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At least 217 records · Page 12

Seeing deep inside engines with X-rays

Argonne National Laboratory outside Chicago is creating a research program that will empower investigators to apply the sensing qualities of X-rays to the challenge of seeing what goes on inside scramjets, rotating detonation engines and other hypersonic propulsion concepts. The program’s architects describe the technology’s heritage and its time- and cost-saving benefits.

42 ENGINEERING↗

Radiochemistry and Trinity

Forty seconds after Trinity detonated, Noble Laureate Enrico Fermi calculated the bomb’s energy release. By measuring the lateral dispersion of small pieces of paper dropped before, during, and after the blast wave passed him, he calculated an explosive yield of ten kilotons. Although Fermi’s estimate was only half of the official yield, it provided immediate confirmation that nuclear fission could be fashioned into a weapon of war.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Effects of Intrusive Confining Units on Groundwater Flow at Pahute Mesa, Nevada National Security Site

Geological, geophysical, hydrogeological, and hydrological evidence indicates that feeder dikes to lava flows play a role as confining units in the groundwater flow system underlying the Pahute Mesa area of underground nuclear testing at the Nevada National Security Site (NNSS). Of geological significance, the Pahute Mesa testing area is largely situated within the Silent Canyon caldera, which includes both tuffs and lavas that were fed by (and are connected to) intrusive rock units such as feeder dikes prior to and during volcanic eruptions (Orkild et al., 1968; Byers et al., 1976). Groundwater modeling results presented in this report support extension of “pool-dam” and “breach scenario” concepts presented in Jackson and Fenelon (2018) and Jackson et al. (2021) to low-permeability intrusive confining units (ICUs) such as feeder dikes that are expected to dissect and ring the caldera. As laterally extensive, steeply-dipping, and sub-parallel planar structures, ICUs can be expected to further compartmentalize groundwater flow in the volcanic aquifers systems at Pahute Mesa beyond the stratigraphically-defined tuff confining units (TCUs). ICUs provide an explanation for changes in water levels before and after the Cheshire test, detonated 2/14/76 (USDOE, 2015), and the unusually high horizontal gradient southwest of Cheshire. These ICU concepts are supported by groundwater modeling results presented in this report. The evidence and groundwater modeling results indicate that the downgradient extent of radionuclide contamination in some areas of Pahute Mesa could be overestimated by ignoring the confining effects of ICUs. On the other hand, contaminant extent could be underestimated by not considering transient flow effects and/or the re-equilibrated flow field caused by breaching of an ICU by an underground nuclear test.

54 ENVIRONMENTAL SCIENCES↗

Type Ia Supernova Nucleosynthesis: Metallicity-dependent Yields

Abstract Type Ia supernova explosions (SN Ia) are fundamental sources of elements for the chemical evolution of galaxies. They efficiently produce intermediate-mass (with Z between 11 and 20) and iron group elements—for example, about 70% of the solar iron is expected to be made by SN Ia. In this work, we calculate complete abundance yields for 39 models of SN Ia explosions, based on three progenitors—a 1.4 M ⊙ deflagration detonation model, a 1.0 M ⊙ double detonation model, and a 0.8 M ⊙ double detonation model—and 13 metallicities, with 22 Ne mass fractions of 0, 1 × 10 −7 , 1 × 10 −6 , 1 × 10 −5 , 1 × 10 −4 , 1 × 10 −3 , 2 × 10 −3 , 5 × 10 −3 , 1 × 10 −2 , 1.4 × 10 −2 , 5 × 10 −2 , and 0.1, respectively. Nucleosynthesis calculations are done using the NuGrid suite of codes, using a consistent nuclear reaction network between the models. Complete tables with yields and production factors are provided online at Zenodo:Yields ( https://doi.org/10.5281/zenodo.8060323 ). We discuss the main properties of our yields in light of the present understanding of SN Ia nucleosynthesis, depending on different progenitor mass and composition. Finally, we compare our results with a number of relevant models from the literature.

