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At least 217 records · Page 12

An Aerosol Extinction-to-Backscatter Ratio Database Derived from the NASA Micro-Pulse Lidar Network: Applications for Space-based Lidar Observations

Backscatter lidar signals are a function of both backscatter and extinction. Hence, these lidar observations alone cannot separate the two quantities. The aerosol extinction-to-backscatter ratio, S, is the key parameter required to accurately retrieve extinction and optical depth from backscatter lidar observations of aerosol layers. S is commonly defined as 4*pi divided by the product of the single scatter albedo and the phase function at 180-degree scattering angle. Values of S for different aerosol types are not well known, and are even more difficult to determine when aerosols become mixed. Here we present a new lidar-sunphotometer S database derived from Observations of the NASA Micro-Pulse Lidar Network (MPLNET). MPLNET is a growing worldwide network of eye-safe backscatter lidars co-located with sunphotometers in the NASA Aerosol Robotic Network (AERONET). Values of S for different aerosol species and geographic regions will be presented. A framework for constructing an S look-up table will be shown. Look-up tables of S are needed to calculate aerosol extinction and optical depth from space-based lidar observations in the absence of co-located AOD data. Applications for using the new S look-up table to reprocess aerosol products from NASA's Geoscience Laser Altimeter System (GLAS) will be discussed.

Welton, Ellsworth J.↗

In Situ Aerosol Profile Measurements and Comparisons with SAGE 3 Aerosol Extinction and Surface Area Profiles at 68 deg North

Under funding from this proposal three in situ profile measurements of stratospheric sulfate aerosol and ozone were completed from balloon-borne platforms. The measured quantities are aerosol size resolved number concentration and ozone. The one derived product is aerosol size distribution, from which aerosol moments, such as surface area, volume, and extinction can be calculated for comparison with SAGE III measurements and SAGE III derived products, such as surface area. The analysis of these profiles and comparison with SAGE III extinction measurements and SAGE III derived surface areas are provided in Yongxiao (2005), which comprised the research thesis component of Mr. Jian Yongxiao's M.S. degree in Atmospheric Science at the University of Wyoming. In addition analysis continues on using principal component analysis (PCA) to derive aerosol surface area from the 9 wavelength extinction measurements available from SAGE III. Ths paper will present PCA components to calculate surface area from SAGE III measurements and compare these derived surface areas with those available directly from in situ size distribution measurements, as well as surface areas which would be derived from PCA and Thomason's algorithm applied to the four wavelength SAGE II extinction measurements.

Source record↗

Dynamic Weakening (Extinction) of Simple Hydrocarbon-air Counterflow Diffusion Flames by Oscillatory Inflows

