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At least 217 records · Page 12

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DOE OSTI2023

Quantitative Insight to Fission Gas Bubble Distribution in Irradiated Annular U-10Zr Metallic Fuel Using Deep Learning

U-10Zr Metal fuel is a promising nuclear fuel candidate for next-generation sodium-cooled fast spectrum reactors. Porosity is one of the key facts to impact the performance of metallic fuel. Additionally, a mechanical understanding of fission gas bubbles evolution behavior is a prerequisite for fuel development and qualification. Previous study of fission gas bubbles relied on a simple threshold method working on low resolution optical microscopy images, which has challenges in recognizing bubble boundaries, and caused inaccurate statistics of bubble properties. In this paper, a pre-trained deep learning model on Scanning Electron Microscopy (SEM) images from an annular U-10Zr fuel (AF1), was applied to another U-10Zr annular fuel (AF2). More accurate fission gas bubble segmentation results were generated, which leads to more precise qualitative analysis on the morphology, size, density, and orientation of bubbles. Furthermore, we investigated the lanthanide movement along the radial temperature gradient and obtained conclusive findings.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Development of machine learning framework for interface force closures based on bubble tracking data

Interfacial force closures in the two-fluid model play a critical role for the predictive capabilities of void fraction distribution. However, the practices of interfacial force modeling have long been challenged by the inherent physical complexity of the two-phase flows. The rapidly expanding computational capabilities in the recent years have made high-fidelity data from the interface-captured direct numerical simulation become more available, and hence potential for data-driven interfacial force modeling has prevailed. In this work, we established a data-driven modeling framework integrated to the HZDR multiphase Eulerian-Eulerian framework for computational fluid dynamics simulations. The data-driven framework is verified in a benchmark problem, where a feedforward neural network managed to capture the non-linear mapping between bubble Reynolds number and drag coefficient and reproduce the void distribution resulting from the baseline model in the test case. The second focus is on utilizing the bubble tracking data set to form a closure for the bubble drag in the turbulent bubbly flow, in which the drag coefficient is set to be correlated with the bubble Reynolds number and the Eötvös number. Pseudo-steady state filtering in the Frenet Frame was carried out to obtain the drag coefficient from the turbulent bubbly flow data. The performance of the data-driven drag model is also examined through a case study, where improvement of model’s prediction near-wall is regarded necessary. In conclusion, discussion and further plans of investigation are provided.

42 ENGINEERING↗

DOE OSTI2023

Effects of transition metal carbide dispersoids on helium bubble formation in dispersion-strengthened tungsten

Abstract The formation of helium bubbles and subsequent property degradation poses a significant challenge to tungsten as a plasma-facing material in future long-pulse plasma-burning fusion reactors. In this study, we investigated helium bubble formation in dispersion-strengthened tungsten doped with transition metal carbides, including TaC, ZrC, and TiC. Of the three dispersoids, TaC exhibited the highest resistance to helium bubble formation, possibly due to the low vacancy mobility in the Group VB metal carbide and oxide phases. Under identical irradiation conditions, large helium bubbles formed at grain boundaries in tungsten, while no bubbles were observed at the interfaces between the carbide dispersoid and tungsten matrix. Moreover, our results showed the interfaces could suppress helium bubble formation in the nearby tungsten matrix, suggesting that the interfaces are more effective in trapping helium as tiny clusters. Our research provided new insights into optimizing the microstructure of dispersion-strengthened tungsten alloys to enhance their performance.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Optical and electrochemical effects of H 2 and O 2 bubbles at upward-facing Si photoelectrodes

The effects of the size, contact-angle, and coverage of gas bubbles on solar fuels devices were characterized at cm-scale, upward-facing planar and microwire-array Si photoelectrodes in stagnant electrolytes. Experimental measurements were supported by ray-tracing simulations of surface attached gas bubble films. A dilute, redox-active tracer allowed for the quantification of the mass-transport effects of bubble coverage during photoanodic O 2 (g) evolution at upward-facing photoanodes in 1.0 M KOH(aq.). Measurements of the gas coverage at upward-facing p-Si photocathodes in 0.50 M H 2 SO 4 (aq.) allowed for the nucleation rate and contact angle of H 2 (g) bubbles to be evaluated for systems having various surface free energies. Under simulated solar illumination, the rapid departure of small O 2 (g) bubbles produced stable photocurrents at upward-facing oxygen-evolving Si photoanodes and yielded increased mass-transport velocities relative to a stagnant electrolyte, indicating that bubbles can provide a net benefit to the photoelectrochemical performance of an upward-facing photoanode in solar fuels devices.

