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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Spatial Heterogeneity in Cloud Condensation Nuclei (SHINE) Field Campaign Report

Multiple land-atmosphere coupling processes influence the spatial distribution of boundary-layer energy, moisture, aerosol, or cloud condensation nuclei (CCN) properties. Accurately quantifying the spatial and temporal distributions of CCN concentrations is essential for investigating aerosol-cloud interactions and reducing uncertainties in aerosol radiative forcing estimates of Earth's system.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Large-Eddy Simulations of Convection Initiation over Heterogeneous, Low Terrain

Abstract Large-eddy simulations are conducted to investigate and physically interpret the impacts of heterogeneous, low terrain on deep-convection initiation (CI). The simulations are based on a case of shallow-to-deep convective transition over the Amazon River basin, and use idealized terrains with varying levels of ruggedness. The terrain is designed by specifying its power-spectral shape in wavenumber space, inverting to physical space assuming random phases for all wave modes, and scaling the terrain to have a peak height of 200 m. For the case in question, these modest terrain fields expedite CI by up to 2–3 h, largely due to the impacts of the terrain on the size of, and subcloud support for, incipient cumuli. Terrain-induced circulations enhance subcloud kinetic energy on the mesoscale, which is realized as wider and longer-lived subcloud circulations. When the updraft branches of these circulations breach the level of free convection, they initiate wider and more persistent cumuli that subsequently undergo less entrainment-induced cloud dilution and detrainment-induced mass loss. As a result, the clouds become more vigorous and penetrate deeper into the troposphere. Larger-scale terrains are more effective than smaller-scale terrains in promoting CI because they induce larger enhancements in both the width and the persistence of subcloud updrafts.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Study of Stratus-Lowering Marine-Fog Events Observed During C-FOG

Two stratus lowering marine fog events observed on 28 September and 04 October 2018 during the Coastal Fog (C-Fog) field campaign that took place offshore of Eastern Canada during 1 September to 6 October 2018 are described. In-situ, profiling and remote sensing observations were made at selected land sites in eastern Newfoundland (NL) and Nova Scotia (NS) as well as aboard the research vessel (R/V) Hugh R. Sharp that cruised in adjoining coastal waters. Synoptic scale analysis showed that both fog episodes were an outcome of the interaction between synoptic-scale surface level low-pressure systems and a contiguous high-pressure system. At the same time, back trajectories revealed that the bulk of the fog layer is formed due to differential advection. Here, the diameter of the fog droplets at the surface gradually decreased from the centre of the fog layer to its leading/trailing edges. The bimodal fog droplet diameter distribution with peaks at 5-10 µm and 20-25 µm provided clues on droplet collision and coalescence processes. The observed difference between microphysical variables and droplet distribution between the two fog events and within same fog layer may have been governed by atmospheric boundary layer conditions (e.g., humidity conditions and turbulence) prevailed in the fog layer. Overall, it is concluded that the life cycle of observed stratus-lowering coastal-fog episodes is dependent on synoptic conditions as well as atmospheric boundary layer characteristics such as stability, cloud top cooling and entrainment.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

The use of idealised experiments in testing a new convective parametrization: Performance of CoMorph-A

CoMorph is a new mass-flux convection parametrization under development at the Met Office designed for use within the Unified Model and its successor model, LFRic. Use of a three-dimensional idealised model enables controlled tests of the performance of the scheme across different regimes. This includes the interaction between the physical parametrizations and the resolved dynamics, allowing study of the emergent organisation of convection on the resolved scale. A selection of well-known cases is revisited here, with the purpose of documenting the extent to which CoMorph captures a range of important, but challenging, behaviour such as the diurnal cycle and sensitivity to tropospheric moisture. Simulations using CoMorph-A, a new physics package, that has been demonstrated to perform well at numerical weather prediction (NWP) and climate scales, are compared against the current global atmosphere configuration and high-resolution results. In addition to an entirely new convection scheme, the package of changes includes significant changes to the cloud, microphysics, and boundary-layer parametrizations. Recognising that CoMorph-A is the first version of a scheme that will continue to be substantially developed and to obtain good performance, compromises in tuning have had to be made. These idealised tests therefore show what works well in this configuration, and what areas will require further work. As such, it is quite a demanding testbed and could be viewed as some of the equipment required for a “convective playground”.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Observations of Aerosol, Cloud, Turbulence, and Radiation Properties at the Top of the Marine Boundary Layer over the Eastern North Atlantic Ocean: The ACORES Campaign

