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NASA NTRS2004

Penetrator Coring Apparatus for Cometary Surfaces

Touch and go impact coring is an attractive technique for sampling cometary nuclei and asteroidal surface on account of the uncertain strength properties and low surface gravities of these objects. Initial coring experiments in low temperature (approx. 153K polycrystalline ice) and porous rock demonstrate that simultaneous with impact coring, measurements of both the penetration strength and constraints on the frictional properties of surface materials can be obtained upon core penetration and core sample extraction. The method of sampling an asteroid, to be deployed, on the now launched MUSES-C mission, employs a small gun device that fires into the asteroid and the resulted impact ejecta is collected for return to Earth. This technique is well suited for initial sampling in a very low gravity environment and deployment depends little on asteroid surface mechanical properties. Since both asteroids and comets are believed to have altered surface properties a simple sampling apparatus that preserves stratigraphic information, such as impact coring is an attractive alternate to impact ejecta collection.

Braun, David F.↗

NASA NTRS2006

Comets, Asteroids, Meteorites, and the Origin of the Biosphere

During the past few decades, the delivery of water, organics, and prebiotic chemicals to the Biosphere of Earth during the Hadean (4.5-3.8 Ga) period of heavy bombardment by comets and asteroids has become more widely accepted. Comets are still largely regarded as frigid, pristine bodies of protosolar nebula material that are devoid of liquid water and therefore unsuitable for life. Complex organic compounds have been observed in comets and on the water-rich asteroid 1998 KY26 and near IR observations have indicated the presence of crystalline water ice and ammonia hydrate on the large Kuiper Belt object (50000) Quaoar that has resurfacing suggesting cryovolcanic outgassing. Spacecraft observations of the chemical compositions and characteristics of the nuclei of several comets (Halley, Borrelly, Wild 2, and Tempel 1) have shown that comets contain complex organic chemicals; that water is the predominant volatile; and that extremely high temperatures (approx. 350-400 K) can be reached on the surfae of the very black (albedo approx. 0.03) nuclei of comets when they approach the Sun. Impact craters and pinnacles observed on comet Wild 2 suggest a thick crust. Episodic outbursts and jets from the nuclei of several comets indicate that localized regimes of liquid water and water vapor can periodically exist beneath the comet crust. The Deep Impact mission found the temperature of the nucleus of comet Tempel 1 at 1.5 AU varied from a minimum of 280 plus or minus 8 K the 330K (57 C) on the sunlit side. In this paper it is argued that that pools and films of liquid water exist (within a wide range of temperatures) in cavities and voids just beneath the hot, black crust. The possibility of liquid water existing over a wide range of temperatures significantly enhances the possibility that comets might contain niches suitable for the growth of microbial communities and ecosystems. These regimes would be ideal for the growth of psychrophilic, mesophilic, and thermophilic photoautotrophs and chemolithotrophs such as the motile filamentous cyanobacteria (e.g., Calothrix, Oscillatoria, Phormidium, and Spirulina) that grow in geothermal springs and geysers of Earth at temperatures ranging fiom 320K to 345K and are also found growing in cold polar desert soils. The mineralized remains of morphotypes of all of these cyanobacteria have also been found in the Orgueil CI1 and the Murchison CN2 carbonaceous meteorites that may derive from cometary parent bodies. Observational results that support the hypothesis that liquid water can in active regions just beneath the surface of comets and that comets, carbonaceous meteorites, and asteroids may have played a significant role in the origin and evolution of the Biosphere and in the distribution of microbial life throughout the Solar System.

Hoover, Richard B.↗

NASA NTRS1979

Dust release and mantle development in comets

A model of dust release and dust mantle development by cometary nuclei is developed to explain the brightness asymmetry observed in comets before and after perihelion. Assuming that the cometary nucleus consists of a uniform mixture of dust and volatile ices and taking into account the differential mass spectrum of the dust and the effect of nuclear gravity, it is shown that the factor which determines whether a comet will be brighter before or after perihelion is the mass ratio of dust to volatiles in the nucleus. If this ratio is greater than about two, the comet will be brighter on the inward path and not lose its mantle near perihelion. Applying the model to comet Halley (dust to volatiles ratio presumed to be less than two), it is predicted that the comet remains without a mantle until it reaches a heliocentric distance of 2.035 AU after perihelion and loses its mantle suddenly at a distance of about 1.45 AU on the inward path, causing it to be brighter after perihelion. Predictions of monochromatic brightness are found to be in fair agreement with total observed brightnesses.

