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At least 217 records · Page 12

Measuring planetary neutron albedo fluxes by remote gamma-ray sensing

In order to measure the planetary neutron albedo fluxes, a neutron-absorbing shield which emits gamma rays of characteristic energy and serves as a neutron detector, is added to a gamma-ray spectrometer (GRS). The gamma rays representing the neutron flux are observed against interference consisting of cosmic gamma rays, planetary continuum and line emission, and gamma rays arising from the interaction of cosmic rays with the GRS and the spacecraft. The uncertainty and minimum detection limits in neutron albedo fluxes are calculated for two missions, a lunar orbiter and a comet nucleus rendezvous. A GRS on a lunar orbiter at 100 km altitude detects a thermal neutron albedo flux as low as 0.002/sq cm/s and an expected flux of about 0.6/sq cm/s is measured with an uncertainty of 0.001/sq cm/s, for a 100 h observation period. For the comet nucleus, again in a 100 h observing period, a thermal neutron albedo flux is detected at a level of 0.006/sq cm/s and an expected flux of about 0.4/sq cm/s is measured with an uncertainty of 0.004/sq cm/s. The expanded geological capabilities made possible by this technique include improvements in H sensitivity, spatial resolution, and measurement depth; and an improved model of induced gamma-ray emission.

Haines, E. L.↗

Evidence for the Sequestration of Hydrogen-Bearing Volatiles Towards the Moons Southern Pole-Facing Slopes

The Lunar Exploration Neutron Detector (LEND) onboard the Lunar Reconnaissance Orbiter (LRO) detects a widespread suppression of the epithermal neutron leakage flux that is coincident with the pole-facing slopes (PFS) of the Moon's southern hemisphere. Suppression of the epithermal neutron flux is consistent with an interpretation of enhanced concentrations of hydrogen-bearing volatiles within the upper meter of the regolith. Localized flux suppression in PFS suggests that the reduced solar irradiation and lowered temperature on PFS constrains volatility to a greater extent than in surrounding regions. Epithermal neutron flux mapped with LEND's Collimated Sensor for Epithermal Neutrons (CSETN) was analyzed as a function of slope geomorphology derived from the Lunar Orbiting Laser Altimeter (LOLA) and the results compared to co-registered maps of diurnally averaged temperature from the Diviner Lunar Radiometer Experiment and an averaged illumination map derived from LOLA. The suppression in the average south polar epithermal neutron flux on equator-facing slopes (EFS) and PFS (85-90 deg S) is 3.3 +/- 0.04% and 4.3 +/- 0.05% respectively (one-sigma-uncertainties), relative to the average count-rate in the latitude band 45-90 deg S. The discrepancy of 1.0 +/- 0.06% between EFS and PFS neutron flux corresponds to an average of approximately 23 parts-per-million-by-weight (ppmw) more hydrogen on PFS than on EFS. Results show that the detection of hydrogen concentrations on PFS is dependent on their spatial scale. Epithermal flux suppression on large scale PFS was found to be enhanced to 5.2 +/- 0.13%, a discrepancy of approximately 45 ppmw hydrogen relative to equivalent EFS. Enhanced poleward hydration of PFS begins between 50 deg S and 60 deg S latitude. Polar regolith temperature contrasts do not explain the suppression of epithermal neutrons on pole-facing slopes. The Supplemental on-line materials include supporting results derived from the uncollimated Lunar Prospector Neutron Spectrometer and the LEND Sensor for Epithermal Neutrons.