14 SOLAR ENERGY↗

DOE OSTI2020

Void-interface wetting to crossing transition owing to bubble to void transformation

Understanding cavity-interface interaction is crucial in designing high-strength, radiation-tolerant nanocomposites. In this work, bubbles near the Cu–Nb interface in Nb could be absorbed by Cu voids wetting the interface due to the high system energy difference produced by the huge pressure difference between the bubbles and voids and high mobility of bubbles, and no bubble-denuded zone forms owing to fast Brownian motion of bubbles, which keeps bubbles distributed homogeneously. However, owing to the low system energy difference generated by the low internal pressure difference and low mobility, voids near the Cu–Nb interface in Nb would simply coalesce with Cu voids wetting the interface, leading to the void-interface wetting to crossing transition and the formation of void-denuded zones due to the negligible migration of internal Nb voids.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Material migration in W and Mo during bubble growth and fuzz formation

Growth of helium (He) induced bubbles and fuzz in tungsten (W) and molybdenum (Mo) is investigated using samples of W films on Mo substrates and Mo films on W substrates exposed to He-containing plasma in the temperature range of 340 to 1075 K, fluence range of 1.0–14 × 10 25 He·m -2 , and incident ion energy of <50 eV. No fuzz (only up to 2 nm diameter bubbles) and no material transport occur in W films at ≤750 K, while precursors-of or fully-developed fuzz and material mixing occur in W and Mo films at ≥800 K. This suggests that fuzz forms in multi-material systems as long as one material meets the conditions for fuzz formation, namely T s / T m ~ 0.27–0.5 where T s and T m are the sample exposure and material melting temperatures, respectively. Larger He bubbles, more material mixing, and further-developed fuzz occur at higher temperature due to increased mobility of He atoms and small He clusters. Accumulation of substrate material at the surface of fuzzy W and Mo thin-film (<80 nm) samples suggests fuzz growth by material transport from the bubble layer in the bulk up to the fiber tip, likely by a two-step process: (i) diffusion of punched dislocation loops in the bulk toward the fuzz base and (ii) diffusion of adatoms along the fuzz base and fiber surface (with effective transport of adatoms upwards due to trapping of adatoms at curved surfaces of fiber tips and/or due to the continuous generation of adatoms at the fuzz base). While the bubble size and fuzz thickness increase with reduced W concentration in Mo thin-film samples at 838 K likely due to an increase in trap mutation and dislocation loop punching in Mo compared to W, the fuzz thickness decreases with reduced W concentration at 1075 K despite an increase in the bubble size likely due to slower diffusion of interstitial loops in Mo.

Physics↗

DOE OSTI2022

Emission from hadronic and leptonic processes in galactic jet-driven bubbles

ABSTRACT We investigate the multiwavelength emission from hadronic and leptonic cosmic rays (CRs) in bubbles around galaxies, analogous to the Fermi bubbles of the Milky Way. The bubbles are modelled using 3D magnetohydrodynamical simulations, and are driven by a 0.3 Myr intense explosive outburst from the nucleus of Milky Way-like galaxies. We compute their non-thermal emission properties at different stages throughout their evolution, up to 7 Myr, by post-processing the simulations. We compare the spectral and spatial signatures of bubbles with hadronic, leptonic, and hybrid hadro-leptonic CR compositions. These each show broadly similar emission spectra, comprised of radio synchrotron, inverse Compton, and non-thermal bremsstrahlung components. However, hadronic and hybrid bubbles were found to be brighter than leptonic bubbles in X-rays, and marginally less bright at radio frequencies, and in γ-rays between ∼0.1 and a few 10s of GeV, with a large part of their emission being driven by secondary electrons formed in hadronic interactions. Hadronic systems were also found to be slightly brighter in high-energy γ-rays than their leptonic counterparts, owing to the π0 decay emission that dominates their emission between energies of 100s of GeV and a few TeV.

