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DOE OSTI2025

A Comparative Study of Cloud Properties Between Northern and Southern High Latitudes Based on ARM Observations and EAMv2 Simulations

Earth's high-latitude regions show a considerable amount of cloud coverage, which significantly affects global radiation budgets. Here, in this study, we examine ground- and ship-based remote sensing observations from two Atmospheric Radiation Measurement (ARM) field campaigns conducted in the high-latitude regions of Northern and Southern Hemispheres (NH and SH). A comparison of macrophysical properties for low, mid-level, high, and deep clouds shows that the cloud top heights and thickness values are higher in the Arctic for each cloud type compared with the Southern Ocean and Antarctic regions, possibly due to higher sea surface temperatures in the north Atlantic. The Arctic also shows lower ice phase occurrence frequencies compared with the SH high latitudes for low clouds. For high, mid-level and deep clouds, the cloud phase distributions as a function of temperature show small geographical variabilities. The observations are then compared with the Department of Energy (DOE) Energy Exascale Earth System Model (E3SM) to evaluate the representations of these cloud properties. Here, the results show that the model captures cloud base and top heights well and reproduces the differences in cloud macrophysical properties between the two hemispheres. But the model underestimates ice phase frequencies for all cloud types. Such model cloud phase bias is strongly correlated with positive relative humidity biases and negative aerosol number concentration biases, indicating an important role of relative humidity and aerosols in modulating cloud phase partitioning in the model.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Insights on sources and formation mechanisms of liquid-bearing clouds over MOSAiC examined from a Lagrangian framework

Understanding Arctic stratiform liquid-bearing cloud life cycles and properly representing these life cycles in models is crucial for evaluations of cloud feedbacks as well as the faithfulness of climate projections for this rapidly warming region. Examination of cloud life cycles typically requires analyses of cloud evolution and origins on short time scales, on the order of hours to several days. Measurements from the recent Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition provide a unique view of the current state of the central Arctic over an annual cycle. Here, we use the MOSAiC radiosonde measurements to detect liquid-bearing cloud layers over full atmospheric columns and to examine the cloud-generating air masses’ properties. We perform 5-day (120 h) back-trajectory calculations for every detected cloud and cluster them using a unique set of variables extracted from these trajectories informed by ERA5 reanalysis data. This clustering method enables us to separate between the air mass source regions such as ice-covered Arctic and midlatitude open water. We find that moisture intrusions into the central Arctic typically result in multilayer liquid-bearing cloud structures and that more than half of multilayer profiles include overlying liquid-bearing clouds originating in different types of air masses. Finally, we conclude that Arctic cloud formation via prolonged radiative cooling of elevated stable subsaturated air masses circulating over the Arctic can occur frequently (up to 20% of detected clouds in the sounding data set) and may lead to a significant impact of ensuing clouds on the surface energy budget, including net surface warming in some cases.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

Regime-specific Cloud Vertical Overlap Characteristics from Radar and Lidar Observations at the ARM sites

Climate and numerical weather prediction models require assumptions to represent the vertical distribution of subgrid-scale clouds, which have radiative transfer implications. In this study, nearly 25 years of ground-based radar and lidar observations of vertical cloud profiles at the Atmospheric Radiation Measurement Program (ARM) Southern Great Plains (SGP) site are utilized to derive cloud vertical overlap characteristics from the Cloud Type (CLDTYPE) data product. Here, the cloud vertical overlap characteristics are further separated by cloud regime by considering seven cloud types (i.e., low cloud, congestus, deep convection, altocumulus, altostratus, cirrostratus, and cirrus) as well as periods of shallow cumulus. The decorrelation length scale (i.e., exponential transition from maximum to random overlap with layer separation) is found to vary by cloud regime, ranging between 0.04 km for cirrostratus paired with cirrus to 4.58 km for low cloud paired with cirrus at SGP. Cloud vertical overlap characteristics are also considered for other ARM sites including the Tropical Western Pacific (TWP), North Slope of Alaska (NSA), and Eastern North Atlantic (ENA) sites amongst other shorter term ARM deployments globally. The decorrelation length scale ranged globally from 1.03 km in the Arctic Ocean to 3.06 km in Manacapuru, Brazil. Globally, the decorrelation length scale by cloud regime exhibited similarities (e.g., for cirrus paired with cirrus) and differences (e.g., congestus paired with cirrus). The results could help inform development of cloud vertical overlap assumptions within operational numerical weather prediction models and potentially improve prediction of radiative fluxes for weather, climate, and renewable energy forecasting.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Evaluating Cloud Properties at Scott Base: Comparing Ceilometer Observations With ERA5, JRA55, and MERRA2 Reanalyses Using an Instrument Simulator

