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Development and validation of a gamma-ray detection response model for neutron-diagnosed subcritical experiments

In a neutron-diagnosed subcritical experiment, a highly sensitive and fast detector is required to accurately determine the true fission γ-ray emission rate from an object composed of special nuclear material under interrogation, in addition to a proper detector response model for use in forward modeling. We present the development of a detector response model that is based in GEANT4 and uses post-processing techniques to include photomultiplier tube time and pulse height response effects. We also define a set of detector performance evaluation metrics that emphasized our experimental objectives. A suite of time and pulse height response measurements for several diverse detector assemblies are described. These assemblies were simulated with this response model and benchmarked against the laboratory measurements. This response model reproduces the pulse height curve shapes and performance hierarchy of the measured detectors well. Additionally, the simulated time response curves exhibit reasonable agreement with counterpart measurements. These measurements and simulation results together suggest that a large volume EJ-299-49 plastic scintillator that is mated to an ultraviolet transmitting plastic light guide and relies on total internal reflection for light transport to the photocathode will provide significantly faster timing, increase pulse height by a factor of 3, and require 25% less γ rays to meet experimental needs, compared to the candidate detector design developed prior to the availability of this response model. Application of this response model and associated performance metrics in the context of large-scale design sensitivity studies is also discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development of an accelerator-based neutron source to prototype Mo-99 production, Part II: A liquid LBE loop under a high vacuum

To provide US domestic supply of Mo-99 without using high-enriched uranium (HEU), a subcritical uranium target assembly (UTA) is irradiated by an accelerator-based neutron source to create Mo-99 through fission. Part I of this work discusses the design of a liquid lead–bismuth eutectic (LBE) windowless target for an accelerator-based neutron source development. Part II discusses how to couple this windowless target to an accelerator operating at an ultra-high vacuum and the subcritical UTA cooled by water at room temperature. Due to the windowless design of the target, the liquid LBE flow shares an ultra-high vacuum (<1.3 × 10 -7 Pa or 10 -9 Torr) space with the accelerator. As a result of this shared vacuum space, the LBE system must operate at a high vacuum (10 -3 ~10 -6 Pa or 10 -5 ~10 -8 Torr). A magnetic rotary motion feedthrough unit utilizes magnetic fluid to allow rotation of the pump while maintaining a high vacuum environment. Prior to testing the LBE system under vacuum, a pump curve measurement is performed to estimate flowrate in the system. This measurement also generates data on orifice loss coefficients, which are compared to correlations in literature. The second experiment investigates vacuum level in the LBE system during operation. High vacuum is maintained (10 -3 ~10 -5 Pa or 10 -5 ~10 -7 Torr) during system operation, and a residual gas analyzer (RGA) scan shows that partial pressures of residual gases in the LBE system lower over the duration of LBE system operations. The third experiment investigates the gravity driven liquid LBE flowing out of the target chamber in the return line, which is partially full. If the liquid LBE is not drained quickly enough, flooding in the target chamber could occur. The coefficient n in the Manning equation is found to be around 0.008 s/m 1/3 . The last experiment performed is a demonstration that a vacuum jacket could provide sufficient thermal insulation to allow coupling between 300 °C LBE loop and a water tank at room temperature. In conclusion, the results from these experiments have influenced the development of the neutron source for the future commercial scale Mo-99 production system.

43 PARTICLE ACCELERATORS↗

Preliminary Thermal-Hydraulic Analysis of the UTA–2 Subcritical Linear Accelerator–Driven System

