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At least 199 records · Page 11

Energy deposition and K-shell ionization of supernovae

We present explicit evaluation of K-shell ionization caused by photoelectric absorption, by Compton scattering, and by electron collisions in supernovae envelopes. Each process derives from the radioactivity that dominates the bolometric luminosity of the model supernovae. We include the ionization by bremsstrahlung. We find that electron-collision ionization with decelerating Compton electrons is the dominant process of K-shell ionization for light elements (lighter than Si) whereas photoelectric K-shell absorption of Comptonized gammas is the dominant process of K-shell ionization for heavy elements (like Fe). The relative importance of the ionization processes also depends upon composition and upon time, as well as upon supernova type. For Type Ia all four ionization sources are of importance. We present fitting formulas for the deposition of radioactive power in each class of models studied. The energy deposition of all mechanisms decreases with time, including the rate of K-shell ionizations of all elements throughout the supernovae model evaluated herein. We compare the relative contributions to the energy deposition and confirm with greater numerical detail results already established.

The, Lih-Sin↗

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r -process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-process Elements (FIRE)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for work on nuclear data (ground-state properties, fission, β-decay), BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from the DOE Office of Science, while national laboratories received funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-process Elements (FIRE)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission In R-process Elements (FIRE) - Quarterly Report (Q2FY22)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Observations of the Bright Star in the Globular Cluster 47 Tucanae (NGC 104)

The Bright Star in the globular cluster 47 Tucanae (NGC 104) is a post-asymptotic giant branch (post-AGB) star of spectral type B8 III. The ultraviolet spectra of late-B stars exhibit myriad absorption features, many due to species unobservable from the ground. The Bright Star thus represents a unique window into the chemistry of 47 Tuc. We have analyzed observations obtained with the Far Ultraviolet Spectroscopic Explorer, the Cosmic Origins Spectrograph aboard the Hubble Space Telescope, and the Magellan Inamori Kyocera Echelle Spectrograph on the Magellan Telescope. By fitting these data with synthetic spectra, we determine various stellar parameters (T {sub eff} = 10,850 ± 250 K, logg=2.20±0.13) and the photospheric abundances of 26 elements, including Ne, P, Cl, Ga, Pd, In, Sn, Hg, and Pb, which have not previously been published for this cluster. Abundances of intermediate-mass elements (Mg through Ga) generally scale with Fe, while the heaviest elements (Pd through Pb) have roughly solar abundances. Its low C/O ratio indicates that the star did not undergo third dredge-up and suggests that its heavy elements were made by a previous generation of stars. If so, this pattern should be present throughout the cluster, not just in this star. Stellar-evolution models suggest that the Bright Star is powered by a He-burning shell, having left the AGB during or immediately after a thermal pulse. Its mass (0.54 ± 0.16M {sub ⊙}) implies that single stars in 47 Tuc lose 0.1–0.2 M {sub ⊙} on the AGB, only slightly less than they lose on the red giant branch.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Fission In R-process Elements (FIRE) (NA-22 Quarterly Report, Q4FY22)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Element Formation in Radiation-hydrodynamics Simulations of Kilonovae

Abstract Understanding the details of r -process nucleosynthesis in binary neutron star merger (BNSM) ejecta is key to interpreting kilonova observations and identifying the role of BNSMs in the origin of heavy elements. We present a self-consistent, two-dimensional, ray-by-ray radiation-hydrodynamic evolution of BNSM ejecta with an online nuclear network (NN) up to a timescale of days. For the first time, an initial numerical relativity ejecta profile composed of the dynamical component and spiral-wave and disk winds is evolved including detailed r -process reactions and nuclear heating effects. A simple model for the jet energy deposition is also included. Our simulation highlights that the common approach of relating in postprocessing the final nucleosynthesis yields to the initial thermodynamic profile of the ejecta can lead to inaccurate predictions. Moreover, we find that neglecting the details of the radiation-hydrodynamic evolution of the ejecta in nuclear calculations can introduce deviations of up to 1 order of magnitude in the final abundances of several elements, including very light and second r -process peak elements. The presence of a jet affects element production only in the innermost part of the polar ejecta, and it does not alter the global nucleosynthesis results. Overall, our analysis shows that employing an online NN improves the reliability of nucleosynthesis and kilonova light-curve predictions.

