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At least 235 records · Page 13

Radiation hardened microprocessor for small payloads

The RH-3000 program is developing a rad-hard space qualified 32-bit MIPS R-3000 RISC processor under the Naval Research Lab sponsorship. In addition, under IR&D Harris is developing RHC-3000 for embedded control applications where low cost and radiation tolerance are primary concerns. The development program leverages heavily from commercial development of the MIPS R-3000. The commercial R-3000 has a large installed user base and several foundry partners are currently producing a wide variety of R-3000 derivative products. One of the MIPS derivative products, the LR33000 from LSI Logic, was used as the basis for the design of the RH-3000 chipset. The RH-3000 chipset consists of three core chips and two support chips. The core chips include the CPU, which is the R-3000 integer unit and the FPA/MD chip pair, which performs the R-3010 floating point functions. The two support whips contain all the support functions required for fault tolerance support, real-time support, memory management, timers, and other functions. The Harris development effort had first passed silicon success in June, 1992 with the first rad-hard 32-bit RH-3000 CPU chip. The CPU device is 30 kgates, has a 508 mil by 503 mil die size and is fabricated at Harris Semiconductor on the rad-hard CMOS Silicon on Sapphire (SOS) process. The CPU device successfully passed tesing against 600,000 test vectors derived directly on the LSI/MIPS test suite and has been operational as a single board computer running C code for the past year. In addition, the RH-3000 program has developed the methodology for converting commercially developed designs utilizing logic synthesis techniques based on a combination of VHDK and schematic data bases.

Shah, Ravi↗

Hot accretion disks with pairs: Effects of magnetic field and thermal cyclocsynchrotron radiation

We show the effects of thermal cyclosynchrotron radiation and magnetic viscosity on the structure of hot, two-temperature accretion disks. Magnetic field, B, is assumed to be randomly oriented and the ratio of magnetic pressure to either gas pressure, alpha = P(sub mag)/P(sub gas), or the sum of the gas and radiation pressures, alpha = (P(sub mag)/P(sub gas) + P(sub rad)), is fixed. We find those effects do not change the qualitative properties of the disks, i.e., there are still two critical accretion rates related to production of e(sup +/-) pairs, (M dot)((sup U)(sub cr)) and (M dot)((sup L)(sub cr)), that affect the number of local and global disk solutions, as recently found by Bjoernsson and Svensson for the case with B = 0. However, a critical value of the alpha-viscosity parameter above which those critical accretion rates disappear becomes smaller than alpha(sub cr) = 1 found in the case of B = 0, for P(sub mag) = alpha(P(sub gas) + P(sub rad)). If P(sub mag) = alpha P(sub gas), on the other hand, alpha(sub cr) is still about unity. Moreover, when Comptonized cyclosynchrotron radiation dominates Comptonized bremsstrahlung, radiation from the disk obeys a power law with the energy spectral index of approximately 0.5, in a qualitative agreement with X-ray observations of active galactic nuclei (AGNS) and Galactic black hole candidates. We also extend the hot disk solutions for P(sub mag) = alpha(P(sub gas) + P(sub rad)) to the effectively optically thick region, where they merge with the standard cold disk solutions. We find that the mapping method by Bjoernsson and Svensson gives a good approximation to the disk structure in the hot region and show where it breaks in the transition region. Finally, we find a region in the disk parameter space with no solutions due to the inability of Coulomb heating to supply enough energy to electrons.