This study compares CL51 ceilometer observations made at Scott Base, Antarctica, with statistics from the ERA5, JRA55, and MERRA2 reanalyses. To enhance the comparison we use a lidar instrument simulator to derive cloud statistics from the reanalyses which account for instrumental factors. The cloud occurrence in the three reanalyses is slightly overestimated above 3 km, but displays a larger underestimation below 3 km relative to observations. Unlike previous studies, we see no relationship between relative humidity and cloud occurrence biases, suggesting that the cloud biases do not result from the representation of moisture. We also show that the seasonal variation of cloud occurrence and cloud fraction, defined as the vertically integrated cloud occurrence, are small in both the observations and the reanalyses. We also examine the quality of the cloud representation for a set of weather states derived from ERA5 surface winds. The variability associated with grouping cloud occurrence based on weather state is much larger than the seasonal variation, highlighting weather state is a strong control of cloud occurrence. All the reanalyses continue to display underestimates below 3 km and overestimates above 3 km for each weather state. But the variability in ERA5 statistics matches the changes in the observations better than the other reanalyses. We also use a machine learning scheme to estimate the quantity of supercooled liquid water cloud from the ceilometer observations. Ceilometer low-level supercooled liquid water cloud occurrences are considerably larger than values derived from the reanalyses, further highlighting the poor representation of low-level clouds in the reanalyses.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Ship‐Based Lidar Evaluation of Southern Ocean Low Clouds in the Storm‐Resolving General Circulation Model ICON and the ERA5 and MERRA‐2 Reanalyses

Global storm resolving models (GSRMs) represent the next generation of global climate models. One of them is a 5-km Icosahedral Nonhydrostatic Weather and Climate Model (ICON). Its high resolution means that parameterizations of convection and clouds, including subgrid-scale clouds, are omitted, relying on explicit simulation but necessarily utilizing microphysics and turbulence parameterizations. Standard-resolution (10–100 km) models, which use convection and cloud parameterizations, have substantial cloud biases over the Southern Ocean (SO), adversely affecting radiation and sea surface temperature. The SO is dominated by low clouds, which cannot be observed accurately from space due to overlapping clouds, attenuation, and ground clutter. We evaluated SO clouds in ICON and the ERA5 and MERRA-2 reanalyzes using approximately 2400 days of lidar observations and 2300 radiosonde profiles from 31 voyages and a Macquarie Island station during 2010–2021, compared to the model and reanalyzes using a ground-based lidar simulator. We found that ICON and the reanalyzes underestimate the total cloud fraction by about 10% and 20%, respectively. ICON and ERA5 overestimate the cloud occurrence peak at about 500 m, associated with underestimated lower tropospheric stability and overestimated lifting condensation level. The reanalyzes strongly underestimate fog and very low-level clouds, and MERRA-2 underestimates cloud occurrence at almost all heights. Outgoing shortwave radiation is overestimated in MERRA-2, implying a “too few, too bright” cloud problem. SO cloud and fog biases are a substantial issue in the analyzed model and reanalyzes and result in shortwave and longwave radiation biases.

