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At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Reduction of scattering using thin all-dielectric shells designed by stochastic optimizer

Adaptive differential evolution method has been used for optimization of all-dielectric multilayer coatings in order to reduce total scattering from spherical targets. The optimal refractive index profiles have been found for various sizes of targets and thicknesses of coatings. Few profile types that appear to be optimal for various geometrical parameters have been identified. Scattering of the target with diameter of 0.75 λ has been reduced by 85% using 0.16 λ thick coating formed by isotropic dielectric materials. For larger targets, scattering reduction becomes smaller, but it still reaches 50% for targets with the diameter of 1.5 λ. The obtained designs provide a route to implement cloaking without the use of magnetic and anisotropic metamaterials.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Scattering evidence of positional charge correlations in polyelectrolyte complexes

Polyelectrolyte complexation plays an important role in materials science and biology. The internal structure of the resultant polyelectrolyte complex (PEC) phase dictates properties such as physical state, response to external stimuli, and dynamics. Small-angle scattering experiments with X-rays and neutrons have revealed structural similarities between PECs and semidilute solutions of neutral polymers, where the total scattering function exhibits an Ornstein–Zernike form. In spite of consensus among different theoretical predictions, the existence of positional correlations between polyanion and polycation charges has not been confirmed experimentally. Here, we present small-angle neutron scattering profiles where the polycation scattering length density is matched to that of the solvent to extract positional correlations among anionic monomers. The polyanion scattering functions exhibit a peak at the inverse polymer screening radius of Coulomb interactions, q* ≈ 0.2 Å –1 . This peak, attributed to Coulomb repulsions between the fragments of polyanions and their attractions to polycations, is even more pronounced in the calculated charge scattering function that quantifies positional correlations of all polymer charges within the PEC. Screening of electrostatic interactions by adding salt leads to the gradual disappearance of this correlation peak, and the scattering functions regain an Ornstein–Zernike form. Experimental scattering results are consistent with those calculated from the random phase approximation, a scaling analysis, and molecular simulations.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS2011

Spectrally-Invariant Approximation Within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These "spectrally invariant relationships" are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud~dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction. and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with ID radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗
NASA NTRS1990

Total cross sections for positrons scattered elastically from helium based on new measurements of total ionization cross sections

An improved technique is presented for employing the 2.3m spectrometer to measure total ionization cross sections, Q sub ion, for positrons incident on He. The new ionization cross section agree with the values reported earlier. Estimates are also presented of total elastic scattering cross section, Q sub el, obtained by subtracting from total scattering cross sections, Q sub tot, reported in the literature, the Q sub ion and Q sub Ps (total positronium formation cross sections) and total excitation cross sections, Q sub ex, published by another researcher. The Q sub ion and Q sub el measured with the 3m high resolution time-of-flight spectrometer for 54.9eV positrons are in accord with the results from the 2.3m spectrometer. The ionization cross sections are in fair agreement with theory tending for the most part to be higher, especially at 76.3 and 88.5eV. The elastic cross section agree quite well with theory to the vicinity of 50eV, but at 60eV and above the experimental elastic cross sections climb to and remain at about 0.30 pi a sub o sq while the theoretical values steadily decrease.

Diana, L. M.↗
NASA NTRS1993

The effect of topography on radar scattering from vegetated areas

This paper shows how the radar scattering from vegetated areas is affected by the topography of the surface underneath the vegetation. It is shown, using a discrete scatterer model, that the dominant scattering mechanism may change drastically when the ground surface is tilted relative to the horizontal. In the case of a horizontal ground surface, total scattering may be dominated by scattering off the tree trunks, followed by a reflection off the ground surface. For a relatively small tilt in the ground surface (about 2 deg from horizontal), the ground-trunk interaction term may be replaced by scattering from the branches alone as the dominant scattering mechanism. We also show that the effect of the topography is more pronounced for scattering by longer wavelengths, and discuss the implications on algorithms designed to infer forest woody biomass and soil and vegetation moisture using polarimetric SAR data. The effect of the topography on the scattering behavior from forested areas is illustrated with images acquired by the NASA/JPL three-frequency polarimetric SAR over the Black Forest in Germany.

