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At least 199 records · Page 11

Canister Helium Leak Detection Based on Temperature Information Using RAMM (Final CRADA Report)

The performance of RAMM-TM in detecting gas leakage from a canister with a small, simulated chloride-induced stress corrosion crack has been demonstrated in a series of experiments conducted at CRIEPI by using a 1/4.5- scale model cask. Leakage of both helium and air from a canister was detected within hours after the start of the leakage. The change in surface temperatures at the top and bottom of the canister (ΔTBT) during gas leakage (depressurization) triggered automatic alarms, providing a sound basis for early detection of gas leakage from the canister. This methodology would enable consequence management through the implementation of mitigatory actions to continue effective aging management, to reduce risks to public safety and health, and to protect the environment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Quantification of Aerosol Transmission through Stress Corrosion Crack-Like Geometries

The formation of a stress corrosion crack (SCC) in the canister wall of a dry cask storage system (DCSS) has been identified as a potential issue for the long-term storage of spent nuclear fuel. The presence of an SCC in a storage system could represent a through-wall flow path from the canister interior to the environment. Modern, vertical DCSSs are of particular interest due to the commercial practice of using more significant backfill pressures in the canister, up to approximately 800 kPa. This pressure differential offers a relatively high driving potential for blowdown of any particulates that might be present in the canister. In this study, the rates of gas flow and aerosol transmission of a spent fuel surrogate through an engineered microchannel with dimensions representative of an SCC were evaluated experimentally using coupled mass flow and aerosol analyzers. The microchannel was formed by mating two gage blocks with a linearly tapering slot orifice nominally 13 μm (0.005 in.) tall on the upstream side and 25 μm (0.0010 in.) tall on the downstream side. The orifice is 12.7 mm (0.500 in.) wide by 8.86 mm (0.349 in.) long (flow length). Surrogate aerosols of cerium oxide, CeO 2 , were seeded and mixed with either helium or air inside a pressurized tank. The aerosol characteristics were measured immediately upstream and downstream of the simulated SCC at elevated and ambient pressures, respectively. These data sets are intended to add to previous testing that characterized SCCs under well-controlled boundary conditions through the inclusion of testing improvements that establish initial conditions in a more consistent way. These ongoing testing efforts are focused on understanding the evolution in both size and quantity of a hypothetical release of aerosolized spent fuel particles from failed fuel to the canister interior and ultimately through an SCC.

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Insert Modeling in UNF ST&DARDS

The Used Nuclear Fuel-Storage, Transportation & Disposal Analysis Resource and Data System (UNF-ST&DARDS) is a software tool that integrates a used nuclear fuel (UNF) or spent nuclear fuel (SNF) relational database and key analysis capabilities to simplify and automate numerous UNF management and fuel cycle–related activities. UNF-ST&DARDS is being developed for the US Department of Energy’s Office of Nuclear Energy Spent Fuel and Waste Disposition program. UNF-ST&DARDS provides an integrated framework that uses advanced modeling and simulation to predict the behavior of SNF over the timescales associated with permanent disposal in a geologic repository. After leaving the spent fuel pool, SNF is transferred to dry storage in a dual-purpose canister (DPC). DPCs are considered “dual purpose” because they are designed for both storage and transportation, removing the need to transfer the fuel to a separate transportation cask. However, much research has been conducted investigating the feasibility of directly disposing of DPCs in geologic repositories. Direct disposal of DPCs could reduce worker exposure during repackaging, reducing the amount of low-level waste from the discarded DPCs and potentially saving billions of dollars. Therefore, direct disposal of as-loaded DPCs is desirable if it can be done safely.

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Review of Experimental Data for Validating Computer Codes Used in Shielding Calculations for Spent Fuel Storage and Transportation Systems

This report presents a review of available radiochemical assay data and shielding benchmarks applicable to spent nuclear fuel (SNF) shielding calculations. The relevant information reviewed herein includes the Spent Fuel Composition (SFCOMPO) database, the Shielding Integral Benchmark Archive and Database (SINBAD), the International Handbook of Evaluated Criticality Safety Benchmark Experiments, and published measurements of external dose rates of casks loaded with SNF. The relevant experimental data identified in this report may be used to support verification and validation of computer codes used in SNF cask/transport shielding applications, as well as development of calculation uncertainties. It should be noted that a relatively small subset of the identified experimental data (e.g., criticality alarm experiments) is available in a standard format established by the international community participating in experimental isotopic and shielding data evaluations. An effort of the SFCOMPO Technical Review Group (TRG) is underway to publish first isotopic evaluations of individual assay data using a standard data evaluation format. The SINBAD TRG has recently initiated benchmark evaluations and modernization of the database. Therefore, more relevant information is expected in the future that will enable users to select quality experimental data in depletion code and shielding code validations for SNF applications.

