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222 records · Page 13

All sources NASA NTRS DOE OSTI

DOE OSTI2023

Development of an accelerator-based neutron source to prototype Mo-99 production, part I: A liquid LBE windowless target

In this article, Molybdenum-99 (Mo-99)’s decay product, technetium-99 (Tc-99 m), is one of the most critical isotopes for medical diagnostics. To provide U.S. domestic supply of Mo-99 without using high-enriched uranium (HEU), a subcritical uranium target assembly (UTA) is irradiated by an accelerator-based neutron source to create Mo-99 through fission. This study discusses the development of the accelerator-based neutron source. The high-energy electrons from the accelerator irradiate a liquid lead-bismuth eutectic (LBE) target to produce neutrons. Part I of this work focuses on numerical and experimental analysis towards the development of a liquid LBE windowless target. Unlike the existing windowless targets in literature, the current design creates a vertical free surface for a beam to irradiate. First, a hydrodynamic analysis of the LBE windowless target is performed. Simplified analytical calculations are assisted by 2D computational fluid dynamics (CFD) simulations to design the target, with the focus on eliminating recirculation zones and avoiding cavitation. With the optimized geometry, the experimental study is performed to investigate the flow hydrodynamics using liquid LBE. The experiments (1) compare pressure drop in the system to correlation predictions; (2) visualize the free surface liquid LBE flow from the beam view; (3) validate the LBE flow profile using temperature sensitive paint from the side view; and (4) validate the liquid LBE film thickness using gamma densitometer measurements. Second, the power handling capability of the designed windowless target is investigated. The divider plate in the current design is susceptible to overheating due to the thin LBE film in front. As LBE erosion and corrosion is likely to occur at an LBE velocity of 2.0 m/s and temperature above 500 °C, a power limit of 10 kW of beam power was established to prevent this corrosion from occurring, which is calculated by a Nusselt number correlation. The divider plate surface temperature at 10 kW agrees well with the 3D CFD simulation results. Part I demonstrates the fundamental physics in liquid LBE windowless target design and associated testing. A companion paper, Part II will demonstrate how to couple this windowless target into the Mo-99 production system, including an accelerator system operating under an ultra-high vacuum and the UTA cooled by water at room temperature.

43 PARTICLE ACCELERATORS↗

NASA NTRS1993

Simulation of preburner sprays, volumes 1 and 2

The present study considered characteristics of sprays under a variety of conditions. Control of these sprays is important as the spray details can control both rocket combustion stability and efficiency. Under the present study Imperial College considered the following: (1) Measurement of the size and rate of spread of the sprays produced by single coaxial airblast nozzles with axial gaseous stream. The local size, velocity, and flux characteristics for a wide range of gas and liquid flowrates were measured, and the results were correlated with the conditions of the spray at the nozzle exit. (2) Examination of the effect of the geometry of single coaxial airblast atomizers on spray characteristics. The gas and liquid tube diameters were varied over a range of values, the liquid tube recess was varied, and the shape of the exit of the gaseous jet was varied from straight to converging. (3) Quantification of the effect of swirl in the gaseous stream on the spray characteristics produced by single coaxial airblast nozzles. (4) Quantification of the effect of reatomization by impingement of the spray on a flat disc positioned around 200 mm from the nozzle exit. This models spray impingement on the turbopump dome during the startup process of the preburner of the SSME. (5) Study of the interaction between multiple sprays without and with swirl in their gaseous stream. The spray characteristics of single nozzles were compared with that of three identical nozzles with their axis at a small distance from each other. This study simulates the sprays in the preburner of the SSME, where there are around 260 elements on the faceplate of the combustion chamber. (6) Design an experimental facility to study the characteristics of sprays at high pressure conditions and at supercritical pressure and temperature for the gas but supercritical pressure and subcritical temperature for the liquid.