Owen, Ellis R. (ORCID:0000000310526439)↗

DOE OSTI2022

Vorticity-induced flow-focusing leads to bubble entrainment in an inkjet printhead: Synchrotron x-ray and volume-of-fluid visualizations

The oscillatory flows present in an inkjet printhead can lead to strong deformations of the air-liquid interface at the nozzle exit. Such deformations may lead to an inward directed air jet with bubble pinch-off and the subsequent entrainment of an air bubble, which is highly detrimental to the stability of inkjet printing. Understanding the mechanisms of bubble entrainment is therefore crucial to improving print stability. Here, in the present work, we use ultrafast x-ray phase-contrast imaging and direct numerical simulations based on the volume-of-fluid method to study the mechanisms underlying the bubble entrainment in a piezoacoustic printhead. We first demonstrate good agreement between experiments and numerics. We then show the different classes of bubble pinch-off obtained in experiments, and that those were also captured numerically. The numerical results are then used to show that the baroclinic torque, which is generated at the gas-liquid interface due to the misalignment of density and pressure gradients, results in a flow-focusing effect that drives the formation of the air jet from which a bubble can pinch off.

42 ENGINEERING↗

DOE OSTI2023

Improved Water Sound Synthesis using Coupled Bubbles

We introduce a practical framework for synthesizing bubble-based water sounds that captures the rich inter-bubble coupling effects responsible for low-frequency acoustic emissions from bubble clouds. We propose coupled-bubble oscillator models with regularized singularities, and techniques to reduce the computational cost of time stepping with dense, time-varying mass matrices. Airborne acoustic emissions are estimated using finite-difference time-domain (FDTD) methods. We propose a simple, analytical surface-acceleration model, and a sample-and-hold GPU wavesolver that is simple and faster than prior CPU wavesolvers. Sound synthesis results are demonstrated using bubbly flows from incompressible, two-phase simulations, as well as procedurally generated examples using single-phase FLIP fluid animations. Our results demonstrate sound simulations with hundreds of thousands of bubbles, and perceptually significant frequency transformations with fuller low-frequency content.

Computer Science↗

DOE OSTI2022

Phase-field simulations of fission gas bubble growth and interconnection in U-(Pu)-Zr nuclear fuel

Abstract The growth and interconnection of fission gas bubbles in the hotter central regions of U-(Pu)-Zr nuclear fuel has been simulated with a phase-field model. The Cahn-Hilliard equation was used to represent the two-phase microstructure, with a single defect species. The volume fraction of the bubble phase and surface area of the bubble-matrix interface were determined during growth and interconnection. Surface area increased rapidly during the initial stages of growth, then slowed and finally decreased as bubble interconnection began and coarsening acted to reduce surface area. The fraction of the bubbles vented to a simulation domain boundary, f V , was quantified as a measure of the microstructure’s interconnectivity and plotted as a function of porosity p . The defect species diffusivity was varied; although changes in diffusivity significantly affected the microstructure, the plots of f V vs. p did not change significantly. The percolation threshold p c was calculated to be approximately 0.26, depending on the assumed diffusivity and using an initial bubble number density based on experimental observations. This is slightly smaller than the percolation threshold for continuum percolation of overlapping 3D spheres. The simulation results were used to parameterize two different engineering-scale swelling models for U-(Pu)-Zr in the nuclear fuel performance code BISON.

