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At least 217 records · Page 12

Resonant Auger decay of dissociating CH 3 I near the I 4d threshold

Resonant Auger processes provide a unique perspective on electronic interactions and excited vibrational and electronic states of molecular ions. Here, new data are presented on the resonant Auger decay of excited CH 3 I in the region just below the I 4d -1 ionization threshold. The resonances include the Rydberg series converging to the five spin–orbit and ligand-field split CH 3 I (I 4d -1 ) thresholds, as well as resonances corresponding to excitation from the I 4d 5/2,3/2 orbitals into the σ* lowest unoccupied molecular orbital. This study focuses on participator decay that populates the lowest lying states of CH 3 I + , in particular, the X̃ 2 E 3/2 and 2 E 1/2 states, and on spectator decay that populates the lowest-lying (CH 3 I 2+ )σ* states of CH 3 I + . The CH 3 I (I 4d -1 )σ* resonances are broad, and dissociation to CH 3 + I competes with the autoionization of the core-excited states. Auger decay as the molecule dissociates produces a photoelectron spectrum with a long progression (up to v 3 + ~ 25) in the C–I stretching mode of the X̃ 2 E 3/2 and 2 E 1/2 states, providing insights into the shape of the dissociative core-excited surface. Further, the observed spectator decay processes indicate that CH 3 I + is formed on the repulsive wall of the lower-lying (CH 3 I 2+ )σ* potentials, and the photon-energy dependence of the processes provides insights into the relative slopes of the (4d -1 )σ* and (CH 3 I 2+ )σ* potential surfaces. Data are also presented for the spectator decay of higher lying CH 3 I (I 4d -1 )nl Rydberg resonances. Photoelectron angular distributions for the resonant Auger processes provide additional information that helps distinguish these processes from the direct ionization signal.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

A rare gas optics-free absolute EUV photon spectrometer for solar system studies

We have developed a prototype spectrometer for space applications which require long term absolute EUV photon flux measurements. In this recently developed spectrometer, the energy spectrum of the incoming photons is transformed directly into an electron energy spectrum by taking advantage of the photoelectric effect in one of several rare gases at low pressures. Using an electron energy spectrometer operating at a few eV, and followed by an electron multiplying detector, pulses due to individual electrons are counted. The overall efficiency of this process is essentially independent of gain drifts in the signal path, and the secular degradation of optical components which is often a problem in other techniques is avoided.

Daybell, M. D.↗

Astrometry in two-photon interferometry using an Earth rotation fringe scan

Optical interferometers may not require a phase-stable optical link between the stations if instead sources of quantum-mechanically entangled pairs could be provided to them, enabling long baselines. We developed a new variation of this idea, proposing that photons from two different astronomical sources could be interfered at two decoupled stations. Interference products can then be calculated in post-processing or requiring only a slow, classical connection between stations. In this work, we investigated practical feasibility of this approach. We developed a Bayesian analysis method for the earth rotation fringe scanning technique and showed that in the limit of high signal-to-noise ratio it reproduced the results from a simple Fisher matrix analysis. Here we identify candidate stair pairs in the northern hemisphere, where this technique could be applied. With two telescopes with an effective collecting area of ~ 2 m 2 , we could detect fringing and measure the astrometric separation of the sources at ~100 μas precision in a few hours of observations, in agreement with previous estimates.

47 OTHER INSTRUMENTATION↗

X-ray multi-probe data acquisition: A novel technique for laser pump x-ray transient absorption spectroscopy

We report the development and implementation of a novel data acquisition (DAQ) technique for synchrotron-based laser pump X-ray Transient Absorption (XTA) spectroscopy, called X-ray Multi-Probe DAQ (XMP DAQ). This technique utilizes high performance analog to digital converters and home-built software to efficiently measure and process the XTA signal from all x-ray pulses between laser excitations. XMP DAQ generates a set of time resolved x-ray absorption spectra at thousands of different pump–probe time delays simultaneously. Two distinct XMP DAQ schemes are deployed to accommodate different synchrotron storage ring filling patterns. Current Integration (CI) DAQ is a quasi-analog technique that implements a fitting procedure to extract the time resolved absorption intensity from the averaged fluorescence detector response. The fitting procedure eliminates issues associated with small drifts in the voltage baseline and greatly enhances the accuracy of the technique. Photon Counting (PC) DAQ is a binary technique that uses a time resolved histogram to calculate the XTA spectrum. While PC DAQ is suited to measure XTA data with closely spaced x-ray pulses (~10 ns) and a low count rate (<1 detected photon/pulse), CI DAQ works best for widely spaced pulses (tens of ns or greater) with a high count rate (>1 detected photon/pulse). XMP DAQ produces a two-dimensional XTA dataset, enabling efficient quantitative analysis of photophysical and photochemical processes from the sub-nanosecond timescale to 100 μs and longer.