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DOE SNF Packaging Demonstration Project: Worktable and Canister Loading Sleeve Design [Slides]

This presentation is a briefing for summer interns and others outside the project, to give them a summary of ongoing design activities. The DOE SNF Packaging Demonstration Project is an effort to develop and demonstrate the designs, technology, processes, and regulatory framework for packaging DOE-managed spent nuclear fuel (SNF) for road ready dry storage (RRDS). The project is to remotely load and seal two types of DOE-managed SNF from the CPP-603 facility into DOE Standard Canisters, place the sealed DOE Standard Canisters into commercial vendor over-canisters (equivalent to commercial MPCs), seal and place the over-canisters into commercial vendor storage overpacks, and place the storage system (over-canister and storage overpack) onto the CPP-2707 cask pad.

42 ENGINEERING↗

Criticality Safety and Fuel Performance Considerations for Enrichment Above 5 Weight Percent in the Uranium Dioxide Fuel Cycle

The U.S. Nuclear Regulatory Commission (NRC) is preparing for anticipated licensing applications requesting fuel enrichments of UO 2 ceramic fuels enriched in excess of 5 weight percent (w/o) 235 U for commercial light-water reactors (LWRs). PNNL has been tasked with providing technical assistance to the NRC related to the review and approval of requests for enrichment increases above the current 5 w/o 235 U enrichment limit. This report will provide the agency with technical assistance to enhance the staff’s knowledge base and to identify developmental needs required to support the licensing of greater than 5 w/o UO 2 ceramic fuels. This report provides a background on increasing enrichment of UO 2 LWR fuel beyond 5 w/o 235 U. The primary concern of increasing enrichment is the impacts to criticality safety. This report will focus on criticality safety as it relates to enrichment, conversion of uranium hexafluoride to UO 2 , fuel assembly fabrication, transportation of fresh/spent fuel assemblies, reactor operations, and storage of fresh/spent fuel assemblies. The report provides a general summary of each of the steps in the UO 2 fuel cycle starting from transportation of enriched UF 6 through dry cask storage of spent fuel assemblies. This report also discusses other impacts of increased enrichment during reactor operation and the surrounding fuel cycle activities. Current needs regarding both data and analytical codes to support the increase above 5 w/o 235 U are identified and discussed.

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Isotope Production for UK PhD Student Visit [Slides]

Overview of INL isotope production work, including organizational structures, the current work and future plans of plutonium fuel supplies, cobalt-60 production, and BRR cask shipping.

07 ISOTOPE AND RADIATION SOURCES↗

Plan for Development and Application of Risk Assessment Approach for Transportation Package Approval of an MNPP for Domestic Highway Shipment

For nuclear reactors, Probabilistic Risk Assessment (PRA) has been conducted since the 1970s [e.g., see WASH-1400 (NRC 1975), NUREG-1150 (NRC 1990), and NUREG-1935 (Chang et al. 2012)]. PRA has also been used to assess a dry cask storage system at a nuclear power plant [see NUREG-1864 (NRC 2007)]. PRA techniques have also been applied to the transportation of spent nuclear fuel, most notably in NUREG/CR-4829 (Fischer et al. 1987), NUREG/CR-6672 (Sprung et al. 2000), and NUREG-2125 (NRC 2014). Additional guidance is provided in International Atomic Energy Agency (IAEA) IAEA-TECDOC-1346 (2003). Transportation PRA was also used in the evaluations of transportation impacts in reports such as the Repository Final Environmental Impact Statement (DOE 2002) and the Repository Final Supplemental Environmental Impact Statement (DOE 2008).

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GaN HEMT Fabrication for Radiation-Hardened Sensing and Communications Electronics

Gallium nitride (GaN), a wide bandgap semiconductor, has vast potential to address two environment conditions associated with the application of electronics to nuclear power: elevated temperatures, and high levels of radiation. A process was developed at The Ohio State University (OSU) to enable fabrication of complex digital and analog electronics circuits for application to nuclear power environments such as locations near or in the reactor core or in spent nuclear fuel casks. Radio frequency (RF)-grade GaN high electron mobility transistor (HEMT) devices were fabricated as part of this process. These were fabricated as depletion mode and enhancement mode devices. They have been electrically characterized and have demonstrated the expected performance. Behavioral models (Verilog-A) were developed from these device measurements to enable electrical simulation of GaN HEMT devices and circuits using common electronics simulation tools based on Simulation Program with Integrated Circuit Emphasis (SPICE). A similar set of GaN HEMT devices is being developed to provide lower speed devices for logic and analog functions. These accomplishments position this technology for effective application to sensor interfacing, signal processing, and data communications in nuclear power plants, including operation in or near the reactor core.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Sensitivity of Spent Fuel Temperatures to Variable Canister Backfills

