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All sourcesNASA NTRSDOE OSTI
NASA NTRS2012

Spectroscopic Characterization of Mineralogy Across Vesta: Evidence of Different Lithologies

The average spectrum of Vesta, obtained by VIR in the range 0.25-5.1 microns, shows clear evidence of absorption bands due to pyroxenes and thermal emissions beyond 3.5 11m. Vesta shows considerable variability across its surface in terms of spectral reflectance and emission, band depths, bands widths and bands centers, reflecting a complex geological history. Vesta's average spectrum and inferred mineralogy resemble those of howardite meteorites. On a regional scale, significant deviations are seen: the south polar 500km Rheasilvia impact crater has a higher diogenitic component, and equatorial regions show a higher eucritic component. This lithologic distribution, with a concentration of Mg-pyroxenes in the Rheasilvia area, reinforces the hypothesis of a deeper diogenitic crust excavated by the impact that formed the Rheasilvia crater, and an upper eucritic crust, whose remnants are seen in the equatorial region. This scenario has implications for Vesta differentiation, consistent with magma ocean models. However, serial magmatism models could also have concentrated pyroxene cumulates in plutons emplaced within the lower crust,

De Sanotis, M. C.↗
NASA NTRS2013

The Use of the Deep Convective Cloud Technique (DCCT) to Monitor On-Orbit Performance of the Geostationary Lightning Mapper (GLM): Use of Lightning Imaging Sensor (LIS) Data as Proxy

The Geostationary Lightning Mapper (GLM) on the next generation Geostationary Operational Environmental Satellite-R (GOES-R) will not have onboard calibration capability to monitor its performance. The Lightning Imaging Sensor (LIS) onboard the Tropical Rainfall Measuring Mission (TRMM) satellite has been providing observations of total lightning over the Earth's Tropics since 1997. The GLM design is based on LIS heritage, making it a good proxy dataset. This study examines the performance of LIS throughout its time in orbit. This was accomplished through application of the Deep Convective Cloud Technique (DCCT) (Doelling et al., 2004) to LIS background pixel radiance data. The DCCT identifies deep convective clouds by their cold Infrared (IR) brightness temperatures and using them as invariant targets in the solar reflective portion of the solar spectrum. The GLM and LIS operate in the near-IR at a wavelength of 777.4 nm. In the present study the IR data is obtained from the Visible Infrared Sensor (VIRS) which is collocated with LIS onboard the Tropical Rainfall Measuring Mission (TRMM) satellite. The DCCT is applied to LIS observations for July and August of each year from 1998-2010. The resulting distributions of LIS background DCC pixel radiance for each July August are very similar, indicating stable performance. The mean radiance of the DCCT analysis does not show a long term trend and the maximum deviation of the July August mean radiance for each year is within 0.7% of the overall mean. These results demonstrate that there has been no discernible change in LIS performance throughout its lifetime. A similar approach will used for monitoring the performance of GLM, with cold clouds identified using IR data from the Advanced Baseline Imager (ABI) which will also be located on GOES-R. Since GLM is based on LIS design heritage, the LIS results indicate that GLM should also experience stable performance over its lifetime.

Buechler, Dennis E.↗
NASA NTRS2013

Mineralogical Composition of the Different Types of Bright Deposits on Vesta

VIR-MS, Dawn's Visible and Infrared Mapping Spectrometer, obtained hyperspectral images of a wide part of Vesta's surface at a variety of spatial resolutions [1]. Vesta spectra are similar to those of the howardite-eucrite-diogenite (HED) meteorites. Moreover, they are characterized by the two iron-bearing pyroxene bands at 0.9 (band I) and 1.9 microns (band II). Vesta surface's is dominated by eucrite/howardite with some diogenitic regions situated in the southern hemisphere near the Rheasilvia basin [2]. The surface is heavily craterized and impacts can expose fresh material, thus generating the Bright Material Deposits (BMD) observed within and surrounding certain craters. BMD can be classified into six different types based on their morphological characteristics: Crater Wall/Scarp Material (CWM), Radial Material (RM), Slope Material (SM), Patchy Material (PM), Spot Material (SpM) and Diffuse Plains Material (DPM) [3]. The most widespread BMD are CWM, SM and RM. CWM, SM, RM originate from impacts. CWM is situated on the edge of the craters. Mass wasting from the crater walls and generates the SM, while RM is associated with the ejecta of the craters [4]. BMD are characterized by albedo greater than that of the vestan average, 0.38 [5]. Therefore the different types of deposits present distinct levels of reflectance respect to the Surrounding Regions (SR), in particular: the CWM and SM is approx.40% brighter, the RM is approx.30- 40% brighter; the SpM is about 20-25% brighter and the PM is about 20% brighter. Near the edge of the Rheasilvia basin it is possible to find some extremely bright areas ~80% brighter than the vestan average [6].

