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Bayes goes fast: Uncertainty quantification for a covariant energy density functional emulated by the reduced basis method
A covariant energy density functional is calibrated using a principled Bayesian statistical framework informed by experimental binding energies and charge radii of several magic and semi-magic nuclei. The Bayesian sampling required for the calibration is enabled by the emulation of the high-fidelity model through the implementation of a reduced basis method (RBM)—a set of dimensionality reduction techniques that can speed up demanding calculations involving partial differential equations by several orders of magnitude. The RBM emulator we build—using only 100 evaluations of the high-fidelity model—is able to accurately reproduce the model calculations in tens of milliseconds on a personal computer, an increase in speed of nearly a factor of 3,300 when compared to the original solver. Besides the analysis of the posterior distribution of parameters, we present model calculations for masses and radii with properly estimated uncertainties. We also analyze the model correlation between the slope of the symmetry energy L and the neutron skin of 48 Ca and 208 Pb. The straightforward implementation and outstanding performance of the RBM makes it an ideal tool for assisting the nuclear theory community in providing reliable estimates with properly quantified uncertainties of physical observables. Such uncertainty quantification tools will become essential given the expected abundance of data from the recently inaugurated and future experimental and observational facilities.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Measurement of the 252 Cf (sf) prompt fission neutron spectrum utilizing 12 C (𝑛, 𝑛) and 9 Be (𝑛, 𝑛) neutron scattering reference measurements
The 252 Cf spontaneous fission (sf), prompt fission neutron spectrum (PFNS) is a fundamental quantity for nuclear physics measurements of neutron-emitting reactions. This energy distribution of neutrons emitted from fission has been considered a neutron data standard for decades and has been utilized as a reference for neutron detection efficiency, validation of Monte Carlo simulations, benchmarking of dosimetry standards, and more. A significant portion of the global collection of nuclear data on neutron-induced reactions is correlated with the 252 Cf (sf) PFNS. Despite the reliance on this quantity by the nuclear physics community, the historical collection of 252 Cf PFNS measurements display systematic disagreements that are not understood or easily explained. These experimental discrepancies could potentially bias the 252 Cf PFNS Standard evaluation. On top of this, these past experiments frequently employed correlated experimental measurement or analysis methods. The artificial intelligence (AI)/machine learning (ML)-informed californium chi-nuclear data experiment (AIACHNE) project was formed to (a) investigate these discrepancies utilizing AI/ML methods to identify outlying regions of literature data, assign these regions to features of the experiment itself, and perform an improved evaluation of the 252 Cf PFNS and (b) perform a new experimental measurement of this quantity designed to improve upon the existing literature database. Here, in this work, we report on the AIACHNE 252 Cf PFNS experiment utilizing a new analysis method uncorrelated with all previous measurements: neutron efficiency determinations based on elastic neutron scattering on 12 C and 9 Be . This new method provides an independent test of the existing literature data and evaluation of the 252 Cf (sf) PFNS. The method is described with detailed covariance quantification procedures, as well as a direct discussion of the sources of uncertainty described as requirements in the “Templates” series of papers. The 252 Cf (sf) PFNS reported in this work agrees well with the overall shape of the existing standard PFNS evaluation as well as many literature measurements, thus verifying the current evaluation utilizing new techniques. However, the results suggest that there are deficiencies in the angle-differential 12 C and 9 Be (𝑛, 𝑛) evaluated nuclear data, which produce unphysical structures in the reported result. While these structures are relatively minor, they become obvious because of the high statistical precision of the data and the expected smooth continuity of the 252 Cf (sf) PFNS.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Experimental study for critical heat flux in 2x2 rod bundles at high pressure conditions
Critical heat flux (CHF) phenomena has been a topic of study for over fifty years yet remains a serious concern across industries and especially in water-cooled nuclear reactor design. CHF data in the high-pressure range is limited, and the effects of bundle geometry and non-uniform heat flux profile are challenging to quantify. In this study, CHF experiments were performed in upward flowing water in a 2 × 2 rod bundle with a cosine profile heat flux. Data were collected between 16.5 and 18 MPa at two mass flux conditions with three inlet subcooling conditions. Under these conditions, average CHF was shown to decrease with increasing pressure. However, pressure had less of an effect than decreasing the inlet subcooling or the mass flux, both of which reduce the CHF value considerably. Of interest, correlations that have been developed for lower pressure continued to predict CHF occurrences with moderate accuracy outside their ranges of validity. Nearly all predicted values were within 20% of experimental values.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Electroweak nuclear radii constrain the isospin breaking correction to V ud