This study of laminar non-premixed HC-air flames used an Oscillatory-input Opposed Jet Burner (OOJB) system developed from a previously well-characterized 7.2-mm Pyrex-nozzle OJB system. Over 600 dynamic Flame Strength (FS) measurements were obtained on unanchored (free-floating) laminar Counterflow Diffusion Flames (CFDF's). Flames were stabilized using plug inflows having steady-plus-sinusoidal axial velocities of varied magnitude, frequency, f, up to 1600 Hz, and phase angle from 0 (most data) to 360 degrees. Dynamic FS is defined as the maximum average air input velocity (U(sub air), at nozzle exit) a CFDF can sustain before strain-induced extinction occurs due to prescribed oscillatory peak-to-peak velocity inputs superimposed on steady inputs. Initially, dynamic flame extinction data were obtained at low f, and were supported by 25-120 Hz Hot-Wire cold-flow velocity data at nozzle exits. Later, expanded extinction data were supported by 4-1600 Hz Probe Microphone (PM) pk/pk P data at nozzle exits. The PM data were first obtained without flows, and later with cold stagnating flows, which better represent speaker-diaphragm dynamics during runs. The PM approach enabled characterizations of Dynamic Flame Weakening (DFW) of CFDF's from 8 to 1600 Hz. DFW was defined as % decrease in FS per Pascal of pk/pk P oscillation, namely, DFW = - 100 d(U(sub air) / U(sub air),0Hz) / d(pkpk P). The linear normalization with respect to acoustic pressure magnitude (and steady state (SS) FS) led to a DFW unaffected by strong internal resonances. For the C2H4/N2-air system, from 8 to 20 Hz, DFW is constant at 8.52 plus or minus 0.20 (% weakening)/Pa. This reflects a quasi-steady flame response to an acoustically induced dU(sub air)/dP. Also, it is surprisingly independent of C2H4/N2 mole fraction due to normalization by SS FS. From 20 to approximately 150 Hz, the C2H4/N2 air-flames weakened progressively less, with an inflection at approximately 70 Hz, and became asymptotically insensitive (DFW approximately 0) at approximately 300 Hz, which continued to 1600 Hz. The DFW of CH4-air flames followed a similar pattern, but showed much greater weakening than C2H4/N2-air flames; i.e., the quasi-steady DFW (8 to approximately 15 Hz) was 44.3 %/Pa, or approximately 5x larger, even though the 0 Hz (SS) FS was only 3.0 x smaller. The quasi-steady DFW's of C3H8-air and C2H6-air were intermediate at 34.8 and 20.9 %Pa, respectively. The DFW profiles of all four fuels, at various frequencies, correlated well but non-linearly with respective SS FS's. Notably, the DFW profile for C3H8 air fell more rapidly in the range greater than 15 to 60 Hz, compared with the 1- and 2-carbon fuels. This may indicate a shift in chemical kinetics, and/or O2 transport to a flame that moved closer to the fuel-side. In conclusion, Dynamic Flame Weakening limits appear significant and unique for each fuel, and correlate closely, but non-linearly, with Steady-State Flame Strengths at any given frequency. For reasons unknown, the dynamic flames didn't weaken more at intermediate frequencies (e.g., at 20-50 Hz) than they did at low frequencies (less than 15 Hz), where quasi-steady weakening appears to dominate. Quasi-steady flame weakening ostensibly represents a transient input strain rate maximum that just exceeds the steady-state strain-rate-limited extinction limit for a few cycles. Clearly, further detailed mechanistic understanding is needed in the fall-off region.

Pellett, G.↗

Extinction-to-Backscatter Ratios of Lofted Aerosol Layers Observed During the First Three Months of CALIPSO Measurements

Case studies from the first three months of the Cloud and Aerosol Lidar and Infrared Pathfinder Spaceborne Observations (CALIPSO) measurements of lofted aerosol layers are analyzed using transmittance [Young, 1995] and two-wavelength algorithms [Vaughan et al., 2004] to determine the aerosol extinction-to-backscatter ratios at 532 and 1064 nm. The transmittance method requires clear air below the layer so that the transmittance through the layer can be determined. Suitable scenes are selected from the browse images and clear air below features is identified by low 532 nm backscatter signal and confirmed by low depolarization and color ratios. The transmittance and two-wavelength techniques are applied to a number of lofted layers and the extinction-to-backscatter ratios are compared with values obtained from the CALIPSO aerosol models [Omar et al., 2004]. The results obtained from these studies are used to adjust the aerosol models and develop observations based extinction-to-backscatter ratio look-up tables and phase functions. Values obtained by these techniques are compared to Sa determinations using other independent methods with a goal of developing probability distribution functions of aerosol type-specific extinction to backscatter ratios. In particular, the results are compared to values determined directly by the High Spectral Resolution Lidar (HSRL) during the CALIPSO CloudSat Validation Experiments (CCVEX) and Sa determined by the application of the two-wavelength lidar Constrained Ratio Aerosol Model-fit (CRAM) retrieval approach [Cattrall et al., 2005; Reagan et al., 2004] to the HSRL data. The results are also compared to values derived using the empirical relationship between the multiple-scattering fraction and the linear depolarization ratio by using Monte Carlo simulations of water clouds [Hu et al., 2006].

Omar, Ali H.↗

The Demonstration of a Light Extinction Tomography System at the NASA Glenn Research Center's Icing Research Tunnel

A prototype light extinction tomography system has been developed for acquiring real-time in-situ icing cloud uniformity and density measurements in the NASA Glenn Research Center's Icing Research Tunnel (IRT). These measurements are currently obtained through periodic manual calibrations of the IRT. These calibrations are time consuming and assume that cloud uniformity and density does not greatly vary between the periodic calibrations. It is envisioned that the new light extinction tomography system will provide the means to make these measurements in-situ in real-time and minimize the need for these manual calibrations. This new system uses the principle of light extinction tomography to measure the spray density and distribution in the test section. The prototype system was installed and successfully demonstrated in the Icing Research Tunnel in early 2018. Data sets were acquired for several standard spray and simulated fault conditions to assess system capability and sensitivity. This paper will describe the prototype light extinction system, the theory behind it, and the results of the demonstration test that was conducted in the IRT.

