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At least 235 records · Page 13

Dynamical Generation of Higher-Order Spin-Orbit Coupling, Topology, and Persistent Spin Texture in Light-Irradiated Altermagnets

Altermagnets have been identified as the third category of magnetic materials, exhibiting momentum-dependent spin splitting characterized by even powers of momentum. Here, in this Letter, we show that when subjected to elliptically polarized light, these materials serve as an exemplary framework for the dynamic generation of topological bands featuring higher-order spin-orbit coupling (SOC). Notably, while the generated Zeeman field remains invariant to the particular altermagnetic ordering, the induced higher-order SOCs are related to the magnitude and symmetry of the altermagnetic order. Specifically, we show that an altermagnet exhibiting 𝐤 2⁢𝑛 -spin splitting can generate odd-in-𝐤 spin-orbit couplings up to 𝐤 2⁢𝑛−1 . In the limit of circularly polarized light, the only correction is 𝑘 2⁢𝑛−1 , with all lower-order contributions being nullified. Interestingly, light-induced SOCs significantly impact the low-energy band topology, where their Chern numbers change by Δ⁢𝐶 = ±1, 2, 3 for 𝑑, 𝑔, 𝑖-wave altermagnets. Finally, we find a critical field in which a persistent spin texture is realized, a highly desirable state with predicted infinite spin lifetime. Our Letter showcases light as a powerful, controllable tool for engineering complex and exciting phenomena in altermagnets.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Double Aperture HTS Dipole Magnet Model for the Persistent Current Operation

Particle accelerators use many different types of magnets. There is an interest in replacing rather low-field conventional resistive magnets with high-temperature superconducting (HTS) magnets. The main goal is to reduce operational expenses, which is critical during the continuously increasing cost of electricity. At Fermilab, several HTS accelerator magnets were built and successfully tested. The paper described a variant of the double-aperture dipole magnet that could be suitable for future Lepton Colliders. A single short-circuited HTS coil of 3.8 kA generates a homogeneous magnetic field of 57 mT in both magnet gaps of 84 mm. The short model magnet was designed, built, and successfully tested at liquid nitrogen temperature. This magnet works in a persistent current mode, which provides additional cost savings when used in particle storage rings operated at a stable magnetic field. The results of design, fabrication, and tests are presented and discussed. The magnet demonstrated a high magnetic field stability in both apertures, efficiency of correction coils, and primary powering circuit.

Kashikhin, Vladimir [Fermilab] (ORCID:000000017249↗

Data-Driven Day-Ahead PV Estimation Using Autoencoder-LSTM and Persistence Model

Inherent variability in photovoltaic (PV) and associated impacts on power systems is a challenging problem for both the PV owners and the grid operators. Existing statistical and machine learning algorithms typically work well for weather conditions similar to historical data. Furthermore, uncertain weather conditions pose a great challenge to the estimation accuracy of the estimation models. With the enhanced integration of intelligent electronic devices and the realization of associated automation in the power grid, renewable energy data is becoming more accessible, which can be utilized by deep learning models and improve the PV power generation estimation accuracy. In this paper, a hybrid deep learning model driven by external weather data is proposed to do day-ahead PV output forecasting at 15-minute-interval. The proposed model is motivated by the recent advancement of Long-Short-Term-Memory (LSTM) networks and AutoEncoder (AE), which estimates uncertainties in sequence while making the prediction for complex weather conditions. Meanwhile, the persistence model (PM) is used to predict continuous sunny weather conditions. The forecasting result is validated with data from multiple locations

42 ENGINEERING↗

Bounds on Optimal Revisit Times in Persistent Monitoring Missions With a Distinct and Remote Service Station</strong

