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At least 217 records · Page 12

AGC-4 Experiment Irradiation Monitoring Data Qualification Final Report

The Graphite Technology Development Program ran a series of six experiments to quantify the effects of irradiation on nuclear grade graphite. This report focuses on the fourth experiment, Advanced Graphite Creep 4 (AGC 4). The Advanced Reactor Development (ARD) Technology Development Office (TDO) Program for research and development activities require documentation of qualified monitoring data to design and license the first high-temperature reactor nuclear plant. Qualified data meets the requirements for use as described in the experiment planning and quality assurance documents. Failed data do not meet the requirements and provide no useable information. Trend data may not meet all requirements but still provide some useable information. Use of Trend data requires assessment of how any deficiencies affect a particular use of the data. AGC-4 began with Advanced Test Reactor (ATR) Cycle 157D on May 30, 2015. After irradiating the graphite for two cycles, the capsule was removed from the reactor after ATR Cycle 158A, which ended on January 2, 2016, due to interference with another experiment. Irradiation was resumed with Cycle 162A on October 7, 2017 after the interfering experiment was removed from the reactor. AGC-4 irradiation completed by the end of Cycle 166B on January 10, 2020. Between Cycles 162A and 166B, AGC-4 capsule was removed from the reactor core during two Powered Axial Locator Mechanism (PALM) Cycles 163A and 165A to avoid overheating. All thermocouples (TCs) have functioned throughout the AGC-4 experiment. A total of 9,256,184 out of all 11,167,213 temperature records (or 82.9%) are Qualified for use by the ARD Program and 1,911,029 missing values are Failed. Argon, helium, and total gas flow data were within expected ranges, except only eight out-of-range values occurred during outages. A total of 21,240,627 out of all 22,288,5103 gas flow rates (or 92.8%) are Qualified for use by the ARD Program and 1,644,476 are Failed records mostly due to missing values. Discharge gas line moisture values were consistently low during full ATR power, except for 162B, when moisture content was increasing to more than 200 ppmv by the end of this cycle. During outages, moisture content reached as high as 700 ppmv. 1,089,941 out of a total of 1,107,331 moisture values (or 98.4%) are within the measurement range of the instrument and are Qualified for use by the ARD Program and 17,390 missing moisture values are Failed. Graphite creep specimens were subjected to one of three loads: 393, 491, or 589 lbf. For a brief period during Cycle 157D between 12:19 on June 2, 2015, and 08:23 on June 11, 2015, the load cells were wired incorrectly, resulting in missing stack load data. Missing stack loads were estimated from measured ram pressures using regression equations developed from the existing data from Cycle 157D. Estimated stack loads during this period are considered to be an accurate representation of actual load applied to the stacks. These loads deviate slightly from the planned loads. This deviation does not prevent the data from being Qualified for use but must be taken into account when analyzing the effect of load on creep. 6,095,728 out of a total of 6,403,985 moisture values (or 95.2%) are within the measurement range of the instrument and are Qualified for use by the ARD Program and 308,257 missing load values are Failed. Stack displacement increased consistently throughout the eight cycles, with total displacement reached highest value of 2.4 in by the end of irradiation. During ATR outages, a set of pneumatic rams raised the stacks of graphite creep specimens to ensure the specimens were not stuck within the test train. This stack raising was performed seven times throughout irradiation. All stacks were raised successfully each time. 4,744,974 out of a total of 6,094,513 displacement values (or 77.9%) are within the measurement range of the instrument and are Qualified for use by the ARD Program and 1,349,539 displacement values are Failed mostly due to missing values. Analyses were conducted on correlations between TCs to look for trends and step changes that might indicate instrument degradation or failure. Correlation analysis was used to identify instances when TCs form short circuits, referred to as virtual junctions, which result in TCs reporting temperatures from some location in the capsule other than the location where they were intended to read. No evidence of virtual junctions was found. Analyses were also conducted on control charts of temperature differences of between two TCs, which are expected to behave consistently throughout the entire irradiation period. Upward or downward trend over time indicates at least one TC in the pair was drifted. Examining control charts for all 66 possible pairs out of twelve TCs installed in the AGC-4 capsules reveal no clear drift failures occurred, except unstable behavior of two TCs in Zone 3, TC-7 and TC-8, over irradiation time. In conclus