Van Zyl, Jakob J.↗
NASA NTRS1992

The effect of topography on radar scattering from vegetated areas

It is shown how radar scattering from vegetated areas is affected by the topography of the surface underneath the vegetation, and that by the use of a discrete scatterer model the dominant scattering mechanism may change drastically when the ground surface is tilted relative to the horizontal. In the case of a horizontal ground surface total scattering may be dominated by scattering off the tree trunks, followed by a reflection off the ground surface. It is shown that for a relatively small tilt in the ground surface the ground-trunk interaction term may be replaced by scattering from the branches alone as the dominant scattering mechanism. The effect of the topography is more pronounced for scattering by longer wavelengths. The implications for algorithms designed to infer forest woody biomass and soil and vegetation moisture using polarimetric synthetic aperture radar (SAR) data are discussed.

Van Zyl, Jakob J.↗
NASA NTRS2011

Spectrally Invariant Approximation within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These spectrally invariant relationships are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud-dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with 1D radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗
DOE OSTI2013

ASYMMETRIC ABSORPTION PROFILES OF Ly{alpha} AND Ly{beta} IN DAMPED Ly{alpha} SYSTEMS

Damped Ly{alpha} systems observed in the quasar spectra are characterized by a high neutral hydrogen column density, N{sub HI} > 2 x 10{sup 20} cm{sup -2}. The absorption wing profiles are often fitted using the Voigt function due to the fact that the scattering cross section near the resonant line center is approximately described by the Lorentzian function. Since a hydrogen atom has infinitely many p states that participate in the electric dipole interaction, the cross section starts to deviate from the Lorentzian in an asymmetric way in the line wing regions. We investigate this asymmetry in the absorption line profiles around Ly{alpha} and Ly{beta} as a function of the neutral hydrogen column density N{sub HI}. In terms of {Delta}{lambda} {identical_to} {lambda} - {lambda}{sub {alpha}}, we expand the Kramers-Heisenberg formula around Ly{alpha} to find {sigma}({lambda}) {approx_equal} (0.5f{sub 12}){sup 2}{sigma}{sub T}({Delta}{lambda}/{lambda}{sub {alpha}}){sup -2}[1 + 3.792({Delta}{lambda}/{lambda}{sub {alpha}})], where f{sub 12} and {sigma}{sub T} are the oscillator strength of Ly{alpha} and the Thomson scattering cross section, respectively. In terms of {Delta}{lambda}{sub 2} {identical_to} {lambda} - {lambda}{sub {beta}} in the vicinity of Ly{beta}, the total scattering cross section, given as the sum of cross sections for Rayleigh and Raman scattering, is shown to be {sigma}({lambda}) {approx_equal} {sigma}{sub T}(0.5f{sub 13}){sup 2}(1 + R{sub 0})({Delta}{lambda}{sub 2}/{lambda}{sub {beta}}){sup -2}[1 - 24.68({Delta}{lambda}{sub 2}/{lambda}{sub {beta}})] with f{sub 13} and the factor R{sub 0} = 0.1342 being the oscillator strength for Ly{beta} and the ratio of the Raman cross section to Rayleigh cross section, respectively. A redward asymmetry develops around Ly{alpha}, whereas a blue asymmetry is obtained for Ly{beta}. The absorption center shifts are found to be almost proportional to the neutral hydrogen column density.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2012

Spectral Invariant Approximation within Atmospheric Radiative Transfer; Applications to EarthCare

Certain algebraic combinations of single-scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These "spectrally-invariant relationships" are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength-independence does not hold in the atmosphere, but in cloud-dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. We identify the conditions under which the spectrally-invariant approximation can accurately describe the extinction and scattering properties of cloudy atmospheres. Validity of the assumptions and accuracy of the approximation is tested with radiative transfer calculations. We discuss the physics behind this phenomenon and possible applications to remote sensing, climate, and the EarthCare, mission in particular.

Marshak, Alexander↗
DOE OSTI2013

Association of scattering matrices in quantum networks

Algorithms based on operations that associate scattering matrices in series or in parallel (analogous to impedance association in a classical circuit) are developed here. We exemplify their application by calculating the total scattering matrix of several types of quantum networks, such as star graphs and a chain of chaotic quantum dots, obtaining results with good agreement with the literature. Through a computational-time analysis we compare the efficiency of two algorithms for the simulation of a chain of chaotic quantum dots based on series association operations of (i) two-by-two centers and (ii) three-by-three ones. Empirical results point out that the algorithm (ii) is more efficient than (i) for small number of open scattering channels. A direct counting of floating point operations justifies quantitatively the superiority of the algorithm (i) for large number of open scattering channels.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2001