Zambon, F.↗
NASA NTRS2013

Mesosiderites on Vesta: A Hyperspectral VIS-NIR Investigation

The discussion about the mesosiderite origin is an open issue since several years. Mesosiderites are mixtures of silicate mineral fragments or clasts, embedded in a FeNi metal matrix. Silicates are very similar in mineralogy and texture to howardites [1]. This led some scientists to conclude that mesosiderites could come from the same parent parent asteroid of the howardite, eucrite and diogenite (HED) meteorites [2, 3]. Other studies found a number of differences between HEDs and mesosiderite silicates that could be explained only by separate parent asteroids [4]. Recently, high precision oxygen isotope measurements of m esosiderites silicate fraction were found to be isotopically identical to the HEDs, requiring common parent body, i.e. 4 Vesta [5]. Another important element in favor of a common origin was given by the identification of a centimeter-sized mesosiderite clast in a howardite (Dar al Gani 779): a metal-rich inclusion with fragments of olivine, anorthite, and orthopyroxene plus minor amounts of chromite, tridymite, and troilite [6]. The Dawn mission with its instruments, the Infrared Mapping Spectrometer (VIR) [7], the Framing Camera [8] and the Gamma-Ray and Neutron Detector (GRaND) [9] confirmed that Vesta has a composition fully compatible with HED meteorites [10]. We investigate here the possibility to discern mesosiderite rich locations on the surface of Vesta by means of hyperspectral IR images.

Palomba, E.↗
NASA NTRS2013

Preliminary Iron Distribution on Vesta

The distribution of iron on the surface of the asteroid Vesta was investigated using Dawn's Gamma Ray and Neutron Detector (GRaND) [1,2]. Iron varies predictably with rock type for the howardite, eucrite, and diogenite (HED) meteorites, thought to be representative of Vesta. The abundance of Fe in howardites ranges from about 12 to 15 wt.%. Basaltic eucrites have the highest abundance, whereas, lower crustal and upper mantle materials (cumulate eucrites and diogenites) have the lowest, and howardites are intermediate [3]. We have completed a mapping study of 7.6 MeV gamma rays produced by neutron capture by Fe as measured by the bismuth germanate (BGO) detector of GRaND [1]. The procedures to determine Fe counting rates are presented in detail here, along with a preliminary distribution map, constituting the necessary initial step to quantification of Fe abundances. We find that the global distribution of Fe counting rates is generally consistent with independent mineralogical and compositional inferences obtained by other instruments on Dawn such as measurements of pyroxene absorption bands by the Visual and Infrared Spectrometer (VIR) [4] and Framing Camera (FC) [5] and neutron absorption measurements by GRaND [6].

Mittlefehldt, David W.↗
NASA NTRS2013

Neutron Absorption Measurements Constrain Eucrite-Diogenite Mixing in Vesta's Regolith

The NASA Dawn Mission s Gamma Ray and Neutron Detector (GRaND) [1] acquired mapping data during 5 months in a polar, low altitude mapping orbit (LAMO) with approx.460-km mean radius around main-belt asteroid Vesta (264-km mean radius) [2]. Neutrons and gamma rays are produced by galactic cosmic ray interactions and by the decay of natural radioelements (K, Th, U), providing information about the elemental composition of Vesta s regolith to depths of a few decimeters beneath the surface. From the data acquired in LAMO, maps of vestan neutron and gamma ray signatures were determined with a spatial resolution of approx.300 km full-width-at-half-maximum (FWHM), comparable in scale to the Rheasilvia impact basin (approx.500 km diameter). The data from Vesta encounter are available from the NASA Planetary Data System. Based on an analysis of gamma-ray spectra, Vesta s global-average regolith composition was found to be consistent with the Howardite, Eucrite, and Diogenite (HED) meteorites, reinforcing the HED-Vesta connection [2-7]. Further, an analysis of epithermal neutrons revealed variations in the abundance of hydrogen on Vesta s surface, reaching values up to 400 micro-g/g [2]. The association of high concentrations of hydrogen with equatorial, low-albedo surface regions indicated exogenic delivery of hydrogen by the infall of carbonaceous chondrite (CC) materials. This finding was buttressed by the presence of minimally-altered CC clasts in howardites, with inferred bulk hydrogen abundances similar to that found by GRaND, and by studies using data from Dawn s Framing Camera (FC) and VIR instruments [8-10]. In addition, from an analysis of neutron absorption, spatial-variations in the abundance of elements other than hydrogen were detected [2].

