Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “nuclear nonproliferation”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Cell design for laser-induced breakdown spectroscopy measurements on reactive gas samples

Uranium hexafluoride (UF 6 ) is the primary material used for the enrichment of uranium in the production of light water nuclear reactor fuels worldwide. Accurate, rapid quantification of uranium isotopic composition in nuclear materials is required for safeguards programs and nonproliferation purposes. One potential technique for isotopic measurements in uranium species in the field is laser induced breakdown spectroscopy (LIBS). Safe and effective application of LIBS to UF 6 for enrichment measurements is uniquely challenging due to the chemical and physical properties of UF 6 , which necessitate specific handling procedures. The objective of this work is to design a cell for isotopic analysis of UF 6 that is (1) compatible with chemical and physical properties of UF 6 , (2) compatible with LIBS laser, and (3) portable-sized for nuclear safeguards applications. Along with cell design, initial testing of the cell for basic performance and chemical compatibility is performed. As designed and constructed, the portable gas cell was gas-tight, chemically compatible with UF 6 , and withstood long-duration laser exposure. In this work, the cell has proven capability for handling reactive gasses, such as UF 6 , with specification application to isotopic analysis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Summary of the Workshop on M400 High-Resolution CZT Detector Safeguards Applications

In September 2023, the US Department of Energy (DOE) National Nuclear Security Administration’s (NNSA’s) Office of Nonproliferation and Arms Control sponsored a workshop on M400 high-resolution cadmium zinc telluride (CZT) detector safeguards applications under its Safeguards Technology Development Program. The workshop brought together internationally recognized subject matter experts (SMEs) in the field of gamma spectrometry and uranium/plutonium isotopic analysis and experts from H3D Inc. (H3D), the vendor for M400.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2024

Shielding an Infrasound Sensor for INL’s Fuel Conditioning Facility

Idaho National Laboratory (INL) has been pyroprocessing spent fuel from the Experimental Breeder Reactor II (EBR-II). This process occurs in the Fuel Conditioning Facility (FCF) which houses the treatment of DOE-owned sodium-bonded metal fuel. The electrometallurgical methods used in FCF treat the spent fuel from EBR-II for recycling of the uranium. The radiation field present inside FCF throughout the pyroprocessing stages affects any electronic sensors and devices that may be used for research. An example of such device is a seismoacoustic sensor which detects sound and vibration waves from the equipment in the facility. Seismoacoustic sensors are of interest to research nonproliferation techniques.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗
DOE OSTI2023

Nevada National Security Site [Slides]

Since 1951, the Nevada National Security Site has ensured the security of the US and its allies by supporting the stewardship of the nuclear deterrent, providing emergency response capability and training, and contributing key nonproliferation and arms control initiatives.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2020

Samarium isotope compositions of uranium ore concentrates: A novel nuclear forensic signature

Uranium ore is mined and milled to produce uranium ore concentrate (UOC), a regulated product of the nuclear fuel cycle. Additionally, diversion of UOC from the fuel cycle into possible weapons production is a key concern in global nonproliferation efforts. As such, the ability to trace the origin of seized nuclear materials is imperative to law enforcement efforts. Although isotopic signatures of UOCs have proven fruitful to pinpoint sample provenance, new isotopic signatures are needed because most existing isotopic signatures are not indicative of the original ore body from which the U is derived. In this work, we developed a new method to separate samarium (Sm) from a U-rich sample matrix and report the first Sm isotope compositions of 32 UOCs derived from a variety of worldwide uranium mines. Relative to terrestrial standards, approximately half the UOCs have resolved and anticorrelated 149 Sm- 150 Sm isotope compositions, consistent with the capture of thermal neutrons by 149 Sm in the ore body. The UOCs with anomalous Sm isotope compositions tend to derive from older (~>1.5Ga) and higher-grade ore bodies, although other factors, such as the presence of neutron moderators like water, also play a role. Nonetheless, the Sm isotope compositions of UOCs directly reflects the neutron fluence over the history of the original ore body and can be used to discern different geologic conditions associated with that ore body. Overall, this work demonstrates the potential use of Sm isotopes as a novel nuclear forensics signature for origin assessment of UOCs.