Hardalupas, Y.↗

NASA NTRS1993

Simulation of preburner sprays, volume 1

Under the present contract a study was made on the characteristics of the sprays of coaxial injectors with particular emphasis on those aspects relevant to the performance of rocket engines. The technical effort was performed primarily by Imperial College of Science and Technology and the details of this effort are contained in the accompanying technical report by Hardalupas and Whitelaw, which forms Vol. 2 of the report. The role of Scientific Research Associates was review of material, initial direction of the technical effort and review of all reports. The study considered characteristics of sprays under a variety of conditions. Control of these sprays is important as the spray details can control both rocket combustion stability and efficiency. Imperial College considered the following: first, measurement of the size and rate of spread of the sprays produced by single coaxial airblast nozzles with axial gaseous stream. The local size, velocity and flux characteristics for a wide range of gas and liquid flowrates were measured and the results were correlated with the conditions of the spray at the nozzle exit. Second, examination of the effect of the geometry of single coaxial airblast atomizers on spray characteristics. The gas and liquid tube diameters were varied over a range of values, the liquid tube recess was varied and the shape of the exit of the gaseous jet was varied from straight to converging. Third, quantification of the effect of swirl in the gaseous stream on the spray characteristics produced by single coaxial airblast nozzles. Fourth, quantification of the effect of reatomization by impingement of the spray on a flat disc positioned around 200 mm from the nozzle exit. This models spray impingement on the turbopump dome during the startup process of the preburner of the Space Shuttle Main Engine (SSME). Fifth, study of the interaction between multiple sprays without and with swirl in their gaseous stream. The spray characteristics of single nozzles were compared with that of three identical nozzles with their axis at a small distance from each other. This study simulates the sprays in the preburner of the SSME, where there are around 260 elements on the faceplate of the combustion chamber. And lastly, design an experimental facility to study the characteristics of sprays at high pressure conditions and at supercritical pressure and temperature for the gas but supercritical pressure and subcritical temperature for the liquid.

Source record↗

NASA NTRS2017

Behavior of a Salt Water Solution Near the Critical Point Under Microgravity Conditions

The Supercritical Water Mixture (SCWM) experiment conducted on the International Space Station (ISS) is designed to study a salt-water solution in the vicinity of the critical transition with a test cell filled with Na2SO4 (aq) 0.5-w. This salt is a Type II salt which undergoes a dramatic decrease in solubility past waters critical point. The paper discusses the liquid-vapor-salt distribution in the test cell for subcritical, trans-critical, and supercritical regimes. In 0-g, the vapor-liquid interface manifests itself by the presence of a large single vapor bubble that is flattened between the two windows. In contrast with pure water, the vapor bubble remains centered in the test cell and is stable for temperatures up to Tc - 50 mK. The processes leading to critical transition during heat-up, as marked by the break-up of the vapor bubble, depends on the applied heating rate. For temperature ramps 1 mKmin, the bubble interface begins to breakup with the formation of a large number of smaller bubbles. For larger temperature ramps (10mKmin), temperature gradients arise in the cell pushing the bubble toward a window surface. As the critical threshold is crossed small variations in cell temperature ( 1 mK) cause an observable spatial variation in density. However, this spatial variation is not discernible as the temperature is increased further into the supercritical regime. The salt precipitation in the vicinity of the critical crossing appears to be heterogeneous in nature with precipitates observable on the cell windows. Direct imaging as well as light scattering indicate a hexagonal structure of the precipitated salt crystals in the near critical regime. The salt deposition is not fully reversible as the temperature is reduced due to window corrosion effects which traps some of the precipitated salt. Critical temperatures as high as 1.9 K above the value for pure water (647.25 K) have been measured. Finally, results on the critical transition phenomena in the presence of an imposed temperature gradient, demonstrating the remarkable stability of the central bubble, are also presented.

near-critical↗

DOE OSTI2023

Transient Efficiency, Flexibility, and Reliability Optimization of Coal-Fired Power Plants - Final Report