Kusunose, Masaaki↗

SpaceCube Demonstration Platform

A document discusses how the HST SM4 SpaceCube flight spare was modified to create an experiment called the Space- Cube Demonstration Platform (SC DP) for use on the MISSE7 Space Station payload (in collaboration with NRL). It is designed to serve as an on-orbit platform for demonstrating advanced fault tolerance technologies. A simple C&DH (command and data handling) system was developed for the Virtex4 FPGAs (field programmable gate arrays). Both Virtex4s on each SpaceCube run the same program, and both receive incoming telemetry. The rad-hard service FPGA performs simple error checking to verify that the incoming telemetry is valid. The SpaceCube framework was modified to allow for new program files to be sent from the ground, to be stored on the SpaceCube, and to be executed through ground commands. Each SpaceCube Virtex4 FPGA has resources set aside for experiments that are functionally isolated from the C&DH system. The experiments communicate to the C&DH system through a set of dual port memories, and this area is where the fault-tolerance experiments are executed. With the use of Xilinx commercial Virtex4 FX60 FPGAs, the fault tolerant framework allows the system to recover from radiation upsets that occur in the rad-soft parts (Virtex4 FPGA logic, embedded PPCs in Virtex4 FPGAs, SDRAM and Flash), the C&DH system that runs simultaneously on both Virtex4 FPGAs that uses a robust telemetry packet structure, checksums, and the rad-hard service FPGA to validate incoming telemetry. The ability to be reconfigured from the ground while in orbit is a novel benefit, as well as is the onboard compression capabilities that allow compressed files from the ground to be uploaded to the SpaceCube.

Espinosa, Daniel↗

ELDRS Characterization for a Very High Dose Mission

Evaluation of bipolar linear parts which may have Enhanced Low Dose Rate Sensitivity (ELDRS) is problematic for missions that have very high dose radiation requirements. The accepted standards for evaluating parts that display ELDRS require testing at a very low dose rate which could be prohibitively long for very high dose missions. In this work, a methodology for ELDRS characterization of bipolar parts for mission doses up to 1 Mrad(Si) is evaluated. The procedure employs an initial dose rate of 0.01 rad(Si)/s to a total dose of 50 krad(Si) and then changes to 0.04 rad(Si)/s to a total dose of 1 Mrad(Si). This procedure appears to work well. No change in rate of degradation with dose has been observed when the dose rate is changed from 0.01 to 0.04 rad(Si)/s. This is taken as an indication that the degradation due to the higher dose rate is equivalent to that at the lower dose rate at the higher dose levels, at least for the parts studied to date. In several cases, significant parameter degradation or functional failure not observed at HDR was observed at fairly high total doses (50 to 250 krad(Si)) at LDR. This behavior calls into question the use of dose rate trend data and enhancement factors to predict LDR performance.

Radiation Damage↗

Mars Science Laboratory Radiation Assessment Detector (MSLRAD) Modeling Workshop Proceedings

The Radiation Assessment Detector (RAD) (Hassler et al., 2012) onboard the Mars Science Laboratory (MSL) Curiosity rover (Grotzinger et al., 2012) has been making detailed measurements of the radiation environment on the surface of Mars since landing on 6 August 2012 (Hassler et al., 2014; Zeitlin et al., 2016). These measurements are the first of their kind on the surface of another planet and are providing essential measurements of the radiation environment on Mars in preparation for a human mission in the coming decades. The objectives of RAD are; 1) to characterize the energetic particle spectrum on the surface of Mars as a function of time in the solar cycle, including direct (galactic cosmic rays and solar energetic particles) and indirect (neutrons, etc.) radiation created in the atmosphere and regolith, 2) to determine the dose and dose‐equivalent rates as a function of time in the solar cycle, and 3) to use these observations to test and validate space radiation transport models. Initial results of the charged particle spectra (Ehresmann et al., 2014) and neutral particle spectrum (Köhler et al., 2014), as well as dose and dose‐equivalent during cruise (Zeitlin et al., 2013) and on the surface (Hassler et al., 2014) have been reported, and with almost five years of continuous measurements, RAD continues to characterize the radiation environment as solar minimum is approached.