79 ASTRONOMY AND ASTROPHYSICS↗

A statistical approach to screening isotopic signatures in monitoring for underground nuclear explosions

The ability to differentiate between atmospheric radionuclide signatures from underground nuclear explosions (UNEs) and signals from other sources, such as medical isotope-production facilities and nuclear reactors, can be critical to the detection and monitoring of unannounced, low-yield nuclear events. Signatures having anomalously high amplitudes, compared to background levels, remain the best indicator in screening for a UNE. However, isotopic composition can further validate a suspected UNE signature, but separation from any atmospheric background composition is first necessary. To date, evaluating the challenges of performing this separation has typically involved comparing an observed background with a highly idealized deterministic model of radioxenon signature production by a UNE that does not consider the influence of post-detonation chemical/physical processes in the detonation cavity or the subsequent gas transport mechanisms that can also affect the isotopic composition of the detected gas signature. In addition, purely deterministic models, as previously employed, overlook the uncertainty inherent in estimating critical parameters characterizing the UNE and its detonation environment. In this paper, we create detailed, multi-parameter models of radionuclide evolution using the widely accepted England and Rider post-detonation radionuclide decay-chain network coupled to detailed models simulating physical production and transport processes affecting the gas signature. Because these models are governed by uncertain parameters including barometric fluctuations, realistic ranges of variation for each of the parameters influencing isotopic composition are then defined. A Latin-Hypercube sampling approach is used to obtain a random distribution of isotopic production and gas transport results associated with a given value of each parameter. We apply these results to background histories of two stations, one providing 4-isotope background measurements and the other providing two-isotope measurements associated with the 2013 DPRK announced UNE.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

U-Pu and Ba-Cs isotopic measurements on Trinitite by laser ablation sampling on the Neoma MC-ICP-MS

In this study we present the results of combined U-Pu and Ba-Cs isotope measurements obtained by laser ablation (LA) sampling of two glassy debris fragments (‘Trinitite’) from the world's first atomic bomb detonation conducted in New Mexico on July 16, 1945. Our primary goal in conducting these measurements was to understand whether examination of the U-Pu and Ba-Cs systematics by direct sampling (e.g. without any chemical separation or purification prior to isotope ratio measurement) could yield meaningful information that would differentiate the Trinitite fragments from glassy material lacking a nuclear fission signature. These measurements were conducted on a ThermoFisher Scientific Neoma multi collector – inductively coupled plasma – mass spectrometer (MC-ICP-MS), which is a relatively new MC-ICP-MS platform, so we also examine the behavior of these isotope systems in standards sampled in solution and via LA. Unsurprisingly, the measurements made on purified solutions of the U, Pu, and Ba isotopic standards produce high precision isotope ratios. Furthermore, this extends to the U-Pu measurements made by LA sampling, with the expected degradation in precision and accuracy related to matrix effects and signal intensity fluctuation. However, the Ba-Cs data acquired by LA is of low precision across all of the matrices examined and bears evidence of complex mass fractionation that will require further investigation to resolve. In total, our results indicate that the observed U-Pu isotope data are of sufficient quality to accurately constrain the U and Pu isotopic composition of glass containing sub-ppm levels of these elements which in turn could be used to differentiate glass containing anthropogenic fission products from natural glass whereas the Ba-Cs LA data cannot be used for this purpose until further methodological refinement is performed.

Ba-Cs↗

Energetic Combustion Devices for Aerospace Propulsion and Power

Chemical reactions have long been the mainstay thermal energy source for aerospace propulsion and power. Although it is widely recognized that the intrinsic energy density limitations of chemical bonds place severe constraints on maximum realizable performance, it will likely be several years before systems based on high energy density nuclear fuels can be placed into routine service. In the mean time, efforts to develop high energy density chemicals and advanced combustion devices which can utilize such energetic fuels may yield worthwhile returns in overall system performance and cost. Current efforts in this vein are being carried out at NASA MSFC under the direction of the author in the areas of pulse detonation engine technology development and light metals combustion devices. Pulse detonation engines are touted as a low cost alternative to gas turbine engines and to conventional rocket engines, but actual performance and cost benefits have yet to be convincingly demonstrated. Light metal fueled engines also offer potential benefits in certain niche applications such as aluminum/CO2 fueled engines for endo-atmospheric Martian propulsion. Light metal fueled MHD generators also present promising opportunities with respect to electric power generation for electromagnetic launch assist. This presentation will discuss the applications potential of these concepts with respect to aero ace propulsion and power and will review the current status of the development efforts.

