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All sourcesNASA NTRSDOE OSTI
NASA NTRS2000

North Atlantic Aerosol Properties and Direct Radiative Effects: Key Results from TARFOX and ACE-2

Aerosol effects on atmospheric radiative fluxes provide a forcing function that can change the climate In potentially significant ways. This aerosol radiative forcing is a major source of uncertainty in understanding the observed climate change of the past century and in predicting future climate. To help reduce this uncertainty, the International Global Atmospheric Chemistry Project (IGAC) has endorsed a series of multiplatform aerosol field campaigns. The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the second Aerosol Characterization Experiment (ACE-2) were the first IGAC campaigns to address the impact of anthropogenic aerosols, Both TARFOX and ACE-2 gathered extensive data sets on aerosol properties and radiative effects, TARFOX focused on the urban-industrial haze plume flowing from the eastern United States over the western Atlantic Ocean, whereas ACE-2 studied aerosols carried over the eastern Atlantic from both European urban/industrial and African mineral sources. These aerosols often have a marked influence on the top-of-atmosphere radiances measured by satellites. Shown there are contours of aerosol optical depth derived from radiances measured by the AVHRR sensor on the NOAA-11 satellite. The contours readily show that aerosols originating in North America, Europe, and Africa impact the radiative properties of air over the North Atlantic. However, the accurate derivation of flux changes, or radiative forcing, from the satellite measured radiances or retrieved optical depths remains a difficult challenge. In this paper we summarize key initial results from TARFOX and, to a lesser extent, ACE-2, with a focus on those results that allow an improved assessment of the flux changes caused by North Atlantic aerosols at middle latitudes.

Russell, P. B.↗
NASA NTRS1998

North Atlantic Aerosol Properties and Direct Radiative Effects: Key Results from TARFOX and ACE-2

Aerosol effects on atmospheric radiative fluxes provide a forcing function that can change the climate in potentially significant ways. This aerosol radiative Forcing is a major source of uncertainty in understanding the observed climate change of the past century and in predicting, future climate. To help reduce this uncertainty, the International Global Atmospheric Chemistry Project (IGAC) has endorsed a series of multiplatform aerosol field campaigns. The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the second Aerosol Characterization Experiment (ACE-2) were the first IGAC campaigns to address the impact of anthropogenic aerosols. Both TARFOX and ACE-2 gathered extensive data sets on aerosol properties and radiative effects. TARFOX focused on the urban-industrial haze plume flowing from the eastern United States over the western Atlantic Ocean, whereas ACE-2 studied aerosols carried over the eastern Atlantic from both European urban/industrial and African mineral sources. These aerosols often have a marked influence on the top-of-atmosphere radiances measured by satellites, as illustrated in Figure 1. Shown there are contours of aerosol optical depth derived from radiances measured by the AVHRR sensor on the NOAA-11 satellite. The contours readily show that aerosols originating in North America, Europe, and Africa impact the radiative properties of air over the North Atlantic. However, the accurate derivation of flux chances, or radiative forcing, from the satellite-measured radiances or 'etrieved optical depths remains a difficult challenge. In this paper we summarize key Initial results from TARFOX and, to a lesser extent ACE-2, with a focus on those results that allow an improved assessment of the flux changes caused by North Atlantic aerosols at middle and high latitudes.

