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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Observation of second harmonic generation in doped polymeric carbon monoxide
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In situ analysis of gas generation in lithium ion batteries with different carbonate-based electrolytes
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Field ionization characteristics of an ion source array for neutron generators
A new deuterium ion source is being developed to improve the performance of existing compact neutron generators. The ion source is a microfabricated array of metal tips with an integrated gate (i.e., grid) and produces deuterium ions by field ionizing (or field desorbing) a supply of deuterium gas. Deuterium field ion currents from arrays at source temperatures of 77 K and 293 K are studied. Ion currents from single etched-wire tips operating under the same conditions are used to help understand array results. I-F characteristics of the arrays were found to follow trends similar to those of the better understood single etched-wire tip results; however, the fields achieved by the arrays are limited by electrical breakdown of the structure. Neutron production by field ionization at 293 K was demonstrated for the first time from microfabricated array structures with integrated gates.
Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films
We experimentally demonstrate efficient third harmonic generation from an indium tin oxide nanofilm (λ/42 thick) on a glass substrate for a pump wavelength of 1.4 μm. A conversion efficiency of 3.3 × 10{sup −6} is achieved by exploiting the field enhancement properties of the epsilon-near-zero mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.
Quadrupole second harmonic generation and sum-frequency generation in ZnO quantum dots
The second harmonic generation (SHG) and the sum frequency generation (SFG) processes are investigated in the conduction band states of the singly charged ZnO quantum dot (QD) embedded in the HfO{sub 2}, and the AlN matrices. With two optical fields of frequency ω{sub p} and ω{sub q} incident on the dot, we study the variation with frequency of the second order nonlinear polarization resulting in SHG and SFG, through the electric dipole and the electric quadrupole interactions of the pump fields with the electron in the dot. We obtain enhanced value of the second order nonlinear susceptibility in the dot compared to the bulk. The effective mass approximation with the finite confining barrier is used for obtaining the energy and wavefunctions of the quantized confined states of the electron in the conduction band of the dot. Our results show that both the SHG and SFG processes depend on the dot size, the surrounding matrix and the polarization states of the pump beams.
Generation of strong pulsed magnetic fields using a compact, short pulse generator
The generation of strong magnetic fields (∼50 T) using single- or multi-turn coils immersed in water was studied. A pulse generator with stored energy of ∼3.6 kJ, discharge current amplitude of ∼220 kA, and rise time of ∼1.5 μs was used in these experiments. Using the advantage of water that it has a large Verdet constant, the magnetic field was measured using the non-disturbing method of Faraday rotation of a polarized collimated laser beam. This approach does not require the use of magnetic probes, which are sensitive to electromagnetic noise and damaged in each shot. It also avoids the possible formation of plasma by either a flashover along the conductor or gas breakdown inside the coil caused by an induced electric field. In addition, it was shown that this approach can be used successfully to investigate the interesting phenomenon of magnetic field enhanced diffusion into a conductor.
Thermoelectric power generation: from new materials to devices
Thermoelectric technology offers the opportunity of direct conversion between heat and electricity, and new and exciting materials that can enable this technology to deliver higher efficiencies have been developed in recent years. This mini-review covers the most promising advances in thermoelectric materials as they pertain to their potential in being implemented in devices and modules with an emphasis on thermoelectric power generation. Classified into three groups in terms of their operating temperature, the thermoelectric materials that are most likely to be used in future devices are briefly discussed. Here, we summarize the state-of-the-art thermoelectric modules/devices, among which nanostructured PbTe modules are particularly highlighted. At the end, key issues and the possible strategies that can help thermoelectric power generation technology move forward are considered.
PV Ramping in a Distributed Generation Environment: A Study Using Solar Measurements; Preprint
Variability in Photovoltaic (PV) generation resulting from variability in the solar radiation over the PV arrays is a topic of continuing concern for those involved with integrating renewables onto existing electrical grids. The island of Lanai, Hawaii is an extreme example of the challenges that integrators will face due to the fact that it is a small standalone grid. One way to study thisproblem is to take high-resolution solar measurements in multiple locations and model simultaneous PV production for various sizes at those locations. The National Renewable Energy Laboratory (NREL) collected high-resolution solar data at four locations on the island where proposed PV plants will be deployed in the near future. This data set provides unique insight into how the solar radiationmay vary between points that are proximal in distance, but diverse in weather, due to the formation of orographic clouds in the center of the island. Using information about each proposed PV plant size, power output was created at high resolution. The team analyzed this output to understand power production ramps at individual locations and the effects of aggregating the production from all fourlocations. Hawaii is a unique environment, with extremely variable events occurring on a daily basis. This study provided an excellent opportunity for understanding potential worst-case scenarios for PV ramping. This paper provides an introduction to the datasets that NREL collected over a year and a comprehensive analysis of PV variability in a distributed generation scenario.