Ices↗

Review of Direct Neutron Conversion and Detection Processes

Commercial and laboratory neutron detection systems use indirect neutron response of materials like pressurized helium-3 (via nuclear reaction 3He(n, p)3H) to measure and count neutrons emanating from a source. Recently a host of semiconductors, especially a ternary semiconductor of lithium indium diselenide (6LiInSe2) and a quaternary alloy of enriched lithium-6, indium, phosphorous, and selenium (6LiInP2Se6), have shown promising neutron counting possibilities by directly converting neutrons into charge-carrying elements within the body of the semiconductor. These semiconductors have high thermal neutron capture cross sections, suitable energy bandgaps (~2.0 electron volts) for room-temperature operations, and a favorable electronic band structure for efficient electron charge transport. The article examines the semiconductor properties of these compounds in terms of their neutron counting capabilities and possible ways to extract neutron energy information from them. Lithium-6 and boron-10 (with thermal neutron absorption cross sections of 938 ± 6 and 3855 ± 26 barns, respectively) produce charged particles to be measured via indirect neutron interactions. The efficiency of indirect conversion neutron detectors is limited because of the inefficiencies in conversion mechanism. In case of direct conversion, the neutrons create charged particles in a single material for neutron capture and charge collection, increasing detection efficiency. Unlike 3He proportional counters, which provide no neutron energy information, the semiconductors can be used as neutron energy spectrometer. Fully resolved neutron energy by 6LiInP2Se6 from a plutonium-beryllium source has been reported in the literature. We will discuss the influence of these multilayered semiconductors’ crystallographic structures and growth techniques on neutron energy determination.

61 RADIATION PROTECTION AND DOSIMETRY↗

Recent progress on the APOLLO3 calculation scheme for the FLUOLE2 experiment

Studies of the neutron fluence on reactor pressure vessel and the correlated reactor lifetime issues require very good knowledge of the neutron source distribution in the reactor core and especially in the peripheral region. The FLUOLE2 experiment offers an appropriate starting configuration to investigate the possibility of using the APOLLO3 deterministic code with a two-step calculation scheme. It enables us to calculate a pin-by-pin neutron source distribution in the core, then to carry out the neutron propagation from the core to neutron detectors. In this paper, we focus on a calculation scheme dedicated to the determination of core neutron source distribution using APOLLO3 with the SHEM281 energy mesh, a Method of Characteristics (MOC) to solve the transport equation for the lattice computation step and a 20-groups 3D computation using the MINARET SN solver of APOLLO3. Reactivity and pin-by-pin reaction rate results have been analyzed. Results obtained with both lattice and core computations show a good agreement with those produced through a reference calculation using the TRIPOLI-4 Monte Carlo transport code. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A search for solar neutrons during solar flares

A new upper limit to the 1-20 MeV neutrons produced at the sun during large solar flares was obtained as a result of measurements made by a neutron detector on board the OGO-6 satellite. It was found that the 1-20 MeV solar neutron flux for the Nov. 2, June 13, June 15, Sept. 25, and Dec. 19, 1969, solar flare events cannot be greater than 0.05 n per sq cm per sec at the 95% confidence level. These measurements are consistent with the models proposed by Lingenfelter (1969) and Lingenfelter and Ramaty (1967) for solar neutron production during solar flares.

Ifedili, S. O.↗

FAST-NEUTRON FLUX IN THE ATMOSPHERE

Neutron flux between one and ten mev from sea level to balloon altitudes, recorded by fast neutron detector insensitive to other radiation

NEUTRON FLUX↗

The response of a 300 micron silicon detector to monoenergetic neutrons determined by the use of the Monte Carlo technique

The response of a 300 micron thick silicon detector to an incident monoenergetic neutron beam is evaluated by the Monte Carlo method for the cases of both a shielded and a bare detector. The result of Monte Carlo calculation, using elastic, inelastic, and absorption reactions indicates that the response of the silicon detector to neutrons is basically due to the elastic scattering. In addition, the gamma rays generated in the shield of the detector will result in a response which is 3 or 4 orders of magnitude smaller than response to incident photons. The response of a bare silicon detector is calculated for neutron energies up to 6 MeV and bias energies from 50 to 250 KeV. It is found that the maximum response for a 300 micron thick silicon detector is less than .004 c/n within this selected neutron and bias energy range. When the pulse height defect is introduced in the calculation the results at low energy neutrons were reduced.

Tahezadeh, M.↗

Quantification of Sub-Pixel Dynamics in High-Speed Neutron Imaging

The high penetration depth of neutrons through many metals and other common materials makes neutron imaging an attractive method for non-destructively probing the internal structure and dynamics of objects or systems that may not be accessible by conventional means, such as X-ray or optical imaging. While neutron imaging has been demonstrated to achieve a spatial resolution below 10 μm and temporal resolution below 10 μs, the relatively low flux of neutron sources and the limitations of existing neutron detectors have, until now, dictated that these cannot be achieved simultaneously, which substantially restricts the applicability of neutron imaging to many fields of research that could otherwise benefit from its unique capabilities. In this work, we present an attenuation modeling approach to the quantification of sub-pixel dynamics in cyclic ensemble neutron image sequences of an automotive gasoline direct injector at a 5 μs time scale with a spatial noise floor in the order of 5 μm.

