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DOE OSTI2020

Strong, Nonresonant Radiation Enhances Cis–Trans Photoisomerization of Stilbene in Solution

Previously, it has been demonstrated that external electric fields may be used to exert control over chemical reactivity. In this paper, the impact of a strong, nonresonant IR field (1064 nm) on the photoisomerization of cis-stilbene is investigated in cyclohexane solution. The design of a suitable reaction vessel for characterization of this effect is presented. The electric field supplied by the pulsed, near-IR radiation (ε 1 = 4.5 × 10 7 V/cm) enhances the cis → trans photoisomerization yield at the red edge of the absorption spectrum (wavelengths between 337 and 340 nm). Within the microliter focal volume, up to 75% of all cis-stilbene molecules undergo isomerization to trans-stilbene in the strong electric-field environment, indicating a significant increase relative to the 35% yield of trans-stilbene under field-free conditions. This result correlates with a 1–3% enhancement in the trans-stilbene concentration throughout the bulk solution. Theoretical analysis suggests that the observed change is the result of dynamic Stark shifting of the ground and first excited states, leading to a significant redshift in cis-stilbene’s absorption spectrum. The predicted increase in the absorption cross section in this range of excitation wavelengths is qualitatively consistent with the experimental increase in trans-stilbene production.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1981

Compact radio source 1413 + 135 is a far-IR extragalactic object

The radio source 1413 + 135 is shown to be one of the strongest known emitters of millimeter radiation. The energy distribution of this object, measured between meter and X-ray wavelengths, reveals that most of the power emitted by this object comes out at millimeter and far-IR wavelengths. If the emission at 1 mm is due to incoherent synchrotron radiation, then the source must be very compact, with a size around 25 micron arc sec, and contain a magnetic field larger than 10 G. The steep spectral index in the near-IR is attributed to a high-energy cutoff in the distribution of synchrotron emitting electrons at a Lorentz factor of approximately 300.

Beichman, C. A.↗
NASA NTRS2001

The Mid and Far IR Universe and Facilities To See It

Although half the luminosity of the universe appears in the band from 20-450 $\mu$m, almost nothing is known about the sources of this radiation. Moreover, many molecules, atoms, and ions of astrophysical interest have some of their strongest lines in this wavelength range. Now Infrared Astronomy Satellite (IRAS) and ISO have flown, Space Infrared Telescope Facility (SIRTF) is nearly ready, SOFIA is under construction, and NGST, ALMA, Herschel, Planck, and a dozen 8 m and a 25 m ground-based visible/near IR telescopes could all be operational by the end of decade. Nevertheless, the mid and far IR region will still not have telescopes that are comparable to neighboring bands in energy sensitivity or angular resolution, despite these many advances. What scientific questions will still be open, and what instrumentation will be required? We anticipate that cold filled-aperture telescopes operating out to 100 $\mu$m and cold imaging interferometers, operating out to about 450 $\mu$m in space could be very powerful, using direct detection rather than heterodyne systems. I will give a brief overview of the scientific questions that may still be open, the main factors governing the choice of equipment, and the technological developments that would be required to actually build and use these new facilities.

Mather, John C.↗
NASA NTRS2005

X-ray Weak Broad-line Qquasars: Absorption or Intrinsic X-ray Weakness

XMM observations of X-ray weak quasars have been performed during 2003 and 2004. The data for all the observations have become available in 2004 (there has been a delay of several months on the initial schedule, due to high background flares which contaminated the observations: as a consequence, most of them had to be rescheduled). We have reduced and analyzed all the data, and obtained interesting scientific results. Out of the eight sources, 4 are confirmed to be extremely X-ray weak, in agreement with the results of previous Chandra observations. 3 sources are confined to be highly variable both in flux (by factor 20-50) and in spectral properties (dramatic changes in spectral index). For both these groups of objects we are completing a publication: 1) For the X-ray weak sources, a paper is submitted with a complete analysis of the X-ray spectra both from Chandra and XMM-Newton, and a comparison with optical and near-IR photometry obtained from all-sky surveys. Possible models for the unusual spectral energy distribution of these sources are also presented. 2) For the variable sources, a paper is being finalized where the X-ray spectra obtained with XMM-Newton are compared with previous X-ray observations and with observations at other wavelengths. It is shown that these sources are high luminosity and extreme cases of the highly variable class of narrow-line Seyfert Is. In order to further understand the nature of these X-ray weak quasars, we submitted proposals for spectroscopy at optical and infrared telescopes. We obtained time at the TNG 4 meter telescope for near-IR observations and at the Hobby-Eberly Telescope for optical high-resolution spectroscopy. These observations have been performed in early 2004. They will complement the XMM data and will lead to understanding of whether the X-ray weakness of these sources is an intrinsic property or is due to absorption by circum-nuclear material. The infrared spectra of the variable sources have been already analyzed and are discussed in the paper by Memola et al. which will be soon submitted.