Magistrelli, Fabio (ORCID:0009000509767851)↗

First results from the Goddard High-Resolution Spectrograph - Element abundances as a function of velocity in the neutral gas toward Xi Persei

Observations of ultraviolet interstellar absorption lines toward Xi Persei obtained with the echelle mode of the Goddard High-Resolution Spectrograph (GHRS) aboard the HST at a resolution of 3.5 km/s are presented. The data for O I, C II, Mg II, S II, Fe II, Si II, Mn II, and Zn II are converted into representations of apparent column density per unit velocity, Na(v), over the velocity range from -30 to +40 km/s. The profiles for ions that are the dominant state of ionization in neutral clouds permit a study of the variation of element abundance with velocity caused by changes in the gas phase depletion in the different absorbing regions situated toward Xi Per. In the denser portions of the diffuse clouds, heavy element depletions are very large. However, in absorbing components near -5 and +25 km/s, the depletions are less severe, with a nearly solar gas phase abundance ratio being found for the gas in the +25 km/s component. The measurements confirm that the GHRS is well suited for diagnostic spectroscopy of interstellar gas.

Savage, Blair D.↗

The Super-TIGER Instrument to Probe Galactic Cosmic Ray Origins

Super-TIGER (Super Trans-Iron Galactic Element Recorder) is under construction for the first of two planned Antarctic long-duration balloon flights in December 2012. This new instrument will measure the abundances of ultra-heavy elements (30Zn and heavier), with individual element resolution, to provide sensitive tests of the emerging model of cosmic-ray origins in OB associations and models of the mechanism for selection of nuclei for acceleration. Super-TIGER builds on the techniques of TIGER, which produced the first well-resolved measurements of elemental abundances of the elements 31Ga, 32Ge, and 34Se. Plastic scintillators together with acrylic and silica-aerogel Cherenkov detectors measure particle charge. Scintillating-fiber hodoscopes track particle trajectories. Super-TIGER has an active area of 5.4 sq m, divided into two independent modules. With reduced material thickness to decrease interactions, its effective geometry factor is approx.6.4 times larger than TIGER, allowing it to measure elements up to 42Mo with high statistical precision, and make exploratory measurements up to 56Ba. Super-TIGER will also accurately determine the energy spectra of the more abundant elements from l0Ne to 28Ni between 0.8 and 10 GeV/nucleon to test the hypothesis that microquasars or other sources could superpose spectral features. We will discuss the implications of Super-TIGER measurements for the study of cosmic-ray origins and will present the measurement technique, design, status, and expected performance, including numbers of events and resolution. Details of the hodoscopes, scintillators, and Cherenkov detectors will be given in other presentations at this conference.

Mitchell, John W.↗

Bimodal abundances in the energetic particles of solar and interplanetary origin

This letter reports the first results from an examination of the daily-averaged abundances of the elements from H through Fe as well as electrons and isotopes of He in energetic particles observed in interplanetary space by the ISEE 3 spacecraft over an 8.5 yr period. The abundances of heavy elements such as Fe/O show, for the first time, clear evidence of the presence of two distinct populations of particles. Earlier observations could be interpreted as extreme variations within a single population. The population with enhanced Fe/O shows correlated enhancements in He-3/He-4, p/e, and He/H. This population is consistent with material that has been processed to high temperatures in the impulsively heated regions of solar flares. The second population, with more normal abundances, is probably accelerated from ambient material by coronal and interplanetary shocks.

Reames, Donald V.↗

Pressurized Adapter for "Shirt-Sleeves" Transfer and Universal Base Expansion (PASSTUBE)

Proposed is a scalable, six-degree-of-freedom, pressurized docking adapter that can connect multiple volumes while resolving all forces within itself. In a large space outpost pass-through connection is needed between multiple volumes to maintain a continuous pressurized cabin for crew access, translation, and egress. Zero-g docking and berthing of elements can be done using robotic arms, thrusters, and simple docking interface hardware because orthogonal mating is only governed by position, orientation, and momentum, but soft capture / hard docking techniques would not work in a gravity environment because modules cannot be brought in square with each other. Gravity docking is problematic in that any two elements have a gravity vector and it is not practical to provide a perfectly flat surface for them to rest on. Any stretch of natural or graded terrain still has surface fluctuations - maneuvering one element in respect to another would constantly be working against a gravity vector, where uneven surfaces would cause modules to come to rest in odd configurations in respect to each other. Manipulation of heavy elements, such as habitats will be difficult to do with precision -- elements may be placed as close as the mobility system can handle but would still leave the elements not in square with each other. The proposed Pressurized Adapter for "Shirt-Sleeve" Transfer and Universal Base Expansion (PASSTUBE) element will connect non-square and skewed elements while resolving all forces internal to itself.

