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208 records · Page 12

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this paper, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke↗

The Tables of Aerosol Optics (TAO) Project

The Table of Aerosol Optics (TAO) project is a community repository of optics computations (extinction, absorption, single-scatter albedo, lidar ratio, etc) that are useful for global models and remote sensing applications. TAO expands upon historical efforts (e.g., Hess et al., 1998) by building an open database that uses recent measurements and new computational techniques for non-spherical particles. The ‘open’ aspect of TAO is important, since the size distributions, hygroscopicities, refractive indices, and morphological recommendations of today will undoubtedly yield to different values in the future; the open framework of TAO allows scientists to keep adding new computations to the database as the science evolves. TAO is meant to be a community repository where specialists can put their computations for other scientists to use. So for instance, some groups are advancing new techniques that can accommodate complex fractal aggregates of black carbon, other groups are working on realistic irregular shapes for mineral dust, and different groups are updating the hygroscopicity of various aerosol types using new techniques. The TAO database gives these scientists a place to distribute their products. As TAO grows, modelers and remote sensing specialists will look to TAO as a place to find a wide variety of choices for testing. Meanwhile, global modelers can also use TAO to lobby for new tables that accommodate their needs. Eventually, TAO will provide mass extinction coefficients, mass absorption coefficients, lidar ratios, etc., at popular remote sensing and global modeling wavelengths (0.25-40 µm) for all pertinent species (sulfate, sea salt, BC, OC, BrC, dust, etc.). TAO will also accept computations for aerosol ‘type’ (e.g., biomass burning, urban, background, etc.) that may include regional and seasonal variability. Multiple tables may be created for each species or type to account for the multiple valid size distributions, hygroscopicities, complex refractive indices, and shapes that can be found in the literature.

Elisabeth Andrews↗

Investigating Drivers of Particulate Matter Pollution Over India and the Implications for Radiative Forcing With GEOS-Chem-TOMAS15

Ambient fine particulate matter (PM 2.5 ) concentrations in India frequently exceed 100 μg/m 3 during fall and winter pollution episodes. We use the GEOS-Chem chemical transport model with the TwO-Moment Aerosol Sectional microphysics scheme with 15 size bins (TOMAS15) to assess PM 2.5 composition and impacts on radiation and cloud condensation nuclei (CCN) during pollution episodes as compared to the seasonal (October-December) average. We conduct high resolution (0.25° × 0.3125°) nested-domain simulations over India for short-duration, high-PM2.5 episodes in the fall of 2015 and 2017. The simulations capture the magnitude and spatial patterns of pollution episodes measured by surface monitors (r PM2.5 = 0.69) although aerosol optical depth is underestimated. During the episodes, near-surface organic matter (OM), black carbon (BC), and secondary inorganic aerosol concentrations increase from seasonal averages by up to 36, 7, and 7 μg/m 3 , respectively. Episodic aerosol increases enhance cooling by lowering the top-of-atmosphere clear-sky direct radiative effect (DRE TOA ) during the 2015 episode (−6 W/m 2 ), with a smaller impact during the 2017 episode (−1 W/m 2 ). Differences in DRE TOA reflect larger increases in scattering aerosols in the column during the 2015 episode (+17 mg/m 2 ) than in 2017 (+13 mg/m 2 ), while absorbing aerosol column enhancements are smaller (+3 mg/m2) in both years. Changes in shortwave radiation at the surface (SW sfc ) are spatially similar to DRE TOA and mostly negative during both episodes. CCN enhancements (0.2% supersaturation) during these episodes occur across the western Indo-Gangetic Plain, coincident with higher PM 2.5 concentrations. Changes in DRE TOA , SW sfc , and CCN during high-PM 2.5 episodes may have implications for crops, the hydrologic cycle, and surface temperature.

