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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Plasmons Enable Ultralow Threshold Solid-State Triplet Fusion Upconversion with a 2D Sensitizer

Solid-state triplet−triplet annihilation (TTA) upconversion has significant potential for application in light harvesting, optoelectronic devices, and bioimaging. However, the high optical powers required to achieve efficient upconversion have inhibited its adoption. In this work, we demonstrate plasmon-enhanced near-infrared (NIR)-to-blue TTA upconversion in a monolayer WSe2/organic heterojunction. Under far-field excitation, the device reaches a threshold of 19 mW/cm 2 and an external quantum efficiency (EQE) of 0.17% with an anti-Stokes shift of 1.1 eV. Plasmon excitation lowers the threshold to 0.9 mW/cm 2 and improves the EQE to 3.6%. We attribute the plasmon enhancement to surface plasmon polariton (SPP) near-field enhancement and dark-exciton absorption. Optimization of the WSe 2 transfer process is identified as a key factor for the device performance. This work demonstrates that plasmon excitation overcomes the low far-field absorption of 2D transition-metal dichalcogenide (TMD) sensitizers. Consequently, monolayer TMDs can achieve solid-state upconversion with a performance among the best reported.

2D materials↗
DOE OSTI2025

Toward Fullerene-Free PIN Perovskite Solar Cells

We highlight opportunities for a transformative shift in perovskite solar cell design by expanding electron transport layers (ETLs) beyond fullerenes. Fullerenes have known limitations, including constraints on open-circuit voltage, stability, and mechanical integrity. Recently, fullerene-free p-i-n cells with power conversion efficiencies exceeding 25% have been demonstrated via both naphthalene diimide-SnO x bilayers and nonfullerene acceptor-based ETLs. Despite successes, fullerenes remain the de facto ETLs for perovskites. Drawing lessons from organic photovoltaics, where it took decades to transition from fullerenes to more broadly available and efficient materials, we explore pathways to accelerate the development and adoption of fullerene-free ETLs. This requires understanding the similarities and differences between organic and perovskite solar cells, which will necessitate carefully designing fullerene replacements with both, high efficiency and also, critically, durability under operation. Here, we incorporate literature data to facilitate comparisons, and independently conduct fracture energy measurements for alternative ETL configurations to motivate their adoption.

14 SOLAR ENERGY↗
DOE OSTI2025

Hot or Not? An Evaluation of Methods for Identifying Hot Moments of Nitrous Oxide Emissions From Soils

Abstract Effectively quantifying hot moments of nitrous oxide (N 2 O) emissions from agricultural soils is critical for managing this potent greenhouse gas. However, we are challenged by a lack of standard approaches for identifying hot moments, including (a) determining thresholds above which emissions are considered hot moments, and (b) considering seasonal variation in the magnitude and frequency distribution of net N 2 O fluxes. We used one year of hourly N 2 O flux measurements from 16 autochambers that varied in flux magnitude and frequency distribution in a conventionally tilled maize field in central Illinois, USA, to compare three approaches to identify hot moment thresholds: standard deviations (SD) above the mean, 1.5x the interquartile range (IQR), and isolation forest (IF) identification of anomalous values. We also compared these approaches on seasonally subdivided data (early, late, and non‐growing seasons) versus the whole year. Our analyses revealed that 1.5x IQR method best identified N 2 O hot moments. In contrast, using 2 or 4 SD both yielded hot moment threshold values too high, and IF yielded threshold values too low, leading to missed N 2 O hot moments or low net N 2 O fluxes mischaracterized as hot moments, respectively. Furthermore, seasonally subdividing the data set not only facilitated identification of smaller hot moments in the late‐ and non‐growing seasons when N 2 O hot moments were generally smaller but it also increased hot moment threshold values in the early growing season when N 2 O hot moments were larger. Consequently, of the methods evaluated here, we recommend using the 1.5x IQR method on whole year data sets to identify N 2 O hot moments.

Stuchiner, Emily R. [Institute for Sustainability,↗
DOE OSTI2024

Comparison of Global Aboveground Biomass Estimates From Satellite Observations and Dynamic Global Vegetation Models

The global forest carbon stocks represent the amount of carbon stored in woody vegetation and are important for quantifying the ability of the global forests to sequester atmospheric CO 2 and to provide ecosystem services (e.g., timber) under climate change. The forest ecosystem carbon pool estimates are highly variable and poorly quantified in areas lacking forest inventory estimates. Here, we compare and analyze aboveground biomass (AGB) estimates from five satellite-based global data sets and nine dynamic global vegetation models (DVGMs). We find that across the data sets, mean AGB exhibits the largest variability around the tropical area. In addition, AGB shows a similar latitudinal trend but large variability among the data sets. Satellite-based AGB estimates are lower than those simulated by DVGMs. The divergence among the satellite-based AGB estimates can be driven by the methodology, input satellite products, and the forested areas used to estimate AGB. The modeled NPP, autotrophic respiration, and carbon allocation mostly drive the variability of AGB simulated by DGVMs. The future availability of a high-quality global forest area map is anticipated to improve AGB estimate accuracy and to reduce the discrepancies among different satellite- and model-based AGB estimates. Furthermore, we suggest the carbon-modeling community reexamine the methodology used to estimate AGB and forested areas for a more robust global forest carbon stock estimation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Interaction of magnetic fields with spinons in a fractionalized state

The 4d-electron trimer lattice Ba₄Nb₁₋ₓRu₃₊ₓO₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures.