Mushotzky, Richard↗
NASA NTRS1983

Voyager photopolarimeter observations of Saturn and Titan

The Voyager 2 photopolarimeter experiment observed the intensity and polarization of scattered sunlight from the atmospheres of Saturn and Titan in the near-UV at 2640 A and in the near-IR at 7500 A. Measurements of Saturn's limb brightening and polarization at several phase angles up to 70 deg indicate that a significant optical depth of UV absorbers are present in the top 100 mbar of Saturn's atmosphere in the equatorial zone and north polar region, and possibly at other latitudes as well. UV absorbers are prominent in polar regions, suggesting that charged particle precipitation from the magnetosphere may be important in their formation. The whole-body polarization of Titan is strongly positive in both the UV and near IR. If spherical particles are responsible for the polarization, no single size distribution or refractive index can account for the polarization at both wavelengths. The model atmosphere proposed by Tomasko and Smith (1982), characterized by a gradient in particle size with altitude, seems capable of explaining the Voyager observations.

West, R. A.↗
NASA NTRS1984

Measuring spectra of arid lands

The principles, instrumentation and data acquisition and interpretation techniques employed in multispectral remote sensing for geological applications are surveyed. Sensing is based on exact measurements of electromagnetic radiation interacting with atoms and molecules in the sensed scene. Absorbed radiation can be used to identify elements in the near-IR bands and emitted or reflected energy can be sensed in the mid- and far-IR. Sunlight normally serves as the exciting source. Wavelength absorptance and emittance characteristics are distinct for the various elements and molecules such as transition metal ions, water, carbonates, etc. The bands for identifying different materials are determined in the laboratory, followed by ground truth field tests. Several hand-held radiometers and spectrometers have been developed for the field trials. Each instrument usually has a limited detection range and serves for developing a data base for subtle distinctions among contiguous minerals with similar radiometric signatures. The data serve for calibrating first airborne and then satellite sensors, e.g., the Landsat MSS and Thematic Mapper. Instruments are also being tested using the Orbiter as the test platform.

Kahle, A. B.↗
NASA NTRS1991

Titan's surface and troposphere, investigated with ground-based, near-infrared observations

Characterizations are presently made of Titan's haze, cloud, surface albedo, and atmospheric H2 abundance on the bases of 4000-5000/cm near-IR spectrum and points from the Fink and Larson (1979) 4000-12,500/cm spectrum. The strength of solar radiation absorption varies significantly with wavelength, facilitating a probing of the various atmospheric levels down to the surface. The present observations suggest the existence of an optically thin CH4 cloud layer, as well as haze and cloud optical depths sufficiently small for surface sensing at 4900, 6250, and 7700/cm. The albedos at these wavenumbers indicate the dominant surface material to be 'dirty' water ice.

Griffith, Caitlin A.↗
NASA NTRS1987

Infrared investigation of water in Comet P/Halley

The results of the investigation of gaseous water, detected in the IR spectra of the Comet Halley's coma taken by the NASA's Kuiper Airborne Observatory, are summarized. High-resolution spectra revealed, near the wavelength of 2.65 microns, solar-pumped fluorescent emission in the (001-000) band of H2O and three lines of the (011-010) 'hot' band. The absolute production rate of H2O and its spatial distribution, temporal variability, and outflow velocity were measured along with the H2O ortho/para ratio. The measured line intensities indicate that water in the coma is rotationally relaxed. The aperture-averaged excitation temperatures for the low-lying rotational transitions were about 40 K, indicating that the coma kinetic temperature is extremely cold. Significant short-term temporal variations in the H2O line intensities were detected together with a strong pre- to postperihelion asymmetry (a factor of about 7) in the water production rate at a heliocentric distance of about 1 AU.