We report persistent monitoring missions require an up-to-date knowledge of the changing state of the underlying environment. Unmannned aerial vehicles (UAVs) can be gainfully employed to continually visit a set of targets representing tasks (and locations) in the environment and collect data therein for long time periods. The enduring nature of these missions requires the UAV to be regularly recharged at a service station. In this article, we consider the case in which the service station is not colocated with any of the targets. An efficient monitoring requires the revisit time, defined as the maximum of the time elapsed between successive revisits to targets, to be minimized. Here, we consider the problem of determining UAV routes that lead to the minimum revisit time. The problem is NP-hard, and its computational difficulty increases with the fuel capacity of the UAV. We develop an algorithm to construct near-optimal solutions to the problem quickly when the fuel capacity exceeds a threshold. We also develop lower bounds to the optimal revisit time and use these bounds to demonstrate (through numerical simulations) that the constructed solutions are, on an average, at most 0.01% away from the optimum.

42 ENGINEERING↗

Characterisation of motor cortex organisation in patients with different presentations of persistent low back pain

Abstract Persistence of low back pain is thought to be associated with different underlying pain mechanisms, including ongoing nociceptive input and central sensitisation. We hypothesised that primary motor cortex (M1) representations of back muscles (a measure of motor system adaptation) would differ between pain mechanisms, with more consistent observations in individuals presumed to have an ongoing contribution of nociceptive input consistently related to movement/posture. We tested 28 participants with low back pain sub‐grouped by the presumed underlying pain mechanisms: nociceptive pain, nociplastic pain and a mixed group with features consistent with both. Transcranial magnetic stimulation was used to study M1 organisation of back muscles. M1 maps of multifidus (deep and superficial) and longissimus erector spinae were recorded with fine‐wire electromyography and thoracic erector spinae with surface electromyography. The nociplastic pain group had greater variability in M1 map location (centre of gravity) than other groups ( p < .01), which may suggest less consistency, and perhaps relevance, of motor cortex adaptation for that group. The mixed group had greater overlap of M1 representations between deep/superficial muscles than nociceptive pain (deep multifidus/longissimus: p = .001, deep multifidus/thoracic erector spinae: p = .008) and nociplastic pain (deep multifidus/longissimus: p = .02, deep multifidus/thoracic erector spinae: p = .02) groups. This study provides preliminary evidence of differences in M1 organisation in subgroups of low back pain classified by likely underlying pain mechanisms. Despite the sample size, differences in cortical re‐organisation between subgroups were detected. Differences in M1 organisation in subgroups of low back pain supports tailoring of treatment based on pain mechanism and motor adaptation.

Elgueta‐Cancino, Edith↗

Persistent enhancement of exciton diffusivity in CsPbBr 3 nanocrystal solids

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons among CsPbBr 3 perovskite nanocrystals (NCs) depends markedly on how recently those NCs were occupied by a previous exciton. Using transient photoluminescence microscopy, we observe a striking dependence of the apparent exciton diffusivity on excitation laser power that does not arise from nonlinear exciton-exciton interactions or thermal heating. We interpret our observations with a model in which excitons cause NCs to transition to a long-lived metastable configuration that markedly increases exciton transport. The exciton diffusivity observed here (>0.15 square centimeters per second) is considerably higher than that observed in other NC systems, revealing unusually strong excitonic coupling between NCs. The finding of a persistent enhancement in excitonic coupling may help explain other photophysical behaviors observed in CsPbBr 3 NCs, such as superfluorescence, and inform the design of optoelectronic devices.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Laurentide Ice Sheet persistence during Pleistocene interglacials

While there are no ice sheets in the Northern Hemisphere outside of Greenland today, it is uncertain whether this was also the case during most other Quaternary interglacials. We show, using in situ cosmogenic nuclides in ice-rafted debris, that the Laurentide Ice Sheet was likely more persistent during Quaternary interglacials than often thought. Low 26 Al/ 10 Be ratios (indicative of burial of the source area) in marine core sediment suggest sediment source areas experienced only brief (on the order of thousands of years) and/or infrequent ice-free interglacials over the past million years. Here these results imply that complete Laurentide deglaciation may have only occurred when climate forcings reached levels comparable to those of the early Holocene, making our current interglacial unusual relative to others of the mid-to-late Pleistocene.