This program developed an advanced model-based monitoring and model-predictive control algorithms for a coal fired power plant (CFPP), and deployed these algorithms in a real-time platform to demonstrate performance benefits for transient flexibility and plant operation efficiency. More specifically, the objectives were successfully achieved through a combination of (i) developing a high-fidelity transient plant model in Apros, which was used as a high-fidelity plant simulation between $100-50\% TMCR$ where TMCR denotes the turbine maximum continuous rating, i.e., baseload, (ii) developing a very fast physics-based reduced-order model (ROM) of the plant, which ran more than $100\times$ faster than real-time, enabling its use as real-time embedded model for model-based estimation (MBE) and model predictive control (MPC) (iii) implementing a real-time MBE based on ROM using a robust unscented Kalman filter (UKF) to continuously tune the ROM to match the measurements from high-fidelity Apros plant model despite significant plant-model mismatch, and thus, obtain a Digital Twin of the plant (iv) designing and implementing a real-time MPC with dual objectives of transient plant load tracking with high ramp rates and minimizing coal consumption, i.e., improving plant efficiency in the baseload-partload operation range of $100-50\% TMCR$. Each key element above was developed and tested individually, and has been reported in corresponding Topical Reports. Finally, all the individual elements were integrated in an overall closed-loop system, that was successfully tested in desktop Simulink test harness simulations with ROM or high-fidelity model as the plant. Thereafter, the Simulink implementation was used to auto-generate C-code and deploy as real-time Docker microservice containers in Linux, and validate that they can run in real-time in the hardware-in-the loop (HIL) setup and produce the same results as in Simulink. The results of the integrated simulation tests in Simulink as well as the real-time HIL deployment are documented in this final report, showing good load tracking for load ramps at $3-4\%/min$ ramp rates, and achieving up to $5.5\%$ reduction in coal relative to baseline operation at $50\% TMCR$ load. The desktop and HIL simulations show successful performance of the overall model based estimation and control solution and achieve the key objectives of the program for flexible, efficient and reliable operation of subcritical coal fired power plants.

20 FOSSIL-FUELED POWER PLANTS↗

DOE OSTI2022

Effects of Chlorine Capture and a Proposed Density Law on the Reactivity of Plutonium Solution Systems

During fissionable material processing, all normal and credible abnormal conditions must remain safely subcritical. Nuclear Criticality Safety (NCS) uses a number of methods to determine subcriticality, one of which is the use of neutron transport codes such as MCNP6. In order to create models for use with MCNP6, both the geometry and materials in fissionable material processes must be known, or assumptions must be made and quantified for the impact to bias. One of the systems with a significant amount of bias due to material modeling assumptions is in the area of aqueous plutonium processing. These solutions are typically plutonium nitrate solutions or plutonium chloride solutions, which are modeled as fictitious plutonium metal-water mixtures because little is known about the actual density of the solution and there is no current predictive capability approved for use at Los Alamos National Laboratory (LANL) for modeling them. This research is currently underway to fill the gap and develop an algorithm for use with MCNP6 to model the density of plutonium chloride solutions. The method is to be validated with experimental data for density, and also validated with critical experiments using MCNP6. Note that the Chlorine Worth Study (CWS) was performed in December 2021 to help bridge the gap in chlorine data for critical experiments, and is currently awaiting International Criticality Safety Benchmark Evaluation Project (ICSBEP) review. This study was performed by LANL at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Site (NNSS). Additional information regarding this experiment may currently be found in LA-UR- 22-29180. Additionally, the Chemistry-Actinide Analytical Chemistry (C-AAC) at LANL has performed a number of solution density measurements for PuCl 3 -HC 1 -H 2 O, allowing for such data be used to create a semi-empirical density via the Pitzer method. The published dataset for the measurements is documented in LA-UR-22-25454. This method has already been tested successfully for aqueous plutonium nitrate solutions in SCALE. Current solution density measurements exist of plutonium concentrations of 0-~142g/L, all at 2M HC1, at temperatures 20-40°C. Additional data was taken for HC1-corrected density values, which essentially mimics the data for a pure PuCl x -water solution. The calculations in this report aim to support the current research by demonstrating the difference in system reactivity for the current modeling method when compared to the new proposed modeling with a density law implementation, which is being written as a Python tool to be used with MCNP6.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