We report on the Azores Stratocumulus Measurements of Radiation, Turbulence and Aerosols (ACORES) campaign, which took place around Graciosa and Pico Islands/Azores in July 2017. The main objective was to investigate the vertical distribution of aerosol particles, stratocumulus microphysical and radiative properties, and turbulence parameters in the eastern North Atlantic. The vertical exchange of mass, momentum, and energy between the free troposphere (FT) and the cloudy marine boundary layer (MBL) was explored over a range of scales from submeters to kilometers. To cover these spatial scales with appropriate measurements, helicopter-borne observations with unprecedented high resolution were realized using the Airborne Cloud Turbulence Observation System (ACTOS) and Spectral Modular Airborne Radiation Measurement System–Helicopter-Borne Observations (SMART-HELIOS) instrumental payloads. Here, the helicopter-borne observations were combined with ground-based aerosol measurements collected at two continuously running field stations on Pico Mountain (2,225 m above sea level, in the FT), and at the Atmospheric Radiation Measurement (ARM) station on Graciosa (at sea level). First findings from the ACORES observations we are discussing in the paper are as follows: (i) we have observed a high variability of the turbulent cloud-top structure on horizontal scales below 100 m with local temperature gradients of up to 4 K over less than 1 m vertical distance, (ii) we have collected strictly collocated radiation measurements supporting the relevance of small-scale processes by revealing significant inhomogeneities in cloud-top brightness temperature to scales well below 100 m, and (iii) we have concluded that aerosol properties are completely different in the MBL and FT with often-complex stratification and frequently observed burst-like new particle formation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Cloud drop number concentrations over the western North Atlantic Ocean: seasonal cycle, aerosol interrelationships, and other influential factors

Cloud drop number concentrations (N d ) over the western North Atlantic Ocean (WNAO) are generally highest during the winter (DJF) and lowest in summer (JJA), in contrast to aerosol proxy variables (aerosoloptical depth, aerosol index, surface aerosol mass concentrations, surface cloud condensation nuclei (CCN) concentrations) that generally peak inspring (MAM) and JJA with minima in DJF. Using aircraft, satellite remote sensing, ground-based in situ measurement data, and reanalysis data, we characterize factors explaining the divergent seasonal cycles and furthermore probe into factors influencing N d on seasonal timescales. The results can be summarized well by features most pronounced in DJF, including features associated with cold-air outbreak (CAO) conditions such as enhanced values of CAO index, planetary boundary layer height (PBLH),low-level liquid cloud fraction, and cloud-top height, in addition to winds aligned with continental outflow. Data sorted into high- and low-N d days in each season, especially in DJF, revealed that all of these conditions were enhanced on the high-N d days, including reduced sea level pressure and stronger wind speeds. Although aerosols may be more abundant in MAM and JJA, the conditions needed to activate those particles into cloud droplets are weaker than in colder months, which is demonstrated by calculations of the strongest (weakest) aerosol indirect effects in DJF (JJA) based on comparing N d to perturbations in four different aerosol proxy variables (total and sulfate aerosol optical depth, aerosol index, surface mass concentration of sulfate). We used three machine learning models and up to 14 input variables to infer about most influential factors related to N d for DJF and JJA, with the best performance obtained with gradient-boosted regression tree (GBRT) analysis. The model results indicated that cloud fraction was the most important input variable, followed by some combination (depending on season) of CAO index and surface mass concentrations of sulfate and organic carbon. Future work is recommended to further understand aspects uncovered here such as impacts of free tropospheric aerosol entrainment on clouds, degree of boundary layer coupling, wet scavenging, and giant CCN effects on aerosol–N d relationships, updraft velocity, and vertical structure of cloud properties such as adiabaticity that impact the satellite estimation of N d .