Kuma, Peter [Stockholm Univ. (Sweden); Univ. of Ca↗

DOE OSTI2025

Downward Convective Moisture Transport Dominated by a Few Overshooting Clouds in Marine and Continental Shallow Convection

Abstract In a previous study (Xiao et al., 2023, https://doi.org/10.1029/2022ms003526 ), we found that ignoring the moist convective downdrafts associated with overshooting clouds in parameterizations can lead to significant biases in the simulated depth and liquid water content of a shallow cloud layer. In this study, we seek to better quantify the properties of the clouds responsible for these moist downdrafts to help improve shallow convection parameterizations. We apply a 3‐D cloud‐tracking algorithm to large‐eddy simulations (LESs) of marine and continental shallow convection. We find that top 1% and 2% of the tracked cloud population ranked by lifetime‐mean cloud‐base mass flux can explain 90%–95% of the total downward moisture transport in the upper cloud layer whereas top 10%–20% is required to explain 90%–95% of the total upward moisture transport near mean cloud base. The vertical structure of the clouds in the top 1% and 2% (the overshooting “deep mode”) is also distinctively different from that of the rest of the cloud population (the “shallow mode”). Shallow convection parameterizations need to capture accurately the properties and convective transports of the clouds in both the deep and shallow modes. To do that, our results suggest that mass‐flux parameterizations need to (a) accurately predict the size and number of the deep‐mode clouds and (b) explicitly represent overshooting cloud updrafts and associated moist downdrafts.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation

Abstract. The Weather Research Forecasting (WRF) version 4.3 model is configured within a Lagrangian framework to quantify the impact of aerosols on evolving cloud fields. Kilometer-scale simulations utilizing meteorological boundary conditions are based on 10 case study days offering diverse meteorology during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA). Measurements from aircraft, the ground-based Atmosphere Radiation Measurement (ARM) site at Graciosa Island in the Azores, and A-Train and geostationary satellites are utilized for validation, demonstrating good agreement with the WRF-simulated cloud and aerosol properties. Higher aerosol concentration leads to suppressed drizzle and increased cloud water content in all case study days. These changes lead to larger radiative cooling rates at cloud top, enhanced vertical velocity variance, and increased vertical and horizontal wind speed near the base of the lower-tropospheric inversion. As a result, marine cloud cell area expands, narrowing the gap between shallow clouds and increasing cloud optical thickness, liquid water content, and the top-of-atmosphere outgoing shortwave flux. While similar aerosol effects are observed in lightly to non-raining clouds, they tend to be smaller by comparison. These simulations show a relationship between cloud cell area expansion and the radiative adjustments caused by liquid water path and cloud fraction changes. The adjustments are positive and scale as 74 % and 51 %, respectively, relative to the Twomey effect. While higher-resolution large-eddy simulations may provide improved representation of cloud-top mixing processes, these results emphasize the importance of addressing mesoscale cloud-state transitions in the quantification of aerosol radiative forcing that cannot be attained from traditional climate models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Comparison of scattering ratio profiles retrieved from ALADIN/Aeolus and CALIOP/CALIPSO observations and preliminary estimates of cloud fraction profiles

The space-borne active sounders have been contributing invaluable vertically resolved information of atmospheric optical properties since the launch of Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) in 2006. To build long-term records from space-borne lidars useful for climate studies, one has to understand the differences between successive space lidars operating at different wavelengths, flying on different orbits, and using different viewing geometries, receiving paths, and detectors. In this article, we compare the results of Atmospheric Laser Doppler INstrument (ALADIN) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) lidars for the period from 28 June to 31 December 2019. First, we build a dataset of ALADIN–CALIOP collocated profiles (Δdist<1°; Δtime<6 h). Then we convert ALADIN's 355 nm particulate backscatter and extinction profiles into the scattering ratio vertical profiles SR(z) at 532 nm using molecular density profiles from Goddard Earth Observing System Data Assimilation System, version 5 (GEOS-5 DAS). And finally, we build the CALIOP and ALADIN globally gridded cloud fraction profiles CF(z) by applying the same cloud detection threshold to the SR(z) profiles of both lidars at the same spatial resolution. Before comparing the SR(z) and CF(z) profiles retrieved from the two analyzed lidar missions, we performed a numerical experiment to estimate the best achievable cloud detection agreement CDA norm (z) considering the differences between the instruments. We define CDA norm (z) in each latitude–altitude bin as the occurrence frequency of cloud layers detected by both lidars, divided by a cloud fraction value for the same latitude–altitude bin. We simulated the SR(z) and CF(z) profiles that would be observed by these two lidars if they were flying over the same atmosphere predicted by a global model. By analyzing these simulations, we show that the theoretical limit for CDA$_{norm}^{theor}$(z) for a combination of ALADIN and CALIOP instruments is equal to 0.81±0.07 at all altitudes. In other words, 19 % of the clouds cannot be detected simultaneously by two instruments due to said differences. The analyses of the actual observed CALIOP–ALADIN collocated dataset containing ~78 000 pairs of nighttime SR(z) profiles revealed the following points: (a) the values of SR(z) agree well up to ~3 km height. (b) The CF(z) profiles show agreement below ~3 km, where ~80 % of the clouds detected by CALIOP are detected by ALADIN as expected from the numerical experiment. (c) Above this height, the CDA$_{norm}^{obs}$(z) reduces to ~50 %. (d) On average, better sensitivity to lower clouds skews ALADIN's cloud peak height in pairs of ALADIN–CALIOP profiles by ~0.5±0.6 km downwards, but this effect does not alter the heights of polar stratospheric clouds and high tropical clouds thanks to their strong backscatter signals. (e) The temporal evolution of the observed CDA$_{norm}^{obs}$(z) does not reveal any statistically significant change during the considered period. This indicates that the instrument-related issues in ALADIN L0/L1 have been mitigated, at least down to the uncertainties of the following CDA$_{norm}^{obs}$(z) values: 68±12 %, 55±14 %, 34±14 %, 39±13 %, and 42±14 % estimated at 0.75, 2.25, 6.75, 8.75, and 10.25 km, respectively.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Composited structure of non-precipitating shallow cumulus clouds

