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At least 217 records · Page 12

High-order harmonics and the reverse of the squaring up process in the triangular-lattice magnet HoPdAl 4 ⁢Ge 2

We uncover high-order harmonics and the reverse of the squaring-up process, in terms of analyzing the evolution of magnetic orders in a centrosymmetric layered triangular-lattice magnet HoPdAl 4 ⁢Ge 2 , based on a detailed study of the crystal structure, magnetic susceptibility, magnetization, heat capacity, and magnetic structure. Temperature dependencies of magnetic susceptibility and heat capacity show two magnetic transitions at T N = 10.5 K and T t = 5.5 K. Below T N , Ho 3+ spins order antiferromagnetically as a transverse spin-density wave with the propagation vector k 1 = (001.5 – δ) with δ ≈ 0.18. Upon further cooling through T t , the high-order harmonics with k n = (001.5 – nδ), n = 3, 5, 7 develop, suggesting a squaring-up process. It is surprising that the squaring-up process does not continue down to 0 K but reverses the trend below 3 K. Magnetic-field-induced metastable transitions were observed in M⁡(H) curves with the fields applied both parallel and perpendicular to the triangular-lattice plane. Neutron-diffraction results suggest that the magnetization process in HoPdAl 4 ⁢Ge 2 involves the conversion of k n = (001.5 – n⁢δ) with n = 1, 3, 5, 7, to a ferromagnetic k F = (000) component. It is worth noting that the already weak seventh harmonic magnetic peak is enhanced by applying a small magnetic field in the ab plane at 1.5 K or warming up to 3 K, accompanied by a slight decrease of δ.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Further rotation reversal studies in C-Mod L-mode plasmas

Studies of core toroidal rotation reversal phenomenology in C-Mod deuterium L-mode plasmas have been expanded to include details of the dependences on plasma current and toroidal magnetic field. Rotation reversal occurs at a critical density, and universal scaling indicates that the product of ncritq95R ∼ BT/2, with ncrit in 1020/m3, R in m, and BT in T. Measurements in H and He plasmas exhibit similar behavior, including a connection with the linear Ohmic confinement/saturated Ohmic confinement transition and the cutoff for non-diffusive heat transport. Electron density and ion cyclotron range of frequencies power modulation experiments suggest that the collisionality ν* is a unifying parameter. Strong impurity puffing causes the critical density to increase, indicating that the situation is more complicated than only collisionality, perhaps involving the details of the effects of dilution on ion temperature gradient mode stability.

Physics↗

Comparison of induced magnetospheres at Venus and Titan

Analyses of the similarities and differences of the magnetic tails of Venus and Titan are presented. Voyager 1 data showed that the Titan bipolar tail is produced by passage through the subsonic plasma flow of Saturn's magnetosphere. Venera 9 and 10 gathered data on the Venus tail, which is produced by the interaction of the Venus atmosphere and ionosphere with the solar wind. Both nonmagnetic bodies have induced two-lobe magnetic tails, field reversal in the tail and display characteristics of decreased energetic electron densities. The plasma flow is supersonic near the Venus tail boundary but not near Titan. Magnetic merging of the tail lobes is continuous behind Titan and irregular in the Venus tail.

Verigin, M. I.↗

Magnetic Control of Solutal Buoyancy Driven Convection

Volumetric forces resulting from local density variations and gravitational acceleration cause buoyancy induced convective motion in melts and solutions. Solutal buoyancy is a result of concentration differences in an otherwise isothermal fluid. If the fluid also exhibits variations in magnetic susceptibility with concentration then convection control by external magnetic fields can be hypothesized. Magnetic control of thermal buoyancy induced convection in ferrofluids (dispersions of ferromagnetic particles in a carrier fluid) and paramagnetic fluids have been demonstrated. Here we show the nature of magnetic control of solutal buoyancy driven convection of a paramagnetic fluid, an aqueous solution of Manganese Chloride hydrate. We predict the critical magnetic field required for balancing gravitational solutal buoyancy driven convection and validate it through a simple experiment. We demonstrate that gravity driven flow can be completely reversed by a magnetic field but the exact cancellation of the flow is not possible. This is because the phenomenon is unstable. The technique can be applied to crystal growth processes in order to reduce convection and to heat exchanger devices for enhancing convection. The method can also be applied to impose a desired g-level in reduced gravity applications.