Brin, G. D.↗

NASA NTRS1984

An improved thermal model for cometary nuclei

A thermal model for cometary nuclei is presented and used in comparisons of predictions with data on Halley's comet. The model considers the surface boundary conditions and heat diffusion equations, the sublimation rate of ice, the energy balance, and the dust production rate. Projections were made for the Halley nucleus over 18 latitudes from -85 to +85 deg, from 185 d before to 110 d after perihelion, and in 20 layers of its surface in 1.3 cm increments. Sublimation is predicted to increase by a factor of 2.2 every orbit, thereby allowing 320 returns for a nucleus with a coma, 710 returns with a bare ice nucleus. The gas production during the Giotto intercept at 0.9 AU will be 4.4 x 10 to the 29th molecules/sec, close to an estimate made during the 1910 return.

Weissman, P. R.↗

NASA NTRS2020

Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs

AEROICESTUDY↗

NASA NTRS1989

Electron beam analysis of particulate cometary material

Electron microscopy will be useful for characterization of inorganic dust grains in returned comet nucleus samples. The choice of instrument(s) will depend primarily on the nature of the samples, but ultimately a variety of electron-beam methods could be employed. Scanning and analytical (transmission) electron microscopy are the logical choise for morphological, mineralogical, and bulk chemical analyses of dust grains removed from ices. It may also be possible to examine unmelted ice/dust mixtures using an environmental scanning electron microscope equipped with a cryo-transfer unit and a cold stage. Electron microscopic observations of comet nuclei might include: (1) porosities of dust grains; (2) morphologies and microstructures of individual mineral grains; (3) relative abundances of olivine, pyroxene, and glass; and (4) the presence of phases that might have resulted from aqueous alteration (layer silicates, carbonates, sulfates).

Bradley, John↗

NASA NTRS1987

Temperatures and minimum thickness of the inactive surface layer of comet Halley

The effects of a nonvolatile mantle on the thermal state of a comet nucleus are investigated. The original computer model was modified so that temperatures can be computed through a thin dust mantle to the center of a 5 km spherical nucleus in the orbit of P/Halley. No attempt is made to simulate the formation of the mantle. Results are obtained for various specified values of initial mantle thickness and thermal conductivity to determine their effects on temperature profiles through the mantle. The minimum thickness of mantle that can withstand ejection by sublimating gasses is also calculated as a function of mantle thermal conductivity. Calculations were performed for ten or more orbits until temperatures in the mantle reached a near steady state. Results indicate that mantles as thin as 4 cm and 14 cm, for thermal conductivities of 600 and 6000 ergs/cm/s K, respectively, will remain intact. Surface temperatures as high as 511 K at perihelion and 400 K at the position of spacecraft encounter were computed at 0 degree latitude for an upright, rotating nucleus. Ice interface temperatures were raised by different amounts during each orbit, depending on mantle thickness and thermal conductivity, until steady state was reached. These results imply that relatively small nonvolatile masses emplaced randomly in comet nuclei could produce an irregular, permanently mantled surface and could also account for the apparently random location of active areas.

Fanale, F. P.↗

NASA NTRS1994

Measurements of Ice Particles in Tropical Cirrus Anvils: Importance in Radiation Balance