Russell, P. B.↗
NASA NTRS1996

Observation of Upper and Middle Tropospheric Clouds

The goal of this research has been to identify and describe the properties of climatically important cloud systems critically important to understanding their effects upon satellite remote sensing and the global climate. These goals have been pursued along several different but complementary lines of investigation: the design, construction, testing and application of instrumentation; the collection of data sets during Intensive Field Observation periods; the reduction and analysis of data collected during IFO's; and completion of research projects specifically designed to address important and timely research objectives. In the first year covered by this research proposal, three papers were authored in the refereed literature which reported completed analyses of FIRE 1 IFO studies initiated under the previous NASA funding of this topic area. microphysical and radiative properties of marine stratocumulus cloud systems deduced from tethered balloon observations were reported from the San Nicolas Island site of the first FIRE marine stratocumulus experiment. Likewise, in situ observations of radiation and dynamic properties of a cirrus cloud layer were reported from first FIRE cirrus IFO based from Madison, Wisconsin. In addition, application techniques were under development for monitoring cirrus cloud systems using a 403 MHz Doppler wind profiler system adapted with a RASS (Radio Acoustic Sounding System) and an infrared interferometer system; these instrument systems were used in subsequent deployments for the FIRE 2 Parsons, Kansas and FIRE 2 Porto Santo, ASTEX expeditions. In November 1991 and in June 1992, these two systems along with a complete complement of surface radiation and meteorology measurements were deployed to the two sites noted above as anchor points for the respective IFO'S. Subsequent research activity concentrated on the interpretation and integration of the IFO analyses in the context of the radiative properties of cloud systems and our ability to remotely observe radiative, thermodynamic and dynamic properties of these cloud systems.

Cox, Stephen K.↗
NASA NTRS1993

Advanced particulate fibrous composite for thermal control of re-entry vehicles

Combining the selectively reflective properties of particulate reflective coatings with the low density and high temperature capability of ceramic fibrous materials results in a novel composite material with useful optical properties. Numerical predictions of the radiative properties of zirconia and silica composites for a range of mixture fractions and wavelengths show the improvements attainable by dispersing spheres throughout a fiber matrix. The radiation conductance is controlled by the percentage of spheres in the composite. Results show that specific wavelength domains are controlled by either the spheres or the fibers, so the optical properties can be tailored for reentry applications.

White, Susan↗
NASA NTRS1990

Inhomogeneities of stratocumulus liquid water

There is a growing body of observational evidence on inhomogeneous cloud structure, most recently from the extensive measurements of the FIRE field program. Knowledge of cloud structure is important because it strongly influences the cloud radiative properties, one of the major factors in determining the global energy balance. Current atmospheric circulation models use plane-parallel radiation, so that the liquid water in each gridbox is assumed to be uniform, which gives an unrealistically large albedo. In reality cloud liquid water occupies only a subset of each gridbox, greatly reducing the mean albedo. If future climate models are to treat the hydrological cycle in a manner consistent with energy balance, a better treatment of cloud liquid is needed. FIRE concentrated upon two cloud types of special interest: cirrus and marine stratocumulus. Cirrus tend to be high and optically thin, thus reducing the effective radiative temperature without increasing the albedo significantly, leading to an enhanced greenhouse heating. In contrast, marine stratocumulus are low and optically thick, thus producing a large increase in reflected radiation with a small change in emitted radiation, giving a net cooling which could potentially mitigate the expected greenhouse warming. The FIRE measurements in California stratocumulus during June and July of 1987 show variations in cloud liquid water on all scales. Such variations are associated with inhomogeneous entrainment, in which entrained dry air, rather than mixing uniformly with cloudy air, remains intact in blobs of all sizes, which decay only slowly by invasion of cloudy air. Two important stratocumulus observations are described, followed by a simple fractal model which reproduces these properties, and finally, the model radiative properties are discussed.

Cahalan, Robert F.↗
NASA NTRS1990

The 27-28 October 1986 FIRE IFO cirrus case study - In situ observations of radiation and dynamic properties of a cirrus cloud layer

Observations are presented of cirrus cloud radiative, microphysical, and dynamic properties, their variability, and apparent scale sizes, as observed from NCAR Sabreliner on October 28, 1986. Broadband mass-absorption coefficients were deduced as a function of depth into the cirrus cloud and found to vary with particle dimension. Broadband volume absorption coefficients were deduced. By employing a diffusivity factor of 1.49 this agreement was maximized. Calculated infrared heating rates were typical of thin cirrus layers. The cloud top cooling and cloud base warming were observed to become more accentuated for the denser portions of cloud. The broadband emittances due to the cloud aerosol were found to approach 0.5 to 0.6. The cirrus clouds were observed to exhibit significant horizontal variability and a significant amount of scatter was evident when attempting to relate the broadband infrared and shortwave radiative properties. It is suggested that these radiative properties, which are modulated by the cloud elements, have their scales determined by the eddies detected in the analysis of wind components.

