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At least 217 records · Page 12

High-resolution time-resolved experiments on mixing and entrainment of buoyant jets in stratified environments

Fluid jets interacting with a stratified layer play an important role in the safety of several reactor designs. In the containment of nuclear power plants, fluid jets dominate the transport and mixing of gaseous species and consequent hydrogen distribution in case of a severe accident. The mixing phenomena in the containment are driven by buoyant high-momentum injections (jets) and low momentum injection plumes. Mixing near the postulated break is initially dominated by high flow velocities. Plumes with moderate flow velocities are instead relevant in the break compartment during the long-term pressurization phase, or in any of the apertures between two connected compartments if the mass flows are sufficiently high and the density differences between efflux and ambient are sufficiently low. Phenomena of interest include free plumes (as produced by the efflux from the break compartment in a larger room or directly from a break flow), wall plumes (such those produced by low mass flows through inter-compartment apertures), and propagating stratification fronts in the ambient (for any stably stratified conditions). These phenomena have been highly ranked about nuclear reactor design, especially regarding of safety protocols. During a Pressurized Thermal Shock (PTS) scenario, the interaction between the cold ECCS injection plume and the stratified fluid present in the cold (or hot) leg is important in order to determine the temperature at the time-dependent temperature at the inlet of the reactor pressure vessel (RPV) and the potential to cause a thermal shock on the RPV wall. In sodium-cooled fast reactors (SFRs), core channels are typically hydro-dynamically isolated so that there exists a considerable temperature variation at the exit of adjacent fuel assemblies. All the above phenomena are characterized by the interaction of buoyant jets with the stratified flow. In stratified layers baroclinic forces create significant redistribution of turbulent kinetic energy and scales, which leads to anisotropy. This important physical phenomenon is highly three dimensional and is challenging to capture even with high-fidelity CFD simulations, due in part to lack of sufficiently resolved validation data. Furthermore, the experimental data available in the open literature do not feature the level of fidelity needed for an extensive validation of turbulence models in lower order CFD. To shed new lights into the crucial phenomena object of the present research project, it was proposed to conduct coordinated experiments and simulations at the University of Michigan and the George Washington University. The project has resulted in an experimental database of high-resolution time-resolved measurements of jets in uniform and stratified environments. The novel experimental data will be used to validate computational fluid dynamic (CFD) codes, including both Large Eddy Simulations (LES) and unsteady Reynolds-averaged Navier-Stokes equations (URANS) methodologies. In the Experimental and Multiphase flow (ECMF) laboratory at Univerisity of Michigan, we built two experimental facilities to investigate also the effect of scaling. The first facility, DESTROJER (DEnsity Stratified Turbulent ROund free Jet ExpeRiment), featuring a contoured jet nozzle with a diameter of D=12.7mm and a 1m×1m×1m cubic tank, which is made of acrylic glass for optical access. The ratio between the tank width and the nozzle diameter is equal to 78, which ensures that there is no direct interaction between the jet and the side walls. A second, modular experimental facility, features three different tank sizes of size 10×10×30, 20×20×30, 30×30×30 cm3 respectively (all tanks have the same height of 30 cm), and a jet diameter of 2mm. For the modular facility, tank-to-nozzle ratio of 50, 100, and 150 are obtained respectively. Experiments with different-density jet impactions and sharp interface with a density difference of 3.16% In the Laboratory at George Washington University, complementary experiments have been carried out at a facility featuring the same dimensions as DESTROYER. Experiments with different jet diameters have been carried out as well. High-resolution time-resolved measurements have been performed at all facilities using high-speed particle image velocimetry (PIV) and planar laser-induced fluorescence (PLIF). In this way, simultaneous measurements of velocity and density fields have been carried out. At the University of Michigan, wire-mesh sensors have been designed and built to gather high-resolution, time-dependent data of the stratified front in the tank. These measurements are important to provide accurate initial conditions for the CFD simulations. An important outcome of the project has been the development of novel techniques to achieve refractive index matching (RIM) of acqueous solutions with high density differences. RIM is crucial if optical techniques such as PIV are used to measure velocity fields. Previous to this project, experiments up to 3% density difference had been reported in the literature. With the methodology developed in this project, we have been able to push the envelop to density differences up to 9%. The experiments have been used to validate Reynolds Averaged Navier-Stokes (RANS) turbulence models and Large Eddy Simulations (LES) models. Both NEK5000 and the commercial CFD code STAR-CCM+ have been used. The experimental data will be made available to the community through the NE-KAMS databasehave been successfully conducted in the scaled facility.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Monitoring Land Surface Albedo and Vegetation Dynamics Using High Spatial and Temporal Resolution Synthetic Time Series from Landsat and the MODIS BRDF/NBAR/Albedo Product