Test Facility↗

The Demonstration of a Light Extinction Tomography System at the NASA Glenn Research Center's Icing Research Tunnel

A prototype light extinction tomography system has been developed for acquiring real-time in-situ icing cloud uniformity and density measurements in the NASA Glenn Research Center's Icing Research Tunnel (IRT). These measurements are currently obtained through periodic manual calibrations of the IRT. These calibrations are time consuming and assume that cloud uniformity and density does not greatly vary between the periodic calibrations. It is envisioned that the new light extinction tomography system will provide the means to make these measurements in-situ in real-time and minimize the need for these manual calibrations. This new system uses the principle of light extinction tomography to measure the spray density and distribution in the test section. The prototype system was installed and successfully demonstrated in the Icing Research Tunnel in early 2018. Data sets were acquired for several standard spray and simulated fault conditions to assess system capability and sensitivity. This paper will describe the prototype light extinction system, the theory behind it, and the results of the demonstration test that was conducted in the IRT.

Tomography↗

The Relationship Of Size Distributions To Spectral (300 - 700 Nm) Extinction Parameterization Of Ambient In Situ Aerosols Measured During FIREX-AQ And The Influence Of Aerosol Composition

Hyperspectral (300 - 700 nm, 0.7 nm resolution) aerosol extinction spectra were measured at seven fires in six states in the western United States during the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) field campaign in July and August 2019. Obtained using an in situ aerosol sampling method, these spectra are directly comparable to other in situ aerosol measurements such as size distribution and composition. A previous deployment of the in situ Spectral Aerosol Extinction (SpEx) instrument that measured fine mode aerosols (50% size cut of 1.3 µm particle diameter) around the Korean peninsula showed that over this spectral range 2nd order polynomials provided a better fit to the logarithmically transformed spectra than linear fits (representative of Ångström exponents). The two fit parameters (a1, a2) of the polynomials are related to the classic Ångström exponent but provide additional information via their two-dimensional parameter space. The previous work was limited by the lack of commensurate size distribution information. Here, using the FIREX-AQ spectra set it is possible to expand on the previous analysis in three specific ways: 1) size distribution information is available to further elucidate how size distribution maps into (a1, a2) space, 2) the sampled size distributions include larger particles than the Korean study, and 3) the FIREX-AQ data set exhibits smoke-related spectral features in the UV part of the spectrum that are not present in background air nor were they observed previously in the Korean study. The UV spectral features are particularly intriguing as they likely arise from the absorption component of the extinction measurement and therefore may be related to composition. The relationships between the ambient in situ aerosol size distributions, the extinction spectra, and composition will be presented.

Carolyn Jordan↗

OMPS LP Version 2.0 Multi-wavelength Aerosol Extinction Coefficient Retrieval Algorithm

The OMPS Limb Profiler (LP) instrument is de-signed to provide high-vertical-resolution ozone and aerosol profiles from measurements of the scattered solar radiation in the 290–1000 nm spectral range. It collected its first Earth limb measurement on 10 January 2012 and continues to provide daily global measurements of ozone and aerosol profiles from the cloud top up to 60 and 40 km, respectively. The relatively high vertical and spatial sampling allow detection and tracking of sporadic events when aerosol particles are injected into the stratosphere, such as volcanic eruptions or pyro cumulonimbus (PyroCb) events. In this paper we discuss the newly released Version 2.0 OMPS multi-wavelength aerosol extinction coefficient retrieval algorithm. The algorithm now produces aerosol extinction profiles at 510, 600, 674, 745, 869 and 997 nm wavelengths. The OMPS LP Version 2.0 data products are compared to the SAGE III/ISS, OSIRIS and CALIPSO missions and shown to be of good quality and suitable for scientific studies. The comparison shows significant improvements in the OMPS LP retrieval performance in the Southern Hemisphere (SH) and at lower altitudes. These improvements arise from use of the longer wavelengths, in contrast with the V1.0 and V1.5 OMPS aerosol retrieval algorithms, which used radiances only at 675 nm and therefore had limited sensitivity in those regions. In particular, the extinction coefficients at 745, 869 and 997 nm are shown to be the most accurate, with relative accuracies and precisions close to 10% and 15%, respectively, while the 675 nm relative accuracy and precision are on the order of 20%. The 510 nm extinction coefficient is shown to have limited accuracy in the SH and is only recommended for use between 20–24 km and only in the Northern Hemisphere. The V2.0 retrieval algorithm has been applied to the complete set of OMPS LP measurements, and the new dataset is publicly available.