47 OTHER INSTRUMENTATION↗

Green Bank and Effelsberg Radio Telescope Searches for Axion Dark Matter Conversion in Neutron Star Magnetospheres

Axion dark matter (DM) may convert to radio-frequency electromagnetic radiation in the strong magnetic fields around neutron stars. The radio signature of such a process would be an ultranarrow spectral peak at a frequency determined by the mass of the axion particle. In this work, we analyze data we collected from the Robert C. Byrd Green Bank Telescope in the L band and the Effelsberg 100-m Telescope in the $\textit{L}$ band and $\textit{S}$ band from a number of sources expected to produce bright signals of axion-photon conversion, including the Galactic center of the Milky Way and the nearby isolated neutron stars RX J0720.4-3125 and RX J0806.4-4123. We find no evidence for axion DM and are able to set constraints on the existence of axion DM in the highly motivated mass range between ~ 5 and 11 μ eV with the strongest constraints to date on axions in the ~10–11 μ eV range.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Direct Detection Doppler Lidar for Spaceborne Wind Measurement

Aerosol and molecular based versions of the double-edge technique can be used for direct detection Doppler lidar spaceborne wind measurement. The edge technique utilizes the edge of a high spectral resolution filter for high accuracy wind measurement using direct detection lidar. The signal is split between an edge filter channel and a broadband energy monitor channel. The energy monitor channel is used for signal normalization. The edge measurement is made as a differential frequency measurement between the outgoing laser signal and the atmospheric backscattered return for each pulse. As a result the measurement is insensitive to laser and edge filter frequency jitter and drift at a level less than a few parts in 10(exp 10). We have developed double edge versions of the edge technique for aerosol and molecular-based lidar measurement of the wind. Aerosol-based wind measurements have been made at Goddard Space Flight Center and molecular-based wind measurements at the University of Geneva. We have demonstrated atmospheric measurements using these techniques for altitudes from 1 to more than 10 km. Measurement accuracies of better than 1.25 m/s have been obtained with integration times from 5 to 30 seconds. The measurements can be scaled to space and agree, within a factor of two, with satellite-based simulations of performance based on Poisson statistics. The theory of the double edge aerosol technique is described by a generalized formulation which substantially extends the capabilities of the edge technique. It uses two edges with opposite slopes located about the laser frequency at approximately the half-width of each edge filter. This doubles the signal change for a given Doppler shift and yields a factor of 1.6 improvement in the measurement accuracy compared to the single edge technique. The use of two high resolution edge filters substantially reduces the effects of Rayleigh scattering on the measurement, as much as order of magnitude, and allows the signal to noise ratio to be substantially improved in areas of low aerosol backscatter. We describe a method that allows the Rayleigh and aerosol components of the signal to be independently determined using the two edge channels and an energy monitor channel. The effects of Rayleigh scattering may then subtracted from the measurement and we show that the correction process does not significantly increase the measurement noise for Rayleigh to aerosol ratios up to 10. We show that for small Doppler shifts a measurement accuracy of 0.4 m/s can be obtained for 5000 detected photon, 1.2 m/s for 1000 detected photons, and 3.7 m/s for 50 detected photons for a Rayleigh to aerosol ratio of 5. Methods for increasing the dynamic range of the aerosol-based system to more than +/- 100 m/s are given.

Korb, C. Laurence↗

Time-resolved momentum imaging of UV photodynamics in structural isomers of iodopropane probed by site-selective XUV ionization

The photodynamics of 1- and 2-iodopropane (1 and 2-IP) were studied in a time-resolved scheme incorporating ultraviolet (UV) excitation and extreme ultraviolet (XUV) probing, which initiates photoionization selectively from the I 4d core orbital. UV absorption in the A-band of both isomers leads to prompt C–I bond fission, with significant disposal of internal energy into the propyl radical product. Site-selective ionization enables a range of charge transfer (CT) processes between the nascent highly charged iodine ions and neutral propyl radicals, dependent on the interfragment distance at the instant of ionization. Subtle differences in the dynamics of these CT processes between the two isomers are observed. In 1-IP, the kinetic energies of iodine ions produced by UV photodissociation and subsequent XUV multiple ionization increased notably over the first few hundred femtoseconds, which could be understood in terms of differing gradients along the photodissociation coordinates of the neutral and polycationic states involved in the pump and probe steps, respectively. Led by a recent report of HI elimination in UV photoexcited 2-IP [Todt et al., Phys. Chem. Chem. Phys., 22(46), 27338 (2020)], we also model the most likely signatures of this process in the present experiment, and can identify signal in the 2-IP data (that is absent or significantly weaker in the data from the unbranched 1-IP isomer) that is consistent with such a process occurring on ultrafast timescales.