Condensed-matter physics↗
DOE OSTI2025

Directly imaging the cooling flow in the Phoenix cluster

In the centres of many galaxy clusters, the hot (approximately 10 7 kelvin) intracluster medium can become dense enough that it should cool on short timescales. However, the low measured star formation rates in massive central galaxies and the absence of soft X-ray lines from the cooling gas suggest that most of this gas never cools. This is known as the cooling flow problem. The latest observations suggest that black hole jets are maintaining the vast majority of gas at high temperatures. A cooling flow has yet to be fully mapped through all the gas phases in any galaxy cluster. Here we present observations of the Phoenix cluster using the James Webb Space Telescope to map the [Ne vi] λ 7.652-μm emission line, enabling us to probe the gas at 10 5.5 kelvin on large scales. These data show extended [Ne vi] emission that is cospatial with the cooling peak in the intracluster medium, the coolest gas phases and the sites of active star formation. Taken together, these imply a recent episode of rapid cooling, causing a short-lived spike in the cooling rate, which we estimate to be 5,000–23,000 solar masses per year. As a result, these data provide a large-scale map of gas at temperatures between 10 5 kelvin and 10 6 kelvin in a cluster core, and highlight the critical role that black hole feedback has in not only regulating cooling but also promoting it.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Atomic lift-off of epitaxial membranes for cooling-free infrared detection

Recent breakthroughs in ultrathin, single-crystalline, freestanding complex oxide systems have sparked industry interest in their potential for next-generation commercial devices. However, the mass production of these ultrathin complex oxide membranes has been hindered by the challenging requirement of inserting an artificial release layer between the epilayers and substrates. Here we introduce a technique that achieves atomic precision lift-off of ultrathin membranes without artificial release layers to facilitate the high-throughput production of scalable, ultrathin, freestanding perovskite systems. Leveraging both theoretical insights and empirical evidence, we have identified the pivotal role of lead in weakening the interface. This insight has led to the creation of a universal exfoliation strategy that enables the production of diverse ultrathin perovskite membranes less than 10 nm. Our pyroelectric membranes demonstrate a record-high pyroelectric coefficient of 1.76 × 10 −2 C m −2 K −1 , attributed to their exceptionally low thickness and freestanding nature. Moreover, this method offers an approach to manufacturing cooling-free detectors that can cover the full far-infrared spectrum, marking a notable advancement in detector technology.

nanoscale materials↗
DOE OSTI2026

Global divergence in urban demographic change and migration patterns

Cities are central to economic development, climate adaptation and social stability, yet globally consistent evidence on how city populations are changing remains limited. Here we analyze annual age- and sex-structured population estimates for more than 10,000 cities worldwide from 2000 to 2020 and show that urban demographic change was highly uneven. Globally, the ratio of children and older adults to working-age adults declined from 0.87 to 0.59, but smaller cities remained consistently younger than larger cities, especially in Africa. We also find pronounced spatial variation in urban sex ratios, including strong male surpluses in parts of the Middle East and North Africa, consistent with patterns of labor migration. Finally, we estimate that 45% of urban population growth was attributable to net migration and 55% to natural increase. These results show that national averages can obscure substantial differences between cities, and highlight the value of globally consistent city-level demographic estimates for understanding regional demographic change and informing locally tailored urban planning.

development studies↗
DOE OSTI2025

Understanding CO 2 adsorption on the surfaces of SrO and its hydroxylated variants Sr(OH) 2 · n H 2 O ( n = 0, 1, 8)

Strontium oxide (SrO) is a promising material for CO 2 capture through a reversible cycle of carbonation and calcination, where SrO reacts with CO 2 to form SrCO 3 and can be regenerated by calcination. In the presence of moisture, SrO forms strontium hydroxide and its hydrates (Sr(OH) 2 ·nH 2 O). Here, this study, which employs density functional theory, investigates the CO 2 adsorption mechanism of these processes on various crystal surfaces, including SrO, Sr(OH) 2 , Sr(OH) 2 ·1H 2 O, and Sr(OH) 2 ·8H 2 O. A significant finding is that the interaction of CO 2 with these surfaces leads to carbonate/bicarbonate formation via electron transfer, with notable differences in CO 2 orientation and bond characteristics between SrO surfaces and its hydroxylated surfaces. To explore the effects of moisture on CO 2 adsorption, H 2 O adsorption on these stable surfaces was investigated. The results showed that H 2 O reacts with the SrO (100) surface to form hydroxyl (OH) groups while it bonds with the surfaces of Sr(OH) 2 ·nH 2 O (n = 0, 1, 8) with hydrogen bonding. A small amount of H 2 O can enhance CO2 adsorption while a large amount of H 2 O could decrease the capability of CO 2 adsorption.