Potential Energy Curves and Transport Properties for the Interaction of He with Other Ground-state Atoms

The interactions of a He atom with a heavier atom are examined for 26 different elements, which are consecutive members selected from three rows (Li - Ne, Na - Ar, and K,Ca, Ga - Kr) and column 12 (Zn,Cd) of the periodic table. Interaction energies are determined wing high-quality ab initio calculations for the states of the molecule that would be formed from each pair of atoms in their ground states. Potential energies are tabulated for a broad range of Interatomic separation distances. The results show, for example, that the energy of an alkali interaction at small separations is nearly the same as that of a rare-gas interaction with the same electron configuration for the dosed shells. Furthermore, the repulsive-range parameter for this region is very short compared to its length for the repulsion dominated by the alkali-valence electron at large separations (beyond about 3-4 a(sub 0)). The potential energies in the region of the van der Waals minimum agree well with the most accurate results available. The ab initio energies are applied to calculate scattering cross sections and obtain the collision integrals that are needed to determine transport properties to second order. The theoretical values of Li-He total scattering cross sections and the rare-gas atom-He transport properties agree well (to within about 1%) with the corresponding measured data. Effective potential energies are constructed from the ab initio energies; the results have been shown to reproduce known transport data and can be readily applied to predict unknown transport properties for like-atom interactions.

Partridge, Harry↗
DOE OSTI2024

Nephelometer Instrument Handbook

The Integrating Nephelometer (Figure 1) is an instrument that measures aerosol light scattering. It measures aerosol optical scattering properties by detecting (with a wide angular integration – from 7 to 170°) the light scattered by the aerosol and subtracting the light scattered by the carrier gas, the instrument walls and the background noise in the detector (zeroing). Zeroing is typically performed for 5 minutes every day at midnight UTC. The scattered light is split into red (700 nm), green (550 nm), and blue (450 nm) wavelengths and captured by three photomultiplier tubes. The instrument can measure total scatter as well as backscatter only (from 90 to 170°) (Heintzenberg and Charlson 1996; Anderson et al. 1996; Anderson and Ogren 1998; TSI 3563 2015) At ARM (Atmospheric Radiation Measurement), two identical Nephelometers are usually run in series with a sample relative humidity (RH) conditioner between them. This is possible because Nephelometer sampling is non-destructive and the sample can be passed on to another instrument. The sample RH conditioner scans through multiple RH values in cycles, treating the sample. This kind of setup allows to study how aerosol particles’ light scattering properties are affected by humidification (Anderson et al. 1996). For historical reasons, the two Nephelometers in this setup are labeled “wet” and “dry”, with the “dry” Nephelometer usually being the one before the conditioner and sampling ambient air (the names are switched for the MAOS measurement site due to the high RH of the ambient air).

47 OTHER INSTRUMENTATION↗
DOE OSTI2014

Exact scattering matrix of graphs in magnetic field and quantum noise

We consider arbitrary quantum wire networks modelled by finite, noncompact, connected quantum graphs in the presence of an external magnetic field. We find a general formula for the total scattering matrix of the network in terms of its local scattering properties and its metric structure. This is applied to a quantum ring with N external edges. Connecting the external edges of the ring to heat reservoirs, we study the quantum transport on the graph in ambient magnetic field. We consider two types of dynamics on the ring: the free Schrödinger and the free massless Dirac equations. For each case, a detailed study of the thermal noise is performed analytically. Interestingly enough, in presence of a magnetic field, the standard linear Johnson-Nyquist law for the low temperature behaviour of the thermal noise becomes nonlinear. The precise regime of validity of this effect is discussed and a typical signature of the underlying dynamics is observed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Research at the University of Kentucky Accelerator Laboratory

The Department of Physics and Astronomy at the University of Kentucky operates a 7-MV CN Van de Graaff accelerator that produces primary beams of protons, deuterons, and helium ions. An in-terminal pulsing and bunching system operates at 1.875 MHz and is capable of providing 1 ns beam bunches at an average current of several microamperes. Nearly all ongoing research programs involve secondary pulsed neutrons produced with gas cells containing deuterium or tritium, as well as with a variety of solid targets. Most experiments are performed at a target station positioned over a deep pit, so as to reduce the background created by backscattered neutrons. Here, recent experiments will be described; these include: measurements of n-p scattering total cross sections from E n = 90 to 1800 keV to determine the n-p effective range parameter; the response of the plastic scintillator BC-418 below 1 MeV to low-energy recoil protons; n-p radiative capture cross sections important for our understanding of nucleosynthesis approximately 2 minutes after the occurrence of the Big Bang; γ-ray spectroscopy following inelastic neutron scattering to study nuclear structure relevant to double-β decay and to understand the role of phonon-coupled excitations in weakly deformed nuclei; and measurements of neutron elastic and inelastic scattering cross sections for nuclei that are important for energy production and for our global understanding of the interaction of neutrons with matter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1991