Cirrus is important in the radiation balance of the global atmosphere, both at solar and thermal infrared (IR) wavelengths. In particular cirrus produced by deep convection over the oceans in the tropics may be critical in controlling processes whereby energy from warm tropical oceans is injected to different levels in the tropical atmosphere to subsequently influence not only tropical but mid latitude climate. Details of the cloud composition may differentiate between a net cooling or warming at these levels. The cloud composition may change depending on the input of nuclei from volcanic or other sources. Observations of cirrus during the FIRE-2 Project over Coffeyville, Kansas and by satellite demonstrate that cirrus, on occasion, is composed not only of larger particles with significant fall velocity (few hundred micrometers, 0.5 m/s) but much more numerous small particles, size 10-20 micrometers, with small fall velocity (cm/s), which may sometimes dominate the radiation field. This is consistent with emissivity measurements. In the thermal IR, ice absorption is strong, so that ice particles only 10 micrometers thick are opaque, at some wavelengths; on the other hand at other wavelengths and in the visible, ice is only moderately to weakly absorbing. It follows that for strongly absorbing wavelengths the average projected area of the ice particles is the important parameter, in weakly absorbing regions it is the volume (mass) of ice which is important. The shape of particles and also their internal structure may also have significant effect on their radiative properties. In order to access the role of cirrus in the radiation budget it is necessary to measure the distribution of ice particles sizes, shapes and concentrations in the regions of interest. A casual observation of any cirrus cloud shows that there is variability down to a scale of at least a few 100 m; this is confirmed by radar and lidar remote sensing. Thus aircraft measurements designed to give insight into the spatial distribution of radiation properties of ice crystals must be capable of examination of concentration, size and shape over a distance ideally of 100 m or less and to detect particles down to a size below which radiative effects are no longer significant.

Foster, Theodore↗

NASA NTRS1981

Structure and origin of cometary nuclei

There is strong evidence that a comet nucleus consists of a single object whose basic structure is Whipple's icy conglomerate. A number of cometary phenomena indicate that the nucleus is a low density, fragile object with a large degree of radial uniformity in structure and composition. Details of the ice-dust pattern are more uncertain. A working model is proposed which is based on theories of accumulation of larger objects from grains. This nucleus is a distorted spherical aggregate of a hierarchy of ice-dust cometesimals. These cometesimals retain some separate identity which lead to comet fragmentation when larger components break off. The outer layers of new comets were modified by cosmic ray irradiation in the Oort Cloud. The evidence for meteorite-comet association is steill controversial. Current dynamical studies do not seem to require a cometary source of meteorites.

Donn, B.↗

DOE OSTI2023

The Role of In-Cloud Wet Removal in Simulating Aerosol Vertical Profiles and Cloud Radiative Forcing

Among the physical processes controlling aerosol vertical profiles, in-cloud wet removal is of utmost importance while its representation in global climate models (GCMs) is crude. In this study, we implement into the Community Atmosphere Model version 6 (CAM6) a physically based aerosol wet removal parameterization scheme that explicitly treats aerosol activation, removal and resuspension. Evaluation against in-situ observations shows that the default scheme substantially overestimates the upper tropospheric black carbon (BC) and sea salt mass. Our physically based scheme reduces BC and sea salt mass by a factor of 10 and 1,000, respectively, in better agreement with observations. Also, the new scheme slightly increases number of aerosol particles between 12 nm and 4.8 μm in diameter, thereby mitigating the aerosol number underestimation in the default scheme. Our new scheme reduces the overestimation of coarse-mode aerosol (0.5–4.8 μm) number. Overall, the aerosol property changes (mass decrease and number increase) reduce the cloud condensation nuclei (CCN) concentration at low supersaturation (i.e., 0.02% and 0.1%), and increase CCN at high supersaturations (i.e., 0.5% and 1%). Consequently, the global annual mean cloud liquid water path increases by 1.89 g m -2 and the ice water path increases by 0.51 g m -2 . The global annual mean shortwave, longwave, and net cloud radiative forcing change by -1.06, 0.57, and -0.48 W m -2 , respectively. Further improvement is needed to reflect the real physics that the removal efficiencies for aerosol mass and number are disproportionate and to advect cloud-borne (activated) aerosols for a complete aerosol lifecycle.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2010