CO2 capture↗
DOE OSTI2016

Long term reliability study and life time model of quantum cascade lasers

Here, we present results of quantum cascade laser lifetime tests under various aging conditions including an accelerated life test. The total accumulated life time exceeds 1.5 × 106 device hours. The longest single device aging time was 46 500 hours without failure in the room temperature aging test. Four failures were found in a group of 19 devices subjected to the accelerated life test with a heat-sink temperature of 60 °C and a continuous-wave current of 1 A. Failure mode analyses revealed that thermally induced oxidation of InP in the semi-insulating layer is the cause of failure. An activation energy of 1.2 eV is derived from the dependence of the failure rate on laser core temperature. The mean time to failure of the quantum cascade lasers operating at a typical condition with the current density of 5 kA/cm2 and heat-sink temperature of 25 °C is expected to be 809 000 hours.

Xie, Feng↗
DOE OSTI2026

Altermagnetic polar metallic phase in ultrathin epitaxially strained RuO 2 films

Altermagnetism refers to a wide class of magnetic orders featuring magnetic sublattices with opposite spins related by rotational symmetries, resulting in nontrivial spin splitting and magnetic multipoles. However, the direct observation of the altermagnetic transition remains elusive. Here, by combining theoretical analysis, electrical transport, X-ray, and optical spectroscopies, we establish a phase diagram in hybrid molecular beam epitaxy-grown RuO 2 /TiO 2 (110) films, mapping symmetries along with altermagnetic/electronic/structural phase transitions as functions of film thickness and temperature. This features an altermagnetic metallic polar phase in epitaxially strained 2 nm films, suggesting a potential link between polar metals and altermagnetic materials. Such a clear signature of a magnetic phase transition at ~500 K is observed exclusively in ultrathin strained films, unlike in bulk RuO 2 single crystals. These results highlight the power of epitaxial heterostructure engineering to induce altermagnetism in systems initially nonmagnetic, opening avenues for realizing emergent quantum phases with multifunctional properties.

RuO2 thin film↗
DOE OSTI2025

Baryon number violation: from nuclear matrix elements to BSM physics

Processes that violate baryon number, most notably proton decay and $n\bar{n}$ transitions, are promising probes of physics beyond the Standard Model (BSM) needed to understand the lack of antimatter in the Universe. To interpret current and forthcoming experimental limits, theory input from nuclear matrix elements to UV complete models enters. Thus, an interplay of experiment, effective field theory, lattice QCD, and BSM model building is required to develop strategies to accurately extract information from current and future data and maximize the impact and sensitivity of next-generation experiments. Here, we briefly summarize the main results and discussions from the workshop ‘INT-25-91W: Baryon Number Violation: From Nuclear Matrix Elements to BSM Physics,’ held at the Institute for Nuclear Theory, University of Washington, Seattle, WA, 13–17 January 2025.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Assessing the numerical stability of physics models to equilibrium variation through database comparisons on DIII-D

High fidelity kinetic equilibria are crucial for tokamak modeling and analysis. Manual workflows for constructing kinetic equilibria are time consuming and subject to user error, motivating development of automated equilibrium reconstruction tools to provide accurate and consistent reconstructions for downstream physics analysis. These automated tools also provide access to kinetic equilibria at large database scales, which enables the quantification of general uncertainties arising from equilibrium reconstruction techniques. In this paper, we compare a large database of DIII-D kinetic equilibria generated manually by physics experts to equilibria from automated kinetic reconstruction tools, assessing the impact of reconstruction method on equilibrium parameters and resulting magnetohydrodynamic stability calculations. We find agreement among scalar parameters, whereas profile quantities, such as the bootstrap current, show larger disagreements. We analyze ideal kink and classical tearing stability with DCON and STRIDE respectively, finding that the kink stability calculation is generally more robust than the tearing index Δ' calculation. We find that in 90% of cases, both kink stability classifications are unchanged between the manual expert and automated kinetic equilibria.