Howe, A. Scott↗

Energy spectra of cosmic rays above 1 TeV per nucleon

Direct measurements of cosmic-ray nuclei above 1 TeV/nucleon have been performed in a series of balloon-borne experiments with emulsion chambers. The observed all-particle spectrum above 20 TeV is consistent with the results of the Proton satellite and many air shower experiments. The proton spectrum is consistent with a power law having an index of 2.76 + or - 0.09 up to at least 100 TeV, but an overabundance of helium by a factor of 2 above 2 TeV per nucleon is found when compared with the extrapolation from the low energies. For heavy elements (C through Fe), the intensities around 1 TeV/nucleon are consistent, within the statistical errors, with the extrapolation from lower energy data using the Spacelab 2 spectral indices. An enhancement for the medium-heavy components (C through Ca) above 200 TeV is indicated. The mean mass above 50 TeV indicates slightly higher values than the results of the air shower experiments.

Burnett, T. H.↗

Comparison of state-interaction and spinor-representation calculations of spin-orbit coupling within exact two-component coupled-cluster theories

Here a benchmark study of state-interaction and spinor-representation calculations of spin-orbit coupling using the exact two-component Hamiltonians with atomic mean-field integrals (the X2CAMF schemes) at the equation-of-motion coupled-cluster singles and doubles level is reported. We adopt a version of the X2CAMF scheme with spin-orbit integrals correct to first order for the state-interaction calculations and a version correct to infinite order for the spinor-representation calculations. The differences between the state-interaction calculations with minimum active spaces to account for (quasi-)degeneracy and the spinor-representation calculations thus correspond to higher-order spin-orbit contributions. This state-interaction approach with scalar-relativistic effects accurately included in the reference functions and in the spin-orbit integrals is shown to exhibit robust performance for elements across the periodic table. On the other hand, the more rigorous spinor representation shows more rapid convergence with respect to the number of correlated electrons and is the preferred choice for accurate calculations for heavy elements.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Intrinsic Bonding and Reactivity of Actinide Clusters Poster

The effect of electronic structure on chemical bonding and reactivity is one of the most important questions in the field of chemistry. Insight into chemical bond formation involving elements that contain f electrons (i.e., the lanthanides and actinides) is critical for solving specific technical challenges, such as development of advanced nuclear fuel cycles and efficient rare earth separations, as well as a broader understanding of bonding across the entire periodic table. The primary technique for studying the fundamentals of lanthanide and actinide bonding is crystallization of metal-ligand compounds followed by structural determination with X-rays and comparison to theory with computational chemistry. While this procedure has yielded significant insights for a wide variety of elements, it is challenging to apply to the heavier trans-uranic actinides such as berkelium and californium because of limited material availability, significant radioactivity, and poorly understood chemical reactivity of these elements. We hypothesize that by forming actinide-ligand clusters in a mass spectrometer and probing their reactivity in the gas-phase, many of the challenges associated with studying the heavier trans-uranic elements can be circumvented. This project will develop a capability to address a wide range of actinide bonding and reactivity phenomena, increasing Idaho National Laboratory’s capability to address fundamental questions at the forefront of heavy element chemical and molecular science.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Systematics of heavy ion enhancements in solar flares

Using Lexan and glass detectors, the composition of solar particles with atomic number 2 or greater was determined as a function of energy from approximately 0.2 to 50 MeV/nucleon in four flares of quite different intensity and during a time when the sun was nearly quiet. Fe is nearly completely stripped. The enhancement factor increases with atomic number at a given energy but decreases with energy. Heavy element enhancements are detectable at higher energies in stronger flares. They occurred in ancient as well as in present-day flares. We have observed Li and Be in one flare. Incomplete ionization, preferential leakage of heavy ions, energy loss by ionization, and nuclear reactions appear to be involved in solar particle production.

Price, P. B.↗