58 GEOSCIENCES↗
DOE OSTI2023

99m Tc Generator Development for Low Specific Activity 99 Mo

Because of aging reactor fleets, complicated regulatory applications for new reactors, unresolved uranium disposition pathways, and the nonproliferation and minimization efforts spearheaded by the National Nuclear Security Administration (NNSA), non-fission-based production of 99 Mo is becoming an attractive alternative.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Inferring UAV Position Relative to Smartphone Sensor Based on Acoustic Characteristics

As commercial and non-commercial unmanned aerial vehicles (UAVs) improve technologically and increase in accessibility, their potential for use in actions antithetical to nuclear non-proliferation efforts increases as well. The ability to identify and locate UAVs using ubiquitous, inexpensive hardware and software would be advantageous as both a deterrent and an initial warning system. Our team looks to utilize smartphones as acoustic sensors to record and characterize UAV movement based on the sound produced while in flight. Multi-rotor UAVs produce identifiable acoustic spectral characteristics with frequencies and harmonics corresponding to motor revolutions per minute and the propeller characteristics. As the source moves closer to the receiver these spectral patterns remain relatively stable (at slow speeds), while the energy observed from the waves increases. The goal of this work is to utilize a small network of smartphone sensors with known, fixed positions to infer the relative position of an in-flight UAV with respect to the position of the smartphones through the variation in acoustic energy.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗
DOE OSTI2023

Multiplicity counting using organic scintillators to distinguish neutron sources: An advanced teaching laboratory

In this advanced instructional laboratory, students explore complex detection systems and nondestructive assay techniques used in the field of nuclear physics. After setting up and calibrating a neutron detection system, students carry out timing and energy deposition analyses of radiation signals. Through the timing of prompt fission neutron signals, multiplicity counting is used to carry out a special nuclear material (SNM) nondestructive assay. Our experimental setup is comprised of eight trans-stilbene organic scintillation detectors in a well-counter configuration, and measurements are taken on a spontaneous fission source as well as two (α,n) sources. By comparing each source's measured multiplicity distribution, the resulting measurements of the (α,n) sources can be distinguished from that of the spontaneous fission source. Such comparisons prevent the spoofing, i.e., intentional imitation, of a fission source by an (α,n) neutron source. This instructional laboratory is designed for nuclear engineering and physics students interested in organic scintillators, neutron sources, and nonproliferation radiation measurement techniques.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Machine learning at the edge to improve in-field safeguards inspections

Artificial intelligence (AI) and machine learning (ML) are near-ubiquitous in day-to-day life; from cars with automated driver-assistance, recommender systems, generative content platforms, and large language chatbots. Implementing AI as a tool for international safeguards could significantly decrease the burden on safeguards inspectors and nuclear facility operators. The use of AI would allow inspectors to complete their in-field activities quicker, while identifying patterns and anomalies and freeing inspectors to focus on the uniquely human component of inspections. Sandia National Laboratories has spent the past two and a half years developing on-device machine learning to develop both a digital and robotic assistant. This combined platform, which we term inspecta, has numerous on-device machine learning capabilities that have been demonstrated at the laboratory scale. Here this work describes early successes implementing AI/ML capabilities to reduce the burden of tedious inspector tasks such as seal examination, information recall, note taking, and more.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2020

Automated Vehicle Detection in a Nuclear Facility Using Low-Frequency Acoustic Sensors

This article presents an analysis of the method of construction and results for a classifier intended to identify vehicles using low-frequency acoustic data collected by a dis-tributed sensor network. This data is collected as part of a venture intended to explore data analytics and multisensor fusion techniques for the monitoring of activities at a test bed nuclear facility located at Oak Ridge National Laboratory in Oak Ridge, Tennessee. We describe the associated target signature and design a classifier based on a multilayer perceptron, followed by an analysis of its results. We discuss how overall accuracy is not the only consideration in constructing this classifier, and how for this application, it is actually desirable to operate at a lower level of accuracy in exchange for a reduction in the false alarm rate, as well as how this relates to the actual deployment of the classifier in practical use.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗
DOE OSTI2022