The National Nuclear Security Administration’s mission includes establishing a reliable supply of 99 Mo without highly enriched uranium. Oak Ridge National Laboratory (ORNL) supports this objective through collaborative research and development with industrial partners. Niowave Inc., a current partner, is currently designing a subcritical linear accelerator-driven system (ADS) and preparing for the US Nuclear Regulatory Commission’s licensing process. Niowave’s system has the potential to efficiently supply medical radioisotopes. The technology includes a superconducting electron accelerator and a pile of both natural and low-enriched uranium (LEU) targets. The process fissions uranium and many valuable isotopes can then be extracted from the targets. Niowave is currently iterating through conceptual and detailed design processes for several system sizes. This report discusses UTA–2, which is at the demonstration stage. UTA–2 will validate numerical modeling results with experimental measurements before progressing to the detailed design of UTA–3, the commercial-sized ADS. The thermal-hydraulic behavior of the UTA–2 core design was numerically investigated using STAR-CCM+, as described in this report. STAR-CCM+, a state-of-the-art computational fluid dynamics (CFD) software that was commercially developed by Siemens, has an extensive user base and a set of validation studies. It is also compliant with the American Society of Mechanical Engineers’ Nuclear Quality Assurance 1 standard. Three cases are investigated in this report. Case 1 quantified the temperature field within the UTA–2 assembly and water tank using only conduction as the method of thermal energy transport. This simplified approach was overly conservative and yielded wetted cladding temperatures above the coolant saturation temperature. In this case, the maximum temperature of the wetted cladding surface of the highest power rod exceeded the saturation temperature of water by 63.8°C. Because of the overly conservative approach taken in Case 1 and its negative subcooled margin, buoyancy-driven natural circulation flow physics were implemented in Case 2. Adding coolant motion significantly distributed the thermal energy of the system through convective heat transfer. This relatively small amount of convective heat transfer significantly reduced system temperatures and increased the subcooled margin from –63.8 to 61.3°C. This margin confirmed that no boiling was expected during normal operation of UTA–2 at 230 W. Case 3 had no additional physics models but considered an overpower event during which the power of each LEU and natural uranium rod was at its respective peak values. This resulted in a study with the total assembly power equal to 176% of the nominal power of 230 W considered in Cases 1 and 2. The resulting natural circulation flows were slightly enhanced. The subcooled margin decreased slightly to 46.3°C, which is still a significant margin to local boiling of the water within the tank. This margin confirmed that no boiling was expected during an abnormal operation of UTA–2 at 406 W.

07 ISOTOPE AND RADIATION SOURCES↗

NASA Tech Briefs, February 2001

The topics include: 1) Application Briefs; 2) National Design Engineering Show Preview; 3) Marketing Inventions to Increase Income; 4) A Personal-Computer-Based Physiological Training System; 5) Reconfigurable Arrays of Transistors for Evolvable Hardware; 6) Active Tactile Display Device for Reading by a Blind Person; 7) Program Automates Management of IBM VM Computer Systems; 8) System for Monitoring the Environment of a Spacecraft Launch; 9) Measurement of Stresses and Strains in Muscles and Tendons; 10) Optical Measurement of Temperatures in Muscles and Tendons; 11) Small Low-Temperature Thermometer With Nanokelvin Resolution; 12) Heterodyne Interferometer With Phase-Modulated Carrier; 13) Rechargeable Batteries Based on Intercalation in Graphite; 14) Signal Processor for Doppler Measurements in Icing Research; 15) Model Optimizes Drying of Wet Sheets; 16) High-Performance POSS-Modified Polymeric Composites; 17) Model Simulates Semi-Solid Material Processing; 18) Modular Cryogenic Insulation; 19) Passive Venting for Alleviating Helicopter Tail-Boom Loads; 20) Computer Program Predicts Rocket Noise; 21) Process for Polishing Bare Aluminum to High Optical Quality; 22) External Adhesive Pressure-Wall Patch; 23) Java Implementation of Information-Sharing Protocol; 24) Electronic Bulletin Board Publishes Schedules in Real Time; 25) Apparatus Would Extract Water From the Martian Atmosphere; 26) Review of Research on Supercritical vs Subcritical Fluids; 27) Hybrid Regenerative Water-Recycling System; 28) Study of Fusion-Driven Plasma Thruster With Magnetic Nozzle; 29) Liquid/Vapor-Hydrazine Thruster Would Produce Small Impulses; and 30) Thruster Based on Sublimation of Solid Hydrazine

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Laser transport and backscatter in low-density SiO 2 and Ta2O 5 foams