The normalized distributions of thermodynamic and dynamical variables both within and outside shallow clouds are investigated through a composite algorithm using large-eddy simulations of oceanic and continental cases. The normalized magnitude is maximum near the cloud centre and decreases outwards. While relative humidity (RH) and cloud liquid water ( q l ) decrease smoothly to match the environment, the vertical velocity, virtual potential temperature (θ v ), and potential temperature (θ) perturbations have more complicated behaviour towards the cloud boundary. Below the inversion layer, θ' v becomes negative before the vertical velocity has turned from an updraft to a subsiding shell outside the cloud, indicating the presence of a transition zone where the updraft is negatively buoyant. Due to the downdraft outside the cloud and enhanced horizontal turbulent mixing across the edge, the normalized turbulent kinetic energy (TKE) and horizontal turbulent kinetic energy (HTKE) decrease more slowly from the cloud centre outwards than the thermodynamic variables. The distributions all present asymmetric structures in response to the vertical wind shear, with more negatively buoyant air, stronger downdrafts, and larger TKE on the downshear side. We discuss several implications of the distributions for theoretical models and parameterizations. Positive buoyancy near the cloud base is mostly due to the virtual effect of water vapour, emphasizing the role of moisture in triggering. The mean vertical velocity is found to be approximately half the maximum vertical velocity within each cloud, providing a constraint to achieve possible power-law distributions for some models. Finally, the normalized distributions for different variables are used to estimate the vertical heat and moisture fluxes within clouds. The results suggest that distributions near the cloud edge and variability of maximum perturbations need careful treatment. The fluxes are underestimated in the inversion layer because cloud-top downdrafts cannot be captured well.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Seasonal Cycle of Idealized Polar Clouds: Large Eddy Simulations Driven by a GCM

The uncertainty in polar cloud feedbacks calls for process understanding of the cloud response to climate warming. As an initial step toward improved process understanding, we investigate the seasonal cycle of polar clouds in the current climate by adopting a novel modeling framework using large eddy simulations (LES), which explicitly resolve cloud dynamics. Resolved horizontal and vertical advection of heat and moisture from an idealized GCM are prescribed as forcing in the LES. The LES are also forced with prescribed sea ice thickness, but surface temperature, atmospheric temperature, and moisture evolve freely without nudging. A semigray radiative transfer scheme without water vapor and cloud feedbacks allows the GCM and LES to achieve closed energy budgets more easily than would be possible with more complex schemes. This enables the mean states in the two models to be consistently compared, without the added complications from interaction with more comprehensive radiation. Furthermore, we show that the LES closely follow the GCM seasonal cycle, and the seasonal cycle of low-level clouds in the LES resembles observations: maximum cloud liquid occurs in late summer and early autumn, and winter clouds are dominated by ice in the upper troposphere. Large-scale advection of moisture provides the main source of water vapor for the liquid-containing clouds in summer, while a temperature advection peak in winter makes the atmosphere relatively dry and reduces cloud condensate. The framework we develop and employ can be used broadly for studying cloud processes and the response of polar clouds to climate warming.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Stratus and Stratocumulus Cloud Microphysics and Drizzle Relationships With CCN Modality