58 GEOSCIENCES↗

Persistent ocean anomalies as a response to Northern Hemisphere heating induced by biomass burning variability

Biomass burning aerosol (BBA) emissions in the Coupled Model Intercomparison Project Phase 6 (CMIP6) historical forcing fields have enhanced temporal variability during the years 1997–2014 compared to earlier periods. Recent studies document that the corresponding inhomogeneous shortwave forcing over this period can cause changes in clouds, permafrost, and soil moisture, which contribute to a net terrestrial Northern Hemisphere warming relative to earlier periods. Here, we investigate the ocean response to the hemispherically asymmetric warming, using a 100-member ensemble of the Community Earth System Model version 2 Large Ensemble forced by two different BBA emissions (CMIP6 default and temporally smoothed over 1990–2020). Differences between the two subensemble means show that ocean temperature anomalies occur during periods of high BBA variability and subsequently persist over multiple decades. In the North Atlantic, surface warming is efficiently compensated for by decreased northward oceanic heat transport due to a slowdown of the Atlantic Meridional Overturning Circulation. In the North Pacific, surface warming is compensated for by an anomalous cross-equatorial cell (CEC) that reduces northward oceanic heat transport. The heat that converges in the South Pacific through the anomalous CEC is shunted into the subsurface and contributes to formation of long-lasting ocean temperature anomalies. The anomalous CEC is maintained through latitude-dependent contributions from narrow western boundary currents and basin-wide near-surface Ekman transport. Furthermore, these results indicate that interannual variability in forcing fields may significantly change the background climate state over long timescales, presenting a potential uncertainty in CMIP6-class climate projections forced without interannual variability.

54 ENVIRONMENTAL SCIENCES↗

Generation and control of phase-locked Bessel beams with a persistent noninterfering region

We present, to the best of our knowledge, a novel method for the generation of multiple Bessel-like (Bessel–Gauss) beams with tilted wavefronts whose optical phases can be controlled independently. In the far field multiple field-free regions develop that are persistent to interference effects and the optical phase. The extent of these field-free regions can be controlled through the tilt angle of the wavefront with a theoretical maximum resolution of 0.1 mrad. Experimentally we employ a spatial light modulator, a lens, and an axicon, each suitable for narrow-band (continuous-wave) and broadband operation. Because of the simplicity in the optical elements, the number of noninterfering Bessel-like beams can be scaled on demand for applications that require multiple sources for coherent imaging or multiple intense beams over a controllable region with the added benefit of a field-free region for detection. Here, for reasons of clarity, we characterized two beams.

Rodnova, Zhanna↗

TEAMER: Performance mapping of Re Vision's Persistance PTO

Contains datasets from experimental measurements that were used to validate Re Vision's Persistence PTO's efficiency and performance. These measurements were obtained using a dynamometer test bench setup. The data includes open-circuit voltage and loss measurements to validate machine characteristics, efficiency mapping tests to determine the generator's performance mapping, and efficiency mapping tests to determine the converter's efficiency over the feasible operating range. This data was collected between June 2023 and September 2023. The data was collected at the National Renewable Energy Laboratory's Flatirons Campus, Colorado, United States. The data was collected using NREL's 5-kW dynamometer test bench, equipped with a torque sensor and various voltage and current sensors fed to a dedicated data acquisition system. Units for the data are included in the data file headers for each data series. A text editor or spreadsheet software such as Excel is required to view the *.csv data. The data are also provided in *.mat files. To view data plots, a Matlab script with *.mat files are provided.