Experiments using a single 527 nm wavelength beam interacting with sub- and supercritical density SiO 2 and Ta 2 O 5 foams examined laser propagation and backscatter from laser–plasma instabilities such as Stimulated Brillouin Scattering (SBS). Two densities of each material were examined, and multiple diagnostics were used to characterize the propagation and backscatter. For 5 mg/cc SiO 2 (n e /n c = 0.375), the laser propagation distance was well approximated by treating the foam as a gas. However, for the 2 mg/cc SiO 2 foam (n e /n c = 0.15), the same model over-predicts the propagation distance by ~40%. Furthermore, existing analytical theories on propagation through subcritical foams were able to account for this difference. The laser heat wave propagated ~1/2 as far in Ta 2 O 5 than SiO 2 foams with similar electron density. We showed that this difference is due to the increased radiation losses in the higher Z foam. The fraction of backscattered light scales linearly with incident laser intensity for the range of intensities examined. Ta 2 O 5 foams had significantly lower levels of backscatter (1–3%) than the SiO 2 (4–8%), which is consistent with estimates of large Landau damping due to the presence of the oxygen atoms. The measured fraction of SBS backscattered laser energy for a 2 mg/cc SiO 2 foam shot was ~4 times lower than predicted by simulations assuming a gas-like foam. We found that we needed to assume increased ion heating such that T i /T e ~1.2–1.5 in the plasma to agree with the measured SBS reflectivity. Analytical models of laser-heated foams predict preferential heating of the ions as has been observed in previous experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A Study of the Kinematic and Dynamic Processes associated with Mesoscale Snowbands in a Midwest United States Snowstorm on 5 February 2020

Mesoscale snowbands are frequently responsible for dumping large amounts of snow over a relatively small region and pose a considerable forecasting challenge. The present study focuses on the mesoscale snowbands observed on 5 February 2020 over the Midwest United States. In order to improve the forecasting of mesoscale snowbands, it is important to understand the processes that organize these features. To this end, we are investigating the kinematic and dynamic processes that shape the mesoscale snowbands using a combination of high-altitude airborne radar, in-situ aircraft measurements, surface observations, and model simulations. This presentation will primarily focus on the three-dimensional structure of the mesoscale snowbands in terms of EXRAD reflectivity and horizontal winds. The horizontal winds are retrieved from the EXRAD scanning-beam Doppler velocities using a VAD technique. These winds, in combination with virtual potential temperature taken from the HRRR operational analysis, are used to compute the bulk Richardson number in order to investigate any contributions to banding features that might be tied to Kelvin-Helmholtz instability. Our analysis does not support the presence of Kelvin-Helmholtz instability. That said, low, but not subcritical, Richardson numbers were found near the top of some banding features in this event and it is possible that the model analysis is smoothing out the virtual potential temperature fields. Finally, we present arguments for using a flight module designed to sample the along-band structures with particular emphasis on observing generating cells and low-level microphysics.

Charles N. Helms↗

Cryogenic on-orbit liquid depot storage acquisition and transfer (COLD-SAT) experiment subsystem instrumentation and wire harness design report

Subcritical cryogens such as liquid hydrogen (LH2) and liquid oxygen (LO2) are required for space based transportation propellant, reactant, and life support systems. Future long-duration space missions will require on-orbit systems capable of long-term cryogen storage and efficient fluid transfer capabilities. COLD-SAT, which stands for cryogenic orbiting liquid depot-storage acquisition and transfer, is a free-flying liquid hydrogen management flight experiment. Experiments to determine optimum methods of fluid storage and transfer will be performed on the COLD-SAT mission. The success of the mission is directly related to the type and accuracy of measurements made. The instrumentation and measurement techniques used are therefore critical to the success of the mission. This paper presents the results of the COLD-SAT experiment subsystem instrumentation and wire harness design effort. Candidate transducers capable of fulfilling the COLD-SAT experiment measurement requirements are identified. Signal conditioning techniques, data acquisition requirements, and measurement uncertainty analysis are presented. Electrical harnessing materials and wiring techniques for the instrumentation designed to minimize heat conduction to the cryogenic tanks and provide optimum measurement accuracy are listed.