This report describes thermal modeling done to understand the effects of a hypothetical loss of backfill to a spent fuel storage canister. A NAC MAGNASTOR system was analyzed using STAR-CCM+ and COBRA-SFS at various heat loads, helium pressures, and air environments. When helium was lost later in life the results showed no safety impact to the thermal performance of the cask system and fuel cladding. However, there were other results of interest from this study. The potential to detect helium leaks using external temperature measurement was considered and found to be a potential area for future technology development. The other major result of interest was the significant change in flow velocities with an air environment. This data will be useful in understanding the potential impacts of a breached canister.

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Neutron Absorber Plate Characterization Plan for Criticality Experiments Design [Slides]

The goal of this presentation is to show the feasibility of performing a critical experiment with a B 4 C/Aluminum alloy neutron absorber plate. The motivation of this experiment is to provide integral data on modern neutron absorber product “Boralcan” by Rio Tinto. In 2020, used in about 20% of spent fuel pools in the US, and in casks for storage and transportation in the US and in Europe. The added value of this experiment: Neutron absorber plate modeling method verification: homogeneous or not, a lot of potential savings by relaxing boron loading credit limits. No available critical benchmark involving Boralcan, other boron-related experiments are relatively old. Nuclear data validation for B, C, and Al in the form of B 4 C in Al matrix.

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Sister Rod Destructive Examinations (FY23) Appendix F3: Uncertainty and Conservative Bias in the Cyclic Integrated Reversible-Bending Fatigue Test

The development and application of the Cyclic Integrated Reversible-Bending Fatigue Tester (CIRFT) has been documented over the past 10 years. The CIRFT system was developed in collaboration with the U.S. Nuclear Regulatory Commission (NRC) to address the concern that high-burnup fuel rod fatigue performance was degraded compared to cladding-only behavior. Fatigue data measured by CIRFT on high-burnup fuel rods were then used by the NRC to develop a fatigue response curve for pressurized water reactor fuel rods with Zircaloy-4 cladding in NUREG-2224. Subsequently, CIRFT has been used in the sister rod project to test whether reoriented hydrides associated with vacuum drying influenced the fatigue lifetime, to extend the fatigue testing database to include fuel rods with ZIRLO cladding, and to add to the experience on both Zircaloy-4 and M5 cladding. These data will be used as a reference for subsequent characterization of fuel rods removed from the high-burnup demonstration cask to better understand the effects of long-term dry storage, which can be thought of as a multiyear elevated temperature anneal. The objective of fatigue testing is to provide data that can be used to develop a best-estimate fatigue curve and a conservative fatigue design curve that accounts for uncertainty and can be compared with actual transportation conditions. The process for defining a design fatigue curve for commercial used fuel rods was developed by Oak Ridge National Laboratory (ORNL) in FY22. One issue noted in the fatigue evaluation was that the calculated combined uncertainty in the strain amplitude values determined from the measured data was large. It was proposed then to directly measure the uncertainty in the strain amplitude to either validate the calculated combined uncertainty or update the uncertainty based on the measurement data. Thus, the purpose of this appendix is to document the measured uncertainty in the strain amplitude data. In the process, it was determined that there has been a conservative bias in the calculated strain amplitude that is small enough to be within the measurement uncertainty. This observation is discussed herein, and a case is made to continue to include the conservative bias in the data.

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Predeployment progress of the Canister Deposition Field Demonstration