Development of 17 N as a time-tagged neutron source for calibration of large antineutrino detectors

Large antineutrino detectors hold the potential for remote nuclear reactor monitoring and discovery, which is of great interest for nonproliferation and treaty verification applications. Correlated-particle calibration sources are especially useful for large-volume designs based on detection of inverse beta-decay events, as the timing information of the coincident particles improves background rejection and event reconstruction. 17 N is a promising calibration source since it emits beta-correlated delayed neutrons and can be produced relatively easily using high-energy neutrons. In this work, we examine the feasibility of 17 N as a time-tagged calibration source for large antineutrino detectors. 17 N was produced using a DT neutron generator from a water sample enriched in 17 O, and the observed production rates were found to be consistent with previous measurements of the 17 O(n,p) 17 N reaction cross-section. As a result, time-tagging of 17 N delayed neutrons is demonstrated via beta-neutron coincidence measurements conducted using a specialized beta detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

ARIES team achieves major milestone in support of nonproliferation

The Advanced Recovery and Integrated Extraction System (ARIES) Program is a great example of LANL’s Weapons and Global Security programs working together to achieve important nuclear security mission goals. Executed at PF-4, a facility better known for its pit production mission, the ARIES Program is helping the nation meet its nonproliferation commitments by preparing surplus weapons-grade plutonium for final disposition. ARIES recently met a major milestone of producing 1 metric ton of plutonium oxide from material removed from surplus pits. The milestone was celebrated in an awards ceremony at LANL on January 28.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2020

Strategic Survey of Antineutrino-based Nonproliferation Technologies

Antineutrinos carry approximately 3% of the total energy released in fission processes. As a consequence, nuclear energy production provides by far the brightest antineutrino sources on Earth. Antineutrino interactions with ordinary matter are weak and these particles cannot be shielded, making them an ideal signature of fissioning systems. However, the same property makes antineutrinos difficult to detect. Antineutrino detection technologies have matured in recent years, and emerging detection approaches warrant further investment. For near-field applications, the major enabling technological advancement, reported in 2018, is the conclusive detection of the antineutrino spectrum in segmented detectors operating at the surface with minimal shielding. For far-field applications, the highlights are the routine detection of reactor antineutrinos at hundreds of kilometer standoff in the kiloton-scale KamLAND and Borexino liquid scintillator detectors, and in particular the observation of the residual South Korean reactor antineutrino flux in KamLAND following the Fukushima disaster that led to shutdown of reactors in Japan

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Improved light yield and growth of large-volume ultrafast single crystal scintillators Cs 2 ZnCl 4 and Cs 3 ZnCl 5

Due to their reported fast decay times, Cs 2 ZnCl 4 and Cs 3 ZnCl 5 are promising candidates for detection of gamma rays and X-rays in high count rate and fast timing applications. In this work, we show that single crystals with better optical quality than previously demonstrated – and larger in size – can be grown via the vertical Bridgman method. Highly transparent Ø7 mm crystals of undoped Cs 2 ZnCl 4 and Cs 3 ZnCl 5 are grown and measured to have light yields surpassing those previously reported, achieving 1980 ± 100 ph/MeV and 1460 ± 70 ph/MeV at 662 keV – a 55% and 232% improvement, respectively. We observe single-component scintillation decay times for both Cs 2 ZnCl 4 (1.66 ns) and Cs 3 ZnCl 5 (0.82 ns) and radioluminescence emission with maximum intensity at ~290 nm. Scalability of these materials is also evaluated based on growth of Ø22 mm crystals. Minimal cracking is observed, and the fast decay times are maintained at this size. Coincidence time resolution of 3 × 3 × 5 mm 3 and 7 × 7 × 10 mm 3 pixels cut from Ø22 mm Cs 2 ZnCl 4 are measured to be 148 ± 1 ps FWHM and 175 ± 1 ps FWHM, respectively. Here, the improved performance and ability to be fabricated in large sizes now place Cs 2 ZnCl 4 and Cs 3 ZnCl 5 on the map as potential contenders for radiation detection applications where BaF 2 – the most commonly used ultrafast inorganic scintillator – is typically considered.

36 MATERIALS SCIENCE↗