16 TIDAL AND WAVE POWER↗

A model of persistent breaking of continuous symmetry

We consider a UV-complete field-theoretic model in general dimensions, including d=2+1, which consists of two copies of the long-range vector models, with O(m) and O(N-m) global symmetry groups, perturbed by double-trace operators. Using conformal perturbation theory we find weakly-coupled IR fixed points for N\geq 6 N ≥ 6 that reveal a spontaneous breaking of global symmetry. Namely, at finite temperature the lower rank group is broken, with the pattern persisting at all temperatures due to scale-invariance. We provide evidence that the models in question are unitary and invariant under full conformal symmetry. Furthermore, we show that this model exhibits a continuous family of weakly interacting field theories at finite N.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Application of electron beam technology to decompose persistent emerging drinking water contaminants: poly- and perfluoroalkyl substances (PFAS) and 1,4-Dioxane

Poly- and perfluoroalkyl substances (PFAS) and 1,4-dioxane are persistent emerging contaminants that are currently under consideration for federal and state-specific regulations in drinking water. Both PFAS and 1,4-dioxane are highly resistant to degradation and are not effectively removed by conventional drinking water treatment systems. Results from the Unregulated Contaminant Monitoring Rule 3 survey showed that >540 sites across the nation are contaminated with both PFAS and 1,4-dioxane. Hence, there is a need to identify technologies that can effectively remove both these contaminants. Water treatment via electron beam (e-beam) has been proven effective at treating a wide range of contaminants, including perfluorooctane sulfonate (PFOS), perfluorooctanoate (PFOA), polychlorinated biphenyls, and trichloroethylene. While the e-beam process is often considered similar to advanced oxidation processes (AOPs), e-beam technology is unique in that it produces both highly oxidizing and reducing species at the same time. The specific objectives of this study were to: (i) determine the effectiveness of 9 MeV electrons provided by the Fermilab’s Accelerator Application Development and Demonstration (A2D2) tool to decompose PFAS and 1,4-dioxane; (ii) assess the formation of byproducts during water treatment; (iii) apply the optimized treatment to field groundwater samples contaminated with PFAS and 1,4-dioxane, and (iv) assess the energy demands for the treatment of these contaminants using e-beam. Results from this study showed that e-beam is effective in treating both 1,4-dioxane and PFAS. Complete degradation of 1,4-dioxane was observed at a dose of 5 kGy for an initial concentration of up to 1 ppm without the need for any sample modification. The electrical energy per order (EEo) for treatment of 1,4-dioxane ranged from 0.46 to 0.72 kWh/m 3 /order and was comparable and even lower, in some cases, than other AOP technologies. Alkaline conditions (pH 13) and low dissolved oxygen concentration (2 mg/L) highly favored the treatment of PFAS by e-beam. Greater than 90% removal of PFOA and PFOS from an initial concentration of 100 to 500 ppb was achieved at a dose of 250 kGy and 500 kGy, respectively, under optimized conditions. The degradation efficiency was not significantly changed when treating other PFAS of fluorinated carbon chain length of 5 to 7 individually at 250 kGy with a removal ranging from 85¬–99% for different compounds. Short chain PFAS (perfluorobutanoate: PFBA and perfluorobutane sulfonate: PFBS) did not degrade under the same conditions at 250 kGy, but 70 to 99% degradation was observed at a higher dose of 1000 kGy. Short chain PFAS (perfluorohexanoate: PFHxA (C5) and perfluoroheptanoate: PFHpA (C6)) were detected after treatment of PFOA, but not after PFOS treatment. Inability to close the mass balance through targeted analysis suggests the presence of other intermediates not detectable by available analytical methods. When treating PFAS mixture containing ten compounds at equimolar concentration of 0.05 µM each, preferential degradation of polyfluorinated compound (6:2 fluorotelomer sulfonate or 6:2 FTS) followed by C8 and C7 compounds was observed as a function of increasing e-beam dose. About 30% degradation of ΣPFAS was observed at 250 kGy and no further removal was observed up to a dose of 1000 kGy. C4 to C6 PFASs showed no degradation, while C3 PFAS (PFBS) showed an increase in concentration by 34% at 1000 kGy due to formation from the breakdown of other long chain PFAS. These results suggested that (a) the reaction kinetics is likely different for different PFAS based on chain length, functional group, and the degree of fluorination of the carbon chain, and (b) there may be intermediates generated from the degradation of 6:2 FTS and C7/C8 compounds that can potentially scavenge hydrated electrons needed for reaction with the untreated PFAS molecules. Treatment of three PFAS-contaminated groundwater samples from two US states showed similar trends as observed in the treatment of equimolar PFAS mixtures. Up to 71% removal of ΣPFAS was achieved in real groundwater samples at 750 kGy and data trend suggested that higher degradation is feasible if higher doses (>1MGy) are applied to treat field samples to overcome matrix effects and competing species. Calculated EEo for PFAS ranged from as low as ~48 to 1081 kWh/m 3 /order depending on the type of PFAS treated. These values are comparable and even lower, in some cases, than other destructive technologies employed for PFAS treatment such as ultrasound, plasma, and photochemical treatment. The results from this study indicate e-beam is a promising approach under favorable conditions and should be explored further as an end-of-train treatment option for PFAS destruction.