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Pinned Clouds over Industrial Sources of Heat during TRACER

An analysis of stereo-camera data from the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign in Houston, Texas, reveals the existence of pinned clouds sitting atop industrial heat sources. These are not plumes of vapor and condensate emanating from stacks: The pinned shallow cumuli have cloud bases at about the lifting condensation of near-surface air. On many mornings, the pinned clouds are the only shallow cumuli in the field of view of the stereo cameras, persisting by themselves for at least an hour. On those mornings, the lower atmosphere straddles the boundary between stable and unstable, and the waste heat from industrial facilities is able to pin moist convection overhead. When solar heating of the surface becomes sufficient later in the morning, those mornings transition to having widespread shallow moist convection. Occurring within the field of view of the stereo cameras and other TRACER instruments, these pinned clouds represent steady plume-like moist convection triggered by known heat sources in a well-characterized atmosphere, making them a rich target for further study. Significance Statement This article introduces steady-state cumulus clouds observed during the Tracking Aerosol Convection Interactions Experiment (TRACER) campaign that were pinned to industrial heat sources. These pinned clouds were present in the early morning only when conditions were primed for moist convection, but for which there was not yet enough solar heating to trigger widespread convection. They persist in a statistical steady state and therefore provide a natural setting to explore the mechanisms controlling convective dynamics, which play a central role in Earth’s atmospheric circulation and radiative balance.

Atmosphere↗
DOE OSTI2026

Aircraft-derived particle fluxes distinguish entrainment zone and decoupled layer nucleation in marine boundary layers

The vertical distribution of freshly nucleated aerosol particles in the marine boundary layer remains poorly constrained, limiting our ability to represent new particle formation in climate models. Here we characterize 3–10 nm particle events, termed small particle events (SPEs), by deriving their vertical turbulent fluxes from aircraft measurements during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign. To overcome stationarity limitations of traditional eddy covariance methods, we applied continuous wavelet transform analysis to data collected during June–July 2017 and January–February 2018 flights over the Azores. Our flux-based analysis revealed two distinct SPE scenarios with different vertical structures and spatial extents. The first featured nucleation in the entrainment zone, where free tropospheric air entrains into the boundary layer. The second showed nucleation in the decoupled layer, a stratified region between the well-mixed surface layer and cloud-topped upper boundary layer. In both cases, convergence of air masses from different layers diluted preexisting aerosol surface area to very low levels, creating conditions favorable for nucleation and generating strong downward particle fluxes. SPEs occurred in 15 % of flights, challenging prevailing theoretical expectations that new particle formation should rarely occur in marine boundary layers due to high condensation and coagulation sink capacity of sea spray aerosols. Aircraft-derived particle fluxes provide first observational constraints on the vertical location and source strength of likely nucleation regions in the remote marine boundary layer, improving aerosol source representations in climate models and reducing uncertainties in aerosol-cloud interactions.

Rasheeda Satheesh, Ajmal [North Carolina State Uni↗
DOE OSTI2023

Sensitivity of Arctic Surface Temperature to Including a Comprehensive Ocean Interior Reflectance to the Ocean Surface Albedo Within the Fully Coupled CESM2