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Report on High Energy Arcing Fault Experiments: Experimental Results from Open Box Enclosures

This report documents an experimental program designed to investigate High Energy Arcing Fault (HEAF) phenomena. The experiments focus on providing data to better characterize the arc to improve the prediction of arc energy emitted during a HEAF event. An open box experiment allow for direct observation of the arc, which allows diagnostic instrumentation to record the phenomenological data needed for better characterization of the arc energy source term. The data collected supports characterization of the arc and arc jet, enclosure breach, material loss, and electrical properties. These results will be used to better characterizing the hazard for improvements in fire probabilistic risk assessment (PRA) realism. The experiments were performed at KEMA Labs located in Chalfont, Pennsylvania. The experimental design, setup, and execution were completed by staff from the NRC, the National Institute of Standards and Technology (NIST), Sandia National Laboratories (SNL) and KEMA Labs. In addition, representatives from the Electric Power Research Institute (EPRI) observed some of the experimental setup and execution. The HEAF experiments were performed between August 22, 2020 and September 18, 2020 on near-identical 51 cm (20 in) cube metal boxes suspended from a Unistrut support structure. The three-phase arcing fault was initiated at the ends of the conductors oriented vertically and located at the center of the box. Either aluminum or copper conductors were used for the conductors. The low-voltage experiments used 1 000 volts AC, while the medium-voltage experiments used 6 900 volts AC consistent with other recently completed experiments. Durations of the experiment ranged from 1 s to 5 s with fault currents ranging from 1 kA to 30 kA. Real-time electrical operating conditions, including voltage, current and frequency, were measured during the experiments. Heat fluxes and incident energies were measured with plate thermometers, radiometers, and slug calorimeters at various locations around the electrical enclosures. The experiments were documented with normal and high-speed videography, infrared imaging and photography.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Criticality Experiments Research Center Futures: A Report of a Workshop held September 6-9, 2022, Los Alamos, NM, November, 2022

Experiments and training with critical assemblies and fissionable material (at or near the critical state) that explore reactivity phenomena are central to a number of national security challenges. From fission energy to nuclear weapons to a broad suite of scientific challenges, it is clear that additional capacity and capability are needed. The National Criticality Experiments Research Center (NCERC) marked 10 years of operations in 2021. This anniversary was an opportune time to celebrate our successes and progress, and to evaluate the remaining and emergent challenges. Against this backdrop, a workshop of approximately 140 national and international leaders in nuclear research was convened in Los Alamos, New Mexico to explore “NCERC Futures.” Therefore, the present workshop focused specifically on needed capabilities and tools to meet the research challenges in eight topical mission areas served by NCERC. As each Topical Group summarized their discussions in the out brief, it was recognized that key challenges could be met through enabling infrastructure investments and new critical assemblies. Enabling infrastructure includes staffing, additional space/buildings, developing an agile bounding safety basis, the ability to keep pace with technological advances in detectors and data acquisition systems (allowing use of those with Bluetooth™ and similar technologies), an expanded set of materials options (especially plutonium), a “Plug and Play” design and implementation mindset, and a facility that enabled free-field measurements. The new critical assemblies that were identified as having the most impact were a bare plutonium (Pu) Critical Assembly, a Horizontal Split Table (HST), a Super Comet, and a Uranium Solution Burst Assembly. NECRC is a unique, one-of-a-kind facility in the United States. If all the improvements were to be made, NCERC would enable the United States and its partners to address many important research questions related to criticality. These include but are not limited to: (1) Covering the entire neutron energy spectrum for both highly enriched uranium (HEU) and Pu in configurations for virtually all conceivable applications; (2) Performing multi-physics solution experiments and irradiations with a Uranium Solution Burst Assembly, which more closely resembles actual criticality accidents; (3) Conducting free-field experiments to make basic fission physics measurements and much cleaner benchmarks with various experimental observables; and (4) Providing more training classes and more experiments annually at greater cost efficiency enabled by additional buildings and machines and an agile, bounding, risk-balanced Safety Basis. In the end, workshop attendees enthusiastically concluded that NCERC Futures are bright and the workshop helped to identify a roadmap of capability gaps that need to be addressed. This report documents the results of those efforts.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Identification and Evaluation for Fueling of NRIC DOME Reactors Report