OMPS↗

An Evaluation of Biomass Burning Aerosol Mass, Extinction, and Size Distribution in Geos Using Observations From Camp2EX

Biomass burning aerosol impacts aspects of the atmosphere and Earth system through radiative forcing, serving as cloud condensation nuclei, and air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in numerical weather prediction and climate models or reanalysis products. Using observations collected as part of the Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) in August through October of 2019, aerosol concentration and optical properties are evaluated within the Goddard Earth Observing System (GEOS) and its underlying aerosol module, GOCART. In the operational configuration, GEOS assimilates aerosol optical depth observations at 550 nm to constrain aerosol fields. Particularly for biomass burning aerosol, without the assimilation of aerosol optical depth, aerosol extinction is underestimated compared to observations collected in the Philippines region during the CAMP2Ex campaign. The assimilation process adds excessive amounts of carbon to account for the underestimated extinction, resulting in positive biases in the mass of black and organic carbon, especially within the boundary layer, relative to in situ observations from the Langley Aerosol Research Group Experiment. Counteracting this, GEOS is deficient in sulphate and nitrate aerosol just above the boundary layer. Aside from aerosol mass, extinction within GEOS is a function of ambient relative humidity and an assumed particle size distribution. The relationship between dry and ambient extinction in GEOS reveals that hygroscopic growth is too aggressive within the model for biomass burning aerosol. An additional concern lies in the assumed particle size distribution for GEOS, which has a mode radius that is too small for organic carbon. Variability in the observed particle size distribution for biomass burning aerosol within a single flight also illuminates the fact that a single assumed particle size distribution is not sufficient and that for a proper representation, a more advanced aerosol module with GEOS may be necessary.

Aerosol Mass↗

Extinction of Solid Diffusion Flame in Microgravity: Details of Quenching and Blowoff Processes

Long duration microgravity experiments aboard the International Space Station determine diffusion flame extinction limits of PMMA spheres. Upon ignition from an electrically-heated coil, the 4-cm-diameter samples are exposed to forced flows ranging from 0.2 to 80 cm/s and an oxygen ranging from 13 to 28% in one atmosphere total pressure. Extinction is reached as oxygen concentration gradually decreases by natural depletion. Five extinction tests are presented at different flow velocities and oxygen concentrations. Quenching at low velocity is observed with the flame tip shrinking upstream and blowoff is observed when a hole forms in the flame at the forward flow stagnation point. However, these processes are not quasistatic. The quenching motion involves periodic flame tip pulsating toward downstream and shrinking upstream with a continually decreasing flame size at the end of each cycle. In blowoff, the flame base pulsates between the flame hole and the downstream location, although with far fewer cycles compared to quenching. The pulsations appear to be the result of a premixed flame front spreading into a combustible mixture. Two specific cases are discussed. In the first, at very low flow velocity (~ 0.4 cm/s) and elevated oxygen, self-sustained flame tip cyclic pulsations are observed for a lengthy period (~15 minutes). In the second case with a higher flow velocity (50 cm/s), the diffusion flame is stabilized at the shoulder of the spherical sample after local stagnation point blowoff. With steady decrease in ambient oxygen due to depletion, spinning flamelets are formed. The long-duration microgravity environment makes it possible to observe. these interesting and detailed extinction processes.