Seasonal vegetation phenology can significantly alter surface albedo which in turn affects the global energy balance and the albedo warmingcooling feedbacks that impact climate change. To monitor and quantify the surface dynamics of heterogeneous landscapes, high temporal and spatial resolution synthetic time series of albedo and the enhanced vegetation index (EVI) were generated from the 500-meter Moderate Resolution Imaging Spectroradiometer (MODIS) operational Collection V006 daily BRDF (Bidirectional Reflectance Distribution Function) / NBAR (Nadir BRDF-Adjusted Reflectance) / albedo products and 30-meter Landsat 5 albedo and near-nadir reflectance data through the use of the Spatial and Temporal Adaptive Reflectance Fusion Model (STARFM). The traditional Landsat Albedo (Shuai et al., 2011) makes use of the MODIS BRDFAlbedo products (MCD43) by assigning appropriate BRDFs from coincident MODIS products to each Landsat image to generate a 30-meter Landsat albedo product for that acquisition date. The available cloud free Landsat 5 albedos (due to clouds, generated every 16 days at best) were used in conjunction with the daily MODIS albedos to determine the appropriate 30-meter albedos for the intervening daily time steps in this study. These enhanced daily 30-meter spatial resolution synthetic time series were then used to track albedo and vegetation phenology dynamics over three Ameriflux tower sites (Harvard Forest in 2007, Santa Rita in 2011 and Walker Branch in 2005). These Ameriflux sites were chosen as they are all quite nearby new towers coming on line for the National Ecological Observatory Network (NEON), and thus represent locations which will be served by spatially paired albedo measures in the near future. The availability of data from the NEON towers will greatly expand the sources of tower albedometer data available for evaluation of satellite products. At these three Ameriflux tower sites the synthetic time series of broadband shortwave albedos were evaluated using the tower albedo measurements with a Root Mean Square Error (RMSE) less than 0.013 and a bias within the range of 0.006. These synthetic time series provide much greater spatial detail than the 500 meter gridded MODIS data, especially over more heterogeneous surfaces, which improves the efforts to characterize and monitor the spatial variation across species and communities. The mean of the difference between maximum and minimum synthetic time series of albedo within the MODIS pixels over a subset of satellite data of Harvard Forest (16 kilometers by 14 kilometers) was as high as 0.2 during the snow-covered period and reduced to around 0.1 during the snow-free period. Similarly, we have used STARFM to also couple MODIS Nadir BRDF-Adjusted Reflectances (NBAR) values with Landsat 5 reflectances to generate daily synthetic times series of NBAR and thus Enhanced Vegetation Index (NBAR-EVI) at a 30-meter resolution. While normally STARFM is used with directional reflectances, the use of the view angle corrected daily MODIS NBAR values will provide more consistent time series. These synthetic times series of EVI are shown to capture seasonal vegetation dynamics with finer spatial and temporal details, especially over heterogeneous land surfaces.

Vegetation Index↗

Probing drift velocity dispersion in MAPbI 3 photovoltaic cells with nonlinear photocurrent spectroscopy

Conventional time-of-flight (TOF) measurements yield charge carrier mobilities in photovoltaic cells with time resolution limited by the RC time constant of the device, which is on the order of 0.1–1 µs for the systems targeted in the present work. We have recently developed an alternate TOF method, termed nonlinear photocurrent spectroscopy (NLPC), in which carrier drift velocities are determined with picosecond time resolution by applying a pair of laser pulses to a device with an experimentally controlled delay time. In this technique, carriers photoexcited by the first laser pulse are “probed” by way of recombination processes involving carriers associated with the second laser pulse. Here, we report NLPC measurements conducted with a simplified experimental apparatus in which synchronized 40 ps diode lasers enable delay times up to 100 µs at 5 kHz repetition rates. Carrier mobilities of ∼0.025 cm 2 /V/s are determined for MAPbI 3 photovoltaic cells with active layer thicknesses of 240 and 460 nm using this instrument. Here, our experiments and model calculations suggest that the nonlinear response of the photocurrent weakens as the carrier densities photoexcited by the first laser pulse trap and broaden while traversing the active layer of a device. Based on this aspect of the signal generation mechanism, experiments conducted with co-propagating and counter-propagating laser beam geometries are leveraged to determine a 60 nm length scale of drift velocity dispersion in MAPbI 3 films. Contributions from localized states induced by thermal fluctuations are consistent with drift velocity dispersion on this length scale.