Abstract Almost all current climate models simplify the ocean surface albedo (OSA) by assuming the reflected solar energy without the ocean interior contribution. In this study, an improved ocean surface albedo scheme is incorporated into the Community Earth System Model version 2 (CESM2) to assess the sensitivity of Arctic surface temperature to including ocean interior reflectance to the OSA. Fully coupled CESM2 simulations with and without ocean interior reflectance are subsequently performed, we focus on the analysis of Arctic surface temperature responses. Incorporating ocean interior reflectance increases absorbed solar radiation and warms the ocean, enhancing seasonal heat storage and release across the Arctic Ocean, and increasing sea ice reduction and positive climate feedbacks that elevates Arctic surface temperature. Seasonal variations in air‐surface temperature differences induce changes in turbulent heat flux patterns, concurrently modifying dynamic advection and moisture processes that affect boundary layer humidity and low clouds, especially in winter. Based on partitioning physical processes in the thermodynamic energy equation, surface air warming is induced primarily through positive heating anomalies of vertical advection, latent heat release, and longwave radiative forcing. Through an examination of the surface energy budget, skin temperature warming is driven predominantly by increased downward longwave radiation, positive surface albedo feedback in summer, and increased conductive heat transport from the ocean particularly in winter. Significant effects of ocean interior reflectance on the Arctic Ocean, including sea surface warming and sea ice reduction, justify the importance of ocean interior reflectance in climate models for better understanding of ongoing Arctic climate changes.

Meteorology & Atmospheric Sciences↗
DOE OSTI2026

ARM Trajectories Data Set Value-Added Product Report

The U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s ARM Trajectories Data Set (ARMTRAJ) Value-Added Product (VAP) provides trajectory data sets initialized at ARM deployment coordinates and configured using ARM data sets. The four trajectory data sets support aerosol, cloud, and planetary boundary-layer research. Trajectory calculations use the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model informed by the European Centre for Medium-Range Weather Forecasts (ECMWF) fifth-generation atmospheric reanalysis (ERA5) data set at its highest spatial resolution (~31 km). HYSPLIT also runs at multiple initial starting locations surrounding ARM deployments (in latitude/longitude and/or vertical coordinates), facilitating an ensemble for each sample in the data sets. The ensemble mean and variability reported in ARMTRAJ improve the fidelity and provide uncertainty estimates of trajectory coordinates, thermodynamic properties, and other output fields.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

PSU-BSEC Doppler Lidar Processed Scans

This data repository includes the processed vertically staring measurements (stare files) made by the Pennsylvania State University (PSU) Doppler Lidar as a part of the Baltimore Social-Environmental Collaborative Urban Integrated Field Laboratory (BSEC UIFL). The PSU Doppler Lidar measures aerosol backscatter intensity (m-1 sr-1), signal-to-noise ratio, and radial velocity (i.e., vertical velocity in the case of stare files, units: m/s) at approximately 1 Hz temporal resolution and 30 m spatial resolution. Future updates will include angled scans, sky cam images, example figures, and the original .hpl files. For further information, please email Nicholas Prince, nec5299@psu.edu.

Air Quality↗
DOE OSTI2024

PSU-BSEC Doppler Lidar Processed Scans

This data repository includes the processed vertically staring measurements (stare files) and the angled scans (profile files) necessary to calculate horizontal winds retrieved by the Pennsylvania State University (PSU) Doppler Lidar as a part of the Baltimore Social-Environmental Collaborative Urban Integrated Field Laboratory (BSEC UIFL). The PSU Doppler Lidar measures aerosol backscatter intensity (m-1 sr-1), signal-to-noise ratio, and radial velocity (i.e., vertical velocity in the case of stare files, units: m/s) at approximately 1 Hz temporal resolution and 30 m spatial resolution. Within the "stare_data" subdirectory there exist example figures of all retrieved data. For further information, please email Nicholas Prince, nec5299@psu.edu.

