DOE OSTI2015
The knowledge of the radionuclide content of radioactive waste is of utmost importance for safety and waste management reasons. Numerical simulations are used at EDF-CIDEN to anticipate the dismantling and the radioactive waste management. The activation scheme by neutron flux developed at EDF-CIDEN comprises four steps. First of all, a 3 dimensional description of the reactor, the chemical composition of each structure, and the neutron sources at nominal power rating conditions are used as the input data to simulate the neutron propagation and to generate a 3 dimensional multi energy group neutron flux distribution in nominal power rating conditions. Secondly, this output data is used with the chemical compositions (including impurities) and the history of the operating conditions to calculate the radiological inventory for each structure. Thirdly, according to the radioactive inventory of each component or sub-component, a waste classification can be made; the classification criteria are based on the levels of radioactivity and radiotoxicity of 143 radionuclides. Finally, comparisons between the calculated radioactive inventories and the results of radio-chemical analyses can be made. These comparisons are made with regards to the activation of 'standard' chemical elements (meaning radionuclides being perfectly modeled with no uncertainty about the chemical concentrations). The results, linked with 'standard' chemical elements, can be used to validate the calculation scheme, including the neutron propagation, the neutron activation and all the other associated simplified assumptions (geometry, history of irradiation, etc). For steel, activation of 'Fe' is retained, and for stainless steel, activation of 'Fe' 'Ni' are retained. Overall, the feedback from Chooz A (Pressurized Water Reactor) shows that numerical simulations produce a slight overestimation of 'Fe-55' and 'Ni-63'. The results linked with minor chemical elements or impurities allowed us to validate the use of the average measured compositions. (authors)
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