The National Reactor Innovation Center (NRIC) has designed a testbed for advanced microreactor experiments that enables and encourages technology developers to bring advanced designs closer to commercial availability. The test bed, Demonstration of Microreactor Experiments (DOME), will be used to facilitate much of the operation experimentation process of the each advanced microreactor including fueling and operational power experiments. This report identifies and evaluates the options for initial fueling the microreactors in DOME. This report also discusses the optional locations that were considered for the initial fueling of microreactor; namely the Transient Reactor Test (TREAT) reactor building, and an unspecified temporary location. But various logistical and construction issues essentially eliminated these other options from further consideration. A brief discussion in this report outlines potential equipment and protocol associated with fueling in DOME.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Signal selection and model-independent extraction of the neutrino neutral-current single 𝜋 + cross section with the T2K experiment

This article presents a study of single 𝜋 + production in neutrino neutral-current interactions (NC⁢1⁢𝜋 + ) using the FGD1 hydrocarbon target of the ND280 detector of the T2K experiment. We report the largest sample of such events selected by any experiment, providing the first new data for this channel in over four decades and the first using a sub-GeV neutrino flux. The signal selection strategy and its performance are detailed together with validations of a robust cross section extraction methodology. The measured flux-averaged integrated cross-section is 𝜎 = (6.07 ± 1.22) × 10 −41 cm 2 /nucleon, 1.3⁢𝜎 above the NEUT v5.4.0 expectation.

Neutrino detection↗

HEU Metal Delayed Critical Experiments with 10 to 19 Inch Thick Graphite Reflectors

Approximately 100 graphite-reflected highly enriched uranium (HEU, 93.14 wt % 235 U) metal annular and cylindrical critical experiments were performed in the early 1960s at the Oak Ridge Critical Experiments Facility (ORCEF). This report presents details from experiment logbooks, experimental data sheets and the author's memory for 44 HEU metal (93.14 wt % 235 U) critical assemblies with graphite reflectors varying from 10 to 19 in. thick, outside diameters varying from 7 to 15 in., inside diameters varying from 7 to 13 in. and critical HEU metal masses varying from 20.4 to 69.0 kg. The data from the 44 experiments described in this report are acceptable for use as criticality safety benchmark experiments for the International Criticality Safety Evaluation Program (ICSBEP) once the uncertainty analysis on the measured k eff is completed. Based on previous ICSBEP benchmarks with this HEU metal at ORCEF, the uncertainties in the measured k eff are expected to be as low as ±0.0004. Preparation of this report is part of an effort at Oak Ridge National Laboratory (ORNL) to document more than 15 undocumented series of critical and subcritical experiments enumerated in Critical and Subcritical NEA Benchmark Possibilities for Measurements at ORCEF and Other US DOE Facilities (Mihalzo, ORNL/TM-2019/1188, 2019) and performed by ORNL at ORCEF and other US Department of Energy critical experiments facilities. More than 500 operational days of critical facility time were used, not including setup and dismantlement time. This documentation for a part of one series of graphite reflected highly enriched uranium metal critical experiments, that used 50 operational days of ORCEF time, was performed using funding received from the DOE Office of Nuclear Energy’s Nuclear Energy University Programs at the University of Tennessee Nuclear Engineering Department. This documentation was also supported by the Nuclear Criticality, Radiation Transport, and Safety programs at ORNL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Application Experiences on a GPU-Accelerated Arm-based HPC Testbed