Spectrally resolved Rayleigh scattering diagnostic for hydrogen-oxygen rocket plume studies

A Rayleigh scattering diagnostic has been developed to measure gas density, temperature, and velocity in the exhaust plume of 100 N thrust class hydrogen-oxygen rockets. The spectrum of argon-ion laser light scattered by the gas molecules in the plume (predominantly water vapor) is measured with a scanning Fabry-Perot interferometer. The gas density is determined from the total scattered power, the gas temperature from the spectral width, and the velocity from the shift in the peak of the spectrum from the frequency of the incident laser light. The diagnostic has been demonstrated in a rocket test cell and a discussion of results is given.

Seasholtz, R. G.↗
DOE OSTI2018

Atomic Dynamics in Simple Liquid: de Gennes Narrowing Revisited

The de Gennes narrowing phenomenon is frequently observed by neutron or x-ray scattering measurements of the dynamics of complex systems, such as liquids, proteins, colloids, and polymers. The characteristic slowing down of dynamics in the vicinity of the maximum of the total scattering intensity is commonly attributed to enhanced cooperativity. In this Letter, we present an alternative view on its origin through the examination of the time-dependent pair correlation function, the van Hove correlation function, for a model liquid in two, three, and four dimensions. We find that the relaxation time increases monotonically with distance and the dependence on distance varies with dimension. We propose a heuristic explanation of this dependence based on a simple geometrical model. Furthermore, this finding sheds new light on the interpretation of the de Gennes narrowing phenomenon and the α-relaxation time.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1998

LASE measurements of aerosols and water vapor during TARFOX

The TARFOX (Tropospheric Aerosol Radiative Forcing Observational Experiment) intensive field campaign was designed to reduce uncertainties in estimates of the effects of anthropogenic aerosols on climate by measuring direct radiative effects and the optical, physical, and chemical properties of aerosols [1]. TARFOX was conducted off the East Coast of the United States between July 10-31, 1996. Ground, aircraft, and satellite-based sensors measured the sensitivity of radiative fields at various atmospheric levels to aerosol optical properties (i.e., optical thickness, phase function, single-scattering albedo) and to the vertical profile of aerosols. The LASE (Lidar Atmospheric Sensing Experiment) instrument, which was flown on the NASA ER-2 aircraft, measured vertical profiles of total scattering ratio and water vapor during a series of 9 flights. These profiles were used in real-time to help direct the other aircraft to the appropriate altitudes for intensive sampling of aerosol layers. We have subsequently used the LASE aerosol data to derive aerosol backscattering and extinction profiles. Using these aerosol extinction profiles, we derived estimates of aerosol optical thickness (AOT) and compared these with measurements of AOT from both ground and airborne sun photometers and derived from the ATSR-2 (Along Track and Scanning Radiometer 2) sensor on ERS-2 (European Remote Sensing Satellite-2). We also used the water vapor mixing ratio profiles measured simultaneously by LASE to derive precipitable water vapor and compare these to ground based measurements.

Ferrare, Richard A.↗
DOE OSTI2021

Magnetic ordering in the Ising antiferromagnetic pyrochlore Nd 2 ScNbO 7

The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behaviour, here we describe a system in which the structural disorder results in long-range antiferromagnetic order due to local symmetry breaking. Nd 2 ScNbO 7 is shown to have a dispersionless gapped excitation observed in other neodymium pyrochlores below T N = 0.37 K through polarized and inelastic neutron scattering. However the dispersing spin waves are not observed. This excited mode is shown to occur in only 14(2)% of the neodymium ions through spectroscopy and is consistent with total scattering measurements as well as the magnitude of the dynamic moment 0.26(2) μB . The remaining magnetic species order completely into the all-in all-out Ising antiferromagnetic structure. This can be seen as a result of local symmetry breaking due disordered Sc +3 and Nb +5 ions about the A-site. From this work, it has been established that B-site disorder restores the dipole-like behaviour of the Nd +3 ions compared to the Nd 2 ScNbO 7 parent series.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