Donald M Hassler↗

Current Active Detectors for Dosimetry and Spectrometry on the International Space Station

We present a high-level overview of two of the most important radiation detection systems currently flying aboard the International Space Station(ISS), ISS-RAD and Timepix. ISS-RAD is a single, large unit that is capable of detecting both chargedand neutral high-energy particles. For most of its first three and a half years of operations onboard Station, ISS-RAD has been periodically moved to different modules, includingtheUSLab, Columbus, JEM, Node2, and Node3. In contrast, the much smaller Timepix-based detectors are deployed in several locations around the station. The first generation of these units were known as REMs, or Radiation Environment Monitors. A second generation has recently been deployed, known as REM-2 units. We will briefly describe the technologies used in these systems and their capabilities.

Cary Zeitlin↗

Status of PEP-X Light Source Design Study

The SLAC Beam Physics group and other SLAC collaborators continue to study options for implementing a near diffraction-limited ring-based light source in the 2.2-km PEP-II tunnel that will serve the SSRL scientific program in the future. The study team has completed the baseline design for a 4.5-GeV storage ring having 160 pm-rad emittance with stored beam current of 1.5 A, providing >10{sup 22} brightness for multi-keV photon beams from 3.5-m undulator sources. The team has also investigated possible 5-GeV ERL configurations which, similar to the Cornell and KEK ERL plans, would have {approx}30 pm-rad emittance with 100 mA current, and {approx}10 pm-rad emittance with 25 mA or less. Now a 4.5-GeV 'ultimate' storage ring having emittance similar to the ERL and operating with {approx}200 mA is under study. An overview of the progress of the PEP-X design study and SSRL's plans for defining performance parameters that will guide the choice of ring options is presented.

43 PARTICLE ACCELERATORS↗

Intensity Effects of the FACET Beam in the SLAC Linac

The beam for FACET (Facility for Advanced aCcelerator Experimental Tests) at SLAC requires an energy-time correlation ('chirp') along the linac, so it can be compressed in two chicanes, one at the midpoint in sector 10 and one W-shaped chicane just before the FACET experimental area. The induced correlation has the opposite sign to the typical used for BNS damping, and therefore any orbit variations away from the center kick the tail of the beam more than the head, causing a shear in the beam and emittance growth. Any dispersion created along the linac has similar effects due to the high (>1.2% rms) energy spread necessary for compression. The initial huge emittances could be reduced by a factor of 10, but were still bigger than expected by a factor of 2-3. Normalized emittance of 3 {micro}m-rad in Sector 2 blew up to 150 {micro}m-rad in Sector 11 but could be reduced to about 6-12 {micro}m-rad, for the vertical plane although the results were not very stable. Investigating possible root causes for this, we found locations where up to 10 mm dispersion was created along the linac, which were finally verified with strong steering and up to 7 mm settling of the linac accelerator at these locations.

43 PARTICLE ACCELERATORS↗

Startup of the New 200 West Pump-and-Treat, Hanford Site, Richland, Washington - 13214