Flame quenching↗

An Assessment of Kinetic Models for Ammonia Flame Extinction

The growing interest in using ammonia as a carbon-neutral replacement fuel has prompted numerous recent research efforts towards understanding fundamental combustion characteristics and chemical kinetics of ammonia oxidation. Despite these recent efforts, there remains a large deficiency in extinction limit data for ammonia flames, particularly under elevated pressure and temperature conditions relevant to gas turbines. Even the literature reaction mechanisms developed specifically for ammonia have been untested under gas turbine relevant conditions, and existing kinetic models have shown large variations in laminar flame speed, extinction strain rate, and speciation predictions for NH3–H2 mixtures at ambient conditions. Recent work by Thomas and co-workers, for example, compared different ammonia kinetic models in the literature for predicting their extinction strain rate measurements for non-premixed NH3-H2 counterflow flames, and again have highlighted the discrepancies in model predictions. Here, our work has undertaken to further highlight important reaction pathways for ammonia oxidation that may be responsible for these discrepancies for extinction strain rate predictions, as well as elucidate sensitive reaction steps with large uncertainties that require further attention. This work points to a need for an improved understanding of ammonia combustion chemistry as well as new datasets at elevated pressure and temperature conditions to better constrain rate expressions for key reaction steps.

ammonia, flame, combustion, kinetic, kinetics↗

Extinction of Premixed Counterflow Ammonia-Air Flames

The effects of radiative heat loss and pressure on premixed counterflow ammonia-air flames have been investigated as a function of equivalence ratio. Non-adiabatic counterflow premixed flame simulations incorporating detailed chemistry, transport and radiative heat transfer in the optically thin limit have been employed to elucidate important underlying physics and extinction characteristics. Non-adiabatic counterflow premixed computations show that the combined effects of positive flame stretch and radiative heat loss for sub-unity Lewis number mixtures lead to the extension of the lean flammability limit for ammonia-air flames, revealing a C-shaped curve near the lean flammability limit that exhibits both radiative-induced and stretch-induced extinction states. The computations compare favorably with the experimentally determined extinction stretch rate values for the stretch-induced extinction states over a wide range of equivalence ratios at different pressures up to 6 atm.

10 SYNTHETIC FUELS↗

Optical Extinction Measurements of Dust Density in the GMRO Regolith Test Bin

A regolith simulant test bin was constructed and completed in the Granular Mechanics and Regolith Operations (GMRO) Lab in 2013. This Planetary Regolith Test Bed (PRTB) is a 64 sq m x 1 m deep test bin, is housed in a climate-controlled facility, and contains 120 MT of lunar-regolith simulant, called Black Point-1 or BP-1, from Black Point, AZ. One of the current uses of the test bin is to study the effects of difficult lighting and dust conditions on Telerobotic Perception Systems to better assess and refine regolith operations for asteroid, Mars and polar lunar missions. Low illumination and low angle of incidence lighting pose significant problems to computer vision and human perception. Levitated dust on Asteroids interferes with imaging and degrades depth perception. Dust Storms on Mars pose a significant problem. Due to these factors, the likely performance of telerobotics is poorly understood for future missions. Current space telerobotic systems are only operated in bright lighting and dust-free conditions. This technology development testing will identify: (1) the impact of degraded lighting and environmental dust on computer vision and operator perception, (2) potential methods and procedures for mitigating these impacts, (3) requirements for telerobotic perception systems for asteroid capture, Mars dust storms and lunar regolith ISRU missions. In order to solve some of the Telerobotic Perception system problems, a plume erosion sensor (PES) was developed in the Lunar Regolith Simulant Bin (LRSB), containing 2 MT of JSC-1a lunar simulant. PES is simply a laser and digital camera with a white target. Two modes of operation have been investigated: (1) single laser spot - the brightness of the spot is dependent on the optical extinction due to dust and is thus an indirect measure of particle number density, and (2) side-scatter - the camera images the laser from the side, showing beam entrance into the dust cloud and the boundary between dust and void. Both methods must assume a mean particle size in order to extract a number density. The optical extinction measurement yields the product of the 2nd moment of the particle size distribution and the extinction efficiency Qe. For particle sizes in the range of interest (greater than 1 micrometer), Qe approximately equal to 2. Scaling up of the PES single laser and camera system is underway in the PRTB, where an array of lasers penetrate a con-trolled dust cloud, illuminating multiple targets. Using high speed HD GoPro video cameras, the evolution of the dust cloud and particle size density can be studied in detail.

lunar simulant↗

Optical Extinction Measurements of Laser Side-Scatter During Tropical Storm Colin