Smith, William L., Jr.↗
NASA NTRS2001

Satellite Imagery Analysis for Nighttime Temperature Inversion Clouds

Clouds play important roles in the climate system. Their optical and microphysical properties, which largely determine their radiative property, need to be investigated. Among several measurement means, satellite remote sensing seems to be the most promising. Since most of the cloud algorithms proposed so far are daytime use which utilizes solar radiation, Minnis et al. (1998) developed a nighttime use one using 3.7-, 11 - and 12-microns channels. Their algorithm, however, has a drawback that is not able to treat temperature inversion cases. We update their algorithm, incorporating new parameterization by Arduini et al. (1999) which is valid for temperature inversion cases. This updated algorithm has been applied to GOES satellite data and reasonable retrieval results were obtained.

Kawamoto, K.↗
NASA NTRS1975

Radiation in the atmosphere

Questions of radiative transfer in realistic atmospheres are considered along with aspects related to radiative energy budgets and the solar constants, the radiative properties of atmosphere and surfaces, radiation instruments and measurements, and radiative interactions in dynamical systems. A number of special topics are discussed, taking into account remote sensing, air pollution, and the effect of turbulence on the propagation of light through the atmosphere. It is pointed out that numerous recent studies have been conducted of the properties and effects of atmospheric aerosols.

Coulson, K. L.↗
NASA NTRS2018

Net Radiative Effects of Dust in the Tropical North Atlantic Based on Integrated Satellite Observations and in Situ Measurements

In this study, we integrate recent in situ measurements with satellite retrievals of dust physical and radiative properties to quantify dust direct radiative effects on shortwave (SW) and longwave (LW) radiation (denoted as DRESW and DRELW, respectively) in the tropical North Atlantic during the summer months from 2007 to 2010. Through linear regression of the CERES-measured top-of atmosphere (TOA) flux versus satellite aerosol optical depth (AOD) retrievals, we estimate the instantaneous DRESW efficiency at the TOA to be -49+/-7.1 W/sq.m AOD(exp -1) and -36+/-4:8W/sq.m AOD(exp -1) based on AOD from MODIS and CALIOP, respectively. We then perform various sensitivity studies based on recent measurements of dust particle size distribution (PSD), refractive index, and particle shape distribution to determine how the dust microphysical and optical properties affect DRE estimates and its agreement with the above-mentioned satellite-derived DREs. Our analysis shows that a good agreement with the observation-based estimates of instantaneous DRESW and DRELW can be achieved through a combination of recently observed PSD with substantial presence of coarse particles, a less absorptive SW refractive index, and spheroid shapes. Based on this optimal combination of dust physical properties we further estimate the diurnal mean dust DRE(sub SW) in the region of -10W/sq.m at TOA and -26W/sq.m at the surface, respectively, of which ~30% is canceled out by the positive DRE(sub LW). This yields a net DRE of about -6:9 and -18.3 W/sq.m at TOA and the surface, respectively. Our study suggests that the LW flux contains useful information on dust particle size, which could be used together with SW observations to achieve a more holistic understanding of the dust radiative effect.

Song, Qianqian↗
NASA NTRS1989

Radiative heat transfer in rocket thrust chambers and nozzles

Numerical models based on the discrete exchange factor (DEF) and the zonal methods for radiative analysis of rocket engines containing a radiatively participating medium have been developed. These models implement a new technique for calculating the direct exchange factors to account for possible blockage by the nozzle throat. Given the gas and surface temperature distributions, engine geometry, and radiative properties, the models compute the wall radiative heat fluxes at different axial positions. The results of sample calculations for a typical rocket engine (engine 700 at NASA), which uses RP-1 (a kerosene-type propellant), are presented for a wide range of surface and gas properties. It is found that the heat transfer by radiation can reach up to 50 percent of that due to convection. The maximum radiative heat flux is at the inner side of the engine, where the gas temperature is the highest. While the results of both models are in excellent agreement, the computation time of the DEF method is found to be much smaller.