Possible Influences of Air Pollution, Dust and Sandstorms on the Indian Monsoon

In Asian monsoon countries, such as China and India, human health and safety problems caused by air pollution are becoming increasingly serious, due to the increased loading of atmospheric pollutants from waste gas emissions and from rising energy demand associated with the rapid pace of industrialization and modernization. Meanwhile, uneven distribution of monsoon rain associated with flash floods or prolonged drought, has caused major loss of human life and damage to crops and.property with devastating societal impacts. Historically, air-pollution and monsoons research are treated as separate problems. However recent studies have suggested that the two problems may be intrinsically linked and need to be studied jointly. Fundamentally, aerosols can affect precipitation through radiative effects cif suspended particles in the atmosphere (direct effect) and/or by interfering and changing: the cloud and precipitation formation processes (indirect effect). Based on their optical properties, aerosols can be classified into two types.: those that absorb solar radiation, and those that do not. Both types of aerosols scatter sunlight and reduce the amount of solar radiation from reaching the Earth's surface, causing it to cool. The surface cooling increases atmospheric stability and reduces convection potential, Absorbing aerosols, however, in addition to cooling the surface, can heat the atmosphere. The heating of the atmosphere may reduce the amount of low clouds by increased evaporation in cloud drops. The heating, however, may induce rising motion, enhance low-level moisture, convergence and, hence, increases rainfall, The latent heating from enhanced rainfall may excite feedback processes in the large-scale circulation, further amplify.the initial response to aerosol heating and producing more rain. Additionally, aerosols can increase the concentration of cloud condensation nuclei (CCN), increase cloud amount and decrease coalescence and collision rates, leading to reduced precipitation. However, in the presence of increasing moist and warm air, the reduced coalescence/collision may lead to supercooled drops at higher altitudes where ice precipitation falls and melts. The latent heat release from freezing aloft and melting below implies greater upward heat transport in polluted clouds and invigorate deep convection. In this way, aerosols may lead to increased local convection. Hence, depending on the ambient large-scale conditions and dynamical feedback processes, aerosols' effect on precipitation can be positive, negative or mixed. In the Asian monsoon and adjacent regions, the aerosol forcing and responses of the water cycle are even more complex, Both direct and indirect effects may take place locally and simultaneously, interacting with each other. in addition to local effects, monsoon rainfall may be affected by aerosols transported from other regions and intensified through large-scale circulation and moisture feedback. Thus, dust transported by the large-scale circulation from the adjacent deserts to northern India may affect rainfall over the Bay of Bengal; sulphate and black carbon front industrial pollution in central, southern China and northern India may affect the rainfall regime over the Korean peninsula and Japan; organic and black carbon front biomass burning from Indo-China may modulate the pre-monsoon rainfall regime over southern China and coastal regions, contributing to variability in differential heating and cooling of the atmosphere and to the land-sea thermal contrast. During the pre-monsoon season and monsoon breaks, it has been suggested that radiative forcing by absorbing aerosols have nearly the same order of magnitude as the forcing due to latent heating from convection and surface fluxes. The magnitude of the total aerosol radiative cooling due to sulphates and soot is of the order of 20-40 W/m2 over the Asian monsoon land region in the pre-monsoon season, compared to about 1-2 W/m2 for global warng. However, the combined forcing at the surface and in the atmosphere, including all species. if aerosols, and details of aerosol mixing, and impacts on the energy and water cycles in the monsoon land regions, are not well known.

Lau, William K. M.↗

NASA NTRS1994

A new derivation of the tensile strength of cometary nuclei: Application to comet Shoemaker-Levy 9

The splitting of comets as exemplified by comet Shoemaker-Levy 9, when it passed near Jupiter, is a common phenomenon. Multiple splitting is also not an uncommon occurrence. It is clear that the comet nucleus is fragile, i.e., its tensile strength is small compared with that of solid materials. We show that aggregates of sub-micron interstellar dust particles presumed to consist of a silicate core, an inner mantle of complex organic refractory molecules, and an outer mantle dominated by H2O ice (Greenberg, 1982) provide the basis for a quantitative derivation of the tensile strength of comet SL9 using molecular interactions at the contact interfaces. In fact, using a mean particle size representing interstellar dust as it would appear in its final presolar state one derives a tensile strength which describes remarkably well the multiple splitting phenomenon. This derivation of the tensile strength of a particle aggregate resulting from molecular interactions is quite general and can be applied to physical situations involving any sorts of aggregates as well as those representing comet nuclei.

Greenberg, J. Mayo↗

NASA NTRS1983

Ice in Comet Bowell

Results of observations of the reflected light in the 1-5 micron region of the spectrum from the Comet Bowell are presented as part of the attempt to directly detect the presence of frozen volatiles in the nucleus of a comet. A deep absorption at 3.25 microns is detected in Comet Bowell which is due to the presence of H2O ice. While other volatile ices have absorption features near 3 microns, it is shown that only H2O ice is a plausible identification at the heliocentric distance of Comet Bowell during the observations (3.4 AU) since only H2O grains are stable enough to have produced the observed absorption. The implications of these findings for models of cometary nuclei are examined.