Aagesen, Larry K. (ORCID:000000034936676X)↗

DOE OSTI2024

Scintillating Bubble Chambers for Direct Dark Matter Detection, and an Update on SBC-LAr10

The Scintillating Bubble Chamber (SBC) Collaboration aims to use the liquid-noble bubble chamber technology as a low-threshold detector for dark matter particles of 1-10 GeV/c2. The detector combines the remarkable electron recoil (ER) discrimination of the bubble chamber with the event-by-event energy resolution provided by liquid argon (LAr) scintillation, with the crucial added benefit that ER discrimination in liquid-noble bubble chambers extends to much lower thresholds than in past freon-filled bubble chambers, with the potential for quasi-background-free operation at thresholds of 100 eV in nuclear recoil (NR) energy. SBC has developed two functionally identical 10 kg detectors: SBC-LAr10 at Fermilab will calibrate low-threshold performance, while the radio-pure SBC-SNOLAB chamber will execute SBC s first deep-underground dark matter search. SBC-LAr10 at Fermilab was recently installed in the MINOS tunnel 100 meters underground, and the first bubbles are expected this fall. I will present the current status of SBC-LAr10 and describe the suite of gamma and neutron calibrations we will execute. The calibrations will confirm the physics reach of this new technology, motivating not just the SBC-SNOLAB chamber now being assembled but also future searches into the solar neutrino fog at 1 GeV/c2.

Sheng, Zhiheng↗

DOE OSTI2025

Benchmark Exercise Report for Experimental Study of Bubble Scrubbing in Sodium Pool

Mechanistic source term (MST) analyses are likely to be an important part of advanced reactor licensing applications. For the purpose, an MST analysis code applicable to newly introduced advanced reactors, called SRT (Simplified Radionuclide Transport) code, has been developed by Argonne National Laboratory. SRT can track overall behaviors of radionuclides especially in metal fuel-based sodium fast reactors (SFRs) and microreactors. Throughout the simulation, migration inside fuel pins before failure, interaction with coolant (for SFR), removal/leakage in cover gas and containment (or confinement), and environmental dose impacts are considered alongside radioactive decay for short-lived nuclides. Among the postulated process, pool scrubbing phenomenon, especially under sodium pool condition, has been identified as high importance with limited supportive data. The phenomenon plays a crucial role in assessing the degree of radiological impacts as radioactive aerosols or vapors are efficiently and effectively removed during the process. To provide validation basis for SRT in assessing pool scrubbing performance inside sodium pools, the University of Wisconsin-Madison performed tests including extensive parametric effects. Separate effect tests were conducted to directly evaluate the SRT models and to estimate degree of contribution by each contributing factor. Specifically, bubble size, aerosol size, aerosol density, aerosol concentration, pool depth, system temperature, and bubble swarm effects were considered. According to the parametric effects, decontamination performance enhances with decreasing bubble size, large density, and deeper pool height. Aerosol concentration provides no effect for the whole range of interest, and pool temperature variation shows minor effects under the considered temperature condition. When multiple bubbles are injected generating a bubble swarm condition, DF performance further enhances by bubble interactions and turbulence characteristics. The measurement shows the exceptional importance of aerosol size range considered, with the lowest decontamination, where most radionuclides are expected to escape.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2023

Simulating vibro-acoustic damping of bubbles in fluids

Bubbles in fluids are common occurrence due to impurities, thermal or flow variations. They are sometimes considered detrimental to the flow and more importantly surrounding structural integrity. On the other hand, bubbles were used positively towards damping vibrations in fluid filled structures [1] and as barriers or curtains in the removal of plastic waste from water ways [2] and also in noise attenuation from offshore windfarms [3]. In the latter two cases, engineers hypothesized these curtains help marine life from sound pollution from surrounding machinery and ships. In this paper the authors discuss two cases to study the effect of bubble size and bubble density. In the first experiment a curtain of air bubbles was introduced in a water body and sound transmission loss (STL) through this curtain was studied. In a second experiment, a stainless-steel tank filled with liquid mercury is infused with helium bubbles and the vibration levels were monitored.