47 OTHER INSTRUMENTATION↗

Preliminary Design of a New Pulsed-Neutron Die--Away Experiments with Absorbers (IER-552 CED-1)

This report presents the preliminary design (CED-1) of IER-552, pulsed-neutron die-away (PNDA) experiments with absorbers, to be conducted by Lawrence Livermore National Laboratory (LLNL). The goal of the PNDA experiments with absorbing materials is to produce high-quality, low-cost integral benchmarks that can be used to validate cross sections that are high priority nuclear data for the Department of Energy’s Nuclear Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them. The original PNDA experiments were set up at LLNL under IER-501. Extending the PNDA experiments to include absorbing materials leverages existing facilities and resources at LLNL to validate cross sections, with a basic experiment design that uses a neutron generator to impinge a short, mono-energetic neutron pulse on a poisoned, moderating target sample. The neutron pulse lasts 100 µs, after which the neutron population in the sample reaches thermal equilibrium and later spatial equilibrium. In this fully equilibrized state, the neutron population has a characteristic decay-time eigenvalue. The eigenvalue can be used as an integral parameter to validate nuclear data involved with neutron scattering and absorption. Two observables can be measured: the neutron population and the population of secondary γ-rays produced by inelastic and capture reactions. This report explores the feasibility of both approaches. For γ-ray measurements, this allows for direct measurement of reactions of interest for validation. During the neutron burst time, inelastic (prompt) γ-rays dominate, and these data can be isolated for validation of neutron inelastic scattering data. After the pulse ends, neutron capture (delayed) γ-rays dominate and are produced by many reaction channels as neutrons slow down to thermal energies. Two sets of γ-ray spectra (inelastic, capture) can be produced for validation. Additionally, the time-dependent decay of the capture γ-ray population when the neutron population is thermalized and in its fundamental mode can be used for validation. Two experiments can be imagined where pulsed neutrons are used to validate the nuclear data of absorbing materials. The first integrates well into the existing PNDA testbed at LLNL. The absorber material would be introduced into a moderating target and the same neutron generator, neutron detectors, electronics, and shielding box used for IER-501 would be employed. From the same experimental setup, many absorbing materials can be validated by simply changing the neutron poison in the moderator. The only significant modification would be the introduction of a γ-ray detector. Such an experiment would primarily serve to validate nuclear data in the thermal energy range. The second kind of experiment would validate the fast and epithermal energy range. It would involve pulsing neutron into a bare assembly of the absorber material and measuring the die-away of neutrons. The fast leakage of such an assembly requires nanosecond neutron-generator pulse widths and fast detectors/electronics that could measure ~200 ns die-away curves. This kind of experiment would ideally be performed at a cyclotron, like that available at Lawrence Berkeley National Laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

4-D Model of CO2 Deposition at North and South of Mars from HEND/Odyssey and MOLA/MGS

The first 1.5 year of neutron mapping measurements onboard Mars Odyssey spacecraft are presented based on High Energy Neutron Detector (HEND) observations. HEND instrument is a part of GRS suite responsible for registration of epithermal and fast neutrons originating in Mars subsurface layer. The scattering of fast neutrons in Mars surface caused by primary cosmic rays is strongly sensitive to presence of hydrogen atoms. Even several percents of subsurface water significantly depress epithermal and fast neutron flux. It turns orbit neutron spectroscopy into one of most efficient methods for finding distribution of subsurface water. The Mars Odyssey observations revealed huge water- ice regions above 60N and 60S latitudes. It was founded that distribution of subsurface water has layered structure at these regions. It is thought that more than 50% wt water ice covered by relatively dry layer with different thickness.