On June 28, 2012, CH2M HILL Plateau Remediation Company (CHPRC) completed the construction and acceptance testing for a new 2,500 gallon-per-minute (gpm) pump-and-treat (P and T) system in the 200 West Area of the Hanford Site in Washington State. This system is designed to remove Tc-99, carbon tetrachloride, trichloroethene (TCE), nitrate, and total and hexavalent chromium from groundwater using ion exchange, anoxic and aerobic bioreactors, and air stripping. The system will eventually remove uranium from groundwater using ion exchange as well. The startup of the P and T system is important because it will ensure that contaminants from the 200 West Area never reach the Columbia River. When fully operational, the 200 West P and T will include approximately 23 extraction wells and 21 injection wells. The extraction wells are 8 inches in diameter, are completed with well screens 100 feet or more in length, and are distributed throughout the central portion of the 5-square-mile carbon tetrachloride plume. The injection wells are also 8 inches in diameter and are installed up-gradient of the plumes to recharge the aquifer and down-gradient of the plumes for flow-path control. Groundwater in the 200 West Area is approximately 250 feet below ground surface, and the aquifer is 200 feet or more in thickness. All of the contaminants (except nitrate) are found within the perimeter of the carbon tetrachloride plume and occur at various depths throughout the aquifer. The 200 West P and T consists of two separate buildings to conduct groundwater treatment. The RAD building contains an ion exchange system to remove Tc-99 from groundwater at a maximum flow rate of 600 gpm. The RAD building only accepts water from those extraction wells showing elevated Tc-99 concentrations. Groundwater initially fills an influent tank, is then pumped through particulate filters (to remove suspended materials), and then passes through two parallel treatment trains containing Purolite{sup R} A530E resin (which has been proven effective in removing Tc-99). The water is then transferred to the biological treatment building for further treatment. When the lead vessel in each of the two treatment trains becomes fully loaded with Tc-99, the Purolite A530E resin is transferred to a separate tank where it is heated to 160 deg. F to remove volatile organics prior to disposal at the Environmental Restoration Disposal Facility. The biological treatment building has a maximum flow capacity of 2,500 gpm. Groundwater from the nonradiological extraction wells and treated groundwater from the RAD building are initially pumped into an equalization tank and then into two parallel fluidized bed reactors (FBRs). The FBRs contain granulated activated carbon in suspension for microbes to populate, a carbon-based food source for the microbes to eat (e.g., MicroCg{sup TM}, molasses, or sodium lactate), and nitrate for the microbes to breathe (represents 'anoxic' conditions that contain little or no dissolved oxygen). The FBRs are maintained at a temperature between 55 deg. F and 90 deg. F, and at a pH between 6.5 and 6.8, to maximize microbial growth. The FBRs break down the nitrate, reduce the hexavalent chromium to trivalent chromium, and break down a good portion of the carbon tetrachloride and TCE. From the FBRs, groundwater is pumped through a carbon separation tank, then through a splitter box that divides the water evenly between four membrane bioreactors (MBRs) that further break down the contaminants. The MBRs have aeration capacity to provide sufficient oxygen for maintaining the aerobic biological process. The MBRs use submerged membranes for filtration. Vertically strung fibers are found in the membrane zone where a vacuum draws water through tiny pores in the fibers. The liquid is then pumped to air strippers to remove any volatile organics that have passed through the bioreactors. Solids from the MBRs are pumped to rotary drum thickeners and centrifuges for dewatering prior to lime being added to kill the bacteria and control odor. The conditioned sludge is then disposed at the Environmental Restoration Disposal Facility. The final treated water is then pumped to the injection well field. The 200 West P and T is a Leadership in Energy and Environmental Design (LEED) gold-certified facility that has an expected 70% energy cost savings over the lifetime of the plant. Fifty percent of the steel used in construction was recycled, 420 tons of recycled concrete were used, and over 75% of construction waste was diverted from landfills. The plant is only staffed one shift per day, and it uses a call-out system if the plant goes down during off-shift hours. Initial sampling results have shown that the 200 West P and T is successfully reducing contaminant levels well below the cleanup levels specified in the Record of Decision, Hanford 200 Area 200-ZP-1 Superfund Site, Benton County, Washington [1]. CHPRC and the U.S. Department of Energy are continuing to look for ways to reduce operational costs, such as testing alternative resins for removing radionuclides and finding less expensive carbon substrate sources. The benefit to others is a LEED gold-certified, 2,500 gpm P and T system that may be used as a model for other complex sites. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Multi-Phased, Post-Accident Support of the Fukushima Dai-Ichi Nuclear Power Plant - 12246