This paper assesses and reports the experience of ten teams working to port, validate, and benchmark several High Performance Computing applications on a novel GPU-accelerated Arm testbed system. The testbed consists of eight NVIDIA Arm HPC Developer Kit systems, each one equipped with a server-class Arm CPU from Ampere Computing and two data center GPUs from NVIDIA Corp. The systems are connected together using InfiniBand interconnect. The selected applications and mini-apps are written using several programming languages and use multiple accelerator-based programming models for GPUs such as CUDA, OpenACC, and OpenMP offloading. Working on application porting requires a robust and easy-to-access programming environment, including a variety of compilers and optimized scientific libraries. The goal of this work is to evaluate platform readiness and assess the effort required from developers to deploy well-established scientific workloads on current and future generation Arm-based GPU-accelerated HPC systems. The reported case studies demonstrate that the current level of maturity and diversity of software and tools is already adequate for large-scale production deployments.

Elwasif, Wael↗

MELCOR Model of the Molten Salt Tritium Transport Experiment (MSTTE)

This report summarizes the FY24 activities to model the Molten Salt Tritium Transport Experiment (MSTTE) using MELCOR. Summarized are the approaches used in construction of the MELCOR methods used for modeling, the construction of the MELCOR deck and the thermohydraulic calculations. The results show good comparison with previously reported calculation data, providing confidence in MELCOR to model experiments in the future.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

EFIT‐AI: Machine Learning and Artificial Intelligence Assisted Equilibrium Reconstruction for Tokamak Experiments and Burning Plasmas (Final Report)

The EFIT-AI project is creating a modern advanced equilibrium reconstruction code suitable for tokamak experiments of burning plasmas. EFIT [1,2] was the first and is the most extensively used equilibrium reconstruction code in the world. This project builds on the production-level experience and adds key elements as follows. 1. A Model Order Reduction (MOR) version of the two-dimensional (2D) Grad-Shafranov equation solver (EFIT-MORNN) using physics-informed neural networks. 2. Improved optimization and data analysis capabilities using a Bayesian framework enhanced with machine learning. 3. A MOR version of the three-dimensional (3D) perturbed equilibrium reconstruction tool.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Experiments on the dynamics and scaling of spontaneous-magnetic-field saturation in laser-produced plasmas

We report in laser-produced high-energy-density plasmas, large-scale strong magnetic fields are spontaneously generated by the Biermann battery effects when temperature and density gradients are misaligned. Saturation of the magnetic field takes place when convection and dissipation balance field generation. While theoretical and numerical modeling provide useful insight into the saturation mechanisms, experimental demonstration remains elusive. In this letter, we report an experiment on the saturation dynamics and scaling of Biermann battery magnetic field in the regime where plasma convection dominates. With time-gated charged-particle radiography and time-resolved Thomson scattering, the field structure and evolution as well as corresponding plasma conditions are measured. In these conditions, the spatially resolved magnetic fields are reconstructed, leading to a picture of field saturation with a scaling of $B ~ 1/L_T$ for a convectively dominated plasma, a regime where the temperature gradient scale ($L_T$) exceeds the ion skin depth.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Constraining computational modeling of indirect drive double shell capsule implosions using experiments

Double shell capsule implosions are an alternative approach to achieving alpha heating on the National Ignition Facility. Current machining techniques construct the outer shell as two hemispheres that are glued together, and the deuterium and tritium (DT) liquid inside the inner shell will be injected by a fill tube. These features introduce asymmetries and jetting that may disrupt the confinement of the DT fuel if not carefully controlled. Simulations indicate that in order to achieve high yields in the laboratory, these features as well as susceptibility to the Rayleigh–Taylor instability (RTI) must be mitigated. Furthermore, due to uncertainties in computational models and the expense of using the best physics models at adequate resolution in three dimensions, our computational modeling must be constrained by experiments. We report on the results of recent hydrogrowth radiography and dual-axis keyhole experiments with double shell targets that have been used to evaluate our modeling of the outer shell joint as well as the impacts of high-energy x-ray preheat that strongly impacts RTI growth. Our simulations show good agreement with the experimental data and inform several important modeling choices.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Progress in Hybrid Plasma Wakefield Acceleration