PM2.5↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke Stratosphere SAGE↗

PTD: Enabling New Space Technologies

Significant advances in the capabilities of small spacecraft over the past 20 years, coupled with improved access to space from a variety of launch platforms have created new opportunities for scientific exploration and commercial application using these high-value (and yet low cost) platforms. Continued development and demonstration of key technologies are improving the performance of the 3U and 6U class CubeSats while expanding the small spacecraft reach into larger platforms, such as 12U and ESPA class missions. The availability and relatively low cost of CubeSat spacecraft allows key technologies to be flight qualified, bridging the TRL 6/7 gap and making truly novel and enabling technologies available to much larger missions in the planning stages at NASA. The key is connecting the technologists with the flight opportunity in a time and cost efficient manner. NASA’s Small Satellite Technology (SST) program is using existing commercial spacecraft to provide a common bus for technology demonstration, taking advantage of their proven platforms and system with proven flight heritage and extensive infrastructure. In this paper we discuss the Pathfinder Technology Demonstrator (PTD) series of four spacecraft and the CubeSat Laser Infrared CrosslinK (CLICK) series of three spacecraft, the approach SST took in facilitating the missions, the successes of those missions as well as lessons learned in the process. NASA’s PTD spacecraft series is demonstrating a variety of new technologies on-orbit, providing proof of the maturity of these significant new technologies, and enhancing the performance of future CubeSats. Each of the four PTD mission consists of one 6-unit (6U) CubeSat weighing approximately 12 kilograms and measuring approximately 30 centimeters x 25 centimeters x 10 centimeters, characterizing its payload within 90 days of orbit insertion. The spacecraft bus, integration and test, and mission operations services are being provided by Terran Orbital. The PTD missions have demonstrated a novel nano-spacecraft compatible propulsion systems (enabling deep space and maneuverable Cubeat missions) and an optical communications system (enabling high data rate collection and communications) already. The CLICK missions are demonstrating compact space-to-space optical communications first with the CLICK A technology demonstrator (already flown) and finally with the CLICK BC dual spacecraft mission. Both projects are part of the SST program within the NASA Space Technology Mission Directorate. SST is chartered to develop and demonstrate technologies to enhance and expand the capabilities of small spacecraft with a particular focus on enabling new mission architectures through the use of small spacecraft, expanding the reach of small spacecraft to new destinations, and augmenting future missions with supporting small spacecraft.

J. Hanson↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

SAGE↗

Recent Trends in Transport of Surface Carbonaceous Aerosols to the Upper-Troposphere-Lower-Stratosphere Linked to Expansion of the Asian Summer Monsoon Anticyclone

Using MERRA-2 re-analyses, we have examined recent trends (2000-2019) in transport of surface carbonaceous aerosols (CA), i.e., organic carbon (OC) and black carbon (BC), to the upper troposphere (UT) and lower stratosphere (LS) during the Asian summer monsoon (ASM). We find a significant increased concentration of UTLS CA, linked to a linear trend in an expansion of the Asian Summer Monsoon Anticyclone (ASMA). Over core monsoon latitudes (25°-35°N), the trends in UTLS CA are enabled by increased upward transport from surface sources via an intensified monsoon meridional circulation, with increased latent heating over the southern Tibetan Plateau and foothill regions, enhanced by feedback processes associated with radiative heating by UTLS CA. In the extra-tropics, increased UTLS CA stems primarily from an extended source of increased wildfire emissions over eastern Siberia and northern Asia, coincident with a large-scale anomalous anticyclone with enhanced surface warming and drying near (80°-120°E, 55°-70°N). Here, carbonaceous aerosols are transported upward from the surface to the LS, likely by increased pyro-convection associated with enhanced wildfires, and enter the tropical UTLS via increased equator ward transport on the eastern flanks of anomalous upper-level anticyclones, coupled to the expanded ASMA. Overall, the increasing UTLS CA trends associated with expansion of the ASMA are consistent with a hydrostatic expansion of a warming troposphere, reflected in a rise in the tropical tropopause and consequential dynamical adjustments of the [ASM subtropical jetstream, modulating the climate of the greater ASM region.

interdecadal trends↗

The Tables of Aerosol Optics (TAO) Project

The Table of Aerosol Optics (TAO) project is a community repository of optics computations (extinction, absorption, single-scatter albedo, lidar ratio, etc) that are useful for global models and remote sensing applications. TAO expands upon historical efforts (e.g., Hess et al., 1998) by building an open database that uses recent measurements and new computational techniques for non-spherical particles. The ‘open’ aspect of TAO is important, since the size distributions, hygroscopicities, refractive indices, and morphological recommendations of today will undoubtedly yield to different values in the future; the open framework of TAO allows scientists to keep adding new computations to the database as the science evolves. TAO is meant to be a community repository where specialists can put their computations for other scientists to use. So for instance, some groups are advancing new techniques that can accommodate complex fractal aggregates of black carbon, other groups are working on realistic irregular shapes for mineral dust, and different groups are updating the hygroscopicity of various aerosol types using new techniques. The TAO database gives these scientists a place to distribute their products. As TAO grows, modelers and remote sensing specialists will look to TAO as a place to find a wide variety of choices for testing. Meanwhile, global modelers can also use TAO to lobby for new tables that accommodate their needs. Eventually, TAO will provide mass extinction coefficients, mass absorption coefficients, lidar ratios, etc., at popular remote sensing and global modeling wavelengths (0.25-40 µm) for all pertinent species (sulfate, sea salt, BC, OC, BrC, dust, etc.). TAO will also accept computations for aerosol ‘type’ (e.g., biomass burning, urban, background, etc.) that may include regional and seasonal variability. Multiple tables may be created for each species or type to account for the multiple valid size distributions, hygroscopicities, complex refractive indices, and shapes that can be found in the literature.