Weaver, H. A.↗
NASA NTRS1993

Possible near-IR channels for remote sensing precipitable water vapor from geostationary satellite platforms

Remote sensing of troposheric water vapor profiles from current geostationary weather satellites is made using a few broadband infrared (IR) channels in the 6-13 micron region. Uncertainties greater than 20% exist in derived water vapor values just above the surface from the IR emission measurements. In this paper, we propose three near-IR channels, one within the 0.94-micron water vapor band absorption region, and the other two in nearby atmospheric windows, for remote sensing of precipitable water vapor over land areas, excluding lakes and rivers, during daytime from future geostationary satellite platforms. The physical principles are as follows. The reflectance of most surface targets varies approximately linearly with wavelength near 1 micron. The solar radiation on the sun-surface-sensor ray path is attenuated by atmospheric water vapor. The ratio of the radiance from the absorption channel with the radiances from the two window channels removes the surface reflectance effects and yields approximately the mean atmospheric water vapor transmittance of the absorption channel. The integrated water vapor amount from ground to space can be obtained with a precision of better than 5% from the mean transmittance. Because surface reflectances vary slowly with time, temporal variation of precipitable water vapor can be determined reliably. High spatial resolution, precipitable water vapor images are derived from spectral data collected by the Airborne Visable-Infrared Imaging Spectrometer, which measures solar radiation reflected by the surface in the 0.4-2.5 micron region in 10-nm channels and has a ground instantaneous field of view of 20 m from its platform on an ER-2 aircraft at 20 km. The proposed near-IR reflectance technique would complement the IR emission techniques for remote sensing of water vapor profiles from geostationary satellite platforms, especially in the boundary layer where most of the water vapor is located.

Gao, B.-C.↗
NASA NTRS1993

Clementine: Anticipated scientific datasets from the Moon and Geographos

The Clementine spacecraft mission is designed to test the performance of new lightweight and low-power detectors developed at the Lawrence Livermore National Laboratory (LLNL) for the Strategic Defense Initiative Office (SDIO). A secondary objective of the mission is to acquire useful scientific data, principally of the Moon and the near-Earth asteroid Geographos. The spacecraft will be in an elliptical polar orbit about the Moon for about 2 months beginning in February of 1994 and it will fly by Geographos on August 31. Clementine will carry seven detectors each weighing less than about 1 kg: two Star Trackers wide-angle uv/vis wide-angle Short Wavelength IR (SWIR) Long-Wavelength IR (LWIR) and LIDAR (Laser Image Detection And Ranging) narrow-angle imaging and ranging. Additional presentations about the mission detectors and related science issues are in this volume. If fully successful Clementine will return about 3 million lunar images, a dataset with nearly as many bits of data (uncompressed) as the first cycle of Magellan and more than 5000 images of Geographos. The complete and efficient analysis of such large data sets requires systematic processing efforts. Described below are concepts for two such efforts for the Clementine mission: global multispectral imaging of the Moon and videos of the Geographos flyby. Other anticipated datasets for which systematic processing might be desirable include multispectral observations of Earth; LIDAR altimetry of the Moon with high-resolution imaging along each ground track; high-resolution LIDAR color along each lunar ground track which could be used to identify potential titanium-rich deposits at scales of a few meters; and thermal IR imaging along each lunar ground track (including nighttime observations near the poles).

Mcewen, A. S.↗
NASA NTRS1999

Near-Infrared Hyperspectral Image Cubes of Mars during the 1999 Opposition

We used the Goddard Space Flight Center, Acousto-Optic Tunable Filter (AOTF) Camera to obtain near-IR spectral image sets of Mars over the 1.6-3.6 micron region during the April 1999 opposition. A complete image set consists of 280 images with a spectral full-width-half maximum of 10 wavenumbers (fixed in frequency), 90 images in H-band (1.55-1.80 micron), 115 images in K-band (1.95-2.50 micron) and 75 images in L-band (2.90-3.70 micron). The short-wavelength limit is set by transmission of AOTF cell and long-wavelength limit is imposed by sensitivity of PICNIC, 256x256, HgCdTe array detector. We will discuss the new array performance and provide preliminary interpretations of some of these results. These measurements were part of a 4-observatory coordinated effort whose overall objective was to assemble a photometrically calibrated, spectrally complete ground-based image cube over the visible and near-IR spectral region. To accomplish this, four observing teams conducted the investigations with instruments spanning 0.4 to 5.0 micron. The instruments and observing facilities were (a) AOTF camera at Apache Point Observatory, 3.5m, f/10, Nasymth focus (this abstract). Primary science targets included the 3 micron water-of hydration feature and CO2, H2O ice (polar regions and clouds); (b) Visible/NIR interference-filter (24 filters) camera at Lowell Observatory, 72" telescope. 430-1050 nm. Science targets were Fe(2+), Fe(3+) mineralogy and coarse grain hematite search; (c) NMSU Tortugas Mountain Observatory, 60 cm telescope, CCD photometry with same filter set as Lowell; (d) KPNO cryogenic grating/slit spectrometer (CRSP/SALLY) at KPNO 2.1 m, f/15 Cassegrain focus (see abstract by D. Glenar, et. al., this meeting). Selected wavelengths in 3-5 micron region (L, M band). Science targets included water-of-hydration feature (3-4 micron long wave extension) and sulfate mineralogy. Observers participating in this campaign included Dave Glenar, John Hillman, Gordon Bjoraker and Fred Espenak from GSFC, Nancy Chanover, Jim Murphy and A. S. MurTell from NMSU, Leslie Young from BU, Diana Blaney from JPL and Dick Joyce from KPNO.