Hammad, K. J.↗
NASA NTRS2000

A Melting Layer Model for Passive/Active Microwave Remote Sensing Applications: Simulation of TRMM Observations - Part 2

The one-dimensional, steady-state melting layer model developed in Part I of this study is used to calculate both the microphysical and radiative properties of melting precipitation, based upon the computed concentrations of snow and graupel just above the freezing level at applicable horizontal gridpoints of 3-dimensional cloud resolving model simulations. The modified 3-dimensional distributions of precipitation properties serve as input to radiative transfer calculations of upwelling radiances and radar extinction/reflectivities at the TRMM Microwave Imager (TMI) and Precipitation Radar (PR) frequencies, respectively. At the resolution of the cloud resolving model grids (approx. 1 km), upwelling radiances generally increase if mixed-phase precipitation is included in the model atmosphere. The magnitude of the increase depends upon the optical thickness of the cloud and precipitation, as well as the scattering characteristics of ice-phase precipitation aloft. Over the set of cloud resolving model simulations utilized in this study, maximum radiance increases of 43, 28, 18, and 10 K are simulated at 10.65, 19.35 GHz, 37.0, and 85.5 GHz, respectively. The impact of melting on TMI-measured radiances is determined not only by the physics of the melting particles but also by the horizontal extent of the melting precipitation, since the lower-frequency channels have footprints that extend over 10''s of kilometers. At TMI resolution, the maximum radiance increases are 16, 15, 12, and 9 K at the same frequencies. Simulated PR extinction and reflectivities in the melting layer can increase dramatically if mixed-phase precipitation is included, a result consistent with previous studies. Maximum increases of 0.46 (-2 dB) in extinction optical depth and 5 dBZ in reflectivity are simulated based upon the set of cloud resolving model simulations.

Olson, William S.↗
NASA NTRS2014

Revised (Mixed-Effects) Estimation for Forest Burning Emissions of Gases and Smoke, Fire/Emission Factor Typology, and Potential Remote Sensing Classification of Types for Ozone and Black-Carbon Simulation

We summarize recent progress (a) in correcting biomass burning emissions factors deduced from airborne sampling of forest fire plumes, (b) in understanding the variability in reactivity of the fresh plumes sampled in ARCTAS (2008), DC3 (2012), and SEAC4RS (2013) airborne missions, and (c) in a consequent search for remotely sensed quantities that help classify forest-fire plumes. Particle properties, chemical speciation, and smoke radiative properties are related and mutually informative, as pictures below suggest (slopes of lines of same color are similar). (a) Mixed-effects (random-effects) statistical modeling provides estimates of both emission factors and a reasonable description of carbon-burned simultaneously. Different fire plumes will have very different contributions to volatile organic carbon reactivity; this may help explain differences of free NOx(both gas- and particle-phase), and also of ozone production, that have been noted for forest-fire plumes in California. Our evaluations check or correct emission factors based on sequential measurements (e.g., the Normalized Ratio Enhancement and similar methods). We stress the dangers of methods relying on emission-ratios to CO. (b) This work confirms and extends many reports of great situational variability in emissions factors. VOCs vary in OH reactivity and NOx-binding. Reasons for variability are not only fuel composition, fuel condition, etc., but are confused somewhat by rapid transformation and mixing of emissions. We use "unmixing" (distinct from mixed-effects) statistics and compare briefly to approaches like neural nets. We focus on one particularly intense fire the notorious Yosemite Rim Fire of 2013. In some samples, NOx activity was not so suppressed by binding into nitrates as in other fires. While our fire-typing is evolving and subject to debate, the carbon-burned delta(CO2+CO) estimates that arise from mixed effects models, free of confusion by background-CO2 variation, should provide a solid base for discussion. (c) We report progress using promising links we find between emissions-related "fire types" and promising features deducible from remote observations of plumes, e.g., single scatter albedo, Angstrom exponent of scattering, Angstrom exponent of absorption, (CO column density)/(aerosol optical depth).

