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Results for “electronic coherence”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12

All sources NASA NTRS DOE OSTI

DOE OSTI2025

Polaron catastrophe within quantum acoustics

The quantum acoustic framework has recently emerged as a nonperturbative, coherent approach to electron–lattice interactions, uncovering rich physics often obscured by perturbative methods with incoherent scattering events. Here, we model the strongly coupled dynamics of electrons and acoustic lattice vibrations within this framework, representing lattice vibrations as coherent states and electrons as quantum wave packets, in a manner distinctively different from tight-binding or discrete hopping-based approaches. We derive and numerically implement electron backaction on the lattice, providing both visual and quantitative insights into electron wave packet evolution and the formation of acoustic polarons. We investigate polaron binding energies across varying material parameters and compute key observables—including mean square displacement, kinetic energy, potential energy, and vibrational energy—over time. Our findings reveal the conditions that favor polaron formation, which is enhanced by low temperatures, high deformation potential constants, slow sound velocities, and high effective masses. Additionally, we explore the impact of external electric and magnetic fields, showing that while polaron formation remains robust under moderate fields, it is weakly suppressed at higher field strengths. These results deepen our understanding of polaron dynamics and pave the way for future studies into nontrivial transport behavior in quantum materials.

Science & Technology - Other Topics↗

DOE OSTI2024

XFEL SASE pulses can enhance time-dependent observables

Abstract X-ray free electron lasers (XFELs) have emerged as powerful sources of short and intense x-ray pulses. We propose a simple and robust procedure which takes advantage of the inherent stochasticity of self-amplified stimulated emission (SASE) pulses to enhance the time-resolution and signal strength of the recorded data. Notably, the proposed method is able to enhance the average signal without knowledge of the signal strength of individual shots. Simple metrics for the probe pulses are introduced, such as an effective pulse duration applicable to SASE pulses characterised in the time domain using e.g. an X-band transverse cavity. The approach is evaluated using simulated and real pulse data in the context of ultrafast electron dynamics in a molecule. Utilising H 2 as a model system, we demonstrate the efficacy of the method theoretically, successfully enhancing the predicted nonresonant ultrafast x-ray scattering signal associated with electron dynamics. The method presented is broadly applicable and offers a general strategy for enhancing time-dependent observables at XFELs.

data analysis↗

DOE OSTI2022

Order fractionalization in a Kitaev-Kondo model

We describe a mechanism for order fractionalization in a two-dimensional Kondo lattice model, in which electrons interact with a gapless spin liquid of Majorana fermions described by the Yao-Lee (YL) model. When the Kondo coupling to the conduction electrons exceeds a critical value, the model develops a superconducting instability into a state with a a spinor order parameter with charge 4 and spin ( = 1 2. The broken symmetry state develops a gapless Majorana Dirac cone in the bulk. By including an appropriate gauge string, we can show that the charge 4, spinorial order develops off-diagonal long range order that allows electrons to coherently tunnel arbitrarily long distances through the spin liquid.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Local condensation of charge-4 ⁢e superconductivity at a nematic domain wall

In the fluctuation regime that precedes the onset of pairing in multi-component superconductors, such as nematic and chiral superconductors, the normal state is generally unstable towards the formation of charge-4e order – an exotic quantum state in which electrons form coherent quartets rather than Cooper pairs. However, charge-4e order is often suppressed by other competing composite orders, such as nematics. Importantly, the formation of nematic domains is unavoidable due to the long-range strains generated, leading to one-dimensional regions where the competing nematic order is suppressed. Here, we employ a real-space variational approach to demonstrate that, in such nematic domain walls, charge-4e order is locally condensed via a vestigial-order mechanism. Here, we explore the experimental manifestations of this effect and discuss materials in which it can be potentially observed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2020

Numerical simulation of terahertz radiation by laser-driven plasma dipole oscillation

