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At least 217 records · Page 12

Coded aperture imaging for fluorescent x-rays

We employ a coded aperture pattern in front of a pixilated charge couple device detector to image fluorescent x-rays (6–25 KeV) from samples irradiated with synchrotron radiation. Coded apertures encode the angular direction of x-rays, and given a known source plane, allow for a large numerical aperture x-ray imaging system. The algorithm to develop and fabricate the free standing No-Two-Holes-Touching aperture pattern was developed. The algorithms to reconstruct the x-ray image from the recorded encoded pattern were developed by means of a ray tracing technique and confirmed by experiments on standard samples.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A qualitative assessment of current CCF guidance based on a review of safety system digital implementation changes with evolving technology - 148

This paper is a summary of a study performed in support of the US Nuclear Regulatory Commission (NRC) to evaluate current policy on software common-cause failure (CCF). The study reported in this paper is one of several that contributed to the technical basis to inform NRC staff. The study first reviewed policies and assessment guidance as discussed in the Staff Requirements Memorandum to the Secretary of the Commission, Office of the NRC (SECY) 93-087, Policy, Technical, and Licensing Issues Pertaining to Evolutionary and Advanced Light Water Reactor (ALWR) Designs, and Branch Technical Position (BTP) 7-19, Guidance on Evaluation of Defense-in-Depth and Diversity in Digital Computer-Based Instrumentation and Control Systems, as well as Chapter 7, 'Instrumentation and Controls', in NUREG-0800, Standard Review Plan for Review of Safety Analysis Reports for Nuclear Power Plants. The study then examined instrumentation and controls (I and C) technology implementations in nuclear power plants in the light of current CCF guidance. The intent was to assess whether the current position on CCF remains appropriate given the evolutions in digital safety system implementations and, if gaps in the guidance were found, to provide recommendations as to how these gaps could be closed. The methodology adopted was to review the vendors' technology and software implementation processes for digital safety systems as technology evolved. The following three representative safety systems were selected to provide illustrative examples: - Eagle 21 was selected to represent vintage microprocessor-based technology used from the 1980's to mid-1990's, - TELEPERM XS (TXS) was selected to represent second generation microprocessor-based technology used from the mid-1990's to the 2000's, and - The advanced logic system (ALS) was selected to represent the latest trend of using technology based on field programmable gate arrays (FPGAs). Technology implementations were reviewed in light of the basic premise of the NRC in BTP 7-19 (Revision 6), that software-based or software-logic-based digital system development errors are a credible source of CCF and therefore are susceptible to CCF because identical copies of the software-based logic and architecture are present in redundant divisions of safety-related systems. BTP 7-19 categorizes firmware and logic developed from software-based development systems all under software. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Effect of high energy electrons on H{sup −} production and destruction in a high current DC negative ion source for cyclotron

Recently, a filament driven multi-cusp negative ion source has been developed for proton cyclotrons in medical applications. In this study, numerical modeling of the filament arc-discharge source plasma has been done with kinetic modeling of electrons in the ion source plasmas by the multi-cusp arc-discharge code and zero dimensional rate equations for hydrogen molecules and negative ions. In this paper, main focus is placed on the effects of the arc-discharge power on the electron energy distribution function and the resultant H{sup −} production. The modelling results reasonably explains the dependence of the H{sup −} extraction current on the arc-discharge power in the experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

R “SHINY” GUI DEVELOPMENT FOR URANIUM ISOTOPIC ANALYSIS WITH MATRIX-ASSISTED IONIZATION MASS SPECTROMETRY

The international nuclear safeguards community continues to seek rapid, accurate, and precise characterization capabilities for the in-field measurement of uranium isotopic compositions in nuclear facilities. Mass spectrometry (MS) is considered the “gold standard” for analysis of relatively long-lived actinides such as uranium (U) and plutonium; however, conventional MS analysis often requires time consuming sample preparation and complex analytical methodologies that are difficult to perform in-field or in-facility. Matrix assisted ionization (MAI) is a novel ambient ionization MS technique (i.e., MAI-MS) that potentially addresses these challenges due to the relative simplicity of the ionization phenomenon and ruggedness of ambient MS instrumentation. Savannah River National Laboratory (SRNL, USA) has demonstrated this technique for nanogram-level 235U/238U isotope ratio measurements within seconds, with percent-level analytical uncertainties capable of discriminating depleted, natural, and low-enriched uranium. Current experimental work on developing MAI methods for uranium isotopic analysis has been enabled by parallel development of a comprehensive MAI-MS data analysis suite at SRNL. Development of this bespoke data analysis software was necessary because commercially available ambient MS software is poorly suited for uranium isotope ratio measurement. The effort leverages the power of R, a popular open-source programming language, and Shiny, an R package providing tools for graphical user interface (GUI) and web interface coding. This software allows researchers without any programming experience to harness and utilize R’s considerable data analysis/visualization power.