In the wake of the March 11 earthquake and tsunami and the subsequent flooding of several of the Fukushima Dai-Ichi reactors, Japan and the Japanese utility TEPCO faced a crisis situation with incredible challenges: substantial amounts of radioactive mixed seawater and freshwater accumulated in the basements of four reactor and other buildings on the site. This water held varying levels of contamination due to the fact that it had been in contact with damaged fuel elements in the cores and with other contaminated components. The overall water inventory was estimated at around 110,000 tons of water with contamination levels up to the order of 1 Ci/l. Time was of the essence to avoid overflow of this accumulated water into the ocean. AREVA proposed, designed and implemented a water treatment solution using a proven chemical coprecipitation process with ppFeNi reagent, which is currently in use for effluent treatment on several nuclear sites including AREVA sites. In addition to the extremely short schedule the other challenge was to adapt the chemical treatment process to the expected composition of the Fukushima water and, in particular, to evaluate the impact of salinity on process performance. It was also necessary to define operating conditions for the VEOLIA equipment that had been selected for implementation of the process in the future facility. The operation phase began on June 17, and by the end of July more than 30,000 tons of highly radioactive saltwater had been decontaminated - the Decontamination Factor (DF) for Cesium was ∼10{sup 4}. It allowed recycling the contaminated water to cool the reactors while protecting workers and the environment. This paper focuses on the Actiflo{sup TM}-Rad water treatment unit project that was part of the TEPCO general water treatment scheme. It presents a detailed look at the principles of the Actiflo{sup TM}-Rad, related on-the-fly R and D, an explanation of system implementation challenges, and a brief summary of operation results to date. AREVA's response to the Fukushima Dai-Ichi crisis was multi-phased: emergency aid and relief supply was sent within days after the accident; AREVA-Veolia engineering teams designed and implemented a water treatment solution in record time, only 3 months; and AREVA continues to support TEPCO and propose solutions for waste management, soil remediation and decontamination of the Fukushima Dai-Ichi site. Despite the huge challenges, the Actiflo{sup TM}-Rad project has been a success: the water treatment unit started on time and performed as expected. The performance is the result of many key elements: AREVA expertise in radioactive effluents decontamination, Veolia know-how in water treatment equipments in crisis environment, and of course AREVA and Veolia teams' creativity. The project success is also due to AREVA and Veolia teams' reactivity and high level of commitment with engineering teams working 24/7 in Japan, France and Germany. AREVA and Veolia deep knowledge of the Japanese industry ensured that the multi-cultural exchanges were not an issue. Finally the excellent overall project management and execution by TEPCO and other Japanese stakeholders was very efficient. The emergency water treatment was a key step of the roadmap towards restoration from the accident at Fukushima Dai-Ichi that TEPCO designed and keeps executing with success. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

2013 LANL Radionuclide Air Emissions Report

This report describes the emissions of airborne radionuclides from operations at Los Alamos National Laboratory (LANL) for calendar year 2013, and the resulting off-site dose from these emissions. This document fulfills the requirements established by the National Emissions Standards for Hazardous Air Pollutants – Emissions of Radionuclides other than Radon from Department of Energy Facilities (40 CFR 61 Subpart H, referred to as the Radionuclide NESHAP or Rad-NESHAP). Compliance with this regulation and preparation of this document is the responsibility of LANL’s Rad-NESHAP compliance program, which is part of the Environmental Protection Division. The information in this report is required under the Clean Air Act and is being submitted to the U.S. Environmental Protection Agency (EPA) Region 6.

54 ENVIRONMENTAL SCIENCES↗

Performance Testing of Tracer Gas and Tracer Aerosol Detectors for use in Radionuclide NESHAP Compliance Testing