Greg Schuster↗

Modeling Atmospheric Brown Carbon in the GISS ModelE Earth System Model

Brown carbon (BrC) is an absorbing organic aerosol (OA), primarily emitted through biomass burning (BB), which exhibits light absorption unique to both black carbon (BC) and other organic aerosols. Despite many field and laboratory studies seeking to constrain BrC properties, the radiative forcing (RF) of BrC is still highly uncertain. To better understand its climate impact, we introduced BrC to the One-Moment Aerosol (OMA) module of the GISS ModelE Earth system model (ESM). We assessed ModelE sensitivity to primary BrC processed through a novel chemical aging scheme and to secondary BrC formed from biogenic volatile organic compounds (BVOCs). Initial results show that BrC typically contributes a top-of-the-atmosphere (TOA) radiative effect of 0.04 W m −2 . Sensitivity tests indicate that explicitly simulating BrC (separating it from other OAs), including secondary BrC, and simulating chemical bleaching of BrC contribute distinguishable radiative effects and should be accounted for in BrC schemes. This addition of prognostic BrC to ModelE allows greater physical and chemical complexity in OA representation with no apparent trade-off in model performance, as the evaluation of ModelE aerosol optical depth against Aerosol Robotic Network (AERONET) and Moderate Resolution Imaging Spectroradiometer (MODIS) retrieval data, with and without the BrC scheme, reveals similar skill in both cases. Thus, BrC should be explicitly simulated to allow more physically based chemical composition, which is crucial for more detailed OA studies like comparisons to in situ measurement campaigns. We include a summary of best practices for BrC representation within ModelE at the end of this paper.

brown carbon aerosols↗

Machine Learning Based Aerosol and Ocean Color Joint Retrieval Algorithm for Multiangle Polarimeters over Coastal Waters

NASA’s Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission, recently launched in February 2024, carries two multiangle polarimeters (MAPs): the UMBC Hyper-Angular Rainbow Polarimeter (HARP2) and SRON Spectropolarimeter for Planetary Exploration One (SPEXone). Measurements from these MAPs will greatly advance ocean ecosystem and aerosol studies as their measurements contain rich information on microphysical properties of aerosols and hydrosols. The Multi-Angular Polarimetric Ocean coLor (MAPOL) joint retrieval algorithm has been developed to retrieve aerosol and ocean color information, which uses a vector radiative transfer (RT) model as the forward model. The RT model is computationally expensive, which makes processing a large amount of data challenging. FastMAPOL was developed to expedite retrieval using neural networks to replace the RT forward models. As a prototype study, FastMAPOL was initially limited to open ocean applications where the ocean Inherent Optical Properties (IOPs) were parameterized in terms of one parameter: chlorophyll-a concentration (Chla). In this study we further expand the FastMAPOL joint retrieval algorithm to incorporate NN based forward models for coastal waters, which use multi-parameter bio-optical models. In addition, aerosols are represented by six components, i.e., fine mode non absorbing insoluble (FNAI), brown carbon (BrC), black carbon (BC), fine mode non absorbing soluble (FNAS), sea salt (SS) and non-spherical dust (Dust). Sea salt and dust are coarse mode aerosols, while the other components are in the fine mode. The sizes and spectral refractive indices are fixed for each aerosol component, while their abundances are retrievable. The multi-parameter bio-optical model and aerosol components are chosen to represent the coastal marine environment. The retrieval algorithm is applied to synthetic measurements in three different configurations ofMAPs in the PACE mission: HARP2 observations only, SPEXone observations only and combined HARP2 and SPEXone observations. The retrieval results from synthetic measurements show that for aerosol retrieval the SPEXone-only configuration works equally well with the HAPR2-only configuration. On the other hand, for ocean color retrieval the SPEXone instrument provides better information due to its larger spectral coverage. For the surface parameters (wind speed), HARP2 measurements provide better information due to its wide field of view. Combined measurement configuration HARP2+SPEXone performed the best to retrieve all aerosol, ocean color and surface parameters. We also studied the impact of sun glint to aerosol and ocean color retrievals. The retrieval test revealed that wind speed and absorbing aerosol retrieval improves significantly when including measurements at glint geometries. Furthermore, the retrieval algorithm is equipped with modules for atmospheric correction and bidirectional reflectance distribution (BRDF) correction to obtain the remote sensing reflectance, which enables ocean biogeochemistry studies using the PACE polarimeter data.

PACE↗