Plasma wakefield accelerators can be driven either by intense laser pulses (LWFA) or by intense particle beams (PWFA). A third approach that combines the complementary advantages of both types of plasma wakefield accelerator has been established with increasing success over the last decade and is called hybrid LWFA→PWFA. Essentially, a compact LWFA is exploited to produce an energetic, high-current electron beam as a driver for a subsequent PWFA stage, which, in turn, is exploited for phase-constant, inherently laser-synchronized, quasi-static acceleration over extended acceleration lengths. The sum is greater than its parts: the approach not only provides a compact, cost-effective alternative to linac-driven PWFA for exploitation of PWFA and its advantages for acceleration and high-brightness beam generation, but extends the parameter range accessible for PWFA and, through the added benefit of co-location of inherently synchronized laser pulses, enables high-precision pump/probing, injection, seeding and unique experimental constellations, e.g., for beam coordination and collision experiments. We report on the accelerating progress of the approach achieved in a series of collaborative experiments and discuss future prospects and potential impact.

43 PARTICLE ACCELERATORS↗

On the adsorption and reactivity of element 114, flerovium

Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Design of Experiments Involving Molybdenum in SNL SPRF/CX Facility

This report is part of the collaboration with the Nuclear Criticality Safety Program and constitutes the “CED-2 report” of the experiments proposed in the SPRF/CX facility of SANDIA National Laboratories to contribute to the validation of Molybdenum in thermal energy spectrum. It supplements the study carried out in the CED-1 report by providing a more precise design of the proposed experiments and presents a complete evaluation of the experimental uncertainties. In the CED-1 report, corresponding to the preliminary design of the experiments, IRSN identified several promising configurations that could be implemented in the SPRF/CX facility of SNL. They use metallic molybdenum either in the form of foils between the UO 2 pellets inside BUCCX rods, or in the form of sleeves surrounding 7uPCX rods. In this CED-2 report, a new design using molybdenum sleeves surrounding BUCCX rods is also analyzed and the experimental uncertainties of all the proposed configurations are estimated. Given the constraints to carry out the experiments and the costs associated with the manufacturing of the foils, the experiments using molybdenum foils are discarded. Similarly, the design using molybdenum sleeves around BUCCX rods leads to significant manufacturing costs which could certainly be partially offset by use of existing grids but which would lead to slightly lower values of the integral sensitivities to the cross sections of molybdenum. Consequently, the design using molybdenum sleeves around 7uPCX rods is favored insofar as it presents higher $k_{eff}$ sensitivities to the molybdenum cross sections and that there is still possibility to reduce the number of sleeves to reduce the cost of experiments. Regarding feedback on nuclear data in support of criticality safety assessment, one of the advantages of the work described here is that the proposed experiments are not correlated with the MIRTE and FP experiments using molybdenum. In addition, they lead to higher sensitivity values in the thermal energy range than the existing experiments and partly “cover” the first resonance of the 95 Mo, which is a real advantage for improving knowledge on molybdenum cross sections.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

FY22 Progress on Multicontinuum Methods in Containment

Estimation of two-phase fluid flow properties is important to understand and predict water and gas movement through the vadose zone for agricultural, hydrogeological, and engineering applications, such as containment transport and/or containment of gases in the subsurface. To estimate rock fluid flow properties and subsequently predict physically realistic processes such as patterns and timing of water, gas, and energy (e.g., heat) movement in the subsurface, laboratory spontaneous water imbibition with simultaneous temperature measurement and numerical modeling methods are presented in the FY22 progress report. A multiple-overlapping-continua conceptual model is used to explain and predict observed complex multi-phenomenological laboratory test behavior during spontaneous imbibition experiments. This report primarily addresses two complexities that arise during the experiments: 1) capturing the late-time behavior of spontaneous imbibition tests with dual porosity; and 2) understanding the thermal perturbation observed at or ahead of the imbibing wetting front, which are associated with adsorption of water in initially dry samples. We use numerical approaches to explore some of these issues, but also lay out a plan for further laboratory experimentation and modeling to best understand and leverage these unique observations.