Prettyman, T. H.↗
NASA NTRS2013

Investigating the Use of Deep Convective Clouds (DCCT) to Monitor On-orbit Performance of the Geostationary Lightning Mapper (GLM) using Lightning Imaging Sensor (LIS) Measurements

There is a need to monitor the on-orbit performance of the Geostationary Lightning Mapper (GLM) on the Geostationary Operational Environmental Satellite R (GOES-R) for changes in instrument calibration that will affect GLM's lightning detection efficiency. GLM has no onboard calibration so GLM background radiance observations (available every 2.5 min) of Deep Convective Clouds (DCCs) are investigated as invariant targets to monitor GLM performance. Observations from the Lightning Imaging Sensor (LIS) and the Visible and Infrared Scanner (VIRS) onboard the Tropical Rainfall Measuring Mission (TRMM) satellite are used as proxy datasets for GLM and ABI 11 m measurements.

Buechler, Dennis E.↗
NASA NTRS2013

Thermal Analysis of Unusual Local-scale Features on the Surface of Vesta

At 525 km in mean diameter, Vesta is the second-most massive object in the main asteroid belt of our Solar System. At all scales, pyroxene absorptions are the most prominent spectral features on Vesta and overall, Vesta mineralogy indicates a complex magmatic evolution that led to a differentiated crust and mantle [1]. The thermal behavior of areas of unusual albedo seen on the surface at the local scale can be related to physical properties that can provide information about the origin of those materials. Dawn's Visible and Infrared Mapping Spectrometer (VIR) [2] hyperspectral images are routinely used, by means of temperature-retrieval algorithms, to compute surface temperatures along with spectral emissivities. Here we present temperature maps of several local-scale features of Vesta that were observed by Dawn under different illumination conditions and different local solar times.

Tosi, F.↗
NASA NTRS2014

Global View of the Bright Material on Vesta

At 525 km in mean diameter, Vesta is the second-most massive and one of the brightest asteroids of the main-belt. Here we give a global view of the bright material (BM) units on Vesta. We classified the BMs according to the normal visual albedo. The global albedo map of Vesta allows to be divided the surface into three principal types of terrains: bright regions, dark regions and intermediate regions. The distribution of bright regions is not uniform. The mid-southern latitudes contain the most bright areas, while the northern hemisphere is poor in bright regions. The analysis of the spectral parameters and the normal visual albedo show a dependence between albedo and the strength (depth) of ferrous iron absorption bands, strong bands correspond with high albedo units. Vesta's average albedo is 0.38, but there are bright material whose albedo can exceed 0.50. Only the E-Type asteroids have albedos comparable to those of the BMs on Vesta. The Dawn mission observed a large fraction of Vesta's surface at high spatial resolution, allowing a detailed study of the morphology and mineralogy of it. In particular, reflectance spectra provided by the Visible and InfraRed spectrometer (VIR), confirmed that Vesta's mineralogy is dominated by pyroxenes. All Vesta spectra show two strong absorption bands at approx 0.9 and 1.9 micron, typical of the pyroxenes and associated with the howardite, eucrite and diogenite (HED) meteorites.

Zambon, F.↗
NASA NTRS2014

Composition of Rheasilvia Basin on Asteroid Vesta

The focus of the present study is the compositional analysis of small-scale surface features within the Rheasil-Aa basin on asteroid Vesta. We are using data acquired by the Visible and InfraRed mapping Spectrometer (VIR) on the Dawn mission. Nominal spatial resolution of the data set considered in this study is 70m/px. The portion of Rheasil-Aa basin below 65degS has a howarditic composition, with the higher concentration of diogenitic versus eucritic material in the region between 45deg and 225degE-lon. However, there are several locations, such as craters Tarpeia and Severina and Parentatio Rupes, with lithologic characteristics different from the surroundings regions. Tarpeia crater has a eucritic patch in the west side of the crater, the bottom part ofthe wall and part of the floor. Severina, located in a region of Mg-rich pyroxene, has some diogenitic units on the walls of the crater. Also the Parentatio Rupes has an ob-AOUS diogenitic unit. These units extend for 10-20km, and their location, especially in the case of the two craters, suggests they formed before the cratering events and also before the Rheasil-Aa impact event. The origin of these units is still unclear; however, their characteristics and locations suggests heterogeneity in the composition of the ancient Vestan crust in this particular location of the surface.