We lay out a novel formalism to connect the isospin-symmetry breaking correction to the rates of superallowed nuclear beta decays, δ C , to the isospin-breaking sensitive combinations of electroweak nuclear radii that can be accessed experimentally. We individuate transitions in the superallowed decay chart where a measurement of the neutron skin of a stable daughter even at a moderate precision could already help discriminating between models used to compute δ C . We review the existing experimental situation and make connection to the existing and future experimental programs.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Accurate temperature diagnostics for matter under extreme conditions
The experimental investigation of matter under extreme densities and temperatures, as in astrophysical objects and nuclear fusion applications, constitutes one of the most active frontiers at the interface of material science, plasma physics, and engineering. The central obstacle is given by the rigorous interpretation of the experimental results, as even the diagnosis of basic parameters like the temperature T is rendered difficult at these extreme conditions. Here, we present a simple, approximation-free method to extract the temperature of arbitrarily complex materials in thermal equilibrium from X-ray Thomson scattering experiments, without the need for any simulations or an explicit deconvolution. Our paradigm can be readily implemented at modern facilities and corresponding experiments will have a profound impact on our understanding of warm dense matter and beyond, and open up a variety of appealing possibilities in the context of thermonuclear fusion, laboratory astrophysics, and related disciplines.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
The impact of 17O + α reaction rate uncertainties on the s-process in rotating massive stars
ABSTRACT Massive stars are crucial to galactic chemical evolution for elements heavier than iron. Their contribution at early times in the evolution of the Universe, however, is unclear due to poorly constrained nuclear reaction rates. The competing 17O(α, γ)21Ne and 17O(α, n)20Ne reactions strongly impact weak s-process yields from rotating massive stars at low metallicities. Abundant 16O absorbs neutrons, removing flux from the s-process, and producing 17O. The 17O(α, n)20Ne reaction releases neutrons, allowing continued s-process nucleosynthesis, if the 17O(α, γ)21Ne reaction is sufficiently weak. While published rates are available, they are based on limited indirect experimental data for the relevant temperatures and, more importantly, no uncertainties are provided. The available nuclear physics has been evaluated, and combined with data from a new study of astrophysically relevant 21Ne states using the 20Ne(d, p)21Ne reaction. Constraints are placed on the ratio of the (α, n)/(α, γ) reaction rates with uncertainties on the rates provided for the first time. The new rates favour the (α, n) reaction and suggest that the weak s-process in rotating low-metallicity stars is likely to continue up to barium and, within the computed uncertainties, even to lead.
79 ASTRONOMY AND ASTROPHYSICS↗
Noniterative finite amplitude methods for E 1 and M 1 giant resonances
The finite amplitude method (FAM) is a very efficient approach for solving the fully self-consistent random-phase approximation (RPA) equations. We use FAM to rederive the RPA matrices for Skyrme functionals, calculate the electric dipole ( E 1) and the magnetic dipole ( M 1) giant resonances, and compare the results with available experimental and evaluated data. For the E 1 transitions in heavy nuclei, the calculations reproduce well the resonance energy of the photoabsorption cross sections. In the case of M 1 transitions, we show that the residual interaction does not affect the transition strength of double-magic nuclei, which suggests that the spin terms in the Skyrme force currently neglected in the present computation could improve the agreement between FAM and experimental data.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Towards Resilient Near Real-Time Analysis Workflows in Fusion Energy Science
Nuclear fusion holds the promise of an endless source of energy. Several research experiments across the world and joint modeling and simulation efforts between the nuclear physics and high performance computing communities are actively preparing the operation of the International Thermonuclear Experimental Reactor (ITER). Both experimental reactors and their simulated counterparts generate data that must be analyzed quickly and in a resilient way to support decision making for the configuration of subsequent runs or prevent a catastrophic failure. However, the cost if the traditional techniques used to improve the resilience of analysis workflows, i.e., replicating datasets and computational tasks, becomes prohibitive with explosion of the volume of data produced by modern instruments and simulations. Therefore, we advocate in this paper for an alternate approach based on data reduction and data streaming. The rationale is that by allowing for a reasonable, controlled, and guaranteed loss of accuracy it becomes possible to transfer smaller amounts of data, shorten the execution time of analysis workflows, and lower the cost of replication to increase resilience. We develop our research and development roadmap towards resilient near real-time analysis workflows in fusion energy science and present early results showing that data streaming and data reduction is a promising way to speed up the execution and improve the resilience of analysis workflows.