14 SOLAR ENERGY↗

Dual transmission grating based imaging radiometer for tokamak edge and divertor plasmas

The designs of single transmission grating based extreme ultraviolet (XUV) and vacuum ultraviolet (VUV) imaging spectrometers can be adapted to build an imaging radiometer for simultaneous measurement of both spectral ranges. This paper describes the design of such an imaging radiometer with dual transmission gratings. The radiometer will have an XUV coverage of 20-200 A with a {approx}10 A resolution and a VUV coverage of 200-2000 A with a {approx}50 A resolution. The radiometer is designed to have a spatial view of 16 Degree-Sign , with a 0.33 Degree-Sign resolution and a time resolution of {approx}10 ms. The applications for such a radiometer include spatially resolved impurity monitoring and electron temperature measurements in the tokamak edge and the divertor. As a proof of principle, the single grating instruments were used to diagnose a low temperature reflex discharge and the relevant data is also included in this paper.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Photocathode characterisation for robust PICOSEC Micromegas precise-timing detectors

The PICOSEC Micromegas detector is a precise-timing gaseous detector based on a Cherenkov radiator coupled with a semi-transparent photocathode and a Micromegas amplifying structure, targeting a time resolution of tens of picoseconds for minimum ionising particles. Initial single-pad prototypes have demonstrated a time resolution below σ = 25 ps, prompting ongoing developments to adapt the concept for High Energy Physics applications, where sub-nanosecond precision is essential for event separation, improved track reconstruction and particle identification. The achieved performance is being transferred to robust multi-channel detector modules suitable for large-area detection systems requiring excellent timing precision. To enhance the robustness and stability of the PICOSEC Micromegas detector, research on robust carbon-based photocathodes, including Diamond-Like Carbon (DLC) and Boron Carbide (B 4 C), is pursued. Results from prototypes equipped with DLC and B 4 C photocathodes exhibited a time resolution of σ ≈ 32 ps and σ ≈ 34.5 ps, respectively. Efforts dedicated to improve detector robustness and stability enhance the feasibility of the PICOSEC Micromegas concept for large experiments, ensuring sustained performance while maintaining excellent timing precision.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

VISAR Analysis in the Frequency Domain

VISAR measurements are typically analyzed in the time domain, where velocity is approximately proportional to fringe shift. Moving to the frequency domain clarifies the limitations of this approximation and suggests several improvements. For example, optical dispersion preserves high-frequency information, so a zero-dispersion (air delay) interferometer does not provide optimal time resolution. Combined VISAR measurements can also improve time resolution. With adequate bandwidth and reasonable noise levels, it is quite possible to achieve better resolution than the VISAR approximation allows.

36 MATERIALS SCIENCE↗

Comprehensive Characterization of Silicon Photomultipliers for Nuclear Security Applications

Scintillation detectors are an essential instrument in a variety of fields, serving as an effective means of detecting radiation for industrial, defense, medical, and basic-research applications. Light sensors are an integral part of all scintillation detectors and can affect detector performance as much as the scintillator itself. The photomultiplier tube (PMT) has been the standard light sensor for over half a century, but alternatives have been developed recently, and the silicon photomultiplier (SiPM) is perhaps the most promising of these new technologies. SiPMs can produce gains of the same order of magnitude as most PMTs and have shown reduced noise levels in the newest generations. Additionally, they posses benefits characteristic of solid-state devices such as insensitivity to magnetic fields, mechanical ruggedness, compactness, low operating voltages, and high quantum efficiencies. The timing properties of light sensors are an important characteristic for many applications, including nuclear security. For example, accurate timing is necessary for time of flight experiments, scatter cameras, and background suppression. This work aims to characterize the time resolution of many commercially available new-generation SiPMs, specifically in a time coincidence setting. SiPMs have been acquired from five leading manufacturers possessing a variety of pixel and microcell sizes. Results are presented with an organic scintillator p-terphenyl and coincidence time resolution of less than 300 picoseconds is achieved. Comparison with PMTs shows that the PMT pair tested has a superior time resolution of 83 picoseconds.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Performance of Pixel and Strip AC-LGAD Sensors with Different Design Parameter on a 120 GeV Proton Beam