The Rad-NESHAP program, part of the Air Quality Compliance team of LANL’s Compliance Programs group (EPC-CP), and the Radiation Instrumentation & Calibration team, part of the Radiation Protection Services group (RP-SVS), frequently partner on issues relating to characterizing air flow streams. This memo documents the most recent example of this partnership, involving performance testing of sulfur hexafluoride detectors for use in stack gas mixing tests. Additionally, members of the Rad-NESHAP program performed a functional trending test on a pair of optical particle counters, comparing results from a non-calibrated instrument to a calibrated instrument. Prior to commissioning a new stack sampling system, the ANSI Standard for stack sampling requires that the stack sample location must meet several criteria, including uniformity of tracer gas and aerosol mixing in the air stream. For these mix tests, tracer media (sulfur hexafluoride gas or liquid oil aerosol particles) are injected into the stack air stream and the resulting air concentrations are measured across the plane of the stack at the proposed sampling location. The coefficient of variation of these media concentrations must be under 20% when evaluated over the central 2/3 area of the stack or duct. The instruments which measure these air concentrations must be tested prior to the stack tests in order to ensure their linear response to varying air concentrations of either tracer gas or tracer aerosol. The instruments used in tracer gas and aerosol mix testing cannot be calibrated by the LANL Standards and Calibration Laboratory, so they would normally be sent off-site for factory calibration by the vendor. Operational requirements can prevent formal factory calibration of some instruments after they have been used in hazardous settings, e.g., within a radiological facility with potential airborne contamination. The performance tests described in this document are intended to demonstrate the reliable performance of the test instruments for the specific tests used in stack flow characterization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

2022 LANL Radionuclide Air Emissions Report (Rev. 2)

This report describes the emissions of airborne radionuclides from operations at Los Alamos National Laboratory (LANL) for calendar year 2022 and the resulting off-site dose from these emissions. This document fulfills the requirements established by the National Emissions Standards for Hazardous Air Pollutants in 40 CFR 61, Subpart H – Emissions of Radionuclides other than Radon from Department of Energy Facilities, commonly referred to as the Radionuclide NESHAP or Rad-NESHAP. Compliance with this regulation and preparation of this document is the responsibility of LANL’s Rad NESHAP compliance program, which is part of the Environmental Protection and Compliance (EPC) Division. The information in this report is required under the Clean Air Act and is being submitted to the U.S. Environmental Protection Agency (EPA) Headquarters and EPA Region 6. The highest effective dose equivalent (EDE) to an off-site member of the public was calculated using procedures specified by the EPA and described in this report. LANL’s EDE was 0.45 for 2022. The annual limit is 10 millirem per year, established by the EPA in 40 CFR 61 Subpart H. All measured air emissions are modeled to a single location, known as the Maximally Exposed Individual (MEI). During calendar year 2022, LANL continuously monitored radionuclide emissions at 27 “major” release points, or stacks. The Laboratory estimates emissions from an additional 34 “minor” release points using radionuclide usage source terms in lieu of stack monitoring. Also, LANL uses an EPA approved network of air samplers around the Laboratory perimeter to monitor ambient airborne levels of radionuclides. To provide data for dispersion modeling and dose assessment, LANL maintains and operates several meteorological monitoring towers. From these various systems, a comprehensive evaluation is conducted to calculate the MEI dose for the Laboratory. The MEI can be any member of the public at any off-site location where there is a residence, school, business, or office. In 2022, this MEI location was a business at 95 Entrada Drive, located in the eastern end of Los Alamos town site. The primary contributors to the off-site dose at this location are the ambient air data at that location combined with radioactive gas emissions from the LANSCE facility and the collected potential emissions from unmonitored (minor) sources. Overall, the MEI dose in 2022 is similar to that which has been observed in recent years, and it remains well below the EPA’s 10 millirem per year limit. Doses reported to the EPA for the past 10 years are shown in Table E1.

54 ENVIRONMENTAL SCIENCES↗

Evaluation of Minimum Detectable Activities for Stack Sample Analyses

The Rad-NESHAP program takes samples at major point sources to track how much of select nuclides are being emitted out of the stack. Samples are taken at the site where the radiological operations are being performed. The samples are then sent to analytical laboratories for analysis to determine what nuclides exist in the sample. However, due to the sensitivity of the instruments, false positives are often reported. To reduce the number of false positives, the results reported from the analytical labs are compared to set detection limits. Anything below the set detection limit is considered part of the background while anything above the limit is considered a positive hit. Therefore, the detection limit must be set low enough that any false negatives do not result in a significant dose missed at the end of the year but high enough that there are not enough false positives to skew the annual dose being reported. All detection limits listed in this section for the analyses below were designed to meet the stated equivalent emissions rate and subsequent off-site doses. These minimum detectable activities (MDAs) were developed in the 1990s and documented in the memo cited for each analysis below. These limits and memos are all currently referenced in the Quality Assurance Project Plan (QAPP) for the Rad-NESHAP Compliance Task, which is being updated to a Project Implementation Plan (PIP) concurrently with this document. As part of this update process, the original MDAs defined in this section needed to be verified that they were still conservative and meet the off-site dose levels stated.