Litchford, Ron J.↗

Gas transport across the low-permeability containment zone of an underground nuclear explosion

Understanding the nature of gas transport from an underground nuclear explosion (UNE) is required for evaluating the ability to detect and interpret either on-site or atmospheric signatures of noble gas radionuclides resulting from the event. We performed a pressure and chemical tracer monitoring experiment at the site of an underground nuclear test that occurred in a tunnel in Nevada to evaluate the possible modes of gas transport to the surface. The site represents a very well-contained, low gaspermeability end member for past UNEs at the Nevada National Security Site. However, there is very strong evidence that gases detected at the surface during a period of low atmospheric pressure resulted from fractures of extremely small aperture that are essentially invisible. Our analyses also suggest that gases would have easily migrated to the top of the high-permeability collapse zone following the detonation minimizing the final distance required for migration along these narrow fractures to the surface. This indicates that on-site detection of gases emanating from such low-permeability sites is feasible while standoff detection of atmospheric plumes may also be possible at local distances for sufficiently high fracture densities. Finally, our results show that gas leakage into the atmosphere also occurred directly from the tunnel portal and should be monitored in future tunnel gas sampling experiments for the purpose of better understanding relative contributions to detection of radioxenon releases via both fracture network and tunnel transport.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Microstructural Effects of PETN on Detonator Performance

The strategic motivation of the project is guided by the Need to understand: material characteristics important to performance; how to most appropriately measure/monitor these characteristics; and, evolution of these characteristics through lifetime and storage conditions.

36 MATERIALS SCIENCE↗

Analysis of 127 Xe tracer measurements using a net counts method

A suite of measurement systems were deployed as part of the Physical Experiment 1 series of experiments, which involved detonating chemical explosives along with radionuclide tracers in an underground cavity, at the Nevada National Security Site (NNSS) in the United States. One of the radionuclide tracers, 127 Xe was released from the containment following the explosion and detected on a SAUNA Q B sampler situated approximately 3.5 km away. The system uses a beta-gamma coincidence detector system to measure fission product radioisotopes of xenon relevant to nuclear explosion monitoring. In this work we use the coincidence measurement data to analyse and interpret the results from the SAUNA Q B system, to calculate the measured 127 Xe activity concentration(s).

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

The Origins of Blast-Loaded Vessels

As the Manhattan Project shifted to the theory of implosion assembly in 1944, plutonium was extremely rare and large uncertainties surrounded the function of the Gadget. For these reasons, a team within the Manhattan Project began another ambitious experiment: to confine the effects of detonating two tons of high explosives and enable the recovery of precious plutonium! No data existed on the subject, and the team faced numerous challenges as they engineered what is believed to be the world’s first blast-loaded confinement vessel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Error Modeling for Prompt Yield Estimation [Slides]

Multi-Phenomenology Explosion Monitoring (MultiPEM) Toolbox provides a capability for post-detonation characterization focusing on yield estimation; Synthesize information from multiple sensor types; Leverage historical databases to inform statistical models; Allows for rapid or comprehensive analysis; Implemented in R code.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Effects of Intrusive Confining Units on Groundwater Flow at Pahute Mesa, Nevada National Security Site

Geological, geophysical, hydrogeological, and hydrological evidence indicates that feeder dikes to rhyolitic lava flows may play a role as confining units in the groundwater flow system underlying the Pahute Mesa (PM) area of underground nuclear testing at the Nevada National Security Site (NNSS) (Figure 1). Of geological significance, the PM testing area is largely situated within the Silent Canyon caldera complex (SCCC), which includes both tuffs and lavas that were fed by (and are connected to) intrusive rock units such as feeder dikes prior to and during volcanic eruptions (Orkild et al., 1968; Byers et al., 1976a). Groundwater modeling results presented in this report support extension of “pool-dam” and “breach scenario” concepts presented in Jackson and Fenelon (2018) and Jackson et al. (2021) to low-permeability intrusive confining units (ICUs) such as feeder dikes that are expected to dissect and ring silicic calderas. As laterally extensive, steeply-dipping, and sub-parallel planar structures, ICUs may further compartmentalize groundwater flow in some areas of the volcanic aquifer system at PM. ICUs may explain unusually high horizontal hydraulic gradient southwest of Cheshire. Breaching of an ICU within which the Cheshire test was emplaced may explain changes in water levels before and after the Cheshire test was detonated in the U-20n emplacement hole on 2/14/76 (USDOE, 2015b). This analysis of the effects of ICUs on groundwater flow at PM addresses a need to evaluate uncertainty in the conceptual model or structural aspects of hydrologic source term (HST) or corrective action unit (CAU) models for groundwater flow and contaminant transport (FFACO, 1996, as amended). At Cheshire and possibly other test locations at PM, downgradient extent of radionuclide contamination may be overpredicted by not including the confining effects of ICUs. On the other hand, contaminant extent may be underpredicted by not considering transient flow effects and/or the re-equilibrated flow field caused by breaching of an ICU by an underground nuclear test. Near Cheshire, the effects of ICUs may be most apparent and impactful to the groundwater flow system at PM because of an unusual combination of thickness, extent, and frequency of dikes transecting the saturated CHLFA4 aquifer and feeding into the overlying unsaturated rhyolite lava of Windy Wash. Chapters 2, 3, and 4 present geological, geophysical, hydrogeological, and hydrological evidence for ICUs at PM. Chapters 5 and 6 examine effects of ICUs on groundwater flow including analysis by groundwater modeling.