Allum, Felix [Deutsches Elektronen-Synchrotron (DE↗

Search for Higgs boson production in association with a high-energy photon via vector-boson fusion with decay into bottom quark pairs at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search is presented for the production of the Standard Model Higgs boson in association with a high-energy photon. With a focus on the vector-boson fusion process and the dominant Higgs boson decay into b-quark pairs, the search benefits from a large reduction of multijet background compared to more inclusive searches. Results are reported from the analysis of 132 fb –1 of pp collision data at $\sqrt{s}$ = 13 TeV collected with the ATLAS detector at the LHC. The measured Higgs boson signal yield in this final-state signature is 1.3 ± 1.0 times the Standard Model prediction. The observed significance of the Higgs boson signal above the background is 1.3 standard deviations, compared to an expected significance of 1.0 standard deviations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Receiver Signal to Noise Ratios for IPDA Lidars Using Sine-wave and Pulsed Laser Modulation and Direct Detections

Integrated path differential absorption (IPDA) lidar can be used to remotely measure the column density of gases in the path to a scattering target [1]. The total column gas molecular density can be derived from the ratio of the laser echo signal power with the laser wavelength on the gas absorption line (on-line) to that off the line (off-line). 80th coherent detection and direct detection IPDA lidar have been used successfully in the past in horizontal path and airborne remote sensing measurements. However, for space based measurements, the signal propagation losses are often orders of magnitude higher and it is important to use the most efficient laser modulation and detection technique to minimize the average laser power and the electrical power from the spacecraft. This paper gives an analysis the receiver signal to noise ratio (SNR) of several laser modulation and detection techniques versus the average received laser power under similar operation environments. Coherent detection [2] can give the best receiver performance when the local oscillator laser is relatively strong and the heterodyne mixing losses are negligible. Coherent detection has a high signal gain and a very narrow bandwidth for the background light and detector dark noise. However, coherent detection must maintain a high degree of coherence between the local oscillator laser and the received signal in both temporal and spatial modes. This often results in a high system complexity and low overall measurement efficiency. For measurements through atmosphere the coherence diameter of the received signal also limits the useful size of the receiver telescope. Direct detection IPDA lidars are simpler to build and have fewer constraints on the transmitter and receiver components. They can use much larger size 'photon-bucket' type telescopes to reduce the demands on the laser transmitter. Here we consider the two most widely used direct detection IPDA lidar techniques. The first technique uses two CW seeder lasers, one on-line and one offline that are intensity modulated by two different frequency sine-waves signals before being amplified by a common laser amplifier. The receiver uses narrowband amplitude demodulation, or lock-in, Signal processing at the given laser modulation frequencies [3,4]. The laser transmitter operates in a quasi CW mode with the peak power equal to twice the average power. The on-line and off-line lasers can be transmitted at the same time without interference. Another direct detection technique uses a low duty cycle pulsed laser modulation [5,6] with the laser wavelengths alternating between on-line and off-line on successive pulses. The receiver uses time resolved detection and can also provide simultaneous target range measurement. With a lower laser duty cycle it requires a much higher peak laser power for the same average power.

Sun, Xiaoli↗

Search for dimuon resonance in the 35 to 75 GeV mass range using 140 fb−1 of 13 TeV pp collisions with the ATLAS detector

A model-independent search for low-mass resonances decaying into pairs of oppositely charged muons is presented. The analysis uses proton-proton collision data corresponding to an integrated luminosity of 140 fb−1, recorded by the ATLAS detector at the Large Hadron Collider between 2015 and 2018. The search targets hypothetical dimuon resonances in the invariant mass range from 35 GeV to 75 GeV. The modelling of this mass region is particularly challenging for conventional analytic background parameterisations. To address this, a Gaussian process regression technique is used to model the background. The dimuon mass spectrum is analysed for potential signals, and no statistically significant excess is observed. Upper limits at the 95% confidence level are set on the fiducial production cross-section of new resonances decaying promptly into muons, ranging from 20 fb to 110 fb, depending on the resonance mass. These results are further interpreted in the context of dark-photon and dark-matter-mediator models, leading to new constraints on their parameter spaces.