Edwards, Lawrence G.↗

Validation and Independent Uncertainty Analysis of the MIX-SOL-THERM-003 ICSBEP Benchmark

The International Criticality Safety Benchmark Evaluation Project (ICSBEP) was started in 1992 by the United States Department of Energy and later in 1995 became an international project with contributions from 22 countries. The project is now organized by the OECD (Organisation for Economic Co-operation and Development) Nuclear Energy Agency (NEA). In its most recent iteration, the ICSBEP handbook contains over five thousand evaluations of critical, near-critical, and subcritical experiments conducted in facilities all around the world. These benchmarks serve as valuable information for criticality safety engineers who can use them to validate calculation techniques and establish minimum subcritical margins for operations with fissionable materials. The benchmarks in the handbook are categorized by their fissile material composition, material form (oxide, solution, or metal), and fission energy spectra. This is especially useful for those looking for benchmarks similar to a system they are working on to compare methods and identify trends. The ICSBEP Handbook Uncertainty Guide is document outlining recommended practices and methods for determining uncertainties in these benchmarks. Quantifying these uncertainties thoroughly is crucial as it allows a higher degree of confidence that data used from them is valid and relevant. The guide stresses the importance of a thorough and well documented uncertainty analysis when evaluating an experiment. All measured values of a system, whether they be dimensions or material compositions, have a certain amount of uncertainty associated with them and can be analyzed one by one to determine their effects on the system. Many evaluated benchmarks in the handbook present this in detail, however some do not, mostly earlier evaluations performed in the 1990’s and early 2000’s. Recently at Los Alamos National Laboratory (LANL), the Nuclear Criticality Safety Division (NCSD) of LANL has been validating MCNP6.2 ® input files of criticality benchmarks for use by Whisper, a criticality safety code developed at LANL. This effort is also part of the OECD NEA Working Party on International Nuclear Data Evaluation Co-operation (WPEC) Subgroup 45, also known as Validation of Nuclear Data Libraries (VaNDaL). The goal of VaNDaL is to compile a set of validated simulation inputs for use in validating nuclear data and simulation codes. As part of these efforts, one of the benchmarks reviewed was the MIX SOL-THERM-003 ICSBEP benchmark. This paper provides an independent uncertainty analysis of this benchmark experiment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Effect of Ice Formations on Propeller Performance

Measurements of propeller efficiency loss due to ice formation are supplemented by an analysis to establish the magnitude of efficiency losses to be anticipated during flight in icing conditions. The measurements were made during flight in natural icing conditions; whereas the analysis consisted of an investIgation of changes in blade-section aerodynamic characteristics caused by ice formation and the resulting propeller efficiency changes. Agreement in the order of magnitude of eff 1- ciency losses to be expected is obtained between measured and analytical results. The results indicate that, in general, efficiency losses can be expected to be less than 10 percent; whereas maximum losses, which will be encountered only rarely, may be as high as 15 or 20 percent. Reported. losses larger than 15 or 20 percent, based on reductions in airplane performance, probably are due to ice accretions on other parts of the airplane. Blade-element theory is used in the analytical treatment, and calculations are made to show the degree to which the aerodynamic characteristics of a blade section. must be altered to produce various propeller efficiency losses. The effects of ice accretions on airfoil-section characteristics at subcritical speeds and their influence on drag-divergence Mach number are examined, and. the attendant maximum efficiency losses are computed. The effect of kinetic heating on the radial extent of ice formation is considered, and its influence on required length of blade heating shoes is discussed. It is demonstrated how the efficiency loss resulting from an icing encounter is influenced by the decisions of the pilot in adjusting the engine and propeller controls.

Neel, C. B., Jr.↗

Equivalent Fundamental-Mode Source Simulations for Spherical Uranium and Plutonium Systems

It is important in neutron noise measurements and reactor startup to understand how the source distribution in a system compares to the equivalent fundamental-mode (EFM) source. Deviation from the fundamental mode source distribution increases as the system $\kappa$ eff increases. A correction factor, g *, is a measure of this deviation, and is the focus of this work. Two methods were utilized to simulate g *. These methods are compared to each other and (where applicable) previous results. The effects associated with nuclear material inner radius, materials of reflectors, and reflector thickness are also investigated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA Tech Briefs, July 2009