M L Litvak↗

Seasonal CO2 Observations on North and South of Mars as Seen by HEND (Mars Odyssey) and MOLA (MGS)

The first year of neutron mapping measurements from the Mars Odyssey spacecraft are presented based on observations from the High Energy Neutron Detector (HEND). The HEND instrument is a part of GRS suite responsible for registration of epithermal and fast neutrons originating in the Mars subsurface layer. The gamma ray and neutron spectrometers measure the scattering of fast neutrons from the Martian surface, which is caused by bombardment of primary cosmic rays and is strongly sensitive to the presence of hydrogen atoms. Even several percent subsurface hydrogen significantly depresses the flux of epithermal and fast neutrons. The recent Mars Odyssey observations detected a considerable amount of hydrogen, almost certainly corresponding to water ice, in the shallow near surface of the southern and northern hemispheres of Mars.

Litvak, M. L.↗

Electrolytic Co-deposition Neutron Production Evaluation

Co-deposition electrochemical cells are a simple means to examine novel nuclear reactions. In this study, palladium and deuterium atoms were co-deposited on a cathode at stoichiometric densities, forming dendritic morphologies. Bubble detector neutron dosimeters were used to measure equivalent dose levels during electrolytic deposition. Standard configuration cells expected to produce excess neutrons were denoted as experimental cells and contained an electrolyte consisting of palladium(II) chloride, lithium chloride, and heavy water. The control cells used copper(II) chloride, lithium chloride, and heavy water electrolyte. Experimental and control cells were supplied current, increasing from 0.1 to 100.0 mA over a period of 20 days. For test days 9 through 20, the standard configuration experimental cells exhibited significantly higher average neutron radiation than the controls at a 99% confidence level. Alternative configurations involving more increasing current over a shortened time scale, substitutions of water in place of heavy water or potassium chloride for lithium chloride, as well as inclusion of depleted uranium near the cell cathodes all resulted in inconclusive evidence for promoting neutron production.

neutron↗

Report on ISR-1 High-Altitude Balloon Flight

To test small technologies at lower cost for space science applications, LANL has developed a small high altitude balloon payload that could, in the future, be regularly and inexpensively launched from LANL. A neutron detector, NEMO, was integrated to evaluate its performance in a space-like mixed-radiation environment and collect neutron data in the atmosphere. In collaboration with EES-14, a high-altitude balloon payload was launched from LANL Technical Area 51 on February 27, 2023 and April 17, 2023. For real-time geolocation, a SAM-M8Q M8 GNSS module was used to get position and time, and an Iridium RockBLOCK 9603 was used to communicate with the ground using the Iridium satellite fleet. These modules were all controlled using an Iteaduino Mega microcontroller board. Finally, a High Altitude Science Eagle Flight Computer with a temperature pressure sensor ran independently, writing data to an SD card. All of these modules were powered by a 5 mAh lithium polymer battery. The battery was attached to the bottom of the payload while the remaining electronics were embedded in the underside of the top of the payload. These modules were wired as seen in Figure 1-2. The Iteaduino Mega microcontroller board was programmed to use the RockBLOCK to send a message once every 10 minutes containing neutron and GPS data read off the NEMO and SAM M8Q, respectively. Once the message send attempt finished, the RockBLOCK would be slept for the rest of the 10 minute interval. The Eagle Flight Computer ran continuously throughout the flight, taking data every 6 seconds. The RockBLOCK message data was set up to be delivered from the Iridium satellite fleet to a website, where it was stored and parsed to create live maps and plots for analysis and balloon retrieval. The RockBLOCK message data was additionally configured to be sent to an email as a fail-safe. The payload was ground-tested successfully for over 50 hours, with multiple revisions occurring to best prepare for conditions at altitude and improve the software and firmware to fix any issues that cropped up with the data pipeline. Additional to the balloon payload, the flight had an attached iMet-4 radiosonde and Garmin T5 GPS Dog Collar. The radiosonde provided GPS and meteorological data. The T5 dog collar is used along with a Garmin Astro 430 to track the balloon at a range of up to 9 miles for retrieval. The balloon itself was initially a 1600 g meteorological balloon with an attached High Altitude Science parachute, both of which can be seen in Figure 1-3. After the first flight, the EES team swapped to a Rocketman parachute.