Hillman, John J.↗
NASA NTRS1990

Multi-waveband observations of colliding galaxies

Colliding galaxies represent a major challenge to both theorists and observers because of the large variety of phenomena which are expected to come into play during the interaction. Strong gravitational fluctuations may drive non-linear waves and instabilities throughout the stars and gas leading to enhanced star formation, nuclear activity and ultimately a mixing of the morphological components of the original galaxies. One relatively uncomplicated class of colliding galaxy where stellar waves play an important role in star formation are ring galaxies. Ring galaxies are probably formed when a companion galaxy passes through the center of a disk system driving circular waves through the disk (Lynds and Toomre 1976, Toomre 1978, Struck-Marcell 1990). Off-center collisions can generate non-circular waves and can be loosely described as banana-shaped although they may exhibit more complex forms as the waves expand into the disk. The propagation of such stellar and gaseous waves through the disk leads to enhanced star formation (e.g., Appleton and Struck-Marcell 1987a; Jeske 1986) and provides a unique probe of the response of the interstellar medium (ISM) to a propagating wave (see Appleton and Struck-Marcell 1987b). Here, the authors report results for 3 systems; the irregular ring Arp 143 (=VV 117); Wakamatsu's Seyfert ring (A0959-755; see Wakamatsu and Nishida 1987) and the brighter member of the pair of ring galaxies comprising of AM 1358-221. The most complete multi-wavelength data is for Arp 143. Optical charge coupled device (CCD) observations made with the 60 inch Palomar telescope at BV and r band, near-IR images at J (1.25 microns), H (1.65 microns) and k (2.2 microns) bands from the infrared camera (IRCAM) InSb array camera on the 3.8m United Kingdon Infrared Telescope (UKIRT) telescope and very large array (VLA) observations at 20cm in both the neutral hydrogen line and radio continuum are described. The observations of Wakamatsu's ring and AM 1358 were made only in the near-IR, and a comparison is made with available optical plate material.

Appleton, P. N.↗
NASA NTRS1992

Scattering of infrared radiation by dust in NGC 7023 and NGC 2023

The contribution of scattered light to the total nebular emission is determined on the basis of linear polarization measurements at 1.25, 1.65, and 2.2 microns of the visual reflection nebulae NGC 7023 and NGC 2023. The percentage polarization of NGC 7023 slowly increases from 0.3 to 1 micron, with peak polarizations of up to 26 percent at 1.25 micron, then rapidly decreases, with values of 4-7 percent at 2.2 microns. This is interpreted as implying that scattered starlight contributes most to the SW emission, while unpolarized emission from small grains or large molecules dominates at longer wavelengths. IR polarization and surface brightness measurements are combined to derive the intensity of scattered light, which is then compared with scattering models. While the near-IR emission of both NGC 2023 and NGC 7023 is dominated by small-grain or large-molecule emission, IR scattered light plays a larger role in NGC 2023 than in NGC 7023.

Sellgren, K.↗
NASA NTRS2003

Solar System Connections to the Organic Material In the ISM

The organic component of the interstellar medium (ISM) has relevance to the formation of the early solar nebula, since our solar system formed out of ISM material. Comparisons of near infrared spectra of the diffuse ISM dust with those of primitive solar system bodies (such as comets and meteorites) show a remarkable similarity, suggesting that perhaps some of the interstellar organic material made its way, unaltered, into our solar system. Tracing the interstellar organic material is necessary to understand how these materials may be important links in the development of prebiotic phenomena. Studies of the ISM reveal that the organic refractory component of the diffuse ISM is largely hydrocarbon in nature, possessing little N or O, with carbon distributed between the aromatic and aliphatic forms. There is a strong similarity in the near IR spectra of the diffuse ISM (the 3.4 micron hydrocarbon bands) and those seen in the Murchison and Orgueil meteorites, however, detailed comparisons at longer wavelengths reveal critical dissimilarities. Here we will present comparisons and discussion of relevant spectra. As we continue to explore, we will gain insight into the connection between planetesimals in the solar system and chemistry in the dusty space between the stars.