Aad, G↗

Kinematically boosted pairs from the nonlinear Breit–Wheeler process in small-angle laser collisions

Here we discuss that a scheme of nonperturbative pair production by high energy photons (ω≳m) in a strong external field is achievable at the next high intensity laser experiments. The pair momentum is boosted, and for ω≳1.2m, the pair yield is increased when the external field is formed by two laser pulses converging at a small angle. These characteristics are nonperturbative in origin and related to the presence of magnetic field in addition to electric field. By enhancing the signal over perturbative backgrounds, these features allow the employment of above-threshold photons ω > 2m, which further increases the pair yield. We note the close relation of this photon-pair conversion mechanism to spontaneous pair creation, recommending it as an accessible stepping stone experiment using state-of-the-art or soon-to-be laser technology.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Single particle detection system for strong-field QED experiments

Abstract Measuring signatures of strong-field quantum electrodynamics (SF-QED) processes in an intense laser field is an experimental challenge: it requires detectors to be highly sensitive to single electrons and positrons in the presence of the typically very strong x-ray and γ -photon background levels. In this paper, we describe a particle detector capable of diagnosing single leptons from SF-QED interactions and discuss the background level simulations for the upcoming Experiment-320 at FACET-II (SLAC National Accelerator Laboratory). The single particle detection system described here combines pixelated scintillation LYSO screens and a Cherenkov calorimeter. We detail the performance of the system using simulations and a calibration of the Cherenkov detector at the ELBE accelerator. Single 3 GeV leptons are expected to produce approximately 537 detectable photons in a single calorimeter channel. This signal is compared to Monte-Carlo simulations of the experiment. A signal-to-noise ratio of 18 in a single Cherenkov calorimeter detector is expected and a spectral resolution of 2% is achieved using the pixelated LYSO screens.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Optimal Energy Measurement in Nonlinear Systems: An Application of Differential Geometry

Design of TES microcalorimeters requires a tradeoff between resolution and dynamic range. Often, experimenters will require linearity for the highest energy signals, which requires additional heat capacity be added to the detector. This results in a reduction of low energy resolution in the detector. We derive and demonstrate an algorithm that allows operation far into the nonlinear regime with little loss in spectral resolution. We use a least squares optimal filter that varies with photon energy to accommodate the nonlinearity of the detector and the non-stationarity of the noise. The fitting process we use can be seen as an application of differential geometry. This recognition provides a set of well-developed tools to extend our work to more complex situations. The proper calibration of a nonlinear microcalorimeter requires a source with densely spaced narrow lines. A pulsed laser multi-photon source is used here, and is seen to be a powerful tool for allowing us to develop practical systems with significant detector nonlinearity. The combination of our analysis techniques and the multi-photon laser source create a powerful tool for increasing the performance of future TES microcalorimeters.

Nonlinear response↗

Nonlinear quantum interferometric spectroscopy with entangled photon pairs

Here, we develop closed expressions for a time-resolved photon counting signal induced by an entangled photon pair in an interferometric spectroscopy setup. Superoperator expressions in Liouville-space are derived that can account for relaxation and dephasing induced by coupling to a bath. Interferometric setups mix matter and light variables non-trivially, which complicates their interpretation. We provide an intuitive modular framework for this setup that simplifies its description. Based on the separation between the detection stage and the light–matter interaction processes, we show that the pair entanglement time and the interferometric time-variables control the observed physics time scale. Only a few processes contribute in the limiting case of small entanglement time with respect to the sample response, and specific contributions can be singled out.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Study of γ γ → γ ψ ( 2 S ) at Belle

Using 980 fb -1 of data at and around the Υ(nS)(n = 1, 2, 3, 4, 5) resonances collected with the Belle detector at the KEKB asymmetric-energy e+e- collider, the two-photon process γγ → γψ(2S) is studied from the threshold to 4.2 GeV for the first time. Two structures are seen in the invariant mass distribution of γψ(2S): one at M R 1 = 3922.4 ± 6.5 ± 2.0 MeV/c 2 with a width of Γ R 1 = 22 ± 17 ± 4 MeV, and another at M R 2 = 4014.3 ± 4.0 ± 1.5 MeV/c 2 with a width of Γ R 2 = 4 ± 11 ± 6 MeV; the signals are parametrized with the incoherent sum of two Breit- Wigner functions. The first structure is consistent with the X(3915) or the χ c2 (3930), and the local statistical significance is determined to be 3.1σ with the systematic uncertainties included. The second matches none of the known charmonium or charmonium like states, and its global significance is determined to be 2.8σ including the look-elsewhere effect. The production rates are Γ γγ B(R 1 → γψ(2S)) = 9.8 ± 3.6 ± 1.2 eV assuming (J PC , |λ|) = (0 ++ , 0) or 2.0 ± 0.7 ± 0.2 eV with (2 ++ , 2) for the first structure and Γ γγ B(R 2 → γψ(2S)) = 6.2 ± 2.2 ± 0.8 eV with (0 ++ , 0) or 1.2 ± 0.4 ± 0.2 eV with (2 ++ , 2) for the second one. Furthermore, the first errors are statistical and the second systematic, and λ is the helicity.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Experimental upper bounds for resonance-enhanced entangled two-photon absorption cross section of indocyanine green