LaBone, Elizabeth D.↗

Threat Sources for Creating Synthetic Urban Search Data

Equivalent point source energy emission distributions were computed for various threat sources for use in simulating the detector responses for urban search scenarios. The sources include standard isotopic sources used in detector testing, medical and industrial sources occasionally encountered in urban searches, and several types of special nuclear materials. Most of the equivalent point source distributions represent small sources inside some amount of shielding, but the special nuclear material sources represent volumetrically distributed sources in spheres of metal. Text-based inputs for emission distributions are available for the Monte Carlo transport codes Monte Carlo N-Particle, SCALE/MAVRIC, and Omnibus/Shift, any of which can easily be converted to other formats. These sources were developed for use in the Radiological Anomaly Detection and Identification (RADAI) project and the follow-on project, the RADAI-Extended project, sponsored by the National Nuclear Security Administration Office of Defense Nuclear Nonproliferation Research and Development.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Analysis of the beam halo in negative ion sources by using 3D3V PIC code

The physical mechanism of the formation of the negative ion beam halo and the heat loads of the multi-stage acceleration grids are investigated with the 3D PIC (particle in cell) simulation. The following physical mechanism of the beam halo formation is verified: The beam core and the halo consist of the negative ions extracted from the center and the periphery of the meniscus, respectively. This difference of negative ion extraction location results in a geometrical aberration. Furthermore, it is shown that the heat loads on the first acceleration grid and the second acceleration grid are quantitatively improved compared with those for the 2D PIC simulation result.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Morpheus Spectral Counter: A computational tool for label-free quantitative mass spectrometry using the Morpheus search engine

Label-free quantitative MS based on the Normalized Spectral Abundance Factor (NSAF) has emerged as a straightforward and robust method to determine the relative abundance of individual proteins within complex mixtures. Here, we present Morpheus Spectral Counter (MSpC) as the first computational tool that directly calculates NSAF values from output obtained from Morpheus, a fast, open-source, peptide-MS/MS matching engine compatible with high-resolution accurate-mass instruments. NSAF has distinct advantages over other MS-based quantification methods, including a higher dynamic range as compared to isobaric tags, no requirement to align and re-extract MS1 peaks, and increased speed. MSpC features an easy to use graphic user interface that additionally calculates both distributed and unique NSAF values to permit analyses of both protein families and isoforms/proteoforms. MSpC determinations of protein concentration were linear over several orders of magnitude based on the analysis of several high-mass accuracy datasets either obtained from PRIDE or generated with total cell extracts spiked with purified Arabidopsis 20S proteasomes. Lastly, the MSpC software was developed in C# and is open sourced under a permissive license with the code made available at http://dcgemperline.github.io/Morpheus_SpC/.

59 BASIC BIOLOGICAL SCIENCES↗

Validation of the EDGES Low-band Antenna Beam Model

The response of the antenna is a source of uncertainty in measurements with the Experiment to Detect the Global Epoch of Reionization Signature (EDGES). We aim to validate the electromagnetic beam model of the low-band (50–100 MHz) dipole antenna with comparisons between models and against data. We find that simulations of a simplified model of the antenna over an infinite perfectly conducting ground plane are, with one exception, robust to changes in the numerical electromagnetic solver code or algorithm. For simulations of the antenna with the actual finite ground plane and realistic soil properties, we find that two out of three numerical solvers agree well. Applying our analysis pipeline to a simulated drift-scan observation from an early EDGES low-band instrument that had a 10 m × 10 m ground plane, we find residual levels after fitting and removing a five-term foreground model from the simulated data binned in local sidereal time (LST) average about 250 mK with ±40 mK variation between numerical solvers. A similar analysis of the primary 30 m × 30 m sawtooth ground plane reduced the LST-averaged residuals to about 90 mK with ±10 mK between the two viable solvers. More broadly we show that larger ground planes generally perform better than smaller ground planes. Simulated data have a power that is within 4% of real observations, a limitation of net accuracy of the sky and beam models. We observe that residual spectral structures after foreground model fits match qualitatively between simulated data and observations, suggesting that the frequency dependence of the beam is reasonably represented by the models. We find that a soil conductivity of 0.02 S m{sup -1} and relative permittivity of 3.5 yield good agreement between simulated spectra and observations. This is consistent with the soil properties reported by Sutinjo et al. for the Murchison Radio-astronomy Observatory, where EDGES is located.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Conception and realization of a parallel-plate free-air ionization chamber for the absolute dosimetry of an ultrasoft X-ray beam