We present the results of an extensive evaluation of strip and pixel AC-LGAD sensors tested with a 120 GeV proton beam, focusing on the influence of design parameters on the sensor temporal and spatial resolutions. Results show that reducing the thickness of pixel sensors significantly enhances their time resolution, with 20- μm-thick sensors achieving around 20 ps. Uniform performance is attainable with optimized sheet resistance, making these sensors ideal for future timing detectors. Conversely, 20-μm-thick strip sensors exhibit higher jitter than similar pixel sensors, negatively impacting time resolution, despite reduced Landau fluctuations with respect to the 50-μm-thick versions. Additionally, it is observed that a low resistivity in strip sensors limits signal size and time resolution, whereas higher resistivity improves performance. This study highlights the importance of tuning the n+ sheet resistance and suggests that further improvements should target specific applications like the Electron-Ion Collider or other future collider experiments. In addition, the detailed performance of four AC-LGADs sensor designs is reported as examples of possible candidates for specific detector applications. These advancements position AC-LGADs as promising candidates for future 4D tracking systems, pending the development of specialized readout electronics.

Lara, Carlos Pérez↗

Results for pixel and strip centimeter-scale AC-LGAD sensors with a 120 GeV proton beam

Here, we present the results of an extensive evaluation of strip and pixel AC-LGAD sensors tested with a 120 GeV proton beam, focusing on the influence of design parameters on the sensor temporal and spatial resolutions. Results show that reducing the thickness of pixel sensors significantly enhances their time resolution, with 20-μm-thick sensors achieving around 20 ps. Uniform performance is attainable with optimized n + sheet resistance, making these sensors ideal for future timing detectors. Conversely, 20-μm-thick strip sensors exhibit higher jitter than similar pixel sensors, negatively impacting time resolution, despite reduced Landau fluctuations with respect to the 50-μm-thick versions. Additionally, it is observed that a low resistivity in strip sensors limits signal size and time resolution, whereas higher resistivity improves performance. This study highlights the importance of tuning the n+ sheet resistance and suggests that further improvements should target specific applications like the Electron–Ion Collider or other future collider experiments. In addition, the detailed performance of four AC-LGADs sensor designs is reported as examples of possible candidates for specific detector applications. These advancements position AC-LGADs as promising candidates for future 4D tracking systems, pending the development of specialized readout electronics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Nonlinear reflection of a spherically divergent N-wave from a plane surface: Optical interferometry measurements in air

Mach stem is a well-known structure typically observed in the process of strong (acoustic Mach numbers greater than 0.4) step-shock waves reflection from a rigid boundary. However, this phenomenon has been much less studied for weak shocks in nonlinear acoustic fields where Mach numbers are in the range from 0.001 to 0.01 and pressure waveforms have more complicated waveforms than step shocks. The goal of this work was to demonstrate experimentally how nonlinear reflection occurs in air for very weak spherically divergent acoustic spark-generated pulses resembling an N-wave. Measurements of reflection patterns were performed using a Mach-Zehnder interferometer. A thin laser beam with sub-millimeter cross-section was used to obtain the time resolution of 0.4 µs, which is 6 times higher than the time resolution of the condenser microphones. Pressure waveforms were reconstructed using the inverse Abel transform applied to the phase of the signal measured by the interferometer. The Mach stem formation was observed experimentally as a result of collision of the incident and reflected shock pulses. It was shown that irregular reflection of the pulse occurred in a dynamic way and the length of the Mach stem increased linearly while the pulse propagated along the surface. Since the front shock of the spark-generated pulse was steeper than the rear shock, irregular type of reflection was observed only for the front shock of the pulse while the rear shock reflection occurred in a regular regime.

42 ENGINEERING↗

Dual wavelength imaging of a scrape-off layer in an advanced beam-driven field-reversed configuration

A dual wavelength imaging system has been developed and installed on C-2U to capture 2D images of a He jet in the Scrape-Off Layer (SOL) of an advanced beam-driven Field-Reversed Configuration (FRC) plasma. The system was designed to optically split two identical images and pass them through 1 nm FWHM filters. Dual wavelength images are focused adjacent on a large format CCD chip and recorded simultaneously with a time resolution down to 10 μs using a gated micro-channel plate. The relatively compact optical system images a 10 cm plasma region with a spatial resolution of 0.2 cm and can be used in a harsh environment with high electro-magnetic noise and high magnetic field. The dual wavelength imaging system provides 2D images of either electron density or temperature by observing spectral line pairs emitted by He jet atoms in the SOL. A large field of view, combined with good space and time resolution of the imaging system, allows visualization of macro-flows in the SOL. First 2D images of the electron density and temperature observed in the SOL of the C-2U FRC are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Molecular Characterization of High Molecular Weight Polyesters by Matrix-Assisted Laser Desorption/Ionization High-Resolution Time-of-Flight Mass Spectrometry Combined with On-plate Alkaline Degradation and Mass Defect Analysis