2019 MDA↗

Notice of Submittal – 2023 Radionuclide Air Emissions Report for Los Alamos National Laboratory

This report describes the emissions of airborne radionuclides from operations at Los Alamos National Laboratory (LANL) for calendar year 2023 and the resulting off-site dose from these emissions. This document fulfills the requirements established by the National Emissions Standards for Hazardous Air Pollutants in 40 CFR 61, Subpart H – Emissions of Radionuclides other than Radon from Department of Energy Facilities, commonly referred to as the Radionuclide NESHAP or Rad-NESHAP. Compliance with this regulation and preparation of this document is the responsibility of LANL’s Rad NESHAP compliance program, which is part of the Environmental Protection and Compliance (EPC) Division. The information in this report is required under the Clean Air Act and is being submitted to the U.S. Environmental Protection Agency (EPA) Headquarters and EPA Region 6. The highest effective dose equivalent (EDE) to an off-site member of the public was calculated using procedures specified by the EPA and described in this report. LANL’s EDE was 0.43 for 2023. The annual limit is 10 millirem per year, established by the EPA in 40 CFR 61 Subpart H. All measured air emissions are modeled to a single location, known as the Maximally Exposed Individual (MEI). During calendar year 2023, LANL continuously monitored radionuclide emissions at 28 “major” release points, or stacks. The Laboratory estimates emissions from an additional 59 “minor” release points using radionuclide usage source terms in lieu of stack monitoring. Also, LANL uses an EPA approved network of air samplers around the Laboratory perimeter to monitor ambient airborne levels of radionuclides. To provide data for dispersion modeling and dose assessment, LANL maintains and operates several meteorological monitoring towers. From these various systems, a comprehensive evaluation is conducted to calculate the MEI dose for the Laboratory. The MEI can be any member of the public at any off-site location where there is a residence, school, business, or office. In 2023, this MEI location was a business at 129 New Mexico State Road 4 (NM-4), located in the northern end of White Rock. The primary contributors to the off-site dose at this location are the ambient air data at that location combined with the collected potential emissions from unmonitored (minor) sources. Overall, the MEI dose in 2023 is similar to that which has been observed in recent years, and it remains well below the EPA’s 10 millirem per year limit. Doses reported to the EPA for the past 10 years are shown in Table E1.

54 ENVIRONMENTAL SCIENCES↗

On the Interplay between CT and Singlet Exciton Emission in Organic Solar Cells with Small Driving Force and Its Impact on Voltage Loss

The interplay between free charge carriers, charge transfer (CT) states and singlet excitons (S 1 ) determines the recombination pathway and the resulting open circuit voltage (V OC ) of organic solar cells. By combining a well-aggregated low bandgap polymer with different blend ratios of the fullerenes PCBM and ICBA, the energy of the CT state (E CT ) is varied by 130 meV while leaving the S 1 energy of the polymer (E S 1 ) unaffected. It is found that the polymer exciton dominates the radiative properties of the blend when approaches E CT , while the V OC remains limited by the non-radiative decay of the CT state. It is concluded that an increasing strength of the exciton in the optical spectra of organic solar cells will generally decrease the non-radiative voltage loss because it lowers the radiative V OC limit (V OC,rad ), but not because it is more emissive. The analysis further suggests that electronic coupling between the CT state and the S 1 will not improve the V OC , but rather reduce the V OC,rad . It is anticipated that only at very low CT state absorption combined with a fairly high CT radiative efficiency the solar cell benefit from the radiative properties of the singlet excitons.