We report the design of a millimeter-sized parallel plate free-air ionization chamber (IC) aimed at determining the absolute air kerma rate of an ultra-soft X-ray beam (E = 1.5 keV). The size of the IC was determined so that the measurement volume satisfies the condition of charged-particle equilibrium. The correction factors necessary to properly measure the absolute kerma using the IC have been established. Particular attention was given to the determination of the effective mean energy for the 1.5 keV photons using the PENELOPE code. Other correction factors were determined by means of computer simulation (COMSOL™and FLUKA). Measurements of air kerma rates under specific operating parameters of the lab-bench X-ray source have been performed at various distances from that source and compared to Monte Carlo calculations. We show that the developed ionization chamber makes it possible to determine accurate photon fluence rates in routine work and will constitute substantial time-savings for future radiobiological experiments based on the use of ultra-soft X-rays.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

NEW TECHNIQUES FOR HIGH-CONTRAST IMAGING WITH ADI: THE ACORNS-ADI SEEDS DATA REDUCTION PIPELINE

We describe Algorithms for Calibration, Optimized Registration, and Nulling the Star in Angular Differential Imaging (ACORNS-ADI), a new, parallelized software package to reduce high-contrast imaging data, and its application to data from the SEEDS survey. We implement several new algorithms, including a method to register saturated images, a trimmed mean for combining an image sequence that reduces noise by up to {approx}20%, and a robust and computationally fast method to compute the sensitivity of a high-contrast observation everywhere on the field of view without introducing artificial sources. We also include a description of image processing steps to remove electronic artifacts specific to Hawaii2-RG detectors like the one used for SEEDS, and a detailed analysis of the Locally Optimized Combination of Images (LOCI) algorithm commonly used to reduce high-contrast imaging data. ACORNS-ADI is written in python. It is efficient and open-source, and includes several optional features which may improve performance on data from other instruments. ACORNS-ADI requires minimal modification to reduce data from instruments other than HiCIAO. It is freely available for download at www.github.com/t-brandt/acorns-adi under a Berkeley Software Distribution (BSD) license.

79 ASTRONOMY AND ASTROPHYSICS↗

Dark matter substructure modelling and sensitivity of the Cherenkov Telescope Array to Galactic dark halos

Hierarchical structure formation leads to a clumpy distribution of dark matter in the Milky Way. These clumps are possible targets to search for dark matter annihilation with present and future γ-ray instruments. Many uncertainties exist on the clump distribution, leading to disputed conclusions about the expected number of detectable clumps and the ensuing limits that can be obtained from non-detection. In this paper, we use the CLUMPY code to simulate thousands of skymaps for several clump distributions. This allows us to statistically assess the typical properties (mass, distance, angular size, luminosity) of the detectable clumps. Varying parameters of the clump distributions allows us to identify the key quantities to which the number of detectable clumps is the most sensitive. Focusing our analysis on two extreme clump configurations, yet consistent with results from numerical simulations, we revisit and compare various calculations made for the Fermi -LAT instrument, in terms of number of dark clumps expected and the angular power spectrum for the Galactic signal. We then focus on the prospects of detecting dark clumps with the future CTA instrument, for which we make a detailed sensitivity analysis using open-source CTA software. Based on a realistic scenario for the foreseen CTA extragalactic survey, and accounting for a post-trial sensitivity in the survey, we show that we obtain competitive and complementary limits to those based on long observation of a single bright dwarf spheroidal galaxy.