Ramachandran, N.↗

Observed relationships between electric fields and auroral particle precipitation.

Simultaneous electric field and plasma observations with the low-altitude polar-orbiting satellite Injun 5 have provided a comprehensive survey of convection electric fields and their association with magnetospheric plasma phenomena. The most prominent features of the convection electric fields are reversals located at high magnetic latitudes, with generally antisunward convection poleward and sunward convection equatorward of the electric field reversal location. The electric field reversal is interpreted as the boundary between open and closed magnetic field lines. During local day the electric field reversal is observed to coincide with the equatorward boundary of the polar cusp. The plasma flow in the dayside polar cusp region is dominantly E-W, away from the stagnation point, the convection velocities typically being about 1 km/sec. At local evening, 'inverted V' electron precipitation bands are observed near or at the position of the electric field reversal. In the local late-evening sector the electric field reversal becomes less distinct, and often no single well-defined electric field reversal can be identified. In all cases the inverted V electron precipitation events are closely associated with large, typically greater than 30 mV/m, irregular electric field fluctuations with time scales of a few seconds or less.

Gurnett, D. A.↗

Modeling of Magnetic Properties of Magnetorheological Elastomers Using JA Hysteresis Model

Magnetorheological elastomers (MREs) are composite materials that consist of magnetically permeable particles in a nonmagnetic polymeric matrix. Under the influence of an external magnetic field, a reversible deformation change occurs in the mechanical properties of these materials. Due to their coupled magnetomechanical response, these materials have been found suitable for a range of applications including tunable vibration absorbers, sensors, and actuators. Notably, improvement of such devices are prerequisites to efficient energy conversion systems, hence the need to understand further the MRE technology. The Jiles-Atherton (JA) theory takes into consideration the magneto-coupling experienced by effective domains in a magnetic material. Algorithm based on the theory yields five model parameters; saturation magnetization (M s ), domain density (a), domain coupling (α), loss coefficient (k), and reversibility (c). Using JA theory, model parameters were calculated and linked to the physical attributes of Fe powder and isotropic MRE. The results show that the calculated Ms for the MRE is reasonably related to that of the Fe powder by a factor of the particle's volume fraction used in the MRE. Further, the calculated k, a, and α provided support for the reduced pinning factor, domain density, and increased domain coupling in the MRE due to the changes in the domain structure between the two materials. From the calculated JA parameters, finite-element modeling (FEM) of the MRE hysteresis loop was performed. The analysis showed that the modeled magnetic properties including coercivity, remanence, and coordinates of the hysteresis loop tip vary with geometric position.

42 ENGINEERING↗

Interface-induced sign reversal of the anomalous Hall effect in magnetic topological insulator heterostructures

The Berry phase picture provides important insights into the electronic properties of condensed matter systems. The intrinsic anomalous Hall (AH) effect can be understood as the consequence of non-zero Berry curvature in momentum space. Here, we fabricate TI/magnetic TI heterostructures and find that the sign of the AH effect in the magnetic TI layer can be changed from being positive to negative with increasing the thickness of the top TI layer. Our first-principles calculations show that the built-in electric fields at the TI/magnetic TI interface influence the band structure of the magnetic TI layer, and thus lead to a reconstruction of the Berry curvature in the heterostructure samples. Based on the interface-induced AH effect with a negative sign in TI/V-doped TI bilayer structures, we create an artificial “topological Hall effect”-like feature in the Hall trace of the V-doped TI/TI/Cr-doped TI sandwich heterostructures. Our study provides a new route to create the Berry curvature change in magnetic topological materials that may lead to potential technological applications.

36 MATERIALS SCIENCE↗

The Heliospheric Magnetic Field Over the Hale Cycle

The concept that open magnetic flux of the Sun (rooted with one and only one footpoint at the Sun) is a conserved quantity is taking root in the heliospheric community. Observations show that the Sun's open magnetic flux returns to the baseline from one solar minimum to the next. The temporary enhancement in the 1AU heliospheric magnetic flux near solar maximum can be accounted for by the temporary creation of closed magnetic flux (with two footpoints at the Sun) during the ejection of coronal mass ejections (CMEs), which are more frequent near solar maximum. As a part of the International Heliophysical Year activities, this paper reviews two recently discussed consequences of open flux conservation: the reversal of open magnetic flux over the solar cycle driven by Coronal Mass Ejections and the impacts of open flux conservation on the global structure of the heliospheric magnetic field. These studies demonstrate the inherent linkages between coronal mass ejections, footpoint motions back at the Sun, and the global structure and evolution of the heliospheric magnetic field.