High resolution extended-range cloud condensation nuclei (CCN) spectral comparisons with cloud microphysics and drizzle of the Physics of Stratocumulus Tops (POST) field experiment confirmed results in the Marine Stratus/Stratocumulus Experiment (MASE). Both of these stratus cloud projects demonstrated that bimodal CCN spectra typically caused by cloud processing were associated with clouds that exhibited higher concentrations of smaller droplets with narrower distributions and less drizzle than clouds associated with unimodal CCN spectra. Resulting brighter clouds and increased cloudiness could enhance both indirect aerosol effects (IAE). These stratus findings are opposite of analogous measurements in two cumulus cloud projects, which showed bimodal CCN associated with fewer larger droplets more broadly distributed and with more drizzle than clouds associated with unimodal CCN. Resulting reduced cumulus brightness and cloudiness could reduce both IAE. Physics of Stratocumulus Tops (POST) flights in air masses with higher CCN concentrations, N CCN , showed more extremes of the stratus characteristics. However, POST flights with lower N CCN showed opposite droplet characteristics similar to the cumulus clouds, yet still showed less drizzle in clouds associated with bimodal CCN, but not as much less as the flights with higher N CCN . Since all MASE clouds were in polluted air masses, while the two cumulus projects were in clean air masses we deduce from these four projects that both the dynamic stratus/cumulus differences (vertical wind) and N CCN are responsible for the microphysics and drizzle differences among these projects. This is because the clean POST characteristics are a hybrid between MASE/POST high N CCN and the two cumulus projects.

bimodality↗

DOE OSTI2025

Marine Boundary Layer Cloud Boundaries and Phase Estimation Using Airborne Radar and In Situ Measurements During the SOCRATES Campaign over Southern Ocean

The Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) was an aircraft-based campaign (15 January–26 February 2018) that deployed in situ probes and remote sensors to investigate low-level clouds over the Southern Ocean (SO). A novel methodology was developed to identify cloud boundaries and classify cloud phases in single-layer, low-level marine boundary layer (MBL) clouds below 3 km using the HIAPER Cloud Radar (HCR) and in situ measurements. The cloud base and top heights derived from HCR reflectivity, Doppler velocity, and spectrum width measurements agreed well with corresponding lidar-based and in situ estimates of cloud boundaries, with mean differences below 100 m. A liquid water content–reflectivity (LWC-Z) relationship, LWC = 0.70Z0.29, was derived to retrieve the LWC and liquid water path (LWP) from HCR profiles. The cloud phase was classified using HCR measurements, temperature, and LWP, yielding 40.6% liquid, 18.3% mixed-phase, and 5.1% ice samples, along with drizzle (29.1%), rain (3.2%), and snow (3.7%) for drizzling cloud cases. The classification algorithm demonstrates good consistency with established methods. This study provides a framework for the boundary and phase detection of MBL clouds, offering insights into SO cloud microphysics and supporting future efforts in satellite retrievals and climate model evaluation.

