SEARCH · Engineering Papers

Results for “Radionuclide”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

SourceResearch connectionFrom yearThrough year

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 217 records · Page 12

All sources NASA NTRS DOE OSTI

NASA NTRS1991

The Cl-36 in the stratosphere

Initial measurements of the cosmogenic radionuclide, Cl-36, in the lower stratosphere were made by accelerator mass spectrometry. Samples were obtained using the large volume LASL air sampling pods on a NASA WB-57F aircraft. Untreated (for collection of particulates only) and tetrabutyl ammonium hydroxide treated (for collection of particulates and HCl) IPC-1478 filters were flown on three flights in the lower stratosphere. Chlorine (Cl) and Cl compounds are important trace constituents for stratospheric chemistry, in particular with respect to O3 destruction. Stratospheric Cl chemistry has recently received increased attention with the observation of strong O3 depletion in the Antarctic winter vortex and in the weaker and more complex Arctic winter vortices. Cosmogenic (Cl-36) is produced by spallation reactions from Ar mainly in the stratosphere, and has had several applications as a geochemical tracer. The large amounts of Cl-36 introduced by nuclear weapon testing have been removed from the stratosphere by now, and measurements in the stratosphere to obtain cosmogenic production rates and concentration distributions is now possible. The use of cosmogenic Cl-36 as a tracer for stratospheric Cl chemistry and for stratospheric/tropospheric exchange processes is investigated. A first attempt to determine stratospheric and tropospheric production rates, the partitioning of Cl-36 among particulate and gaseous Cl compounds, and the respective inventories and removal rates is being made. Results from a flight at 13.7 km, 30-33 degrees N, 97-107 degrees W, and from a second flight at 17.7 km, 43-45-36 degrees N, 92-94 degrees W, for the untreated and treated filters respectively are presented.

Deck, Bruce↗

NASA NTRS1991

Profiles of alpha 13 C and alpha D in methane from the lower stratosphere

Methane is an important greenhouse gas of biogenic and anthropogenic origin for which global budgets are being constructed from a variety of data. One approach to the global methane budget is the use of the stable isotopes C-13 and D, and the radionuclide C-14 as tracers. The authors measured the isotopic composition of methane from various sources and in tropospheric air for a number of locations. Here, the authors report on the isotopic composition of methane from the lower stratosphere. Measurements of this concentration in the stratosphere can yield estimates for the kinetic isotope effects in the methane destruction reactions. These effects have to be known for quantitative isotopic methane budgets.

Wahlen, Martin↗

NASA NTRS1990

Medium and high-energy neutrino physics from a lunar base

Neutrino astronomy at high energy levels conducted from the moon is treated by considering 'particle astronomy' as a part of physics and the moon as a neutrino detector. The ability to observe the Galactic center is described by means of a 1-1000 TeV 'window' related to the drop in flux of atmospheric neutrinos from the earth. The long-baseline particle physics which are described in terms of a lunar observatory are found to be possible exclusively from a lunar station. The earth's neutrinos can be eliminated for the observations of astrophysical sources, and other potential areas of investigation include neutrino oscillation and the moon's interior. Neutrino exploration of the earth-moon and antineutrino radionuclide imaging are also considered. The moon is concluded to be a significantly more effective orbital platform for the study of neutrino physics than orbiting satellites developed on earth.

Wilson, Thomas L.↗

NASA NTRS1991

Analysis of surfaces from the LDEF A0114, phase 4

Progress made from 1 Mar. to 31 Aug. 1991 is presented. The work concentrated on profilometry measurements of eroded and corroded sample surfaces, optical transmission measurements, analysis of the pinhole camera, and x-ray photoelectron spectroscopic (XPS) analysis of some samples. The following papers are presented: (1) observation of Be-7 on the surface of the Long Duration Exposure Facility (LDEF) Spacecraft; (2) measurement of the passive attitude control performance of a recovered spacecraft; (3) effects on LDEF exposed copper flim and bulk; (4) measurements of erosion characteristics for metal and polymer surfaces using profilometry; (5) the interactions of atmospheric cosmogenic radionuclides with spacecraft surfaces; (6) pinhole cameras as sensors for atomic oxygen in orbit; and (7) interaction of atomic oxygen with solid surfaces in low earth orbit- results from LDEF experiment A0114.