Schwardron, N. A.↗

Minimum dissipation rates in magnetohydrodynamics

Minimum dissipation rate states are explored for a current-carrying channel of magnetofluid, supported by a dc magnetic field and driven by an applied electric field. The minimization is carried out subject to the constraints of constant axial (toroidal) magnetic flux and constant time-averaged rate of supply of magnetic helicity. The solutions of the resulting Euler-Lagrange equations are sensitive to boundary conditions on the current density j. One set of boundary conditions on j leads to the same consequences as Taylor's 'minimum-energy' theory. A different set leads to significantly different consequences, including a departure from the 'force-free' magnetic profile and a toroidal component of current density that does not reverse at the wall when the toroidal magnetic field reverses.

Montgomery, David↗

Subminiature micropower digital recorder

High-density digital data, collected periodically or randomly from multiplicity of sensors, are recorded by subminiature recorder. Magnetic recording head is energized with suitable pulsatile signals to reverse polarization on magnetically-sensitive tape while tape is immobilized at recording head. Prior to next recording, set tape so new area of tape is at recording head.

Goodman, R. M.↗

Logical and Physical Reversibility of Conservative Skyrmion Logic

Magnetic skyrmions are nanoscale whirls of magnetism that can be propagated with electrical currents. The repulsion between skyrmions inspires their use for reversible computing based on the elastic billiard ball collisions proposed for conservative logic in 1982. In this letter, we evaluate the logical and physical reversibility of this skyrmion logic paradigm, as well as the limitations that must be addressed before dissipation-free computation can be realized.

42 ENGINEERING↗

Observed relationships between electric fields and auroral particle precipitation

Simultaneous electric field and plasma observations with the low altitude, polar orbiting satellite Injun (Hawkeye) 5 provided a comprehensive survey of convection electric fields and their association with magnetospheric plasma phenomena. The most prominent features of the convection electric fields are reversals located at high magnetic latitudes, with generally anti sunward convection poleward convection equatorward of the electric field reversal location. The electric field reversal is interpreted as the boundary between open and closed magnetic field lines. To investigate the electric field and plasma interrelationships during a polar magnetic substorm, a series of passes obtained prior to and during a substrom is presented. Large, anti sunward convection velocities were detected over the polar cap several tens of minutes before the onset of the expansive phase of the substrom. These convection velocities gradually decreased during the decay phase of the substrom. Measurements of enhanced anti sunward flow over the polar cap region are generally consistent with concepts of the origin of substroms.

Gurnett, D. A.↗

Mars Crustal Remanent Magnetism: An Extinct Dynamo Leaves a Record of Field Reversals in the Heavily Cratered Highlands

The Mars Global Surveyor spacecraft, in a highly elliptical polar orbit about Mars, obtained vector magnetic field measurements just above the surface of Mars (altitudes > 100 kilometers). Crustal magnetization, largely confined to the most ancient, heavily cratered Mars highlands, is frequently organized in east-west trending linear features, the largest of which extends over 2000 km. A representative set of survey passes are modeled using uniformly magnetized thin plates and a generalized inverse methodology. Crustal remanent magnetization exceeds that deduced for the largest terrestrial magnetic anomalies by more than an order of magnitude. Groups of quasi-parallel linear features of alternating magnetic polarity are found. They are reminiscent of similar magnetic features associated with sea floor spreading and crustal genesis on Earth but with a much larger spatial scale.