Ammannito, Eleonora↗
NASA NTRS2014

Constraints on Vesta's Interior Structure Using Gravity and Shape Models from the Dawn Mission

We use the shape and gravity field of Vesta determined from observations of the Dawn spacecraft to place constraints on the asteroid's interior structure. We compute a three-layer interior structure model by minimizing the power of the residual gravity anomaly. The densities of the mantle and crust are based on constraints derived from the Howardite-Eucrite-Diogenite (HED) meteorites. Vesta's present-day shape is not in hydrostatic equilibrium. The Rheasilvia and Veneneia impact basins have a large effect on Vesta's shape and are the main source of deviation from hydrostatic shape. Constraining a pre-giant-impact rotation rate and orientation of the spin axis from an ellipsoidal fit to the parts of Vesta unaffected by the giant impacts, and using the theory of figure, we can constrain the shape of the core. Our solution for Vesta's crust-mantle interface reveals a belt of thick crust around Rheasilvia and Veneneia. The thinnest crust is in the floor of the two basins and in the Vestalia Terra region. Our solution does not reveal an uplift of the crust-mantle boundary to the surface in the largest basins. This, together with the lack of olivine detected by the Visible and Infrared Spectrometer (VIR) data in Rheasilvia and Veneneia, indicates that Vesta's presumed olivine mantle was either not brought to the surface by these large impacts or was covered by ejecta from subsequent impacts.

Interiors↗
DOE OSTI2025

An Atomistic Study of Reactivity in Solid-State Electrolyte Interphase Formation for Li/Li7P3S11

Lithium metal batteries offer superior volumetric and gravimetric specific capacities compared to those based on traditional graphite anodes. Although advancements in solid-state electrolytes address safety concerns, challenges remain, particularly regarding interphase formation in lithium metal anodes. This work presents a computational framework based on high-throughput first-principles density functional theory and machine-learning interatomic potentials (MLIPs) including automated iterative, active learning to enable robust computational exploration of interphase formation between lithium metal anodes and an inorganic solid-state electrolyte. As a demonstration, we apply the framework to a Li/Li7P3S11 interface and find that it accurately identifies the experimentally observed, thermodynamically stable interphase products as well as their overall spatial arrangement within a heterogeneous, amorphous layered structure, with Li2S domains of nanocrystallinity. Our simulations show two stages, a fast and slow diffusion reaction regime, that corroborate the relative phase formation rate of Li x P, Li2S, and Li3P. Using the Onsager transport theory, we capture time-dependent ionic diffusion within the reacting interface, including cross-correlation effects. We found that cross-correlation effects between Li-P and P-S ionic motion significantly influence P-ion diffusion, making it highly sensitive to the local environment and potentially leading to "kinetic trapping" of Li-P phases. The passivation of the interface is shown as the ionic fluxes all approach zero, effectively halting interphase growth.

Diffusion↗
DOE OSTI2022

Observation of a phase transition within the domain walls of ferromagnetic Co3Sn2S2

Abstract The ferromagnetic phase of Co 3 Sn 2 S 2 is widely considered to be a topological Weyl semimetal, with evidence for momentum-space monopoles of Berry curvature from transport and spectroscopic probes. As the bandstructure is highly sensitive to the magnetic order, attention has focused on anomalies in magnetization, susceptibility and transport measurements that are seen well below the Curie temperature, leading to speculation that a “hidden” phase coexists with ferromagnetism. Here we report spatially-resolved measurements by Kerr effect microscopy that identify this phase. We find that the anomalies coincide with a deep minimum in domain wall (DW) mobility, indicating a crossover between two regimes of DW propagation. We demonstrate that this crossover is a manifestation of a 2D phase transition that occurs within the DW, in which the magnetization texture changes from continuous rotation to unidirectional variation. We propose that the existence of this 2D transition deep within the ferromagnetic state of the bulk is a consequence of a giant quality factor for magnetocrystalline anisotropy unique to this compound. This work broadens the horizon of the conventional binary classification of DWs into Bloch and Néel walls, and suggests new strategies for manipulation of domain walls and their role in electron and spin transport.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Ion correlations explain kinetic selectivity in diffusion-limited solid-state synthesis reactions