Gregory, John C.↗

NASA NTRS1992

Surface activation of Concorde by Be-7

Activation analysis of two airframe components from the Concorde aircraft has identified the presence of Be-7, a nuclide found by other investigators that was deposited on the forward edge of the Long Duration Exposure Facility (LDEF) structure. The results of the Concorde analysis indicate that this phenomenon is very much a surface effect, and that the areal densities of the Be-7 are comparable to those found for LDEF. The collection of Be-7 by the aircraft must be greater than in the case of LDEF (since duration for which Concorde is accumulating the nuclide is shorter) and is of the order of 1.2 to 41 nuclei/sq cm(-)s(exp -1) depending upon assumptions made regarding the altitude at which collection becomes appreciable, and the efficiency of the process which removes the radionuclide.

Truscott, P. R.↗

NASA NTRS1992

How Mars lost its atmosphere

There is a widespread suspicion that Mars thin atmosphere is in some way attributable to the planet's size. Another possibility is that the atmosphere was never degassed or outgassed in the first place. I prefer escape. Hydrodynamic escape (vigorous thermal escape) and impact erosion (expulsion of atmosphere by impacts) are two processes that should have been operative early. Although in principle hydrodynamic escape could have shrunk Mars atmosphere a hundredfold while leaving the composition of the remnant atmosphere nearly unaltered, very high escape fluxes are required. The implicated escape mechanism must have been efficient, nearly non-fractionating, and vastly more potent for Mars than for Earth or Venus. Impact erosion is an appealing candidate. Noble gases are the obvious first test. Noble gases are the most volatile elements and so are the most likely to have been affected by impact erosion and the easiest to address quantitatively. Xenon in particular imposes three constraints on how Mars lost its atmosphere: (1) the very low abundance of nonradiogenic Xe abundance of nonradiogenic Xe compared to Earth, Venus, and likely meteoritic sources; (2) its nonradiogenic isotopes distinct from likely meteoritic sources; and (3) the relatively high absolute abundance of radiogenic daughter of the extinct radionuclide I-129 (half-life 17 Myr). In impact erosion, the first two become constraints on the composition, mass distribution, and orbital elements of the impactors. The third requires that Mars lost its nonradiogenic Xe early, probably before it was 100 Myr old. Impact erosion can explain Mars by any of three stories. (1) Mars in unlikely. In a sort of planetary brinkmanship, impact erosion almost removed the entire atmosphere but was arrested just in time. (2) Martian noble gases are cometary and cometary Xe is as isotopically mass fractionated as Martian and terrestrial Xe. This is most easily accomplished if a relatively thick geochemically controlled CO2 atmosphere protected trace atmophiles against escape. (3) Mars was indeed stripped of its early atmosphere but a small remnant was safely stored in the regolith, later released as a byproduct of water mobilization.

Zahnle, Kevin↗

NASA NTRS1992

Radioactive 7Be materials flown on LDEF

Following the discovery of the atmospheric cosmogenic radionuclide Be-7 on the Long Duration Exposure Facility (LDEF), we began a search for other known nuclides produced by similar mechanisms. None of the others have the narrow gamma-ray line emission of Be-7 decay which enable its rapid detection and quantification. A search for Be-10 atoms on LDEF clamp plates using accelerator mass spectrometry is described. An unexpected result was obtained.