A side-scatter imaging (SSI) technique using a 447 nm, 500 mW laser and a Nikon D80 camera was tested at Kennedy Space Center, Florida during the passing of a rain band associated with Tropical Storm Colin. The June 6, 2016, 22:00 GMT rain event was intense but short-lived owing to the strong west-to-east advection of the rain band. An effort to validate the optical extinction measurement was conducted by setting up a line of three tipping rain gauges along an 80 m east-west path and below the laser beam. Differences between tipping bucket measurements were correlated to the extinction coefficient profile along the lasers path, as determined by the SSI measurement. In order to compare the tipping bucket to the optical extinction data, a Marshall-Palmer DSD model was assumed. Since this was a daytime event, the laser beam was difficult to detect in the camera images, pointing out an important limitation of SSI measurements: the practical limit of DSD density that can be effectively detected and analyzed under daylight conditions using this laser and camera, corresponds to a fairly moderate rainfall rate on the order of 20 mmh (night measurements achieve a much improved sensitivity). The SSI analysis model under test produced promising results, but in order to use the SSI method for routine meteorological studies, improvements to the math model will be required.

optical extinction↗

Extinction Monitoring of Pulsed Proton Beams Using FPGA-Based Peak Detection

The Mu2e experiment at Fermilab imposes stringent requirements on the elimination of out-of-time beam in its pulsed proton beam - a requirement known as "extinction". We present a method to measure the out-of-time particle rates to calculate the level of extinction in the inter-pulse gaps. The proposed method utilizes an array of quartz Cherenkov radiators and photomultiplier tubes to detect particles scattered from a vacuum chamber in the M4 transfer beamline at Fermilab.The measurement will employ a new μTCA-based FPGA system for data acquisition and signal processing, utilizing real-time peak detection algorithms to count scattered beam particles. By integrating data over many transfers, the time profile of the out-of-time beam will be resolved to fractional levels relative to that of the in-time beam. These results are compared with G4beamline simulations to validate models of beam transport, dynamics, and extinction, providing critical input for optimizing beam delivery to Mu2e.

Hensley, Ryan [UC, Davis]↗

Extinction and scattering by several types of silicate sphere of radius 0.05-1.0 micron, for the wavelength range 0.21-50 microns.

The exact calculation of scattering and absorption by various sub-micron sized silicate spheres is presented here, using accurately determined optical constants in the wavelength range from 50 to 0.21 microns. The extinction features near 10 and 20 microns for various samples are discussed. It is found that the ratio of peak extinction at 20 microns to that at 10 microns is constant for small particles up to 0.4-micron radius, but is less for particles of 1-micron radius. The ratio of maximum extinction in the ultraviolet to that at 10 microns decreases with increasing particle size.

Bromage, G. E.↗

Pulsar extinction

The radiation properties of pulsars are reinvestigated in the context of the 'PCFB' model, according to which the radiation originates at the polar caps and the magnetic-field lines change from a closed to an open configuration at the 'force-balance' or 'corotation' radius. Major attention is given to the condition for electron-positron pair creation, which leads, in turn, to an extinction condition whereby any pulsar will cease to be a radio emitter after its period has increased beyond a certain value. This extinction condition is derived on the basis of a model where the magnetic field is the same as that of a point dipole located at the center of the star; effects of dipole distortion are also considered. A comparison of the results with observational data shows that most pulsars satisfy or nearly satisfy the pair-creation condition for undistorted dipoles and seem to satisfy the extinction condition. It is noted that pulsars which should be extinguished according to the undistorted-dipole model need not be if the magnetic field is sufficiently distorted at the polar caps.

Sturrock, P. A.↗

The relation between carbon monoxide emission and visual extinction in cloud L134

Emission from the J = 1-0 transition of carbon monoxide has been mapped over an area of 40 by 55 arcmin in cloud L134, and visual extinctions over the entire cloud have been obtained by means of star counts. Line intensities of at least 2 K are observable down to an extinction level of about one magnitude. From observations of the J = 1-0 transition of the (C-13)O isotopic species at 18 locations in the cloud, a linear correlation is found between the local thermodynamic equilibrium (LTE) column densities of (C-13)O and magnitudes of visual extinction.

Tucker, K. D.↗