CAKE↗
DOE OSTI2020

Measurement of the integrated luminosity of the Phase 2 data of the Belle II experiment

From April to July 2018, a data sample at the peak energy of the Υ(4S) resonance was collected with the Belle II detector at the SuperKEKB electron-positron collider. This is the first data sample of the Belle II experiment. Using Bhabha and digamma events, we measure the integrated luminosity of the data sample to be (496.3±0.3±3.0)pb –1 , where the first uncertainty is statistical and the second is systematic. This work provides a basis for future luminosity measurements at Belle II.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Observation of the decays 𝐵 + → Σ 𝑐 ⁢(2455) ++ $\bar{Ξ}^-_c$ and 𝐵 0 → Σ 𝑐 ⁢(2455) 0⁢ $\bar{Ξ}^0_𝑐$

We report the first observation of the two-body baryonic decays 𝐵 + → Σ 𝑐 ⁢(2455) ++ $\bar{Ξ}^-_c$ and 𝐵 0 → Σ 𝑐 ⁢(2455) 0⁢ $\bar{Ξ}^0_𝑐$ with significances of 7.3⁢𝜎 and 6.2⁢𝜎, respectively, including statistical and systematic uncertainties. The branching fractions are measured to be ℬ⁡(𝐵 + → Σ 𝑐 ⁢(2455) ++ $\bar{Ξ}^-_c$) = (5.74 ± 1.11 ± 0.4⁢2$^{+2.47}_{−1.53}$) ×10 −4 and ℬ⁡(𝐵 0 → Σ 𝑐 ⁢(2455) 0⁢ $\bar{Ξ}^0_𝑐$) = (4.83 ± 1.12 ± 0.3⁢7$^{+0.72}_{−0.60}$) ×10 −4 . The first and second uncertainties are statistical and systematic, respectively, while the third ones arise from the absolute branching fractions of $\bar{Ξ}^-_c$ or $\bar{Ξ}^0_𝑐$ decays. The data samples used for this analysis have integrated luminosities of 711 fb −1 and 365 fb −1 , and were collected at the ϒ⁡(4⁢𝑆) resonance by the Belle and Belle II detectors operating at the KEKB and SuperKEKB asymmetric-energy 𝑒 + ⁢𝑒 − colliders, respectively.

branching fraction↗
DOE OSTI2025

Search for a Dark Higgs Boson Produced in Association with Inelastic Dark Matter at the Belle II Experiment

Inelastic dark matter models that have two dark matter particles and a massive dark photon can reproduce the observed relic dark matter density without violating cosmological limits. The mass splitting between the two dark matter particles 𝜒 1 and 𝜒 2 , with 𝑚⁡(𝜒 2 ) >𝑚⁡(𝜒 1 ), is induced by a dark Higgs field and a corresponding dark Higgs boson ℎ′. We present a search for dark matter in events with two vertices, at least one of which must be displaced from the interaction region, and missing energy. Using a 365 fb −1 data sample collected at Belle II, which operates at the SuperKEKB 𝑒 + ⁢𝑒 − collider, we observe no evidence for a signal. We set upper limits on the product of the production cross section 𝜎⁡(𝑒 + ⁢𝑒 − → ℎ′⁡𝜒 1 ⁢𝜒 2 ), and the product of branching fractions ℬ⁡(𝜒 2 → 𝜒 1⁢ 𝑒 + ⁢𝑒 − ) ×ℬ⁡(ℎ′ → 𝑥 + ⁢𝑥 − ), where 𝑥 + ⁢𝑥 − indicates 𝜇 + ⁢𝜇 − , 𝜋 + ⁢𝜋 − , or 𝐾 + ⁢𝐾 − , as functions of ℎ′ mass and lifetime at the level of 10 −1 fb. We set model-dependent upper limits on the dark Higgs mixing angle at the level of 10 −5 and on the dark photon kinetic mixing parameter at the level of 10 −3 . This is the first search for dark Higgs bosons in association with inelastic dark matter.

dark matter↗
DOE OSTI2025

Measurement of the 𝐶⁢𝑃 asymmetry in 𝐷 + → 𝜋 + ⁢𝜋 0 decays at Belle II

We measure the 𝐶⁢𝑃 asymmetry in 𝐷 + → 𝜋 + ⁢𝜋 0 decays reconstructed in 𝑒 + ⁢𝑒 − collisions at the Belle II experiment using a dataset corresponding to an integrated luminosity of 428 fb −1 . A control sample of 𝐷 + → 𝜋 + ⁢𝐾$^0_𝑆$ decays is used to correct for detection and production asymmetries. The result 𝐴 𝐶⁢𝑃 ⁡(𝐷 + → 𝜋 + ⁢𝜋 0 ) = (−1.8 ± 0.9 ± 0.1)%, where the first uncertainty is statistical and the second systematic, is the most precise determination to date. It agrees with the prediction of 𝐶⁢𝑃 symmetry from the standard model and with results of previous measurements.

CP violation↗