Topics covered include: Dual Cryogenic Capacitive Density Sensor; Hail Monitor Sensor; Miniature Six-Axis Load Sensor for Robotic Fingertip; Improved Blackbody Temperature Sensors for a Vacuum Furnace; Wrap-Around Out-the-Window Sensor Fusion System; Wide-Range Temperature Sensors with High-Level Pulse Train Output; Terminal Descent Sensor Simulation; A Robust Mechanical Sensing System for Unmanned Sea Surface Vehicles; Additive for Low-Temperature Operation of Li-(CF)n Cells; Li/CFx Cells Optimized for Low-Temperature Operation; Number Codes Readable by Magnetic-Field-Response Recorders; Determining Locations by Use of Networks of Passive Beacons; Superconducting Hot-Electron Submillimeter-Wave Detector; Large-Aperture Membrane Active Phased-Array Antennas; Optical Injection Locking of a VCSEL in an OEO; Measuring Multiple Resistances Using Single-Point Excitation; Improved-Bandwidth Transimpedance Amplifier; Inter-Symbol Guard Time for Synchronizing Optical PPM; Novel Materials Containing Single-Wall Carbon Nanotubes Wrapped in Polymer Molecules; Light-Curing Adhesive Repair Tapes; Thin-Film Solid Oxide Fuel Cells; Zinc Alloys for the Fabrication of Semiconductor Devices; Small, Lightweight, Collapsible Glove Box; Radial Halbach Magnetic Bearings; Aerial Deployment and Inflation System for Mars Helium Balloons; Steel Primer Chamber Assemblies for Dual Initiated Pyrovalves; Voice Coil Percussive Mechanism Concept for Hammer Drill; Inherently Ducted Propfans and Bi-Props; Silicon Nanowire Growth at Chosen Positions and Orientations; Detecting Airborne Mercury by Use of Gold Nanowires; Detecting Airborne Mercury by Use of Palladium Chloride; Micro Electron MicroProbe and Sample Analyzer; Nanowire Electron Scattering Spectroscopy; Electron-Spin Filters Would Offer Spin Polarization Greater than 1; Subcritical-Water Extraction of Organics from Solid Matrices; A Model for Predicting Thermoelectric Properties of Bi2Te3; Integrated Miniature Arrays of Optical Biomolecule Detectors; A Software Rejuvenation Framework for Distributed Computing; Kurtosis Approach to Solution of a Nonlinear ICA Problem; Robust Software Architecture for Robots; R4SA for Controlling Robots; Bio-Inspired Neural Model for Learning Dynamic Models; Evolutionary Computing Methods for Spectral Retrieval; Monitoring Disasters by Use of Instrumented Robotic Aircraft; Complexity for Survival of Living Systems; Using Drained Spacecraft Propellant Tanks for Habitation; Connecting Node; and Electrolytes for Low-Temperature Operation of Li-CFx Cells.

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Experimental validation of a high fidelity Monte Carlo neutron transport model of the MIT graphite exponential pile

High-fidelity modeling and simulation were performed for the MIT graphite exponential pile (MGEP) using Monte Carlo neutron transport codes OpenMC and MCNP, and the results were validated by experimental data. The MGEP is being used as the test bed for the design of an autonomous control system for the pile's neutron flux distribution. The main contribution of this work is to generate the training data sets of neutron flux distributions with different locations of control rods that perturb the neutron flux profiles. First, code -to-code cross verification between OpenMC and MCNP was performed to ensure consistency of the numerical modeling within statistical uncertainties. To validate the accuracy of this high-fidelity model, a series of neutron flux measurements were conducted using a Helium-3 (He-3) neutron detector on a mobile platform that is placed inside the pile. Second, the neutron flux profiles were measured in four vertical layers of interest, and compared to the corresponding simulation results. The comparison results shows that the root mean square error is less than 2.5% in the two upper layers, and less than 4.5% in all four measured layers. Here the results validated the accuracy of the modeling and simulation. Finally, the relative change of the neutron flux profiles from moving control rods was analyzed, which identified the layer that has the best sensitivity regarding the control rods movements. Thus, this work identified and provided training data sets of both simulated and experimental neutron flux profiles in the most sensitive layer, paving the path forward to the real-time experimental demonstration of the autonomous control system.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Validation of an All-Pressure Fluid Drop Model: Heptane Fluid Drops in Nitrogen