79 ASTRONOMY AND ASTROPHYSICS↗

The Nuclear Reaction Network WinNet

Abstract We present the state-of-the-art single-zone nuclear reaction network WinNet , which is capable of calculating the nucleosynthetic yields of a large variety of astrophysical environments and conditions. This ranges from the calculation of the primordial nucleosynthesis, where only a few nuclei are considered, to the ejecta of neutron star mergers with several thousands of involved nuclei. Here we describe the underlying physics and implementation details of the reaction network. We additionally present the numerical implementation of two different integration methods, the implicit Euler method and Gears method, along with their advantages and disadvantages. We furthermore describe basic example cases of thermodynamic conditions that we provide together with the network and demonstrate the reliability of the code by using simple test cases. With this publication, WinNet will be publicly available and open source at GitHub and Zenodo.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ON THE FERMI LARGE AREA TELESCOPE SURPLUS OF DIFFUSE GALACTIC GAMMA-RAY EMISSION

Recent observations of diffuse Galactic γ-ray emission (DGE) by the Fermi Large Area Telescope (Fermi-LAT) have shown significant deviations, above a few GeV to about 100 GeV, from DGE models that use the GALPROP code for the propagation of cosmic ray (CR) particles outside their sources in the Galaxy and their interaction with the target distributions of the interstellar gas and radiation fields. The surplus of radiation observed is most pronounced in the inner Galaxy, where the concentration of CR sources is strongest. The present study investigates this 'Fermi-LAT Galactic Plane Surplus' by estimating the γ-ray emission from the sources themselves, which is disregarded in the above DGE models. It is shown that the expected hard spectrum of CRs, still confined in their sources (source cosmic rays, SCRs), can indeed explain this surplus. The method is based on earlier studies regarding the so-called EGRET GeV excess, which by now is generally interpreted as an instrumental effect. The contribution from SCRs is also predicted to increasingly exceed the DGE models above 100 GeV, up to γ-ray energies of about 10 TeV, where the corresponding surplus exceeds the hadronic part of the DGE by about one order of magnitude. Above such energies, the emission surplus should decrease again with energy due to the finite lifetime of the assumed supernova remnant sources. Observations of the DGE in the inner Galaxy at 15 TeV with the ground-based Milagro γ-ray detector and, at TeV energies, with the ARGO-YBJ detector are interpreted to provide confirmation of a significant SCR contribution to the DGE.

79 ASTRONOMY AND ASTROPHYSICS↗

The small-angle neutron scattering extension in MCNPX and the SANS cross section for nanodiamonds

Detonation nanodiamonds provide an intriguing prospect for the development of a very cold neutron (VCN) source or as a high albedo material for VCN reflection helping to control leakage of cold and very cold neutrons in a moderator. The investigation of source and reflector designs necessitates the development of new simulation tools for existing Monte Carlo codes that include small angle neutron scattering (SANS). The SANS extension in MCNPX 2.7 provides an analytical model of hard-sphere scattering with variable scattering particle sizes, size distributions, and packing fractions in order to supplement currently existing scattering kernels as well as the capability to read an experimentally determined small angle neutron scattering profile from a data file. The SANS extension is discussed and compared to nanodiamond SANS measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A New Safeguards Technique for Spent Fuel Verification in Dry Storage by Using He-4 Detectors - 18262

It is demanded to find key issues and critical paths for verifying and monitoring a spent nuclear fuel cask or storage with a purpose of non-proliferation of nuclear weapon. However, unfortunately there are no reliable methods to verify the containment in a spent nuclear fuel cask or storage. Therefore, research and development (R and D) has been continuously required to develop new and alternative technologies for searching and verifying undeclared nuclear materials, activities, and facilities. Therefore, the present authors have developed a new safeguards technique of passively scanning a spent fuel cask or storage using pressurized He-4 scintillation neutron detectors. A new approach is to quickly verify content in a spent nuclear fuel cask or presence of all special nuclear materials in unknown packages by comparing experimental and computational results. For that, the present authors have developed a new algorithm and user-interface coupled ORIGEN-ARP and MCNP codes, and the prototype safeguards apparatus employing the array of He-4 fast neutron detectors has been designed, built, and tested. The feasibility test of this new apparatus has been performed with Cf-252 neutron sources and the laboratory scale model cask, minimized by a factor of ten compared to the actual dimension of a KN-21 cask. This technique has several advantages over current methods based on neutron and gamma detection; (1) incident neutron energy information is preserved, (2) disturbance of gamma-ray is excellently rejected (discriminated), and (3) much higher neutron counts and operational cost and space-effectiveness are expected since no moderator is required for fast neutrons. The final goal of this study will (1) conduct a prototype instrument and employ it to monitor a nuclear spent fuel cask or storage at a commercial nuclear power reactor facilities, (2) use spectral-specific measurement data to show proof of concept for measurable data successfully converted to quantifiable signatures, such as diversion/removal of fuel, and maintenance of fuel and cask integrity of fuel, and (3) develop a cask imaging capability. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Nitrogen ion implantation into various materials using 28 GHz electron cyclotron resonance ion source