Remote sensing↗
NASA NTRS1998

Validation of POLDER/ADEOS data using a ground-based lidar network: Preliminary results for semi-transparent and cirrus clouds

At mid and tropical latitudes, cirrus clouds are present more than 50% of the time in satellites observations. Due to their large spatial and temporal coverage, and associated low temperatures, cirrus clouds have a major influence on the Earth-Ocean-Atmosphere energy balance through their effects on the incoming solar radiation and outgoing infrared radiation. At present the impact of cirrus clouds on climate is well recognized but remains to be asserted more precisely, for their optical and radiative properties are not very well known. In order to understand the effects of cirrus clouds on climate, their optical and radiative characteristics of these clouds need to be determined accurately at different scales in different locations i.e. latitude. Lidars are well suited to observe cirrus clouds, they can detect very thin and semi-transparent layers, and retrieve the clouds geometrical properties i.e. altitude and multilayers, as well as radiative properties i.e. optical depth, backscattering phase functions of ice crystals. Moreover the linear depolarization ratio can give information on the ice crystal shape. In addition, the data collected with an airborne version of POLDER (POLarization and Directionality of Earth Reflectances) instrument have shown that bidirectional polarized measurements can provide information on cirrus cloud microphysical properties (crystal shapes, preferred orientation in space). The spaceborne version of POLDER-1 has been flown on ADEOS-1 platform during 8 months (October 96 - June 97), and the next POLDER-2 instrument will be launched in 2000 on ADEOS-2. The POLDER-1 cloud inversion algorithms are currently under validation. For cirrus clouds, a validation based on comparisons between cloud properties retrieved from POLDER-1 data and cloud properties inferred from a ground-based lidar network is currently under consideration. We present the first results of the validation.

Chepfer, H.↗
NASA NTRS2021

Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) Science Plan

Coastal cities provide the opportunity to characterize marine clouds and the substantial effects of manmade particles on cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties. The focus of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) is to characterize the extent, radiative properties, aerosol interactions, and precipitation characteristics of stratocumulus clouds in the Eastern Pacific across all four seasons at a coastal location, the Scripps Pier and the Scripps Mt. Soledad sites in La Jolla. An important enhancement to this study will be the collection of simultaneous in-cloud aerosol and droplet measurements to investigate the differences in these cloud properties during regional polluted and clean marine conditions. The combined observations will provide an unprecedented set of constraints for the following questions: 1. Cloud and Aerosol Climatology: What are the seasonal and diurnal cycles of marine stratocumulus cloud and aerosol properties on the northeastern Pacific coast? 2. Cloud Radiative Fluxes: How do cloud properties, including the ratio of direct-to-diffuse radiation, change as coastal clouds are advected inland? 3. Aerosol-Cloud Interactions: Will retrieved cloud properties reflect the regional signatures of aerosol?

Eastern Pacific Cloud Aerosol Precipitation Experi↗
NASA NTRS2004

Small-Scale Variability of Large Cloud Drops

Cloud droplet size distribution is one of the most fundamental subjects in cloud physics. Understanding of spatial distribution and small-scale fluctuations of cloud droplets is essential for both cloud physics and atmospheric radiation. For cloud physics, it relates to the coalescence growth of raindrops while for radiation, it has a strong impact on a cloud's radiative properties. Most of the existing cloud radiation and precipitation formation models assume that the mean number of drops with a given radius varies proportionally to volume. The analysis of microphysical data on liquid water drop sizes shows that, for sufficiently small volumes, the number is proportional to the drop size dependent power of the volume. For abundant small drops present, the exponent is 1 as assumed in the conventional approach. However, for rarer large drops, the exponents fall below unity. At small scales, therefore, the mean number of large drops decreases with volume at a slower rate than the conventional approach assumes, suggesting more large drops at these scales than conventional models account for; their impact is consequently underestimated. Size dependent models of spatial distribution of cloud drops that simulate the observed power laws show strong drop clustering, the more so the larger the drops. The degree of clustering is determined by the observed exponents. The strong clustering of large drops arises naturally from the observed power-law statistics. Current theories of photon-cloud interaction and warm rain formation will need radical revision in order to produce these statistics; their underlying equations are unable to yield the observed power law.