Suter, Fred↗
Physics and Chemistry of Te and HgTe-based Ternary Melts
Historically, the theoretical treatment of the liquid phases has always been more difficult and complicated than that for solid and gas phases. A liquid has no lattice structure as crystalline solids and the atoms/molecules in the liquid can migrate through it relatively rapidly. On the other hand, it is also interacting with many other atoms/molecules so that the simplifications of the kinetic theory of gases cannot be employed. For more complicated liquids, such as the liquids of high ionicity and those containing hydrogen bonds and electric dipoles, the understanding is far from complete. At the same time, accurate information on the physics and chemistry of semiconductor melts is needed for the quantitative descriptions of the process of crystal growth from melt. The pre-crystallization phenomena in the liquid phase are critical because the properties of the grown crystals depend on the state and structure of the melt as well as the thermal history of the melt during solidification process. However, the data on the liquid phase, such as thermophysical properties of semiconductor melts are scarce, especially for the HgTe-based II-VI ternary compound semiconductors because of their high vapor pressure and extreme toxicity. Analysis of the thermophysical properties of the melt can provide information about structural transitions of the melt during the solidification process. From a broader point of view, the structure of liquids is much more complicated than the crystalline solids, especially the relaxation behavior through different thermal histories. The theory of hetero-phase fluctuations of liquids is applicable to any many-body systems including condensed-matter physics, field theory, physics of nuclear-matter, cosmology, biology and even sociology. This book summarizes the physics and chemistry from the experimental measurements and theoretical analyses of phase diagram, thermodynamic properties, density, thermal conductivity, viscosity, and electrical conductivity on the binary, pseudo-binary and ternary melts of the most advanced IR-detector material systems of HgCdTe and HgZnTe as well as the analyses of these results. The main objectives of this study are: (1) to provide the phase diagrams and thermodynamic properties of Hg-Cd-Te and Hg-Zn-Te systems through quantitatively fitting the experimental data by assuming an associated solution model for the liquid phase, (2) to experimentally measure the thermophysical properties of the Hg-Cd-Te and Hg-Zn-Te melts, including density, viscosity, electrical conductivity and thermal conductivity as functions of temperature and composition and (3) to enhance the fundamental knowledge of hetero-phase fluctuations and relaxation phenomena in the melts and extend our understanding of the solidification process in order to interpret the experimental results of crystal growth so as to improve the melt growth processes of the compound semiconductor. The physics and chemistry of Te and HgTe-based ternary melts were explored through the studies of the structural transformation during melting, the supercooling during solidification, the relaxation phenomena after rapid cooling of the melts and the metal-semiconductor transition in the melts through the analyses of electrical conductivity and Lorenz number. An in-depth study on the thermophysical properties and their time-dependent structural dynamic processes taking place in the vicinity of the solid-liquid phase transition of the narrow homogeneity range HgTe-based ternary semiconductors as well as the analysis of the homogenization process in the melt will also be presented.
Thermophysical properties↗
The FLUKA code for space applications: recent developments
The FLUKA Monte Carlo transport code is widely used for fundamental research, radioprotection and dosimetry, hybrid nuclear energy system and cosmic ray calculations. The validity of its physical models has been benchmarked against a variety of experimental data over a wide range of energies, ranging from accelerator data to cosmic ray showers in the earth atmosphere. The code is presently undergoing several developments in order to better fit the needs of space applications. The generation of particle spectra according to up-to-date cosmic ray data as well as the effect of the solar and geomagnetic modulation have been implemented and already successfully applied to a variety of problems. The implementation of suitable models for heavy ion nuclear interactions has reached an operational stage. At medium/high energy FLUKA is using the DPMJET model. The major task of incorporating heavy ion interactions from a few GeV/n down to the threshold for inelastic collisions is also progressing and promising results have been obtained using a modified version of the RQMD-2.4 code. This interim solution is now fully operational, while waiting for the development of new models based on the FLUKA hadron-nucleus interaction code, a newly developed QMD code, and the implementation of the Boltzmann master equation theory for low energy ion interactions. c2004 COSPAR. Published by Elsevier Ltd. All rights reserved.