Gregory, John C.↗

NASA NTRS1991

Lunar ferroan anorthosites and mare basalt sources - The mixed connection

Global overturn of a hot, gravitationally unstable lunar mantle immediately following the solidification of a magma ocean explains several characteristics of lunar petrology. Lunar mare basalt sources are inferred to be depleted in europium and alumina. These depletions are consensually attributed to complementary plagioclase floating from a magma ocean. However, in contrast to the mare basalt source parent magma, the ferroan anorthosite parent magma was more evolved by virtue of its lower Mg/Fe ratio and Ni abundances, although less evolved in its poverty of clinopyroxene constituents, flat rare earth pattern, and lower incompatible element abundances. The europium anomaly in mare sources is inferred to be present at 400 km depth, too deep to have been directly influenced by plagioclase crystallization. Massive overturning of the post-magma ocean mantle would have carried down clinopyroxene, ilmenite, and phases containing fractionated rare earths, europium anomalies, and some heat-producing radionuclides.

Ryder, Graham↗

NASA NTRS1991

Exposure histories of lunar meteorites - ALHA81005, MAC88104, MAC88105, and Y791197

The cosmogenic radionuclides Ca-41, Cl-36, Al-26, and Be-10 in the Allan Hills 81005, MacAlpine Hills 88104, MacAlpine Hills 88105, and Yamato 791197 meteorites were measured by accelerator mass spectrometry. Mn-53 in Allan Hills 81005 and Yamato 791197 was measured by neutron activation. These four lunar meteorites experienced similar histories. They were ejected from near the surface of the moon ranging in depth down to 400 g/sq cm and had very short transition times (less than 0.1 Ma) from the moon to the earth. A comparison of the cosmogenic nuclide concentrations in MacAlpine Hills 88104 and MacAlpine Hills 88105 clearly indicates that they are a pair from the same fall.

Nishiizumi, K.↗

NASA NTRS1991

Exposure histories of the lunar meteorites - MAC88104, MAC88105, Y791197, and Y86032

Four lunar meteorites were analyzed for the cosmogenic radionuclides Be-10, Al-26, Cl-36, and Ca-41. Histories of exposure to cosmic rays were modelled in terms of two-stage irradiations, each with a long first stage on the moon, lasting a time T sub 2pi greater than 5 Ma at a burial depth d sub 2pi(g/sq cm), followed by a second stage in space, i.e., the transit time between the moon and the earth, lasting a time T sub 4pi (Ma) in a body of typical metereological size. It is inferred that the production rate is of the order of 5/Ma and the arrival rate worldwide is about 3,000,000 meteorites/Ma. It is concluded that each impact event large enough to produce lunar meteorites sends a large number of them to the earth.

Vogt, S.↗

NASA NTRS1992

On the modulation of X ray fluxes in thunderstorms

The production of X-ray fluxes in thunderstorms has been attributed to bremsstrahlung. Assuming this, another question arises. How can a thunderstorm modulate the number density of electrons which are sufficiently energetic to produce X-rays? As a partial answer to this question, the effects of typical thunderstorm electric fields on a background population of energetic electrons, such as produced by cosmic ray secondaries and their decays or the decay of airborne radionuclides, are considered. The observed variation of X-ray flux is shown to be accounted for by a simple model involving typical electric field strengths. A necessary background electron number density is found from the model and is determined to be more than 2 orders of magnitude higher than that available from radon decay and a factor of 8 higher than that available from cosmic ray secondaries. The ionization enhancement due to energetic electrons and X-rays is discussed.

Mccarthy, Michael P.↗

NASA NTRS1991

Solar-cosmic-ray fluxes during the last ten million years

The fluxes of energetic (E is greater than or approximately equal to 10 MeV) solar particles in the vicinity of the earth in the past can be determined from nuclides that they produced in the top centimeter of lunar rocks. Activity-vs-depth profiles of short-lived radioactivities measured in the top centimeter of lunar rocks agree with profiles calculated with directly measured solar-proton fluxes since about 1965 and were used with indirect observations to get solar-proton fluxes back to 1956. Lunar-rock profiles for long-lived radionuclides have been used to infer solar-proton fluxes averaged over several time periods in the past. New results are reported for solar-proton-produced Kr-81 measured in lunar rock 68815. Activities of 76,000-yr Ni-59 can be used to get fluxes of solar alpha particles averaged over the last 100,000 yr. The average solar-proton fluxes in the past are not greatly different from those observed during the last three 11-yr solar cycles. The work that needs to be done to determine more and better fluxes of energetic particles from the sun in the past is discussed.

