic-ray exposure ages are 103 + or - 3 m.y. for 71135 and 134 + or - 7 m.y. for 71569. An approach is outlined to deducing complex exposure histories from rare-gas data using depth profiles of the production rates of the cosmogenic rare-gas isotopes. Examination of the Xe isotopes by means of a 'concordia' plot suggests that 71569 may have a simple one-stage exposure history whereas 71135 has a more complex history. An attempt is made to construct exposure models for these two rocks which account for the abundances of all the cosmogenic rare gases, the Xe isotopic compositions, and the apparent (Kr-81)-Kr exposure ages. This study demonstrates the depreciation of (Kr-81)-Kr ages for rocks exposed at shallow depths, caused by the relatively rapid variation of the Kr-81 production as the rock is eroded. Possible implications of the tentative results for the formation age of the Central Cluster unit are discussed.

Niemeyer, S.↗
NASA NTRS1975

Krypton and xenon in Apollo 14 samples - Fission and neutron capture effects in gas-rich samples

Gas-rich Apollo 14 breccias and trench soil are examined for fission xenon from the decay of the extinct isotopes Pu-244 and I-129, and some samples have been found to have an excess fission component which apparently was incorporated after decay elsewhere and was not produced by in situ decay. Two samples have excess Xe-129 resulting from the decay of I-129. The excess is correlated at low temperatures with excess Xe-128 resulting from neutron capture on I-127. This neutron capture effect is accompanied by related low-temperature excesses of Kr-80 and Kr-82 from neutron capture on the bromine isotopes. Surface correlated concentrations of iodine and bromine are calculated from the neutron capture excesses.

Drozd, R.↗
NASA NTRS1978

s-process studies - Xenon and krypton isotopic abundances

We propose an analysis of the s-process contributions to the isotopes of xenon and krypton. The object is to aid studies of the possibility that meteorites may contain gas that was carried in presolar grains that were grown in stellar ejecta and that were not degassed prior to incorporation into parent bodies. That model suggests routine interstellar fractionation of s-isotopes from r-isotopes owing to differential incorporation into dust. We show that a deficiency of s-process nuclei cannot yield details of Xe-X, but the gross similarities are strong enough to lead one to think that such a deficiency may play a role in a more complicated explanation. We predict the existence of an s-rich complement somewhere if fractional separation of this type has played a role in Xe-X. We show that the analogous decomposition of krypton is more uncertain, and we call for measurements of neutron-capture cross sections to alleviate these uncertainties.

Clayton, D. D.↗
NASA NTRS1979

LaRC results on nuclear pumped noble gas lasers

The recent experiment and theoretical results obtained for noble gas nuclear laser systems are presented. It is shown that the noble gas lasers are among the easiest systems to pump by nuclear excitation and as a result, all of the noble gases except He have lased under nuclear excitation. The noble gas systems are not ideal for high-power applications but they do give valuable insight into the operation and pumping mechanisms associated with nuclear lasers. At present, the Ar-Xe system is the best noble gas candidate for (U-235)F6 pumping. It appears that the quenching of Ar-Xe lasing is a result of the fluorine and not the uranium or fission fragments themselves. Thus, to achieve lasing with UF6, a fluorine compatible system must be found.

Deyoung, R. J.↗
NASA NTRS1980

Rare gases in the past and present solar wind

The elemental abundances, fluxes and isotopic compositions of rare gases in the past and present-day solar wind are discussed on the basis of direct measurements and fossil evidence in lunar and meteorite samples. Spacecraft measurements of the abundances of He, O, Si, Fe, Ne, and Ar with respect to H in the solar wind are shown to agree with relative abundance measurements of these elements in the solar photosphere and corona, while the lack of evidence of systematic depletion with increasing ionic mass suggests solar abundances of the much less abundant Kr and Xe in the solar wind. Relative He, Ne and Ar abundances in the ancient solar wind as derived from lunar ilmenite and the Pesyanoe meteorite are similar to present-day values, except for a factor of two underabundance of He, while the heavy rare gases appear to be enriched by up to a factor of five. The isotopic compositions of solar wind Ar, Kr and Xe have apparently been fairly constant over most of the solar lifetime, whereas He and possibly Ne show evidence of an increasing abundance of their heavy isotopes with increasing solar wind age.

Pepin, R. O.↗