Laser-plasma interactions have many theoretical and technological applications. One is the use of coherently accelerated electrons to provide novel sources of THz radiation. Our research focuses on simulating the cross/self-interactions between two high intensity, ultra-short, counter propagating and detuned laser pulses and an initial neutral target for controlled ionization. Unlike our previous studies of laser-matter interaction over preformed plasma, we explore the injection and collision of laser pulses to induce background plasma driven by the self-guided laser wakefield mechanism, which is then used to perturb the plasma resulting in induced dipole oscillations leading to transverse radiation. Inducing a cylindrical spatial plasma column within the laser beam radius regime provides a stable, spatially localized plasma channel. The emitted radiation from the plasma dipole oscillation (PDO) will not be affected by surrounding plasma absorption, resulting in effective radiation distribution. Finally, results include 3D EM-PIC simulations and a comparison of the self- ionizing plasma against the preformed plasma to assess the efficiency of the mechanisms.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1974

The SNS Josephson junction with a third terminal

Discussion of the operating characteristics of a three-terminal thin-film SNS Josephson junction whose diameter is much greater than the electron pair coherence length in the N metal. It is shown that a junction of this type is essentially a two-terminal device even though the third terminal of the junction supplies the control current. The mechanism underlying this finding is discussed.

Prans, G. P.↗

NASA NTRS1985

Semiconductor Laser Phased Array

Oscillations synchronized and modulated individually for beam steering. Phased array of GaAs infrared lasers put out powerful electronically-steerable coherent beam. Fabricated as integrated circuit on GaAs chip, new device particularly suited to optical communications, optical data processing and optical detection and ranging systems.

Katz, J.↗

NASA NTRS1984

Perturbations of subionospheric LF and MF signals due to whistler-induced electron precipitation bursts

Increasing attention is now being devoted to the problem of the pitch angle scattering and resulting precipitation of magnetospheric energetic electrons by coherent waves. The present investigation has the objective to report the first evidence of a correlation between whistlers and amplitude perturbations on low-frequency (LF) signals at 37.2 kHz and medium-frequency (MF) signals at 780 kHz. Whistler-correlated amplitude perturbations were observed on a 780-kHz MF signal propagating on an approximately 1800 km path from South America to Palmer. The observed MF perturbations were of order 50 percent in amplitude and developed much more quickly than other changes of comparable magnitude on the signal.

Carpenter, D. L.↗

NASA NTRS1987

A cyclotron-maser instability associated with a nongyrotropic distribution

A stability analysis for the cyclotron-maser instability in the presence of a nongyrotropic electron distribution is presented. The model configuration describes a uniformly magnetized cold ambient plasma that contains a relatively diffuse suprathermal electron component coherently bunched in gyrophase. The stability of perturbations propagating parallel to the ambient magnetic field is considered, and substantial growth rates are found to occur. The results are contrasted with those found for a comparable gyrotropic loss-cone distribution, and it is found that the nongyrotropic instability is characterized by substantially higher growth rates.

Freund, H. P.↗

DOE OSTI2021

New methodology for measuring electron density perturbations caused by plasma coherent modes using profile reflectometry: Magnitudes and radial profiles in DIII-D

New capabilities of fast-sweep frequency-modulated profile reflectometry are explored to measure electron density ne perturbation magnitudes and radial profiles due to plasma coherent modes in DIII-D. The first approach is based on the frequency analysis of phase perturbations associated with high frequency (~MHz) Alfvén eigenmodes (AEs). The measurement of ~5.5 MHz fast-ion-driven global Alfvén eigenmodes (GAEs) is demonstrated in a neutral beam-heated DIII-D plasma. The GAE induced a broad radial distribution of phase perturbations in the profile reflectometer data. Analysis of these data determined the effective cutoff location displacement and the estimated ne fluctuation profile. In the second approach, high resolution ne profiles are used directly to determine the radial structure of ne perturbations due to a neo-classical tearing mode. These new measurements broaden the application of profile reflectometry and advance the development of AE spectroscopy as a tool for non-invasive diagnosis of fast-ion-driven modes in DIII-D and burning plasmas such as ITER.

47 OTHER INSTRUMENTATION↗

DOE OSTI2020

Bayesian Optimization of a Free-Electron Laser

The Linac Coherent Light Source X-ray free-electron laser is a complex scienti c apparatus which changes con gurations multiple times per day, necessitating fast tuning strategies to reduce setup time for successive experiments. To this end, we employ a Bayesian approach to maximizing X- ray laser pulse energy by controlling groups of quadrupole magnets. A Gaussian process model provides probabilistic predictions for the machine response with respect to control parameters, enabling a balance of exploration and exploitation in the search for the global optimum. We show that the model parameters can be learned from archived scans, and correlations between devices can be extracted from the beam transport. Furthermore, the result is a sample-e cient optimization routine, combining both historical data and knowledge of accelerator physics to signi cantly outperform existing optimizers.