Marshak, Alexander↗
NASA NTRS2004

Contrail Coverage Over the USA Derived from NOAA and EOS Satellite Data

Contrails, like natural cirrus clouds, can cause a warming of the Earth-atmospheric system by absorbing longwave radiation from the surface and lower troposphere and radiating additional radiation back to the surface. They can also produce some cooling of the surface during the daytime by reflecting some sunlight back to space. Recently, Minnis et al. (2004) determined from surface observations of cirrus cloud cover that the overall impact appears to be a warming that is consistent with theoretical calculations, at least over the United States of America (USA) and surrounding areas. This finding highlights the need to better understand the formation and persistence of contrails and their radiative properties. To better assess the climatic impact of contrails, it is essential to determine the variability of the contrail microphysical properties, their impact on the atmospheric radiation budget, and their relationship to the atmospheric state. To that end, this paper continues the analyses of Advanced Very High Resolution Radiometer (AVHRR) data from the NOAA-15 (N15), NOAA-16 (N16), and NOAA-17 (N17) satellites, Moderate Resolution Imaging Spectroradiometer (MODIS) data from the Terra and Aqua satellites. The combination of these satellites provides a relatively comprehensive coverage of the daily cycle of air traffic. Thus, it should be possible to use these data to help understand the impact of air traffic on the upper tropospheric humidity during the day as well as determine the local-time variability of contrail coverage. The results will be valuable for developing models of contrail effects and methods for mitigating the impact of aviation on climate.

Palikonda, Rabindra↗
NASA NTRS1997

Characterization of Aircraft Produced Soot and Contrails Near the Tropopause

Participation in the SUCCESS project primarily involved development and deployment of specific instruments for characterizing jet aircraft exhaust emissions as particulates and their subsequent evolution as contrail particles, either liquid or solid, as cirrus. Observations can be conveniently considered in two categories - close or distant from the aircraft. Thus close to the aircraft the exhaust is mixing through the engine turbulence with a much drier and colder environment and developing water/ ice supersaturation along the trail depending on circumstances (near field), whereas distant from the aircraft (far field) the exhaust has cooled essentially to ambient temperature, the turbulence has decayed and any particle growth or evaporation is controlled by the prevailing ambient conditions. Intermediate between these two regions the main aircraft vortices form (one on each side of the aircraft) which tend to inhibit mixing under some conditions, a region extending from a few aircraft lengths to sometimes a hundred times this distance. Our approach to the problem lay in experience gained in characterizing the smoke from hydrocarbon combustion in terms of its cloud forming properties and its potential influence on the radiation properties of the smoke and subsequent cloud from the viewpoint of reduction (absorbtion and scattering ) of solar radiation flux leading to significant global cooling (Hudson et al 1991; Hallett and Hudson 1991). Engine exhaust contains a much smaller proportion of the fuel carbon than is sometimes present in ordinary combustion (less than 0.01% compared with 10%) and influences condensation in quite different ways, to be characterized by the Cloud Condensation Nucleus, CCN - supersaturation spectrum. The transition to ice is to be related to the dilution of solution droplets to freeze by homogeneous nucleation at temperatures somewhat below -40C (Pueschel et al 1998). The subsequent growth of ice particles depends critically on temperature, supersaturation and to some extent pressure, as is demonstrated in an NSF funded project being carried out in parallel with the work reported here. As will be discussed below, nucleation processes themselves and also exhaust impurities also influence the growth of ice particles and may control some aspects of growth of ice in contrails. Instrumentation was designed to give insight into these questions and to be flown on the NASA DC- 8 as a platform. In addition a modest program was undertaken to investigate the properties of laboratory produced smoke produced under controlled conditions from the viewpoint of forming both CCN and CN. The composition of the smoke could inferred from a thermal characterization technique; larger particles were captured by formvar replicator for detailed analysis; ice particles were captured and evaporated in flight on a new instrument, the cloudscope, to give their mass, density and impurity content.

Hallett, John↗