Matrix-assisted laser desorption ionization high-resolution time-of-flight mass spectrometry (MALDI HR TOF MS) is a powerful tool for the molecular characterization of industrial polymers. However, accurate mass determination and resolution of isobaric ions are possible for oligomer samples only typically below m/z 3000. To cut long polymer chains into oligomers suitable for high-resolution mass spectrometry, we propose a simple “on-plate” alkaline degradation of polyesters as a sample pretreatment technique prior to the MALDI TOF MS measurement. This pretreatment can be performed on a MALDI target using a small amount of sample (μg or less) and 1 μL of alkaline reagent by simple pipetting. Informative mass spectra in the oligomeric mass range are successfully recorded but complicated by the variation of end-groups and the copolymeric composition of the degradation products. Data processing is assisted by a series of advanced Kendrick mass defect (KMD) analyses recently proposed by the authors to plot visually understandable two-dimensional maps. On-plate degradation pretreatment, high-resolution MALDI TOF MS measurements, and advanced KMD analyses are innovatively combined for the compositional characterization of bacterial poly(3-hydroxybutyric acid-co-3-hydroxyvaleric acid) and industrial poly(ethylene terephthalate) samples. .

74 ATOMIC AND MOLECULAR PHYSICS↗

Digital data acquisition system implementation at the National Superconducting Cyclotron Laboratory

A Digital Data Acquisition System (DDAS) composed of 16-channel FPGA-programmable modules running 12-bit 100 Mega-Samples Per Second (MSPS) ADCs has been implemented on three different experimental arrays at the National Superconducting Cyclotron Laboratory (NSCL) encompassing charged particle spectroscopy, high and low energy-resolution photon detection, and neutron time-of-flight measurements. DDAS has increased the experimental capabilities of each array by providing energy and time measurements with nearly zero dead-time, low energy thresholds, and large dynamic range. The performance of the DDAS Analog-to-Digital Converters (ADC)s was characterized, and energy and time resolutions were compared with traditional analog systems. We have demonstrated a 14- to 15-bit peak-sensing equivalent resolution when applied to semiconductor detectors and 500 ps time resolution for LaBr 3 detectors measuring coincident radiation with signal amplitudes of ≈13% of the input range of the ADC. Details regarding the operation of the system at NSCL including digital filtering, triggering, clock distribution, and event-building are discussed along with applications to selected detector systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Studies of uniformity of 50 μ m low-gain avalanche detectors at the Fermilab test beam

In this study, we report measurements of the uniformity of time resolution, signal amplitude, and charged particle detection efficiency across the sensor surface of low-gain avalanche detectors (LGAD). Comparisons of the performance of sensors with different doping concentrations and different active thicknesses are presented, as well as their temperature dependence and radiation tolerance up to 6 x 10 14 n/cm 2 . Results were obtained at the Fermilab test beam facility using 120 GeV proton beams, and a high precision pixel tracking detector. LGAD sensors manufactured by the Centro Nacional de Microelectrónica (CNM) and Hamamatsu Photonics (HPK) were studied. The uniformity of the sensor response in pulse height before irradiation was found to have a 2% spread. The signal detection efficiency and timing resolution in the sensitive areas before irradiation were found to be 100% and 30–40 ps, respectively. A “no-response” area between pads was measured to be about 130 μm for CNM and 170μm for HPK sensors. After a neutron fluence of 6 x 10 14 n/cm 2 the CNM sensor exhibits a large gain variation of up to a factor of 2.5 when comparing metalized and non-metalized sensor areas. An irradiated CNM sensor achieved a time resolution of 30 ps for the metalized area and 40 ps for the non-metalized area, while a HPK sensor irradiated to the same fluence achieved a 30 ps time resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Application of high-resolution time-of-flight chemical ionization mass spectrometry measurements to estimate volatility distributions of α-pinene and naphthalene oxidation products