Campins, H.↗

NASA NTRS1980

Laboratory investigations of cloud nuclei from combustion of Space Shuttle propellant

Small quantities of solid rocket motor propellant, of the type to launch the Space Shuttle, were burned at ambient pressure in the laboratory to provide aerosol samples for characterization. A portion of each sample was injected into an isothermal cloud chamber and the remainder into a 770-liter holding tank. Portable ice nucleus (IN) counters, filter devices for IN determinations and a cloud condensation nucleus (CCN) counter sampled from the tank. The measurements show that particles resulting from the combustion of the propellant are active IN (3.3 times 10 to the 8th to 1.5 times 10 to the 11th/g active at 20 C). The portable counters and filters detected significantly fewer IN than the isothermal cloud chamber. The propellant aerosol is a prolific source of CCN that swamped the instrument.

Hindman Ii, E. E.↗

NASA NTRS2001

A Model for the Breakup of Comet Linear (C/1999 S4)

We propose a mechanism based on the rubble-pile hypothesis of the cometary nucleus (Weissman 1986) to explain the catastrophic breakup of comet LINEAR (C/1999 S4) observed during July-August 2000. We suggest that a solid nucleus made up of 10-100 m "cometesimals" (Weidenschilling 1997) contains a network of inter-connected voids in the inter-cometesimal regions. The production of super-volatile (i.e., species more volatile than water) gases into these voids occurs due to the thermal wave propagating through the nucleus and associated phase transitions of water ice. The network of voids provides an efficient pathway for rapid propagation of these gases within the nucleus resulting in gas pressure caused stresses over a wide regime of the nucleus. This provides a mechanism for catastrophic breakups of small cometary nuclei such as comet LINEAR (C/1999 S4) as well as for some observed cometary outbursts including those that occur at large heliocentric distances (e.g., West et al. 1991). We emphasize the importance of techniques such as radar reflection tomography and radiowave transmission tomography (e.g., Kofman et al. 1998) aboard cometary missions to determine the three dimensional structure of the nucleus in particular the extent of large scale voids.

Samarasinha, Nalin H.↗

DOE OSTI2020

Aerosol-Ice Formation Closure Pilot Study (AEROICSTUDY) Field Campaign Report

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2012

Chemical and Hydrodynamical Models of Cometary Comae

Multi-fluid modelling of the outflowing gases which sublimate from cometary nuclei as they approach the Sun is necessary for understanding the important physical and chemical processes occurring in this complex plasma. Coma chemistry models can be employed to interpret observational data and to ultimately determine chemical composition and structure of the nuclear ices and dust. We describe a combined chemical and hydrodynamical model [1] in which differential equations for the chemical abundances and the energy balance are solved as a function of distance from the cometary nucleus. The presence of negative ions (anions) in cometary comae is known from Giotto mass spectrometry of 1P/Halley. The anions O(-), OH(-), C(-), CH(-) and CN(-) have been detected, as well as unidentified anions with masses 22-65 and 85-110 amu [2]. Organic molecular anions such as C4H(-) and C6H(-) are known to have a significant impact on the charge balance of interstellar clouds and circumstellar envelopes and have been shown to act as catalysts for the gas-phase synthesis of larger hydrocarbon molecules in the ISM, but their importance in cometary comae has not yet been fully explored. We present details of new models for the chemistry of cometary comae that include atomic and molecular anions and calculate the impact of these anions on the coma physics and chemistry af the coma.

Charnley, Steven↗

NASA NTRS1989

Cirrus crystal nucleation by homogeneous freezing of solution droplets

A numerical model consisting of a system of differential equations is used to study cirrus crystal nucleation in a rising parcel containing a distribution of cloud condensation nuclei. The evolution of the particle population and the thermodynamic variables in the parcel are examined. The results suggest that, if homogeneous freezing is not considered, liquid water should be detected below -40 C. If homogeneous freezing is considered, the rapid growth of ice crystals and vapor depletion prevent water saturation from being reached. It is shown that the likelihood of a droplet being frozen is increased by lower temperatures, larger droplet diameter, or lower solution density.

Heymsfield, Andrew J.↗