Air Quality↗
DOE OSTI2021

Evaluating the Lagrangian Evolution of Subtropical Low Clouds in GCMs Using Observations: Mean Evolution, Time Scales, and Responses to Predictors

In this work, a Lagrangian framework is developed to show the daily-scale time evolution of low clouds over the eastern subtropical oceans. An identical framework is applied to two general circulation models (GCMs): the CAM5 and UKMET and a set of satellite observations. This approach follows thousands of parcels as they advect downwind in the subtropical trade winds, comparing cloud evolution in time and space. This study tracks cloud cover, in-cloud liquid water path (CLWP), droplet concentration $N_d$, planetary boundary layer (PBL) depth, and rain rate as clouds transition from regions with predominately stratiform clouds to regions containing mostly trade cumulus. The two models generate fewer clouds with greater $N_d$ relative to observations. Models show stronger Lagrangian cloud cover decline and greater PBL deepening when compared with observations. In comparing frequency distributions of cloud variables over time, it is seen that models generate increasing frequencies of nearly clear conditions at the expense of overcast conditions, whereas observations show transitions from overcast to cloud amounts between 50% and 90%. Lagrangian decorrelation time scales ($\mathcal{e}$-folding time $\tau$) of cloud cover and CLWP are between 11 and 19 h for models and observations, although they are a bit shorter for models. A Lagrangian framework applied here resolves and compares the time evolution of cloud systems as they adjust to environmental perturbations in models and observations. Increasing subsidence in the overlying troposphere leads to declining cloud cover, CLWP, PBL depth, and rain rates in models and observations. Modeled cloud responses to other meteorological variables are less consistent with observations, suggesting a need for continuing mechanical improvements in GCMs.

58 GEOSCIENCES↗
DOE OSTI2023

Analysis of an Arctic cold air outbreak during autumn and related air mass transformations forced by surface changes and advection in higher altitudes

During marine cold air outbreaks (MCAOs), cold and dry Arctic air masses are transported from the central Arctic southward across the closed sea ice and much warmer open oceans. They experience significant transformations including a rapid heating and moistening, often leading to cloud formation. While intense wintertime MCAOs have been analyzed widely, the air mass transformations during other seasons have been studied sparsely. We address this gap by investigating an MCAO case observed in September 2020. To study the transformation processes, we combine the fifth generation of atmospheric reanalyses of the global climate (ERA5), trajectory calculations, as well as shipborne and airborne measurements. In the central Arctic, observations acquired from aboard the research vessel (RV) Polarstern during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition characterized the initial state of the air mass over closed sea ice. Trajectories indicated the pathway the air mass took from RV Polarstern southward to the Fram Strait. For the first 24 h of the southbound drift, the air masses remained quasi-stationary. Then, still 15 h ahead of the marginal sea ice zone, differential advection across the boundary layer flow introduced humidity and clouds at higher altitudes between 1.5 and 2.5 km. ERA5-derived temperature and humidity tendencies indicated complex vertical interactions. Radiative cloud-top cooling, entrainment, and turbulence were significantly reduced in the lower and enhanced in the upper advected cloud layer. Eventually, the lower cloud deck dissipated. After this confluence of 2 different air masses, observations gathered by Polar 5 in Fram Strait as part of the MOSAiC Airborne observations in the Central Arctic campaign revealed cloudy, moist layers throughout the lowest 3.5 km and an increasing boundary layer height. Comparing the initial with the final state 48 h later, the largest net heating of +8 K was found close to the surface, yet the largest net moistening of +2.5 g kg -1 at an altitude of 1 km, as the initial profile was exceptionally dry here. We conclude that the observed air mass transformations were driven by the surface changes from sea ice to open ocean but additionally strongly impacted by the differential advection of clouds and moisture across the near-surface MCAO flow.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Sunlight-absorbing aerosol amplifies the seasonal cycle in low-cloud fraction over the southeast Atlantic