Pendleton, Yvonne J.↗
NASA NTRS2011

CANDELS: The Cosmic Assembly Near-Infrared Deep Extragalactic Legacy Survey

The Cosmic Assembly Near-IR Deep Extragalactic Legacy Survey (CANDELS) is designed to document the first third of galactic evolution, from z approx. 8 - 1.5. It will image > 250,000 distant galaxies using three separate cameras on the Hubble Space Tele8cope, from the mid-UV to near-IR, and will find and measure Type Ia supernovae beyond z > 1.5 to test their accuracy as standard candles for cosmology. Five premier multi-wavelength sky regions are selected, each with extensive ancillary data. The use of five widely separated fields mitigates cosmic variance and yields statistically robust and complete samples of galaxies down to a stellar mass of 10(exp 9) solar mass to z approx. 2, reaching the knee of the UV luminosity function of galaxies to z approx. 8. The survey covers approximately 800 square arc minutes and is divided into two parts. The CANDELS/Deep survey (5(sigma) point-source limit H =27.7mag) covers approx. 125 square arcminutes within GOODS-N and GOODS-S. The CANDELS/Wide survey includes GOODS and three additional fields (EGS, COSMOS, and UDS) and covers the full area to a 50(sigma) point-source limit of H ? or approx. = 27.0 mag. Together with the Hubble Ultradeep Fields, the strategy creates a three-tiered "wedding cake" approach that has proven efficient for extragalactic surveys. Data from the survey are non-proprietary and are useful for a wide variety of science investigations. In this paper, we describe the basic motivations for the survey, the CANDELS team science goals and the resulting observational requirements, the field selection and geometry, and the observing design.

Grogin, Norman A.↗
NASA NTRS2017

Cosmic Infrared Background Fluctuations and Zodiacal Light

We performed a specific observational test to measure the effect that the zodiacal light can have on measurements of the spatial fluctuations of the near-IR (near-infrared)background. Previous estimates of possible fluctuations caused by zodiacal light have often been extrapolated from observations of the thermal emission at longer wavelengths and low angular resolution or from IRAC (Infrared Array Camera) observations of high-latitude fields where zodiacal light is faint and not strongly varying with time. The new observations analyzed here target the COSMOS (Cosmic Evolution Survey) field at low ecliptic latitude where the zodiacal light intensity varies by factors of approximately 2 over the range of solar elongations at which the field can be observed. We find that the white-noise component of the spatial power spectrum of the background is correlated with the modeled zodiacal light intensity. Roughly half of the measured white noise is correlated with the zodiacal light, but a more detailed interpretation of the white noise is hampered by systematic uncertainties that are evident in the zodiacal light model. At large angular scales (greater than or approximately equal to 100 arcseconds) where excess power above the white noise is observed, we find no correlation of the power with the modeled intensity of the zodiacal light. This test clearly indicates that the large-scale power in the infrared background is not being caused by the zodiacal light.

cosmology: observations aEuro" diffuse radiation a↗
NASA NTRS1974

Observational constraints on model atmospheres for Uranus and Neptune

We have re-examined the visible and near-IR regions of the spectra of Uranus and Neptune to provide additional data for constructing atmospheric models. We find that a true continuum exists only at wavelengths below 4700 A, that the 6420 A absorption previously attributed to hydrogen is probably caused by methane, that there is no evidence for ammonia, ethylene or ethane absorptions in our spectra, and that the abundance of methane is probably much higher than previous estimates suggest. This last finding implies that the value of H/C in the atmospheres of both planets is much less than 1/10 the solar (or Jovian) value. Clear, Rayleigh-scattering model atmospheres are not compatible with the observations, but more work is needed to establish viable alternatives.

Encrenaz, T.↗
NASA NTRS1985

Infrared emission from desorbed NO2(*) and NO(*)

Infrared photons from the radiative cascade accompany both the gas phase NO2 continuum chemiluminescence (which originates from its 2B2 and 2B1 states) and the NO beta bands. When these upper electronic states are excited by recombination/desorption at surfaces of low Earth orbiting spacecraft, similar IR emission spectrums will be observed. The principal NO2 features (other than the long wavelength tail of its electronic transitions) are the nu sub 3 fundamental sequence near 6.2 microns and nu sub 1 + nu sub 3 intercombination bands near 3.6 microns; NO would emit the delta v=1 and delta v=2 systems above 5.3 and 2.7 microns. Because of the long radiative lifetimes of the upper vibrational states, the infrared radiances in projections parallel to the vehicle surface (which we estimate) are substantially less than those of the visible and ultraviolet glows.

Kofsky, I. L.↗