Connerney, John E.↗

Modeling and Measuring the Stress Distribution in Soft Magnetic Cores due to Epoxy Impregnation and Curing

Understanding the effects of viscoelastic relaxation of stresses is critical in electric motor and inductor applications, where the magnetic material is fully or partially comprised of an amorphous phase and impregnated in an epoxy. Magnetic Amorphous Nanocomposites (MANCs) are a class of recently developed high-frequency magnetic materials that exhibit low magnetic hysteresis, high saturation flux density and very low AC magnetic losses. MANCs are formed as long, thin ribbons, a shape factor that minimizes eddy current-induced self-heating. This feature, in addition to their 1 GPa strength, and makes them attractive candidates for high-speed, high-power density, electric motors. MANCs are used in the form of tape-wound cores (TWCs). During the manufacturing process, the cores are impregnated with liquid epoxy between each layer of ribbon. Validated knowledge of the stresses imposed by the manufacturing process and during operation is necessary to understand motor performance limitations with respect to strength. Magnetostriction, the strain imposed by reversal of the magnetic field, also affects performance. When the epoxy cures, it contracts volumetrically by 8%, imposing radial and circumferential stresses that vary along the radial direction. To date, these stresses have received little attention in the literature. Here, we model the stress distribution throughout a TWC due to epoxy curing. Strain gauge measurements reported here indicate substantially lower tangential strain than model values, which is beneficial and which we attribute to viscoelastic relaxation of the epoxy layers. We will incorporate a constitutive model of this viscoelastic relaxation, and conduct more detailed strain measurements to understand how this takes

24 POWER TRANSMISSION AND DISTRIBUTION↗

Intrinsic even-odd thickness-driven anomalous Hall effect in epitaxial MnBi2⁢Te4 thin films

We demonstrate precise control of magnetism in MnBi2⁢Te4 thin films through careful synthesis by molecular beam epitaxy, achieving minimal defects and accurate layer thickness control. By optimizing Mn-Bi-Te ratios and growth temperatures, we minimize detrimental self-doping effects and accurately target integer-layer films. X-ray diffraction and reflectivity provide quantitative measures of film quality and thickness. When these macroscale probes of structure and thickness are integrated with magnetotransport measurements, a striking even-odd layer dependence of the anomalous Hall effect is revealed. Odd-layer films exhibit a large hysteresis up to the Néel temperature (∼25K), consistent with noncompensated antiferromagnetism, while even-layer films show minimal response, as expected for an antiferromagnet. The sign of the anomalous Hall effect exhibits a sign reversal for intrinsic magnetism versus magnetism associated with defects. This work identifies critical factors for inducing pure, noncompensated ferromagnetism and reveals the characteristics of the intrinsic anomalous Hall effect in MnBi2⁢Te4, which together is a step toward realizing the zero-field quantum anomalous Hall effect in topological materials.

Mallick, Deb [ORNL] (ORCID:000900005806411X)↗

Coercive Fields Exceeding 30 T in the Mixed-Valence Single-Molecule Magnet (Cp iPr5 ) 2 Ho 2 I 3

Mixed-valence dilanthanide complexes of the type (Cp iPr5 ) 2 Ln 2 I 3 (Cp iPr5 = pentaisopropylcyclopentadienyl; Ln = Gd, Tb, Dy) featuring a direct Ln–Ln σ-bonding interaction have been shown to exhibit well-isolated high-spin ground states and, in the case of the Tb and Dy variants, a strong axial magnetic anisotropy that gives rise to a large magnetic coercivity. Here, we report the synthesis and characterization of two new mixed-valence dilanthanide compounds in this series, (Cp iPr5 ) 2 Ln 2 I 3 (1-Ln; Ln = Ho, Er). Both compounds feature a Ln–Ln bonding interaction, the first such interaction in any molecular compounds of Ho or Er. Like the Tb and Dy congeners, both complexes exhibit high-spin ground states arising from strong spin–spin coupling between the lanthanide 4f electrons and a single σ-type lanthanide–lanthanide bonding electron. Beyond these similarities, however, the magnetic properties of the two compounds diverge. In particular, 1-Er does not exhibit observable magnetic blocking or slow magnetic relaxation, while 1-Ho exhibits magnetic blocking below 28 K, which is the highest temperature among Ho-based single-molecule magnets, and a spin reversal barrier of 556(4) cm –1 . Additionally, variable-field magnetization data collected for 1-Ho reveal a coercive field of greater than 32 T below 8 K, more than 6-fold higher than observed for the bulk magnets SmCo 5 and Nd 2 Fe 14 B, and the highest coercive field reported to date for any single-molecule magnet or molecule-based magnetic material. Multiconfigurational calculations, supported by far-infrared magnetospectroscopy data, reveal that the stark differences in magnetic properties of 1-Ho and 1-Er arise from differences in the local magnetic anisotropy of the lanthanide centers.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