Abstract. The mean altitude of the smoke loading over the southeast Atlantic moves from the boundary layer in July to the free troposphere by October. This study details the month-by-month changes in cloud properties and the large-scale environment as a function of the biomass burning aerosol loading at Ascension Island (8∘ S, 14.5∘ W) from July to October, based on island measurements, satellite retrievals, and reanalysis. In July and August, the smoke loading predominantly varies within the boundary layer. During both months, the low-cloud fraction is less and is increasingly cumuliform when more smoke is present, with the exception of a late morning boundary layer deepening that encourages a short-lived cloud development. The meteorology varies little, suggesting aerosol–cloud interactions explain the cloudiness changes. September marks a transition month during which midlatitude disturbances can intrude into the Atlantic subtropics, constraining the free tropospheric aerosol closer to the African coast. Stronger boundary layer winds on cleaner days help deepen, dry, and cool much of the marine boundary layer compared to that on days with high smoke loadings, with stratocumulus reducing everywhere but at the northern deck edge. The September free troposphere is better mixed on smoky days compared to October. Longwave cooling rates, generated by a sharp water vapor gradient at the aerosol layer top, encourage a small-scale vertical mixing that could help maintain the well-mixed smoky September free troposphere. The October meteorology primarily varies as a function of the strength of the free tropospheric winds advecting aerosol offshore. The free tropospheric aerosol loading is less than in September, and the moisture variability is greater. Low-level clouds increase and are more stratiform in October when the smoke loadings are higher. The increased free tropospheric moisture can help sustain the clouds through a reduction in evaporative drying during cloud-top entrainment. Enhanced subsidence above the coastal upwelling region, increasing cloud droplet number concentrations, may further prolong cloud lifetime through microphysical interactions. Reduced subsidence underneath stronger free tropospheric winds at Ascension Island supports slightly higher cloud tops during smokier conditions. Overall, the monthly changes in the large-scale aerosol and moisture vertical structure act to amplify the seasonal cycle in low-cloud amount and morphology. This is climatically important, as cloudiness changes dominate changes in the top-of-atmosphere radiation budget.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

On the Relationship Between the Marine Cold Air Outbreak M Parameter and Low-Level Cloud Heights in the Midlatitudes

Focusing on conditions of subsidence when low clouds are present, ground-based observations in both the North Atlantic and the Southern Ocean reveal strong relationships between cloud boundary (base and top heights) and different measures of lower tropospheric instability. The difference in potential temperature between the surface and 800 hPa (a metric called M) provides a stronger relationship than measures of inversion strength such as the lower tropospheric stability and estimated inversion strength. This is because (1) inversion strength itself does not correlate well with cloud boundaries, and (2) M contains information that appears important for cloud boundaries. These include the surface forcing through the use of sea surface rather than near-surface air temperature and an upper level close to the real cloud top. These results expand upon previous work on the importance of M as a predictor of cloud morphology. However, important differences are found in low-cloud conditions for the North Atlantic as compared to the Southern Ocean (for a given value of M): stronger inversions, deeper boundary layers, and much larger sea level pressures. Therefore, the relationship between cloud boundaries and M differs between the two regions. A general circulation model provides similar relationships as observed between M and both cloud top height and temperature but tends to place clouds higher and at colder temperatures than observed for a given M. This might cause issues with the representation of precipitation, cloud cover and radiation in the Southern Ocean.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Constraining effects of aerosol-cloud interaction by accounting for coupling between cloud and land surface

Aerosol-cloud interactions (ACIs) are vital for regulating Earth’s climate by influencing energy and water cycles. Yet, effects of ACI bear large uncertainties, evidenced by systematic discrepancies between observed and modeled estimates. This study quantifies a major bias in ACI determinations, stemming from conventional surface or space measurements that fail to capture aerosol at the cloud level unless the cloud is coupled with land surface. We introduce an advanced approach to determine radiative forcing of ACI by accounting for cloud-surface coupling. By integrating field observations, satellite data, and model simulations, this approach reveals a drastic alteration in aerosol vertical transport and ACI effects caused by cloud coupling. In coupled regimes, aerosols enhance cloud droplet number concentration across the boundary layer more homogeneously than in decoupled conditions, under which aerosols from the free atmosphere predominantly affect cloud properties, leading to marked cooling effects. Our findings spotlight cloud-surface coupling as a key factor for ACI quantification, hinting at potential underassessments in traditional estimates.

54 ENVIRONMENTAL SCIENCES↗