Kappagantu, Ramana↗

NASA NTRS1976

Flight 1 technical report for experiment 74-36: Thermal migration of bubbles and their interaction with solidification interfaces

Specimens of gas saturated carbon tetrabromide were directionally solidified in a transparent furnace using a gradient freeze technique. The original temperature gradient was 5 C/cm and the cooling rate was 40 C/h. Progress of the experiment was monitored photographically. Gas bubbles were generated at the advancing solidification front in each of the three specimens. The gas bubbles were observed to increase in size, coalesce, and eventually be grown into the solid specimen under low gravity conditions. No bubble detachment from the interface was observed. Identical specimens processed in the laboratory showed bubble nucleation, bubble growth, and eventual bubble detachment due to buoyancy forces. Examination of the specimens showed a significantly greater void content in the low gravity processed samples. The grain size was observed to be finer in the low gravity processed samples.

Papazian, J. M.↗

NASA NTRS1977

The interaction of bubbles with solidification interfaces

The behavior of bubbles at a dendritic solidification interface was studied during the coasting phase of a sounding rocket flight. Sequential photographs of the gradient freeze experiment showed nucleation, growth and coalescence of bubbles at the moving interface during both the low-gravity and one-gravity tests. In the one-gravity test the bubbles were observed to detach from the interface and float to the top of the melt. However, in the low-gravity tests no bubble detachment from the interface or steady state bubble motion occurred and large voids were grown into the crystal. These observations are discussed in terms of the current theory of thermal migration of bubbles and in terms of their implications on the space processing of metals.

Papazian, J. M.↗

NASA NTRS1978

Topside sounder observations of equatorial bubbles

Large scale regions of depleted equatorial ionospheric plasma, called equatorial bubbles, are investigated using topside sounder data. The sounder's unique remote measuring capability enables the magnetic field-aligned nature of the bubbles to be investigated. A search of all available Alouette 2 and ISIS 1 ionograms during nighttime perigee passes near the magnetic equator has revealed a variety of echo signatures associated with bubbles. In addition to a sudden drop in electron density, these signatures usually include in situ spread F and ducted traces. The ducted traces have been used to determine the electron density distribution and to infer changes in ion composition along the magnetic field line within the duct associated with the bubble. In some cases it can be determined that the bubble is asymmetric with respect to the magnetic equator. Even though such features require 3 dimensional models for their explanation, the great field-aligned extent of the bubbles (relative to their cross section) suggests that current theories, which ignore variations along the magnetic field, are still applicable.

Dyson, P. L.↗

NASA NTRS1982

Bubble in a corner flow

The distortion of a two-dimensional bubble (or drop) in a corner of angle delta, due to the flow of an inviscid incompressible fluid around it, is examined theoretically. The flow and the bubble shape are determined as functions of the angle delta, the contact angle beta and the cavitation number gamma. The problem is formulated as an integrodifferential equation for the bubble surface. This equation generalized the integrodifferential equations derived by Vanden-Broeck and Keller. The shape of the bubble is found approximately by using the slender body theory for bubbles. When gamma reaches a critical value gamma sub 0 (beta, delta), opposite sides of the bubble touch each other. Two different families of solution for gamma gamma sub 0 are obtained. In the first family opposite sides touch at one point. In the second family contact is allowed along a segment.

Vanden-Broeck, J. M.↗

NASA NTRS1982

Bubble migration in a rotating, liquid-filled sphere

Results and analysis of ground-based experiments performed to aid in designing experiments on the behavior of bubbles in a rotating liquid body on board the Shuttle in free fall are presented. Spherical shells filled with silicone oil containing a small gas bubble were spun and filmed by high speed motion picture photography. The rotation of the shell and the trajectory of the bubble motion were recorded and the film was exposed to a motion analyzer connected to a keypunch. The analyzer measured Cartesian coordinates as well as angle, frame number, and rotation rate. Optical correction equations were employed to determine the apparent bubble trajectory relative to an inertial frame of reference. An analytical model for the bubble motion was defined, yielding predictions of velocity and position at different times. Rotation of the fluid container is concluded to aid in centering the bubbles.

Annamalai, P.↗