42 ENGINEERING↗

Northern and Southern Permafrost Regions on Mars with High Content of Water Ice: Similarities and Differences

The measurements by neutron detectors on Odyssey have revealed two large poleward regions with large depression of flux of epithermal and high energy neutrons [1-3]. The flux of neutrons from Mars is known to be produced by the bombardment of the surface layer by galactic cosmic rays. The leakage flux of epithermal and fast neutrons has regional variation by a factor of 10 over the surface of Mars (e.g. see [3- 5]). These variations are mainly produced by variations of hydrogen content in the shallow subsurface. On Mars hydrogen is associated with water. Therefore, the Northern and Southern depressions of neutron emission could be identified as permafrost regions with very high content of water ice [1-5]. These regions are much larger than the residual polar caps, and could contain the major fraction of subsurface water ice. Here we present the results of HEND neutron data deconvolution for these regions and describe the similarities and differences between them.

Mitrofanov, I. G.↗

Northern and Southern Permafrost Regions on Mars with High Content of Water Ice: Similarities and Differences

The measurements by neutron detectors on Odyssey have revealed two large poleward regions with large depression of flux of epithermal and high energy neutrons. The flux of neutrons from Mars is known to be produced by the bombardment of the surface layer by galactic cosmic rays. The leakage flux of epithermal and fast neutrons has regional variation by a factor of 10 over the surface of Mars. These variations are mainly produced by variations of hydrogen content in the shallow subsurface. On Mars hydrogen is associated with water. Therefore, the Northern and Southern depressions of neutron emission could be identified as permafrost regions with very high content of water ice. These regions are much larger than the residual polar caps, and could contain the major fraction of subsurface water ice. Here we present the results of HEND neutron data deconvolution for these regions and describe the similarities and differences between them.

Mitrofanov, I. G.↗

A Ce-Doped LiI Scintillator Film-Based High Rate, High Spatial Resolution Neutron Anger Camera for Neutron Scattering Facilities

The 2-D position sensitive neutron detectors featuring a significantly improved count rate capacity and a sub-mm spatial resolution are in high demand by neutron scattering facilities, especially the next generation high-flux spallation neutron sources (SNSs). They are anticipated to play a crucial role in fully utilizing the unprecedentedly high neutron brightness offered by these sources. In this work, a high rate and high spatial resolution neutron Anger camera has been successfully developed based on a Ce-doped microcolumnar LiI scintillator film and the PETsys TOFPET2 ASIC readout electronics. The performance evaluation was conducted in a standard laboratory environment as well as the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) with regard to light yield, γ-ray sensitivity, neutron detection efficiency, count rate capability, spatial resolution, and position linearity. The LiI:Ce scintillator was found to have a higher light yield and a lower γ-ray sensitivity than GS20 (i.e., 11729 versus 6000 photons/n and 1.67 × 10 −5 versus on the order of 10 −4 ). The neutron detection efficiency was measured to be 63% at 4.2 Å. This camera demonstrated an exceptional count rate capability, up to at least 481 kHz without rate loss. The spatial resolution was as good as 0.47 mm. Here, the position linearity was also enhanced.

High rate↗

Epithermal Neutron Resonance Analysis Using a Compact D-T Generator

Nuclear material identification and isotopic composition analysis are important capabilities for safeguards and the verification of nuclear arms control and nonproliferation treaties. Epithermal neutron resonance imaging has been proposed for spent fuel assay measurements, and the development of a mobile neutron imaging system could provide such a tool for on-site applications. This technique is highly sensitive to isotopes of interest for safeguards applications (e.g. 235,238 U, 238,239,240 Pu) and yields unique transmission spectra for a target containing actinides and some mid- and high-Z elements. Paired with a position-sensitive neutron detector, such a system could provide spatial information of the target isotopic composition. Recent progress in the development of high intensity neutron sources could make mobile epithermal neutron imaging designs increasingly feasible to serve as a tool for nuclear inspectors. In this work, Monte Carlo (MC) simulations were performed to further optimize a previous design for an epithermal neutron resonance-based analysis apparatus using a D-T portable neutron generator. Additionally, experimental work is being performed to test the feasibility of this method. The MC simulations of moderation time distributions for different moderator compositions and thicknesses were measured to provide a multi-group correction for neutron time-of-flight energy reconstruction.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