1,4-Dioxane↗

Application of electron beam technology to decompose persistent emerging drinking water contaminants: poly- and perfluoroalkyl substances (PFAS) and 1,4 dioxane.

Fermi Research Alliance, LLC (FRA) operates Fermilab under contract with the U.S. Department of Energy and has patents on technologies and applications of a novel mobile electron beam accelerator. A high-power version of this mobile accelerator based on FRA-developed SRF technology is under development at Illinois Accelerator Research Center (IARC) and can enable several new applications that have significant commercial potential. One such application is the e-beam treatment of persistent emerging contaminants in drinking water. The contaminants of concern are poly- and perfluoroalklyl substances (PFAS) and 1,4-dioxine. Both PFAS and 1,4-D are highly resistant to degradation and are not effectively removed by conventional drinking water treatment systems. Existing technologies, such as granular activated carbon (GAC) filters and reverse osmosis (RO) systems do not decompose. The Center for Clean Water Technology (CCWT) at Stony Brook University (SBU) is in the process of identifying and testing effective technologies to remove PFAS and/or 1,4-D from drinking waters. se PFAS, but rather concentrate them either by adsorption (GAC) or membrane rejection (RO). The Center for Clean Water Technology (CCWT) at Stony Brook University (SBU) is in the process of identifying and testing effective technologies to remove PFAS and/or 1,4-D from drinking waters to demonstrate the full-scale application of novel water treatment technologies and is experienced in conducting research to understand treatment performance with a particular focus on 1,4-D and PFAS contamination.

43 PARTICLE ACCELERATORS↗

Worth More Dead than Alive? Quantifying Necromass Persistence for Terrestrial Carbon Storage

The continuous cycle of plant-associated microbial biomass growth, death, and decay provides a consistent supply of necromass-C throughout the rooting zone of the soil profile. These inputs are obviously important for resource allocation and soil quality, but microbial necromass-C may play a critical, but currently unknown, role in mitigating the impacts of climate change through atmospheric decarbonization. Microbial necromass is the largest terrestrial sink of persistent carbon in soils, thus its fate and preservation will have a major impact on global C budgets. Our current understanding of the ecosystem controls on necromass generation, biogeochemical transformation, and stabilization is lacking. The objective of this project is to explore the specific influence of rhizosphere and necromass inputs on soil carbon pools.

54 ENVIRONMENTAL SCIENCES↗

Persistent DynAMICS

Persistent DynAMICS is a lightweight software platform that enables distributed sensing systems to operate as a unified, responsive network. It integrates with existing sensors, data systems, and processing tools as an overlay, without requiring hardware replacement or increasing user burden. As data is collected, the system identifies situations that require additional attention and directs selected sensors to gather more information. For example, if a sensor detects an unusual condition along a pipeline, the system can task nearby sensors or different sensing modalities to confirm the event and focus data collection where it is needed. To support this, the platform forms temporary groups of sensors that work together to address specific objectives. Once complete, these groups are dissolved and resources are reassigned as needed. Communication is handled through an integrated messaging framework with client and server components, enabling reliable operation and data continuity even in low-bandwidth or intermittent connectivity environments.