Non-NASA Center↗
California Bridge to the Electron-Ion Collider (EIC) (Final Technical Report)
This report summarizes the activities and outcomes of DOE Grant DE-SC0022358, a traineeship program designed to prepare students for future nuclear physics research at the Electron-Ion Collider. The project leveraged the California EIC Consortium and statewide academic networks to provide immersive research experiences spanning universities and national laboratories. Participants engaged in theoretical, computational, and experimental research related to EIC physics and took part in professional meetings and collaborative research activities. The program supported student preparation for advanced study and research careers in nuclear physics.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
First Measurement of Differential Charged Current Quasielastic-like $\nu_\mu$–Argon Scattering Cross Sections In Kinematic Imbalance Variables With The MicroBooNE Detector
We report the first measurement of flux-integrated multi-differential cross sections for charged-current events with muon neutrinos scattering on argon with solely a muon and a single proton in the final state as a function of kinematic imbalance variables. The measurement was carried out using the Booster Neutrino Beam at Fermi National Accelerator Laboratory within the MicroBooNE Liquid Argon Time Projection Chamber detector with an exposure of 6.79 × 10 20 protons on target. Events were selected to enhance the contribution of charged-current mesonless interactions with one proton detected in the final state. The data discussed here are reported in terms of multidifferential cross sections in kinematic imbalance variables, which are generally sensitive to nuclear effects. The double-differential results in these variables can provide an excellent handle to disentagle specific nuclear aspects not easily isolated via single differential cross sections. Our results pave a path towards identifying regions of the phase-space where future interaction modeling development and Monte Carlo neutrino generator tuning efforts should concentrate. EVENT SELECTION Neutrino oscillation measurements aim to extract neutrino mixing angles, mass differences, the value of the chargeparity violating phase in the lepton sector, and to search for new physics beyond the Standard Model [1, 2]. For that to be achieved, an unprecedented understanding of neutrino-argon interactions is of utmost importance since a growing number of neutrino oscillation experiments employ Liquid Argon Time Projector Chamber (LArTPC) neutrino detectors [3–6]. The accuracy to which these experiments can extract neutrino oscillation parameters requires a good understanding of the neutrino energy. Experimentally, this energy is deduced from the measured kinetic energies of particles that are emitted following the neutrino interaction in the detector. The kinematic properties of such finalstate particles reflect complex dynamics due to nuclear and initial-state effects of the interaction [7]. However, certain categories of nuclear effects can be isolated by variables built specifically to characterize the degeneracy between such effects [8–10]. This note reports cross sections in kinematic variables sensitive to nuclear effects using events with one detected muon with momentum 0.1 < pµ < 1.2 GeV/c, and exactly one proton with 0.3 < pp < 1 GeV/c. This signal definition includes events with any number of protons below 300 MeV/c, neutrons at any momenta, and charged pions with momentum lower than 70 MeV/c. This choice is guided by the fact that their experimental signature of correlated muon-proton pairs is fairly straightforward to reconstruct [11–22]. Such events primarily originate from chargedcurrent (CC) neutrino-nucleon quasielastic (QE) scattering interactions where the neutrino removes a single intact nucleon from the nucleus without producing any additional particles. This definition can also include contributions from interactions that lead to the production of additional particles that are absent from the final state due to nuclear effects, such as pion absorption, or have momenta that are below the experimental detection threshold.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Charged Lepton Flavour Violations searches with muons: present and future
Charged-lepton flavor violation (cLFV) is one of the most powerful probes for New Physics (NP). Since lepton flavor conservation is an accidental symmetry in the Standard Model (SM), it is naturally violated in many NP models, with contributions at the level of the current experimental sensitivities. Moreover, the negligible SM contributions would make the observation of cLFV unambiguous evidence of NP. It makes these searches extremely sensitive and, at the same time, extremely pure. Thanks to the intense muon beams currently available, their intriguing upgrade programs, and the progress in the detection techniques, cLFV muon processes are the golden channels in this field. Experimental programs to search for $\mu^+ \to e^+ \gamma$, $\mu^+ \to e^+ e^+ e^-$ and the $\mu \to e$ conversion in the nuclear field are currently ongoing. We review the current status and the strategic plans for future searches. This document is an update of the prior cLFV submission to the 2018 European Strategy for Particle Physics (ESPP); the earlier submission should be consulted for more experimental details.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Initial Delayed Critical Configuration of SHEBA I and Subcritical Measurements by Californium Source-Driven Noise Analysis