Reedy, Robert C.↗

NASA NTRS1992

Beryllium 7 and lead 210 in the Western Hemisphere Arctic atmosphere - Observations from three recent aircraft-based sampling programs

Concentrations of the natural radionuclides Be-7 and Pb-210 in the Western Hemisphere Arctic atmosphere were determined during the recent NOAA Arctic Gas and Aerosol Sampling Program (AGASP 3) and NASA Global Tropospheric Experiment/Arctic Boundary Layer Expeditions (GTE/ABLE 3A and ABLE 3B) missions. Be-7 concentrations measured during the AGASP 3 mission north and west of Norway are in accord with previous results for high northern latitudes, but suggest that the 'stratospheric' air masses sampled at the highest elevations reached were significantly diluted with tropospheric air. Higher resolution sampling in the free troposphere of the North American Arctic during ABLE 3B revealed a layer of elevated Be-7 concentrations near 5 km. The distribution of Pb-210 in the high-altitude troposphere of North America during the summer was quite similar to distributions of more frequently measured aerosol species.

Dibb, Jack E.↗

NASA NTRS1993

On the Bur Gheluai H5 chondrite and other meteorites with complex exposure histories

Isotopic concentrations and track densities measured in 13 samples of the Bur Gheluai meteorite fall are presented. Experimental methods are described and results are presented for isotopic ratios of noble gases and cosmogenic radionuclide contents. Evidence for complex irradiation is discussed and a model for two-stage exposure histories is presented. The duration of each irradiation stage and possible effects on isotope production rates are considered. Explanations are suggested for the discrepant Ne production rates.

Vogt, S. K.↗

NASA NTRS1993

Al-26-Mg-26 ages of iron meteorites

An exposure age for an iron meteorite can be calculated from measurements of a radioactive nuclide and a stable nuclide that are produced by similar sets of nuclear reactions, provided that the stable nuclide is present with low initial abundance. The standard methods rely on either K-40 (t(sub 1/2) = 1.26 Gy), K-39, and K-41 or on a shorter-lived radionuclide and a stable, noble gas isotope. Widely used pairs of this type include Cl-36/Ar-36 and Al-26/Ne-21. Other pairs that may serve the purpose for iron meteorites contain many stable isotopes besides those of K and the noble gases that are produced partly by cosmic rays. We consider here the calculation of exposure ages, t(sub 26), from measurements of Al-26 (t(sub 1/2) = 0.7 My) and (stable) Mg-26. Ages based on Al-26/Mg-26 ratios, like those based on Cl-36/Ar-36 ratios, are 'buffered' against changes in relative production rates due to shielding because decay of the radioactive nuclide accounts for a good part of the inventory of the stable nuclide.

Herzog, G. F.↗

NASA NTRS1993

On possible Mn-53 heterogeneity in the early solar system

The effects of influence of shock wave propagation on the energy spectrum of accelerated particles that lead to different production rates of radionuclides, in particular, Mn-53, on small scales in the early solar system are shown. Search for evidence for extinct Mn-53 has stimulated investigations of Cr isotope anomalies in meteorites. The linear correlation between the magnitude of the Cr-53* excesses and the Mn/Cr ratio that unambiguously proves the in situ decay of Mn-53 was detected, really, in different mineral phases of some carbonaceous and enstatite chondrites, primitive achondrites, pallasites and iron meteorites. However, the data on the Cr-53* excess rarely defines a single linear array on a Mn-53-Cr-52 evolution diagram even for meteorites of the same chemical group. A clear isochron with Mn-53/Mn-55 = 4.4 plus or minus 1.0 x 10(exp -5) (in range of approximately 2.4 to approximately 9 x 10(exp -5)) is observed for CAI of the Allende C3-chondrite while the data for the Murchison C2- and Orgueil C1-chondrites fall much lower corresponding rather to Mn-53/Mn-55 less than 2 x 10(exp -5). In the case of iron meteorites it ranges from less than 5 x 10(exp -8) to less than 5 x 10(exp -5).