Shape Memory Alloys and their Applications in Power Generation and Refrigeration
The shape memory effect is closely related to the reversible martensitic phase transformation, which is diffusionless and involves shear deformation. The recoverable transformation between the two phases with different crystalline symmetry results in reversible changes in physical properties such as electrical conductivity, magnetization, and elasticity. Accompanying the transformation is a change of entropy. Fascinating applications are developed based on these changes. In this paper, the history, fundamentals and technical challenges of both thermoelastic and ferromagnetic shape memory alloys are briefly reviewed; applications related to energy conversion such as power generation and refrigeration as well as recent developments will be discussed.
InDEEP, DEEC-Tec, and Direct Generation Synergies for Ocean Wave Energy: Wave Energy Scotland's Direct Generation Programme Review
The presentation highlights: (i) how DEEC-Tec, advanced through the U.S. DOE's InDEEP Prize, holds the potential to redefine ocean wave energy conversion through modular, embedded energy conversion; (ii) a global scan that identified 158 participants and 35 promising concepts, showcasing strong international momentum; (iii) InDEEP's innovation-first approach and how it complements Wave Energy Scotland's structured Direct Generation research; and (iv) the ongoing and possible future collaborative pathways for co-funded trials, joint metric/standards developments, and maturation of these technologies toward and real-world deployment.
Generation of extremely low frequency chorus in Van Allen radiation belts: ELF CHORUS GENERATION
Recent studies have shown that chorus can efficiently accelerate the outer radiation belt electrons to relativistic energies. Chorus, previously often observed above 0.1 equatorial electron gyrofrequency f ce , was generated by energetic electrons originating from Earth's plasmasheet. Chorus below 0.1 f ce has seldom been reported until the recent data from Van Allen Probes but its origin has not been revealed so far. Because electron resonant energy can approach the relativistic level at extremely low frequency relativistic effects should be considered in the formula for whistler-mode wave growth rate. Here we report high-resolution observations during the 14 October 2014 small storm and firstly demonstrate, using a fully relativistic simulation, that electrons with the high energy tail population and relativistic pitch angle anisotropy can provide free energy sufficient for generating chorus below 0.1 f ce . The simulated wave growth displays a very similar pattern to the observations. Finally, the current results can be applied to Jupiter, Saturn and other magnetized planets.
Inter‐Fullerene Electronic Coupling Controls the Efficiency of Photoinduced Charge Generation in Organic Bulk Heterojunctions
Photoinduced charge generation (PCG) dynamics are notoriously difficult to correlate with specific molecular properties in device relevant polymer:fullerene organic photovoltaic blend films due to the highly complex nature of the solid state blend morphology. Here, this study uses six judiciously selected trifluoromethylfullerenes blended with the prototypical polymer poly(3‐hexylthiophene) and measure the PCG dynamics in 50 fs–500 ns time scales with time‐resolved microwave conductivity and femtosecond transient absorption spectroscopy. The isomeric purity and thorough chemical characterization of the fullerenes used in this study allow for a detailed correlation between molecular properties, driving force, local intermolecular electronic coupling and, ultimately, the efficiency of PCG yield. The findings show that the molecular design of the fullerene not only determines inter‐fullerene electronic coupling, but also influences the decay dynamics of free holes in the donor phase even when the polymer microstructure remains unchanged.
Controlled Generation of Singlet Oxygen in Living Cells with Tunable Ratios of the Photochromic Switch in Metal–Organic Frameworks
Abstract Development of a photosensitizing system that can reversibly control the generation of singlet oxygen ( 1 O 2 ) is of great interest for photodynamic therapy (PDT). Recently several photosensitizer–photochromic‐switch dyads were reported as a potential means of the 1 O 2 control in PDT. However, the delivery of such a homogeneous molecular dyad as designed (e.g., optimal molar ratio) is extremely challenging in living systems. Herein we show a Zr‐MOF nanoplatform, demonstrating energy transfer‐based 1 O 2 controlled PDT. Our strategy allows for tuning the ratios between photosensitizer and the switch molecule, enabling maximum control of 1 O 2 generation. Meanwhile, the MOF provides proximal placement of the functional entities for efficient intermolecular energy transfer. As a result, the MOF nanoparticle formulation showed enhanced PDT efficacy with superior 1 O 2 control compared to that of homogeneous molecular analogues.