Despite the fact that supercritical fluids occur both in nature and in industrial situations, the fundamentals of their behavior is poorly understood because supercritical fluids combine the characteristics of both liquids and gases, and therefore their behavior is not intuitive. There are several specific reasons for the lack of understanding: First, data from (mostly optical) measurements can be very misleading because regions of high density thus observed are frequently identified with liquids. A common misconception is that if in an experiment one can optically identify "drops" and "ligaments", the observed fluid must be in a liquid state. This inference is incorrect because in fact optical measurements detect any large change (i.e. gradients) in density. Thus, the density ratio may be well below Omicron(10(exp 3)) that characterizes its liquid/gas value, but the measurement will still identify a change in the index of refraction providing that the change is sudden (steep gradients). As shown by simulations of supercritical fluids, under certain conditions the density gradients may remain large during the supercritical binary fluids mixing, thus making them optically identifiable. Therefore, there is no inconsistency between the optical observation of high density regions and the fluids being in a supercritical state. A second misconception is that because a fluid has a liquid-like density, it is appropriate to model it as a liquid. However, such fluids may have liquid-like densities while their transport properties differ from those of a liquid. Considering that the critical pressure of most fuel hydrocarbons used in Diesel and gas turbine engines is in the range of 1.5 - 3 MPa, and the fact that the maximum pressure attained in these engines is about 6 Mps, it is clear that the fuel in the combustion chamber will experience both subcritical and supercritical conditions. Studies of drop behavior over a wide range of pressures were performed in the past, however none of these studies identified the crucial differences between the subcritical and supercritical behavior. In fact, in two of these studies, it was found that the subcritical and supercritical behavior is similar as the drop diameter decreased according to the classical d(exp 2)-law over a wide range of pressures and drop diameters. The present study is devoted to the exploration of differences in fluid-behavior characteristics under subcritical and supercritical conditions in the particular case of heptane fluid drops in nitrogen; these substances were selected because of the availability of experimental observations for model validation.

Harstad, K.↗

Bifurcation and Hysteresis of the Magnetospheric Structure with a varying Southward IMF: Field Topology and Global Three-dimensional Full Particle Simulations

Using a three-dimensional full electromagnetic particle model (EMPM), we have performed global simulations of the interaction between the solar wind and the terrestrial magnetosphere, and have investigated its asymptotic stability. The distance between the dayside magnetopause subsolar point and the Earth center, R(sub mp) is measured, as the intensity of southward IMF |B(sub z)| is slowly varying. Based on the field topology theory, one analyzes the variation of R(sub mp) as a reference index of the dynamics of this interaction, when IMF |B(sub z)| successively increases and decreases to its original value. Two striking results are observed. First, as the IMF |B(sub z)| increases above a critical value, the variation of R(sub mp) suddenly changes (so called 'bifurcation' process in field topology). Above this critical value, the overall magnetic field topology changes drastically and is identified as being the signature of magnetic reconnection at the subsolar point on the magnetopause. Second, this subsolar point recovers its original location R(sub mp) by following different paths as the IMF |B(sub z)| value increases (from zero to a maximum fixed value) and decreases (from this maximum to zero) passing through some critical values. These different paths are the signature of 'hysteresis' effect, and are characteristic of the so-called 'subcritical-type' bifurcation. This hysteresis signature indicates that dissipation processes take place via an energy transfer from the solar wind to the magnetosphere by some irreversible way, which leads to a drastic change in the magnetospheric field topology. This hysteresis is interpreted herein as a consequence of the magnetic reconnection taking place at the dayside magnetopause. The field topology reveals to be a very powerful tool to analyze the signatures of three-dimensional magnetic reconnection without the obligation for determining the mechanisms responsible for, and the consequences of the reconnection on the overall magnetospheric dynamics.