MBL clouds over Southern Ocean↗

DOE OSTI2026

Response of marine post-frontal clouds to Gulf Stream variability

Understanding how Gulf Stream variation influences cloud morphology is critical for evaluating cloud feedback in the western North Atlantic Ocean and beyond, where mesoscale air-sea interactions dominate. This study investigates the impact of altered mean sea surface temperature (SST) and SST gradients on post-frontal cloud characteristics during cold-air outbreaks, using the Weather Research and Forecasting (WRF) model. Three sensitivity experiments are conducted: a control simulation (default SST), Plus4 (uniform SST increase of 4 K), and Gradplus (SST gradient enhanced by 25 %, centered around mean SST). Results reveal distinctly different responses in boundary layer dynamics and cloud macro-physics. In Plus4, a warmer and moister boundary layer reduces total cloud cover but promotes larger cloud sizes and elongated cloud streets, with diminished liquid water and enhanced ice-phase hydrometeors. Conversely, Gradplus amplifies impacts in the upwind colder SST regions, yielding a drier, colder boundary layer, weaker energy transport, and higher liquid water path but reduced ice water content and cloud lines. Tracer analysis highlights that SST modifications alter airmass sources near cloud tops due to the entrainment of ambient air, with Plus4 amplifying boundary layer contributions to cloud-top regions. These findings underscore the spatially varying effects of SST gradients and mean SST on cloud organization and microphysics, emphasizing the need to resolve ocean-atmosphere coupling in global models to improve the prediction of marine cloud feedback under warming scenarios.

AIR-SEA INTERACTION↗

DOE OSTI2026

Prognostic simulations of mixed-phase clouds with model AC-1D v1.0: the impact of aerosol types and freezing parameterizations on ice crystal budgets

Mixed-phase clouds at high latitudes contribute to the uncertainty in predicting cloud feedbacks and climate sensitivity, mainly due to the complexity of microphysical processes that influence the partitioning between the supercooled liquid and ice phases, and hence, cloud radiative effects on regional scales. Particularly in Arctic mixed-phase clouds, the activation of ice-nucleating particles (INPs) from various aerosol populations remains a leading source of uncertainty. We developed an aerosol-cloud one-dimensional (AC-1D) model, which provides a novel framework to prognostically treat INP and ice crystal budgets while explicitly accounting for polydisperse and multicomponent aerosol that activate INPs following different freezing parameterizations. The AC-1D model is informed by large-eddy simulations to probe the impact of INP representation on predicted ice crystal number concentrations (N i ) and ice crystal budgets in mixed-phase Arctic stratus. We apply three immersion freezing (IMF) parameterizations, two time-independent (singular) and one time-dependent (classical nucleation theory), to predict the evolution of the INP reservoir and resulting ice crystal budget from polydisperse mineral dust, organic (humic-like substances), and sea spray aerosol particle size distributions. Our analysis focuses on how variations in aerosol number concentration and cloud system parameters such as cloud cooling rate, cloud-top entrainment rate, and ice crystal fall speed influence the INP reservoir and ice crystal budgets. Furthermore, this study investigates the competitive ice nucleation dynamics in mixed aerosol environments and provides a process-level quantification of the INP budget terms, which directly controls ice crystal budgets. For all studied case scenarios, the aerosol types and associated particle size distributions significantly impact INP and N i , and the choice between a time-dependent and a singular freezing description yields orders-of-magnitude differences in the predicted INP and N i over the 10 h simulation time, reflecting typical cloud lifetimes. Our results show that the influence of cloud cooling, INP entrainment, and sedimentation varies significantly depending on the chosen freezing parameterization. These findings underscore the critical need for robust IMF parameterizations and precise cloud system observations to enhance the accuracy of models in predicting mixed-phase cloud structure and evolution.

Arctic clouds↗

DOE OSTI2021

Observations of Clouds, Aerosols, Precipitation, and Surface Radiation over the Southern Ocean: An Overview of CAPRICORN, MARCUS, MICRE, and SOCRATES

Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation, and radiative processes, and their interactions. Projects between 2016 and 2018 used in situ probes, radar, lidar, and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN), and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF–NCAR G-V aircraft flying north–south gradients south of Tasmania, at Macquarie Island, and on the R/V Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multilayered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of dynamics and turbulence that likely drive heterogeneity of cloud phase. Satellite retrievals confirmed low clouds were responsible for radiation biases. Furthermore, the combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

An Overview of Atmospheric Features Over the Western North Atlantic Ocean and North American East Coast—Part 2: Circulation, Boundary Layer, and Clouds