58 GEOSCIENCES↗

Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments Execution Plan (IER-518 CED-3a)

As part of the experiment design and planning, the critical experiment design team (CEDT), as well as additional stakeholders, convened a series of meetings to discuss the goals and requirements of execution for this experiment. The slides from these meetings are attached in Appendix A. The following sections summarize the outcome of those discussions and present the planned experimental configurations and measurements. The stated goals of this experiment are as follows: 1) Measure time-tagged list-mode data for configurations exceeding neutron multiplication of 100; 2) Provide intercomparison between LLNL, LANL, and IRSN detector systems and methodologies; 3) Generate experiment execution report(s) useful to a fundamental physics benchmark for the ICSBEP; 4) Leverage existing critical experiment and detector system benchmarks to limit required modeling and uncertainty analysis.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Search for Θ+ in KLp→K+n reaction in KLF at JLab

The possibility of the existence of multiquark hadrons made of 4-quarks for mesons and 5-quarks for baryons was predicted by Gell-Mann [Phys. Lett. 8, 214 (1964)]. The renewed interest for the search for exotic pentaquark states was initiated by the paper by Diakonov, Petrov, and Polyakov [Z. Phys. A 359, 305 (1997)]. The 2003 experimental reports on the observation of [Formula: see text] pentaquark with [Formula: see text] quark content created a great excitement and many following experiments have reported its observation [K. H. Hicks, Eur. Phys. J. H 37, 1 (2012)]. After high-statistics experiments at JLab, which did not confirm previous claims by the CLAS collaboration, the community concluded that the [Formula: see text] pentaquark either does not exist at all or has an extremely small cross-section, making it currently unobserved. There were different review papers on this subject, questioning the existence of [Formula: see text] or trying to explain the reasons why reaching a conclusion based on production experiments is challenging [M. Amaryan, Eur. Phys. J. Plus 137, 684 (2022)]. To address the challenge of minimal 3-body final states, a formation experiment with a projectile-kaon beam is proposed. In the following, we discuss how the [Formula: see text] could be observed in the [Formula: see text] reaction in the KLF experiment at JLab [M. Amaryan et al. [KLF Collaboration], arXiv:2008.08215 [nucl-ex]].

Astronomy & Astrophysics↗

Final Design of a New Pulsed-Neutron Die-Away Experimental Testbed for Thermal Scattering Law Benchmarks (PNDA) (IER-501 CED-2)

This report presents the final design (CED-2) of IER-501, a testbed for pulsed-neutron die-away (PNDA) experiments at Lawrence Livermore National Laboratory (LLNL). The PNDA experiments will be high-quality benchmarks that serve to optimize and validate thermal neutron scattering laws (TSLs), which are high-priority nuclear data for the Department of Energy’s Nuclear Criticality Safety Program (NCSP). This CED-2 was guided by experimental results gathered from a prototype experimental set-up rather than with detailed simulations as is typically done for criticality experiments. The report presents the PNDA design and its equipment, and it documents the methodology used to postprocess the measured data. It discusses how experimental configurations influenced the decay-constant eigenvalue, or the integral parameter, of the experiment. The studied variations included the distance from the target to the generator, the orientation of the generator relative to the box, the orientation of the target to the generator, the effect of HDPE lining in the shielding box, the settings of the generator, and finally the benefits of using a low-scatter facility. From these results, a final configuration for the target, detectors, shielding box, and neutron generator was chosen. Two factors particularly influenced the chosen configuration: the reproducibility of the experiment’s geometry for benchmark modeling, and the minimization of measured neutrons scattered off the shielding box.

42 ENGINEERING↗