In September 1980, the initial delayed critical configuration of the Solution High-Energy Burst Assembly (SHEBA I) was assembled, and the US Department of Energy’s Oak Ridge National Laboratory (ORNL) staff performed near critical and subcritical measurements using the californium source-driven noise analysis (CSDNA) method at the Los Alamos National Laboratory (LANL) Critical Experiments Facility. An unreflected 56 cm outside diameter stainless-steel cylindrical tank was partially filled with uranyl fluoride solution (235U enrichment was 4.95 wt %) until delayed criticality was achieved. Then, measurements were performed for various fuel solution heights from delayed critical to 60% of the height required for delayed criticality. The stainless-steel tank had an inside diameter of 54.6 cm and a height of 105 cm and was partially (20–36.5 cm) filled with an aqueous solution of uranyl fluoride (with a density of 2.162 g/cm 3 ). The density of the uranium in solution was 1.042 g/cm 3 , and the solution had a H/U atomic ratio of 20.43. The tank had a 6.35 mm wall thickness and an axial reentrant tube with an inside diameter of 6.02 cm and wall thickness of 0.165 cm. The tank was essentially unreflected on the top and sides because it was in a thin metal shed. The reactivity of the near–delayed critical configuration was −10.4 cents, which corresponds to a k eff value of 0.99922. In addition to the CSDNA measurements, the prompt neutron decay constants were determined from break frequency noise analysis (BNFA) measurements. The subcritical neutron multiplication factors from CSDNA and BFNA compared extremely well. These data can be used as the basis of International Nuclear Criticality Safety Evaluation benchmark for the near-critical configuration, and the k eff values at various subcritical configurations can be used as subcritical benchmarks. Furthermore, the measured prompt neutron decay constants can be used as reactor physics benchmarks. This report documents the experimental information for the measurements performed so that, at a later date, researchers could perform the required uncertainty and calculational analyses and documentation to use these data for an International Criticality Safety Benchmark Evaluation Program (ICSBEP) or Nuclear Energy Agency benchmarks. The measured prompt neutron decay constants can be used as the basis of a benchmark for the International Reactor Physics Evaluation Program (IRPhEP). The data from these measurements are available from the ORNL Records Management Services Department, and the logbook is available from ICSBEP at Idaho National Laboratory.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Many-body Nuclear Dynamics
The principal goal of this work was to better understand the fusion of neutron-rich nuclei a topic relevant to the fields of both nuclear physics and nuclear astrophysics. The work provides insight into the structure and reactions of neutron-rich nuclei namely the extent of their neutron density distribution and its polarizability. By comparing the fusion excitation functions for a chain of isotopes with a common target nucleus changes in the attractive nuclear potential are assessed. This change in the attractive potential is related to changes in the neutron density distribution with increasing number of neutrons or changes in fusion dynamics with increasing neutron number. The impact of the pairing of valence neutrons and protons on the fusion cross-section is also examined. Measurement of an isotopic chain is a powerful tool to address this topic. The experimental program made use of several different accelerator facilities. The core of the experimental work involved experiments at the ReA3 accelerator and the Facility for Rare Isotope Beams (FRIB) situated at Michigan State University, at GANIL, the French national nuclear physics laboratory, and the University of Notre Dame. At ReA3 the degree to which α-clusters associated with fusion of 28,30,32 Si + 28 Si result from the collision dynamics or reflect an initial α-cluster structure was explored. Alpha clusters observed in fusion reactions exceed the predictions of the standard statistical model. This experiment provides a measure of how clusterization is impacted by the increasing neutron-richess of the system. In the experiment at GANIL we investigated fusion in 19 O + 12 C and 20 O + 12 C. This experiment utilized the recently developed active-target detector MuSIC@Indiana. Using this proven, highly efficient, active-target detector we measured the fusion excitation function for these neutron-rich systems. Grounded by these experimental measurements, theoretical models were used to examine the role of unpaired valence neutrons on the fusion cross-section at energies just above the fusion barrier.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Pump depletion in Raman lasing in a graded index multimode fibre
We examine multimode diode laser pump depletion in a graded index multimode (MM) fibre Raman laser generating a high-quality Stokes beam. Spatial ‘hole burning’ in the transmitted pump beam is demonstrated. A balance model is constructed for interaction of the pump and Stokes waves in the MM Raman laser. Analytical formulas are derived and used in calculations demonstrating qualitative agreement with experimental data. The origin of the observed quantitative discrepancies is discussed. (paper)
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Beam Stability Overview [Slides]
Radiographic spot size is affected by many factors, including beam motion due to instabilities. Instabilities and effects that can influence the radiation-source spot size are being evaluated for the Scorpius flash-radiography accelerator. The Scorpius LIA design has a direct influence on beam stability. Many features of the design were specifically incorporated to mitigate instability. The major beam dynamics concerns for high-current LIAs are being evaluated for the long, 102-cell Scorpius design. For these results, all tools available were used including experimental data, analytic theory, and physics simulation codes.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