Establishing viable solid-state synthesis pathways for novel inorganic materials remains a major challenge in materials science. Previous pathway design methods using pairwise reaction approaches have navigated the thermodynamic landscape with first-principles data but lack kinetic information, limiting their effectiveness. This gap leads to suboptimal precursor selection and predictions, especially for reactions forming competing phases with similar formation energies, where ion diffusion is a critical influence. Here we demonstrate an inorganic synthesis framework by incorporating machine learning-derived transport properties through ‘liquid-like’ product layers into a thermodynamic cellular reaction model. In the Ba–Ti–O system, known for its competitive polymorphism, we obtain accurate predictions of phase formation with varying BaO:TiO2 ratios as a function of time and temperature. We find that diffusion–thermodynamics interplay governs phase compositions, with cross-ion transport coefficients critical for predicting diffusion-limited selectivity. This work bridges length scales and timescales by integrating solid-state reaction kinetics with first-principles thermodynamics and spatial reactivity.

Atomistic models↗
DOE OSTI2020

Superdiffusive transport of energy in one-dimensional metals

Metals in one spatial dimension are described at the lowest energy scales by the Luttinger liquid theory. It is well understood that this free theory, and even interacting integrable models, can support ballistic transport of conserved quantities including energy. In contrast, realistic one-dimensional metals, even without disorder, contain integrability-breaking interactions that are expected to lead to thermalization and conventional diffusive linear response. We argue that the expansion of energy when such a nonintegrable Luttinger liquid is locally heated above its ground state shows superdiffusive behavior (i.e., spreading of energy that is intermediate between diffusion and ballistic propagation), by combining an analytical anomalous diffusion model with numerical matrix-product–state calculations on a specific perturbed spinless fermion chain. Different metals will have different scaling exponents and shapes in their energy spreading, but the superdiffusive behavior is stable and should be visible in time-resolved experiments.

Bulchandani, Vir B.↗
DOE OSTI2021

Let it rip: The mechanics of self-bisection in asexual planarians determines their population reproductive strategies

Asexual freshwater planarians reproduce by transverse bisection (binary fission) into two pieces. This process produces a head and a tail, which fully regenerate within 1-2 weeks. How planarians split into two offspring - using only their musculature and substrate traction – is a challenging biomechanics problem. We found that three different species, Dugesia japonica, Girardia tigrina and Schmidtea mediterranea, have evolved three different mechanical solutions to self-bisect. Using time lapse imaging of the fission process, we quantitatively characterize the main steps of division in the three species and extract the distinct and shared key features. Across the three species, planarians actively alter their body shape, regulate substrate traction, and use their muscles to generate tensile stresses large enough to overcome the ultimate tensile strength of the tissue. Moreover, we show that how each planarian species divides dictates how resources are split among its offspring. This ultimately determines offspring survival and reproductive success. Furthermore, heterospecific differences in the mechanics of self-bisection of individual worms explain the observed differences in the population reproductive strategies of different planarian species.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

Hydrodynamics of quantum spin liquids

Quantum spin liquids are topological states of matter that arise in frustrated quantum magnets at low temperatures. At low energies, such states exhibit emergent gauge fields and fractionalized quasiparticles and can also possess enhanced global symmetries compared to their parent microscopic Hamiltonians. Here we study the consequences of this emergent gauge and symmetry structure for the hydrodynamics of quantum spin liquids. Specifically, we analyze two cases, the U(1) spin liquid with a Fermi surface and the SU(4)-symmetric “algebraic” spin liquid. We show that the emergent degrees of freedom in the spin liquid phase lead to a variety of additional hydrodynamic modes compared to the high-temperature paramagnetic phase. We identify a hydrodynamic regime for the internal U(1) gauge field common to both states, characterized by slow diffusion of the internal transverse photon.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Dynamics and transport in the boundary-driven dissipative Klein-Gordon chain

Motivated by experiments on chains of superconducting qubits, we consider the dynamics of a classical Klein-Gordon chain coupled to coherent driving and subject to dissipation solely at its boundaries. As the strength of the boundary driving is increased, this minimal classical model recovers the main features of the "dissipative phase transition" seen experimentally. Between the transmitting and non-transmitting regimes on either side of this transition (which support ballistic and diffusive energy transport respectively), we observe additional dynamical regimes of interest. These include a regime of superdiffusive energy transport at weaker driving strengths, together with a "dissipative breather crystal" regime at stronger driving strengths, which is characterized by emergent translation symmetry, ballistic energy transport, and coherent oscillations of a nonlinear normal mode. Here, we propose a non-local Lyapunov exponent as an experimentally measurable diagnostic of many-body chaos in this system, and more generally in open systems that are only coupled to an environment at their boundaries.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