This report updates the high-level test plan for evaluating surface deposition on three commercial 32PTH2 spent nuclear fuel (SNF) canisters inside NUTECH Horizontal Modular Storage (NUHOMS) Advanced Horizontal Storage Modules (AHSMs) from Orano (formerly Transnuclear Inc.) and provides a summary of the surface sampling activities that have been conducted to date. The details contained in this report represent the best designs and approaches explored for testing as of this publication. Given the rapidly developing nature of this test program, some of these plans may change to accommodate new objectives or requirements. One goal of this testing is to collect defensible and detailed dust deposition measurements from the surface of dry storage canisters in a marine coastal environment to guide chloride-induced stress corrosion cracking (CISCC) research. Another goal is to provide data for the validation of computational fluid dynamics (CFD) based deposition modeling. To facilitate surface sampling, the otherwise highly prototypic dry storage systems will not contain SNF but rather will be electrically heated to mimic the decay heat and thermal hydraulic environment. Test and heater design is supported by detailed CFD modeling. Instrumentation throughout the canister, storage module, and environment will provide extensive information about the thermal-hydraulic behavior of horizontal dry cask storage systems. Manual sampling over a comprehensive portion of the canister surface at regular time intervals will offer detailed quantification and composition of the deposited particulates from a realistic storage environment. Discussions of a potential host site for the Canister Deposition Field Demonstration (CDFD) are ongoing. Until a host site is chosen, testing of key CDFD hardware components including the heater assemblies, power skid, and remote data acquisition system will continue. Functional testing of the finalized heater assemblies and test apparatus started this fiscal year. These initial heater tests have shown the assemblies are performing within design specifications. Staged surface sampling of a mockup of a canister outside the AHSM on a transfer skid was also performed. Refinements to the sampling procedures and techniques were captured from observation of these activities and lessons-learned debriefs. These updated sampling procedures and techniques are planned to be tested again in the field using the mockup in order to assure personnel are using the most accurate and repeatable methods possible prior to deployment for actual CDFD testing.

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Testing of Microchannels and Lab-Grown Stress Corrosion Cracks for Quantification of Aerosol Transmission

The formation of a stress corrosion crack (SCC) in the canister wall of a dry cask storage system (DCSS) has been identified as a potential issue for the long-term storage of spent nuclear fuel. The presence of an SCC in a storage system could represent a through-wall flow path from the canister interior to the environment. Modern, vertical DCSSs are of particular interest due to the commercial practice of using higher backfill pressures in the canister, up to approximately 800 kPa, compared to their horizontal counterparts. This pressure differential offers a relatively high driving potential for blowdown of any particulates that might be present in the canister. In this study, the rates of gas flow and aerosol transmission of a spent fuel surrogate through an engineered microchannel with dimensions representative of an SCC were evaluated experimentally using coupled mass flow and aerosol analyzers. The microchannel was formed by mating two gage blocks with a linearly tapering slot orifice nominally 13 μm (0.005 in.) tall on the upstream side and 25 μm (0.0010 in.) tall on the downstream side. The orifice is 12.7 mm (0.500 in.) wide by 8.86 mm (0.349 in.) long (flow length). Surrogate aerosols of cerium oxide, CeO 2 , were seeded and mixed with either helium or air inside a pressurized tank. The aerosol characteristics were measured immediately upstream and downstream of the simulated SCC at elevated and ambient pressures, respectively. These data sets are intended to add to previous testing that characterized SCCs under well-controlled boundary conditions through the inclusion of testing improvements that establish initial conditions in a more consistent way. While the engineered microchannel has dimensions similar to actual SCCs, it does not reproduce the tortuous path the aerosol laden flow would have to traverse for eventual transmission. SCCs can be rapidly grown in a laboratory setting given the right conditions, and initial characterization and clean-flow testing has begun on lab grown crack samples provided to Sandia National Laboratories (SNL). Many such samples are required to produce statistically relevant transmission results, and SNL is developing a procedure to produce samples in welded steel plates. These ongoing testing efforts are focused on understanding the evolution in both size and quantity of a hypothetical release of aerosolized spent fuel particles from failed fuel to the canister interior and ultimately through an SCC.

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Code of Record: DOE Standard Canister (DOESC)

The United States Department of Energy (DOE) Spent Nuclear Fuel (SNF) Packaging Demonstration seeks to develop and demonstrate the designs, technology, processes, and regulatory framework for packaging DOE SNF for road-ready dry storage (RRDS); and establish the processes that will be used in a future production facility. The Packaging Demonstration will utilize the DOE Standard Canister (DOESC) for packaging select DOE-managed SNF types for interim storage, transportation and disposal as part of RRDS. Placing DOE-managed SNF into RRDS is part of the strategic framework for SNF on the Idaho National Laboratory (INL) site. To comply with DOE, INL and Nuclear Regulatory Commission (NRC) requirements, this Code of Record establishes the American Society of Mechanical Engineers (ASME) Boiler and Pressure Vessel Code (BPVC), Section III, Division 3 as the Code that will govern DOESC and internal support structure constructioni, with certain clarifications. This Code of Record establishes a rationale for proceeding without construction certification of the DOESC (i.e., “N-stamping) and the extent to which a Registered Professional Engineer is required for the DOE Spent Fuel Packaging Demonstration. Given the (i) standard industry practice to pursue independent licensure of commercial storage casks and transportation packages by the NRC in lieu of ASME certification and (ii) guidance provided by 10 CFR 830, DOESC construction activities need not be certified (i.e., “stamped”) to the ASME BPVC. However, additional quality assurance requirements will apply as outlined in this Code of Record.