The installation of the 28 GHz electron cyclotron resonance ion source (ECRIS) ion implantation beamline was recently completed at the Korea Basic Science Institute. The apparatus contains a beam monitoring system and a sample holder for the ion implantation process. The new implantation system can function as a multipurpose tool since it can implant a variety of ions, ranging hydrogen to uranium, into different materials with precise control and with implantation areas as large as 1–10 mm{sup 2}. The implantation chamber was designed to measure the beam properties with a diagnostic system as well as to perform ion implantation with an in situ system including a mass spectrometer. This advanced implantation system can be employed in novel applications, including the production of a variety of new materials such as metals, polymers, and ceramics and the irradiation testing and fabrication of structural and functional materials to be used in future nuclear fusion reactors. In this investigation, the first nitrogen ion implantation experiments were conducted using the new system. The 28 GHz ECRIS implanted low-energy, multi-charged nitrogen ions into copper, zinc, and cobalt substrates, and the ion implantation depth profiles were obtained. SRIM 2013 code was used to calculate the profiles under identical conditions, and the experimental and simulation results are presented and compared in this report. The depths and ranges of the ion distributions in the experimental and simulation results agree closely and demonstrate that the new system will enable the treatment of various substrates for advanced materials research.

36 MATERIALS SCIENCE↗

Investigation of the hard x-ray background in backlit pinhole imagers

Hard x-rays from laser-produced hot electrons (>10 keV) in backlit pinhole imagers can give rise to a background signal that decreases signal dynamic range in radiographs. Consequently, significant uncertainties are introduced to the measured optical depth of imaged plasmas. Past experiments have demonstrated that hard x-rays are produced when hot electrons interact with the high-Z pinhole substrate used to collimate the softer He-α x-ray source. Results are presented from recent experiments performed on the OMEGA-60 laser to further study the production of hard x-rays in the pinhole substrate and how these x-rays contribute to the background signal in radiographs. Radiographic image plates measured hard x-rays from pinhole imagers with Mo, Sn, and Ta pinhole substrates. The variation in background signal between pinhole substrates provides evidence that much of this background comes from x-rays produced in the pinhole substrate itself. A Monte Carlo electron transport code was used to model x-ray production from hot electrons interacting in the pinhole substrate, as well as to model measurements of x-rays from the irradiated side of the targets, recorded by a bremsstrahlung x-ray spectrometer. Inconsistencies in inferred hot electron distributions between the different pinhole substrate materials demonstrate that additional sources of hot electrons beyond those modeled may produce hard x-rays in the pinhole substrate.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

MITgcm-AD v2: Open source tangent linear and adjoint modeling framework for the oceans and atmosphere enabled by the Automatic Differentiation tool Tapenade

The Massachusetts Institute of Technology General Circulation Model (MITgcm) is widely used by the climate science community to simulate planetary atmosphere and ocean circulations. A defining feature of the MITgcm is that it has been developed to be compatible with an algorithmic differentiation (AD) tool, TAF, enabling the generation of tangent-linear and adjoint models. These provide gradient information which enables dynamics-based sensitivity and attribution studies, state and parameter estimation, and rigorous uncertainty quantification. Importantly, gradient information is essential for computing comprehensive sensitivities and performing efficient large-scale data assimilation, ensuring that observations collected from satellites and in-situ measuring instruments can be effectively used to optimize a large uncertain control space. As a result, the MITgcm forms the dynamical core of a key data assimilation product employed by the physical oceanography research community: Estimating the Circulation and Climate of the Ocean (ECCO) state estimate. Although MITgcm and ECCO are used extensively within the research community, the AD tool TAF is proprietary and hence inaccessible to a large proportion of these users. The new version 2 (MITgcm-AD v2) framework introduced here is based on the source-to-source AD tool Tapenade, which has recently been open-sourced. Another feature of Tapenade is that it stores required variables by default (instead of recomputing them) which simplifies the implementation of efficient, AD-compatible code. The framework has been integrated with the MITgcm model’s main branch and is now freely available.

Adjoints↗