47 OTHER INSTRUMENTATION↗

DOE OSTI2026

Long-lived polaritonic coherence and polaron decoupling effects in 2D electronic spectra

Molecular polaritons, formed by coupling molecular excitons with cavity photons, offer a promising platform for exploring quantum phenomena. A key challenge is understanding how these hybrid states maintain coherence in the presence of environmental vibrations. Here, we show theoretically that collective coupling of many molecular excitons in a cavity can protect polariton coherence from phonon-induced decoherence. Under realistic conditions, the coherence time can extend up to 200 fs at room temperature, compared with 15 fs for typical molecular systems. Simulations of two-dimensional electronic spectra reveal prolonged oscillations between upper and lower polariton states, and reduced vibrational coupling as indicated by changes in the nodal line slope of the lower polariton peak. These findings provide guidance for experimental efforts to realize long-lived polaritons, such as coupling CdSe nanoplatelets to optical cavities.

2D electronic spectroscopy↗

DOE OSTI2021

Unveiling the spatial distribution of molecular coherences at conical intersections by covariance X-ray diffraction signals

Significance Monitoring the real-space motion of the electrons directly involved in ultrafast molecular dynamics is a challenging goal, hindered by the strong contributions of the remaining inactive electrons. Molecular quantum coherences can provide a direct window into elementary electronic dynamics, but they could not be separately imaged so far. Here, we demonstrate a time- and frequency-resolved X-ray diffraction technique, which can employ existing stochastic X-ray pulses to separately image the coherence contributions. The technique can selectively follow the relevant electrons involved in the ultrafast dynamics and identify the confined molecular regions covered by their motion. It enables readily feasible measurements and can be straightforwardly extended to full three-dimensional imaging via X-ray and electron diffraction.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2020

Polaritons and excitons: Hamiltonian design for enhanced coherence

The primary questions motivating this report are: Are there ways to increase coherence and delocalization of excitation among many molecules at moderate electronic coupling strength? Coherent delocalization of excitation in disordered molecular systems is studied using numerical calculations. The results are relevant to molecular excitons, polaritons, and make connections to classical phase oscillator synchronization. In particular, it is hypothesized that it is not only the magnitude of electronic coupling relative to the standard deviation of energetic disorder that decides the limits of coherence, but that the structure of the Hamiltonian—connections between sites (or molecules) made by electronic coupling—is a significant design parameter. Inspired by synchronization phenomena in analogous systems of phase oscillators, some properties of graphs that define the structure of different Hamiltonian matrices are explored. The report focuses on eigenvalues and ensemble density matrices of various structured, random matrices. Some reasons for the special delocalization properties and robustness of polaritons in the single-excitation subspace (the star graph) are discussed. The key result of this report is that, for some classes of Hamiltonian matrix structure, coherent delocalization is not easily defeated by energy disorder, even when the electronic coupling is small compared to disorder.

Science & Technology - Other Topics↗

DOE OSTI2023

Toward a fully coherent tender and hard X-ray free-electron laser via cascaded EEHG in fourth-generation synchrotron light sources