The Western North Atlantic Ocean (WNAO) is a complex land-ocean-atmosphere system that experiences a wide range of atmospheric phenomena, which in turn drive unique aerosol transport pathways, cloud morphologies, and boundary layer variability. This work, Part 2 of a 2-part paper series, provides an overview of the atmospheric circulation, boundary layer variability, three-dimensional cloud structure, and precipitation over the WNAO; the companion paper (Part 1) focused on chemical characterization of aerosol, gas, and wet deposition. Seasonal changes in the circulation and sea surface temperature explain a clear transition in cloud morphologies from small shallow cumulus clouds, convective clouds, and tropical storms in summer, to stratus/stratocumulus and multi-layer cloud systems associated with winter storms. Synoptic variability in cloud fields is estimated using satellite-based weather states, and the role of postfrontal conditions (cold-air outbreaks) in the development of stratiform clouds is further analyzed. Precipitation is persistent over the ocean, with a regional peak over the Gulf Stream path, where offshore sea surface temperature gradients are large and surface fluxes reach a regional peak. Satellite data show a clear annual cycle in cloud droplet number concentration along the coast in winter, and minima in summer, suggesting a marked annual cycle in aerosol-cloud interactions. The performance of four climate models are assessed against satellite cloud retrievals. The models qualitatively reproduce the annual cycle in cloud cover and liquid water path, but with large discrepancies across models, especially in the extra-tropics. The paper concludes with a summary of outstanding issues and recommendations for future work.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Characterizing the magnetic fields of nearby molecular clouds using submillimeter polarization observations

Of all the factors that influence star formation, magnetic fields are perhaps the least well understood. The goal of this paper is to characterize the 3D magnetic field properties of nearby molecular clouds through various methods of statistically analysing maps of polarized dust emission. Our study focuses on nine clouds, with data taken from the Planck Sky Survey as well as data from the Balloon-borne Large Aperture Submillimeter Telescope for Polarimetry observations of Vela C. We compare the distributions of polarization fraction (p), dispersion in polarization angles ($\mathcal {S}$), and hydrogen column density (N H ) for each of our targeted clouds. To broaden the scope of our analysis, we compare the distributions of our clouds’ polarization observables with measurements from synthetic polarization maps generated from numerical simulations. We also use the distribution of polarization fraction measurements to estimate the inclination angle of each cloud’s cloud-scale magnetic field. We obtain a range of inclination angles associated with our clouds, varying from 16° to 69°. We establish inverse correlations between p and both $\mathcal {S}$ and NH in almost every cloud, but we are unable to establish a statistically robust $\mathcal {S}$ versus NH trend. By comparing the results of these different statistical analysis techniques, we are able to propose a more comprehensive view of each cloud’s 3D magnetic field properties. These detailed cloud analyses will be useful in the continued studies of cloud-scale magnetic fields and the ways in which they affect star formation within these molecular clouds.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

Theory of In-Cloud Activation of Aerosols and Microphysical Quasi-Equilibrium in a Deep Updraft

The microphysical quasi-equilibrium in an ascending adiabatic parcel is elucidated by an analytical theory in 0D with drastic simplifications. The theory predicts how in-cloud activation is most likely to be triggered by the onset of precipitation during sufficient ascent, with the ascent only needing to approach almost twice the cloud-base updraft speed aloft. The precipitation and cloud condensate mass fields are coupled in a closed system in a simplified version of the model. The initial state of no precipitation is unstable with respect to a perturbation. In the 2D phase space of both mass fields, there is a neutral line. Unstable growth of precipitation mass drives the system to cross the line into a regime of stability. An attractor is then approached consisting of precipitation mass balanced by accretion of cloud mass and fallout. The cloud-particle number concentration also approaches a stable equilibrium governed by the balance between in-cloud activation aloft from the inexorably increasing supersaturation during vertical acceleration and accretion of cloud droplets by precipitation. Dimensionless numbers characterizing the microphysical equilibria and their stability are derived mathematically, including a condensation–precipitation efficiency and an in-cloud activation efficiency. The theory explains common observations of the orders of magnitude of liquid water content in convective and stratiform clouds. Finally, sensitivity tests of the numerically integrated theoretical equations are documented with respect to variations in cloud condensation nucleus (CCN) aerosols and updraft speed. In conclusion, it is shown that this theory of in-cloud activation, with an increasing supersaturation during ascent, applies to both ice-only and liquid-only cloud.

54 ENVIRONMENTAL SCIENCES↗