14 SOLAR ENERGY↗

Patient Radiation Dose Reduction Considerations in a Contemporary Interventional Radiology Suite

PurposeWe sought to evaluate patient radiation exposure during complex liver interventional procedures performed with newer angiography equipment.Materials and MethodsWe conducted a retrospective study of transjugular intrahepatic portosystemic shunt (TIPS) creations and liver tumor embolizations performed in our new angiography suite (Discovery IGS740, GE Healthcare). T tests were used to compare air kerma-area product (P{sub KA}) and reference plane air kerma (K{sub a,r}) in the new room versus data from historical rooms and previous studies (including the RAD IR study). Results were expressed as medians [interquartile ranges (Q1, Q3)].ResultsFrom February 2015 to June 2016, 134 complex liver interventional procedures were performed in the new room, including 14 TIPS creations, 60 hepatic tumor arterial embolizations (HAEs), 26 Y90 mappings (Y90m), and 34 Y90 radioembolizations (Y90). K{sub a,r} (Gy) values were as follows: TIPS, 0.65 (0.24, 1.15); HAE, 0.89 (0.49, 1.49); Y90m, 0.54 (0.38, 0.94); Y90, 0.46 (0.21, 1.06). P{sub KA} (Gy·cm{sup 2}) values were as follows: TIPS, 148.2 (66.7, 326.5); HAE, 142.6 (88, 217.8); Y90m, 148.3 (98.2, 247); Y90, 90.8 (43.9, 161.5). K{sub a,r} and P{sub KA} were lower in the new room than in historical rooms [K{sub a,r} and P{sub KA} reductions: TIPS, 58 and 49%; HAE, 31 and 39%; Y90m, 58 and 52%; Y90, 49 and 56% (p < 0.05)] and versus the RAD IR study [K{sub a,r} and P{sub KA} reductions: TIPS, 64 and 43%; HAE, 26 and 40% (p < 0.05)].ConclusionsUsing the latest technology and image processing tools enables significant reduction in radiation exposure during complex liver interventional procedures.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

A comprehensive study of non-adaptive and residual-based adaptive sampling for physics-informed neural networks

Physics-informed neural networks (PINNs) have shown to be effective tools for solving both forward and inverse problems of partial differential equations (PDEs). PINNs embed the PDEs into the loss of the neural network using automatic differentiation, and this PDE loss is evaluated at a set of scattered spatio-temporal points (called residual points). The location and distribution of these residual points are highly important to the performance of PINNs. However, in the existing studies on PINNs, only a few simple residual point sampling methods have mainly been used. Here, we present a comprehensive study of two categories of sampling for PINNs: non-adaptive uniform sampling and adaptive nonuniform sampling. We consider six uniform sampling methods, including (1) equispaced uniform grid, (2) uniformly random sampling, (3) Latin hypercube sampling, (4) Halton sequence, (5) Hammersley sequence, and (6) Sobol sequence. We also consider a resampling strategy for uniform sampling. To improve the sampling efficiency and the accuracy of PINNs, we propose two new residual-based adaptive sampling methods: residual-based adaptive distribution (RAD) and residual-based adaptive refinement with distribution (RAR-D), which dynamically improve the distribution of residual points based on the PDE residuals during training. Hence, we have considered a total of 10 different sampling methods, including six non-adaptive uniform sampling, uniform sampling with resampling, two proposed adaptive sampling, and an existing adaptive sampling. We extensively tested the performance of these sampling methods for four forward problems and two inverse problems in many setups. Our numerical results presented in this study are summarized from more than 6000 simulations of PINNs. Here, we show that the proposed adaptive sampling methods of RAD and RAR-D significantly improve the accuracy of PINNs with fewer residual points for both forward and inverse problems. Furthermore, the results obtained in this study can also be used as a practical guideline in choosing sampling methods.

97 MATHEMATICS AND COMPUTING↗