Free-electron-laser-based beamlines utilize fully coherent laser pulses with extremely narrow bandwidth allowing direct use of X-rays without monochromators. This could be very beneficial for all users of current and future fourth-generation diffraction-limited synchrotron light sources (DL-SLSs) who need narrowband full-coherence high-brightness X-ray pulses. Based on our previous finding, i.e. that separating the two stages of echo-enabled harmonic generation (EEHG) with a few extra bending-magnet sections provides an effective way to increase the momentum compaction of chicane 1, one can simultaneously achieve adequate prebunching at extremely high harmonics as well as keep the energy modulation to the ideal minimum. This could open the door for cascaded EEHG, toward fully coherent tender and hard X-ray wavelengths. Built on our compact design of a twin-pulse seeding electron beam with an adjustable delay and timing jitter at the level of a few femtoseconds, a cascaded EEHG can be implemented, which includes two EEHG beamlines, where the radiation pulse generated by the first beamline with harmonic $h$ 1 could be used as the input seed laser pulse to the second beamline with harmonic $h$ 2 . Hence, the second radiator could potentially reach very high harmonics [$h$ = $h$ 1 (20)$h$ 2 (25–100)] from 500 to 2000, corresponding to tender and hard X-ray wavelengths. It is demonstrated that the cascaded EEHG scheme is compatible with almost any current or planned fourth-generation DL-SLS, with significant benefits for space-limited storage rings in particular. The main advantage is that this scheme requires almost no change of the storage-ring lattice and is fully compatible with other beamlines. Current proposals for rings with much longer straight sections would add self-amplified spontaneous emission as another viable option for storage-ring-based free-electron lasers.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Interferometric bunch length measurements of 3 MeV picocoulomb electron beams

We report picosecond bunch length measurements using an interferometric method for a 3 MeV electron beam having bunch charge ranging from 1 to 14 pC. The method senses the single-cycle sub-terahertz (THz) pulse emitted by each electron bunch as coherent transition radiation which, in turn, is analyzed using a Michelson-type interferometer, forming an interferogram that is then processed to yield the nominal electron bunch length. This sub-THz coherent radiation intensity was measured using a quasi-optical detector (QOD) operated at room temperature. This experiment was quite challenging since the divergence angle of the sub-THz pulse emitted by the low-energy electron bunch exceeds ±10°, and its pulse energy at the entrance to the detector was as low as 100 pJ. When compared to a conventional helium-cooled silicon composite bolometer designed for frequencies above 0.5 THz, the QOD provided much better signal-to-noise ratio in the ~80 GHz frequency range, which was critical for the successful measurement of the bunch length.

36 MATERIALS SCIENCE↗

NASA NTRS1986

Radio wavelength observations of magnetic fields on active dwarf M, RS CVn and magnetic stars

The dwarf M stars, YZ Canis Minoris and AD Leonis, exhibit narrow-band, slowly varying (hours) microwave emission that cannot be explained by conventional thermal radiation mechanisms. The dwarf M stars, AD Leonis and Wolf 424, emit rapid spikes whose high brightness temperatures similarly require a nonthermal radiation process. They are attributed to coherent mechanisms such as an electron-cyclotron maser or coherent plasma radiation. If the electron-cyclotron maser emits at the second or third harmonic gyrofrequency, the coronal magnetic field strength equals 250 G or 167 G, and constraints on the plasma frequency imply an electron density of 6 x 10 to the 9th/cu cm. Radio spikes from AD Leonis and Wolf 424 have rise times less than or equal to 5 ms, indicating a linear size of less than or equal to 1.5 x 10 to the 8th cm, or less than 0.005 of the stellar radius. Although Ap magnetic stars have strong dipole magnetic fields, they exhibit no detectable gyroresonant radiation, suggesting that these stars do not have hot, dense coronae. The binary RS CVn star UX Arietis exhibits variable emission at 6 cm wavelength on time scales ranging from 30 s to more than one hour.

Lang, Kenneth R.↗

NASA NTRS1983

Quasi-relativistic electron precipitation due to interactions with coherent VLF waves in the magnetosphere

The equations of motion for the cyclotron resonance interaction between coherent whistler mode waves and energetic particles are rederived with the inclusion of relativistic effects. The pitch angle scattering of the near-loss-cone quasi-relativistic electrons trapped in the magnetosphere is studied using a test particle method employing these relativistic equations, and the precipitated energy spectrum due to the wave-induced perturbations of a full distribution of particles is computed. Results show that the full width at half maximum peak width of the rms scattering pattern of the near-loss-cone particles would give an upper bound to the peak width of the associated precipitated energy spectrum under the conditions of moderate wave intensities in the low L shell region. In addition, it is found that the peak widths are within the upper limit values measured by recent satellite experiments. It is concluded that interactions of inner radiation belt particles with monochromatic waves could produce precipitated fluxes with relatively sharp spectral widths, and that therefore the L-dependent narrow peaks observed by low altitude satellite particle detectors could be caused by such interactions.

Chang, H. C.↗