54 ENVIRONMENTAL SCIENCES↗

Long-Term Surveillance and Maintenance Plan for the Salmon, Mississippi, Site

The U.S. Department of Energy (DOE) Office of Legacy Management (LM) prepared this Long-Term Surveillance and Maintenance Plan (LTS&M Plan) for the Salmon, Mississippi, Site (the Salmon site) to describe LM’s plan and policy for future site activities. The Salmon site consists of 1470 acres in Lamar County, Mississippi, approximately 10 miles west of Purvis, Mississippi, and about 21 miles southwest of Hattiesburg, Mississippi. The site is located over a large subsurface salt formation referred to as the Tatum Salt Dome. Two nuclear tests (Project Dribble) and two gas explosive tests (Project Miracle Play) were conducted in the salt dome between 1964 and 1970. Salmon, the first nuclear test, was conducted on October 22, 1964, and created a cavity approximately 2700 feet (ft) below ground surface (bgs). The second nuclear test, Sterling, was conducted on December 3, 1966. The Sterling test and the two gas explosions—Diode Tube on February 2, 1969, and Humid Water on April 19, 1970—were all conducted in the cavity created by the Salmon test. The four explosions were conducted as part of the U.S. Atomic Energy Commission’s (AEC’s) Vela Uniform program. Testing at the site ended in 1970 after the second gas detonation. The tests resulted in residual contamination and postdetonation features that require long-term oversight.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

A section 110 evaluation of the huron king test chamber, area 3, nevada national security site, nye county, nevada

The U.S. Department of Energy, National Nuclear Security Administration Nevada Field Office tasked Desert Research Institute (DRI) with the identification and evaluation of the Huron King Test Chamber as part of their cultural resources program obligations under Section 110 of the National Historic Preservation Act. The Huron King nuclear test was a vertical line-of-sight weapons effects test that took place in Area 3 on June 24, 1980. Unique to this event was a specially designed aboveground test chamber that held a model defense communications satellite in a vacuum tank meant to replicate the space environment. Sponsored by the Defense Nuclear Agency, the purpose of the experiment was to understand the response of the satellite and its materials and equipment to an electromagnetic pulse and attendant radiation. Between July and August 2022, DRI conducted an archival review on the Huron King experiment and its associated test chamber. Subsequently, pedestrian fieldwork was undertaken at the Huron King Test Chamber by DRI on September 29, 2022. During fieldwork, the outside of the test chamber was documented using a Nevada State Historic Preservation Office Architectural Resource Assessment form. This effort included verifying the substructures that compose the test chamber as determined by the archival review, as well as obtaining a detailed photographic recordation of the exterior and assessing its current condition. Notably, the site where the Huron King test took place has been abandoned and almost entirely naturalized. All of the portable instrumentation trailers, communications and data cabling, and winch systems used to retract the test chamber following the detonation were removed after completion of the experiment in 1980. Only the subsidence crater and the test chamber remain as physical evidence of this experiment. Based on these findings, DRI recommends that the Huron King Test Chamber is eligible for listing in the National Register of Historic Places (NRHP) at the local level under Significance Criteria A and C and that it meets Criteria Consideration G for properties less than 50 years old.

54 ENVIRONMENTAL SCIENCES↗

Summary of FY25 activities on the project Realistic Reaction Evaluations for Fission Products Off Stability (RREFPOS)

Applications such nonproliferation, post-detonation forensics, spent-fuel assay, reactor burnup and design, as well as astrophysics, rely on the accurate description of the neutron interaction with unstable fission products. Current neutron-induced cross-section descriptions for these nuclei are either non-existent or based on simplified assumptions, leading to unquantified impacts on predicted cross-sections. The goal of the Realistic Reaction Evaluations for Fission Products Off Stability (RREFPOS) project is to develop a reproducible methodology leading to a more predictive and realistic new set of evaluated nuclear data, improving the reliability of applications involving fission products off stability. The current report documents the activities related to the RREFPOS project in its first year, corresponding to the Fiscal Year of 2025 (FY25).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