Recent developments in high-resolution time-of-flight chemical ionization mass spectrometry (HR-ToF-CIMS) have made it possible to directly detect atmospheric organic compounds in real time with high sensitivity and with little or no fragmentation, including low-volatility, highly oxygenated organic vapors that are precursors to secondary organic aerosol formation. Here, using ions identified by high-resolution spectra from an HR-ToF-CIMS with acetate reagent ion chemistry, we develop an algorithm to estimate the vapor pressures of measured organic acids. The algorithm uses identified ion formulas and calculated double bond equivalencies, information unavailable in quadrupole CIMS technology, as constraints for the number of possible oxygen-containing functional groups. The algorithm is tested with acetate chemical ionization mass spectrometry (acetate-CIMS) spectra of O 3 and OH oxidation products of α-pinene and naphthalene formed in a flow reactor with integrated OH exposures ranged from 1.2 × 10 11 to 9.7 × 10 11 molec s cm −3 , corresponding to approximately 1.0 to 7.5 days of equivalent atmospheric oxidation. Measured gas-phase organic acids are similar to those previously observed in environmental chamber studies. For both precursors, we find that acetate-CIMS spectra capture both functionalization (oxygen addition) and fragmentation (carbon loss) as a function of OH exposure. The level of fragmentation is observed to increase with increased oxidation. The predicted condensed-phase secondary organic aerosol (SOA) average acid yields and O/C and H/C ratios agree within uncertainties with previous chamber and flow reactor measurements and ambient CIMS results. While acetate reagent ion chemistry is used to selectively measure organic acids, in principle this method can be applied to additional reagent ion chemistries depending on the application.

54 ENVIRONMENTAL SCIENCES↗

Results from the commissioning of a multi-modal endoscope for ultrasound and time of flight PET

The EndoTOFPET-US collaboration has developed a multi-modal imaging system combining Ultrasound with Time-of-Flight Positron Emission Tomography into an endoscopic imaging device. The objective of the project is to obtain a coincidence time resolution of about 200 ps FWHM and to achieve about 1 mm spatial resolution of the PET system, while integrating all the components in a very compact detector suitable for endoscopic use. This scanner aims to be exploited for diagnostic and surgical oncology, as well as being instrumental in the clinical test of new biomarkers especially targeted for prostate and pancreatic cancer. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Time- and angle-resolved x-ray diffraction to probe structural and chemical evolution during Al-Ni intermetallic reactions

We present novel time- and angle-resolved x-ray diffraction (TARXD) capable of probing structural and chemical evolutions during rapidly propagating exothermic intermetallic reactions between Ni-Al multilayers. The system utilizes monochromatic synchrotron x-rays and a two-dimensional (2D) pixel array x-ray detector in combination of a fast-rotating diffraction beam chopper, providing a time (in azimuth) and angle (in distance) resolved x-ray diffraction image continuously recorded at a time resolution of {approx}30 {micro}s over a time period of 3 ms. Multiple frames of the TARXD images can also be obtained with time resolutions between 30 and 300 {micro}s over three to several hundreds of milliseconds. The present method is coupled with a high-speed camera and a six-channel optical pyrometer to determine the reaction characteristics including the propagation speed of 7.6 m/s, adiabatic heating rate of 4.0 x 10{sup 6} K/s, and conductive cooling rate of 4.5 x 10{sup 4} K/s. These time-dependent structural and temperature data provide evidences for the rapid formation of intermetallic NiAl alloy within 45 {micro}s, thermal expansion coefficient of 1.1 x 10{sup -6} K for NiAl, and crystallization of V and Ag{sub 3}In in later time.

36 MATERIALS SCIENCE↗

Application of spatially resolved high resolution crystal spectrometry to inertial confinement fusion plasmas

High resolution ({lambda}/{Delta}{lambda}{approx} 10 000) 1D imaging x-ray spectroscopy using a spherically bent crystal and a 2D hybrid pixel array detector is used world wide for Doppler measurements of ion-temperature and plasma flow-velocity profiles in magnetic confinement fusion plasmas. Meter sized plasmas are diagnosed with cm spatial resolution and 10 ms time resolution. This concept can also be used as a diagnostic of small sources, such as inertial confinement fusion plasmas and targets on x-ray light source beam lines, with spatial resolution of micrometers, as demonstrated by laboratory experiments using a 250-{mu}m {sup 55}Fe source, and by ray-tracing calculations. Throughput calculations agree with measurements, and predict detector counts in the range 10{sup -8}-10{sup -6} times source x-rays, depending on crystal reflectivity and spectrometer geometry. Results of the lab demonstrations, application of the technique to the National Ignition Facility (NIF), and predictions of performance on NIF will be presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