97 MATHEMATICS AND COMPUTING↗

Persistence Control of Engineered Functions in Complex Soil Microbiomes (PerCon SFA), Secure Biosystems Design Project Data Catalog at PNNL DataHub

The Persistence Control of Engineered Functions in Complex Soil Microbiomes Project (PerCon SFA) at Pacific Northwest National Laboratory (PNNL) is a Genomic Sciences Program Biosystems Design, Science Focus Area research project consortium. Collaborating across highly integrated institutions, PerCon SFA scientists are exploring how environmental niches can be sculpted using the mechanisms of genome reduction and metabolic addiction to drive secure rhizosphere community design for robust biomass cropping in challenging environments. The PerCon SFA DataHub project repository contains publication-relevant digital dataset and metadata DOI packages, enabling exploration and download of integrated experimental dataset catalogs publicly available to a global scientific community. and metadata repository allow for exploring and downloading integrated experimental biodesign omics dataset catalogs, including experimental protocols and/or workflows, raw and/or processed data, as required by the repository, and other relevant supporting materials and/or metadata required for research reproducibility and reporting.

59 BASIC BIOLOGICAL SCIENCES↗

Antibiotic resistance and host immune system-induced metal bactericidal control are key factors for microbial persistence in the developing human preterm infant gut microbiome

The human gut microbiome, which develops and stabilizes during the early stages of infant life, plays an essential role in host health through the production of metabolic resources and the stimulation and training of the immune system. To study colonization and community functional dynamics of the microbiota based on responses to host immune processes during the normal and dysbiotic establishment of the gut, metaproteomics was conducted on 91 fecal samples collected over the first 90 days of life from 17 hospitalized premature infants. Microbial responses to antibiotic administration and host-imposed metal bactericidal control correlated with community assembly and resiliency of microbes in the developing preterm gut. Specifically, proteins related to antibiotic resistance and metal homeostasis mechanisms were predominant in persisting members in the infant gut environment over the first several weeks of life. Overall, this metaproteomics study provides a unique approach to examine the temporal expansion and resilience of microbial colonization, as it allows simultaneous examination of both host and microbial metabolic activities. Understanding the interplay between host and microbes may elucidate the microbiome’s potential immunomodulatory roles relevant to necrotizing enterocolitis and other dysbiotic conditions in preterm infants.

59 BASIC BIOLOGICAL SCIENCES↗

Genomic Diversity and Phenotypic Variation in Fungal Decomposers Involved in Bioremediation of Persistent Organic Pollutants

Fungi work as decomposers to break down organic carbon, deposit recalcitrant carbon, and transform other elements such as nitrogen. The decomposition of biomass is a key function of wood-decaying basidiomycetes and ascomycetes, which have the potential for the bioremediation of hazardous chemicals present in the environment. Due to their adaptation to different environments, fungal strains have a diverse set of phenotypic traits. This study evaluated 320 basidiomycetes isolates across 74 species for their rate and efficiency of degrading organic dye. We found that dye-decolorization capacity varies among and within species. Among the top rapid dye-decolorizing fungi isolates, we further performed genome-wide gene family analysis and investigated the genomic mechanism for their most capable dye-degradation capacity. Class II peroxidase and DyP-type peroxidase were enriched in the fast-decomposer genomes. Gene families including lignin decomposition genes, reduction-oxidation genes, hydrophobin, and secreted peptidases were expanded in the fast-decomposer species. This work provides new insights into persistent organic pollutant removal by fungal isolates at both phenotypic and genotypic levels.

59 BASIC BIOLOGICAL SCIENCES↗