Cai, DongSheng↗

Numerical simulation of fluid flow and heat transfer in a thin liquid film over a stationary and rotating disk and comparison with experimental data

In the first section, improvements in the theoretical model and computational procedure for the prediction of film height and heat-transfer coefficient of the free surface flow of a radially-spreading thin liquid film adjacent to a flat horizontal surface of finite extent are presented. Flows in the presence and absence of gravity are considered. Theoretical results are compared to available experimental data with good agreement. In the presence of gravity, a hydraulic jump is present, isolating the flow into two regimes: supercritical upstream from the jump and subcritical downstream of it. In this situation, the effects of surface tension are important near the outer edge of the disk where the fluid experiences a free fall. A region of flow separation is present just downstream of the jump. In the absence of gravity, no hydraulic jump or separated flow region is present. The variation of the heat-transfer coefficient for flows in the presence and absence of gravity are also presented. In the second section, the results of a numerical simulation of the flow field and associated heat transfer coefficients are presented for the free surface flow of a thin liquid film adjacent to a horizontal rotating disk. The computation was performed for different flow rates and rotational velocities using a 3-D boundary-fitted coordinate system. Since the geometry of the free surface is unknown and dependent on flow rate, rate of rotation, and other parameters, an iterative procedure had to be used to ascertain its location. The computed film height agreed well with existing experimental measurements. The flow is found to be dominated by inertia near the entrance and close to the free surface and dominated by centrifugal force at larger radii and adjacent to the disk. The rotation enhances the heat transfer coefficient by a significant amount.

Faghri, Amir↗

Modifications to the Bubble experiment and preparation for additional irradiations

SHINE Medical Technologies is planning to use neutron-induced fission in a subcritical low-enriched-uranium uranyl sulfate target solution for production of 99 Mo. During this operation, the solution will undergo self-heating due to fissioning of the uranium, radiolytic decomposition of the water, and circulation due to thermal gradients generated in the solution, and will be cooled by cooling tubes running through the annulus and from cooling outside the annulus. Because the formation of the radiolysis-induced bubbles (H 2 and O 2 ) and their size and dynamics will impact the operational parameters of the liquid target, an understanding of bubble behavior is critical for the ability to predict the behavior of the target solution during this operation. It is also important to be able to predict the thermal gradients and the circulation in the vessel. Researchers at Argonne National Laboratory have designed an experimental setup to study radiolytic gas formation in uranyl sulfate under direct electron beam irradiation and have conducted initial experiments. Results of those experiments provided invaluable information on thermal hydraulic behavior of the solution and some information on bubble formation and behavior, but those initial experiments fell short in the measurements of the gas generation rates and bubble behavior. To address the shortcomings of the original experiment, the irradiation setup was modified to improve our abilities to measure gas generation rates and measure the temperature distribution in the solution with better precision. Modifications to the experimental setup and preparation for the irradiations are described below.

07 ISOTOPE AND RADIATION SOURCES↗

Fluid dynamics and low gravity effects of chemical vapor deposition

Based on the comparison between experimental data and numerical results for the growth of GaAs from TMGa, it was shown that 3D simulations are necessary to simulate rectangular CVD reactors even when operated under subcritical (Ra) conditions. The important points found are summarized in the three attached reprints. The experimental studies of mixed convection in horizontal channels have shown three regimes of high Ra (22,220) number flows. At Re = 18.5, the rolls develop very quickly, significantly modulating the axial velocity even before it reaches the beginning of the hot plate. A few centimeters downstream, the velocities become asymmetric about the vertical centerplane and at x = 12 cm, become unsteady. These asymmetries were predicted theoretically, but experimental evidence has not been published prior to this work. At Re = 36, the axial velocity is only slightly modified at x = 0. Although the flow remains steady and symmetric about the vertical centerplane, there is a small spatial oscillation in the velocities over the length of the channel. The period of this oscillation was around 5 cm. At Re = 54, the longitudinal rolls developed smoothly over a length of 30 cm, with no asymmetries, unsteadiness, or spatial oscillations. Comparison of numerical simulations of these flows to experiments has revealed the importance and difficulty of setting proper thermal boundary conditions on the sidewalls. Calculated flows and experimentally measured flows showed very similar profiles, but at different axial locations, with the rolls developing more rapidly in the experiments. This is directly attributable to partially conducting sidewalls of the apparatus being hotter in the entrance section than the adiabatic walls of the simulations. A thorough comparison of the experimental data and numerical results for a variety of sidewall boundary conditions is in preparation.

Nyce, Thomas A.↗