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Preliminary Simulations of Commercial Drying Cycles Using the Advanced Drying Cycle Simulator

The purpose of this report is to document updates on the apparatus to simulate commercial vacuum drying procedures at the Nuclear Energy Work Complex at Sandia National Laboratories. Validation of the extent of water removal in a dry spent nuclear fuel storage system based on drying procedures used at nuclear power plants is needed to close existing technical gaps. Operational conditions leading to incomplete drying may have potential impacts on the fuel, cladding, and other components in the system during subsequent storage and disposal. A general lack of data suitable for model validation of commercial nuclear canister drying processes necessitates well-designed investigations of drying process efficacy and water retention. Scaled tests that incorporate relevant physics and well-controlled boundary conditions are essential to provide insight and guidance to the simulation of prototypic systems undergoing drying processes. This report documents fiscal year 2023 (FY23) updates on the Advanced Drying Cycle Simulator (ADCS). This apparatus was built to simulate commercial drying procedures and quantify the amount of residual water remaining in a pressurized water reactor (PWR) fuel assembly after drying. The ADCS was constructed with a prototypic 17×17 PWR fuel skeleton and waterproof heater rods to simulate decay heat. These waterproof heaters are the next generation design to heater rods developed and tested at Sandia National Laboratories in FY20. In FY23, a series of four simulated commercial drying tests was completed. This report presents the temperature and pressure histories of the drying tests as well as axial temperature profiles that can be compared to data from the Electric Power Research Institute (EPRI) High Burnup Demonstration TN-32B cask. Water content measurements and dew point calculations from a Hiden Analytical HPR-30 mass spectrometer are also presented in this report. Due to familiarization with this first-of-a-kind system, refinements to equipment calibration and test procedures have been identified to better match commercial drying cycles for future simulated tests. However, the presented data demonstrate the successful construction and operation of a viable research platform for quantifying residual water content closely approaching that expected in dry storage canisters during commercial drying procedures.

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Final Seismic Shake Table Test Plan

The Spent Fuel Waste Disposition (SFWD) program is planning to conduct a full-scale seismic shake table test on the dry storage systems of spent nuclear fuel (SNF) to close the gap related to seismic loads on fuel assemblies in dry storage systems. This test will allow for quantifying the strains and accelerations on surrogate fuel assembly hardware and cladding during earthquakes of different magnitudes and frequency content. Full-scale testing is needed because a dry storage system is a complex and highly nonlinear system making it hard to predict (model) the responses to seismic excitations. The non-linearity arises from the multiple spatial gaps in the system – between fuel rods and the basket, between the basket and dry storage canister, between the dry storage canister and the storage cask (overpack), and ventilation gaps. The non-linearities pose significant limitations on the value of tests with scaled systems.

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Characterization of Lab-Grown Cracks for Aerosol Transmission Testing

Motivation: Determine the length and opening of two lab-grown cracks, designated as LT-14 and LT-28, representative of stress corrosion cracks in spent nuclear fuel dry storage casks to supplement future testing of gas and aerosol transport. Problem: The extreme aspect ratio of the crack length to opening requires that imaging occurs in stages with the results merged before final analysis. Method: High magnification (1500x) optical images of both sides of the two plates were acquired. 20x stitched images with LSCM were acquired, fully stitched along the length, and leveled with newly developed PLATES Method in MATLAB®. Conclusion for LT-14: Side 1 is 47.25 mm long and has 366 separate crack features with an average length of 23.50 µm and an average opening of 8.27 µm. Side 2 is 69.44 mm long and has 550 separate crack features with an average length of 81.63 µm and an average opening of 67.70 µm. Conclusion for LT-28: Side 1 is 71.95 mm long and has 1,127 separate crack features with an average length of 42.27 µm and an average opening of 10.31 µm. Side 2 is 74.88 mm long and has 520 separate crack features with an average length of 98.13 µm and an average opening of 14.99 µm. The adjacent crack on side 1 is 18.95 mm long and has 37 separate crack features with an average length of 17.46 µm and an average opening of 10.42 µm. The adjacent crack on side 2 is 26.40 mm long and has 55 separate crack features with an average length of 87.26 µm and an average opening of 48.29 µm. Each adjacent crack is approximately 26 mm from the main crack.

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