Lavrukhina, A. K.↗

NASA NTRS1993

Al-26 production profile and model comparisons in Canyon Diablo

The large preatmospheric size of the Canyon Diablo meteorite, a radius of about 15 m, makes it especially suitable for systematic studies of cosmogenic nuclide production rates of iron objects in a 2 pi geometry. To reconstruct the exposure history of the meteoroid, Heymann et al. investigated several fragments recovered from known geographic locations around the crater for their shock features and cosmogenic nobel gases. They applied the Signer-Nier noble gas production rate model to establish the preatmospheric depth of the specimens in the meteoroid. Cosmic ray exposure ages suggested a multi-episodic irradiation, with 170 or 540 Ma being inferred for most of the samples studied while two anomalous specimens indicated a possible third exposure age at 940 Ma. Be-10 and Cl-36 have been measured in a number of these same samples by accelerator mass spectrometry (AMS), with use being made of the preatmospheric depths determined in Heymann et al. to construct production profiles. The present study extends the cosmogenic radionuclide data to Al-26 and compares the results with both the production rate model of Reedy and Arnold and production rates determined from the cross sections used by the Reedy-Arnold model (for the major nuclear reactions making Al-26) in combination with differential fluxes calculated using the Los Alamos High Energy Transport (LAHET) Code System. Model calculations for Be-10 and Cl-36 have also been obtained.

Michlovich, E.↗

NASA NTRS1993

FE-60 and the evolution of eucrites

We have recently presented evidence for the existence of live Fe-60 in the early solar system. This evidence comes from observations of 2.4 to 50 epsilon unit (1 part in 10(exp 4)) relative excesses of Ni-60 measured in samples from the eucrite Chervony Kut (CK). These isotopic excesses have been produced by the decay of the short-lived radionuclide Fe-60 (T(sub 1/2) = 1.5 Ma). Because CK originates from a planetesimal which was totally molten and its high Fe/Ni ratio is due to a planet-wide Fe-Ni fractionation during metal-silicate segregation, the presence of the Fe-60 decay product indicates the large scale abundance of Fe-60 in the early solar system and its presence during differentiation of this planetesimal. The observed variable Ni-60 excesses in different bulk samples and mineral separates from CK can only be understood if some Fe-60 was still alive at the time when basaltic magma had solidified on the eucrite parent body. The lack of a correlation between Ni-60 and the respective Fe/Ni ratios in different mineral fractions from CK indicates a metamorphic remobilization of Ni after essentially all Fe-60 has decayed. However, Ni-60 from three bulk samples from different locations within the meteorite appears to correlate reasonably well with the respective Fe/Ni ratios. If we regard this correlation as an isochron then its slope yields a Fe-60/Fe-56 ratio f (3.9 +/- 0.6) x 10(exp -9) and an initial Ni-60 of 3.2 plus or minus 0.9 epsilon units at the time of crystallization of CK. Estimates based on these values and a approximately 10 Ma time interval between CK solidification and formation of the earliest condensates in the solar system followed by rapid accretion of planetary bodies indicate that the decay of Fe-60 could produce sufficient heat to melt these planetesimals. If Al-26 was present on a planetary scale as Fe-60 and at abundances close to values observed in Allende inclusions then melting of small early formed planets is inevitable. As an attempt to further explore the Fe-60/Ni-60 isotope system as an early solar system chronometer we studied another noncumulate eucrite, Juvinas (JUV) (sample USNM 1051), which belongs to the same subgroup as CK.

Shukolyukov, A.↗