Resonant intermediate states have been proposed to increase the efficiency of entangled two-photon absorption (ETPA). Although resonance-enhanced ETPA (r-ETPA) has been demonstrated in atomic systems using bright squeezed vacuum, it has not been studied in organic molecules. We investigate for the first time r-ETPA in an organic molecular dye, indocyanine green (ICG), when excited by broadband entangled photons in near-IR. Similar to many reported virtual state mediated ETPA (v-ETPA) measurements, no r-ETPA signals are measured, with an experimental upper bound for the cross section placed at 6(±2) × 10 −23 cm 2 . In addition, the classical resonance-enhanced two-photon absorption (r-TPA) cross section of ICG at 800 nm is measured for the first time to be 20(±13) GM, where 1 GM equals 10 −50 cm 4 s, suggesting that having a resonant intermediate state does not significantly enhance two-photon processes in ICG. Furthermore, the spectrotemporally resolved emission signatures of ICG excited by entangled photons are also presented to support this conclusion.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Electron ionization via dark matter-electron scattering and the Migdal effect

There are currently several existing and proposed experiments designed to probe sub-GeV dark matter (DM) using electron ionization in various materials. The projected signal rates for these experiments assume that this ionization yield arises only from DM scattering directly off electron targets, ignoring secondary ionization contributions from DM scattering off nuclear targets. We investigate the validity of this assumption and show that if sub-GeV DM couples with comparable strength to both protons and electrons, as would be the case for a dark photon mediator, the ionization signal from atomic scattering via the Migdal effect scales with the atomic number Z and 3-momentum transfer q as Z 2 q 2 . The result is that the Migdal effect is always subdominant to electron scattering when the mediator is light, but that Migdal-induced ionization can dominate over electron scattering for heavy mediators and DM masses in the hundreds of MeV range. We put these two ionization processes on identical theoretical footing, address some theoretical uncertainties in the choice of atomic wave functions used to compute rates, and discuss the implications for DM scenarios where the Migdal process dominates, including for XENON10, XENON100, and the recent XENON1T results on light DM scattering.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Simplified Architecture for Precise Aiming of a Deep-Space Communication Laser Transceiver

The simplified architecture is a minimal system for a deep-space optical communications transceiver. For a deepspace optical communications link the simplest form of the transceiver requires (1) an efficient modulated optical source, (2) a point-ahead mechanism (PAM) to compensate for two-way light travel, (3) an aperture to reduce the divergence of the transmit laser communication signal and also to collect the uplink communication signal, and (4) a receive detector to sense the uplink communication signal. Additional components are introduced to mitigate for spacecraft microvibrations and to improve the pointing accuracy. The Canonical Transceiver implements this simplified architecture (see figure). A single photon-counting smart focal plane sensor combines acquisition, tracking, and forward link data detection functionality. This improves optical efficiency by eliminating channel splits. A transmit laser blind sensor (e.g. silicon with 1,550-nm beam) provides transmit beam-pointing feedback via the two-photon absorption (TPA) process. This vastly improves the transmit/receive isolation because only the focused transmit beam is detected. A piezoelectric tiptilt actuator implements the required point-ahead angle. This point-ahead mechanism has been demonstrated to have near zero quiescent power and is flight qualified. This architecture also uses an innovative 100-mHz resonant frequency passive isolation platform to filter spacecraft vibrations with voice coil actuators for active tip-tilt correction below the resonant frequency. The canonical deep-space optical communications transceiver makes synergistic use of innovative technologies to reduce size, weight, power, and cost. This optical transceiver can be used to retire risks associated with deep-space optical communications on a planetary pathfinder mission and is complementary to ongoing lunar and access link developments.

Ortiz, Gerard G.↗