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At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Synthesis and characterization of the novel breathing pyrochlore compound Ba 3 ⁢Tm 2⁢ Zn 5⁢ O 11

In this study, a novel material from the rare-earth based breathing pyrochlore family, Ba 3 ⁢Tm 2 ⁢Zn 5 ⁢O 11 , was successfully synthesized. Powder x-ray diffraction and high-resolution powder neutron diffraction confirmed phase purity and the $F\bar4$3⁢𝑚 breathing pyrochlore crystal structure, while thermogravimetric analysis revealed incongruent melting behavior compared to its counterpart, Ba 3 ⁢Yb 2⁢ Zn 5⁢ O 11 . High-quality single crystals of Ba 3 ⁢Tm 2 ⁢Zn 5 ⁢O 11 were grown using the traveling solvent floating zone technique and assessed using Laue x-ray diffraction and single crystal x-ray diffraction. Further, thermodynamic characterization indicated paramagnetic behavior down to 0.05 K, and inelastic neutron scattering measurements identified distinct dispersionless crystal electric field energy bands, with the fitted crystal electric field model predicting a single-ion singlet ground state and an energy gap of ∼9 meV separating it from the first excited (singlet) state. Additional low-energy excitation studies on single crystals revealed dispersionless bands at 0.8 and 1 meV. Computed phonon dispersions from first-principles calculations ruled out phonons as the origin of these modes, further illustrating the puzzling and unique properties of Ba 3 ⁢Tm⁢ 2 Zn 5 ⁢O 11 .

36 MATERIALS SCIENCE↗
DOE OSTI2022

1 GW peak power and 100 J pulsed operation of a diode-pumped Tm:YLF laser

We report on the generation of high energy, high power pulses in a tabletop diode-pumped Tm:YLF-based laser system, which delivers amplified pulse energies up to 108 J, as well as GW peak power performance when seeded with nanosecond duration pulses. Furthermore, the high power and efficiency capabilities of operating Tm:YLF in the multi-pulse extraction (MPE) regime were explored by seeding the experimental setup with a multi-kHz burst of pulses exhibiting a low individual pulse fluence, resulting in a 3.6 kW average power train of multi-joule-level pulses with an optical-to-optical efficiency of 19%.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

Demonstration of a compact, multi-joule, diode-pumped Tm:YLF laser

We report the demonstration of a diode-pumped Tm:YLF laser operating at 1.88 µm that produces pulse energies up to 3.88 J in 20 ns. The compact system consists of a Q-switched cavity-dumped oscillator generating 18 mJ pulses, which are then amplified in a 4-pass power amplifier. Energies up to 38.1 J were obtained with long-pulse amplifier operation. These results illustrate the high energy storage and extraction capabilities of diode-pumped Tm:YLF, opening the path to high peak and average power mid-infrared solid-state lasers

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Demonstration of a 1 TW peak power, joule-level ultrashort Tm:YLF laser

Here we report on the demonstration of a diode-pumped, Tm:YLF-based, chirped pulse amplification laser system operating at λ ≈ 1.9 µm that produces amplified pulse energies exceeding 1.5 J using a single 8-pass power amplifier. The amplified pulses are subsequently compressed to sub-300 fs durations by a diffraction grating pair, producing record >1 TW peak power pulses. To the best of our knowledge, this is the highest peak power demonstrated for any solid-state, near-2 µm laser architecture and illustrates the potential of Tm:YLF for the next generation of high-power, diode-pumped ultrashort lasers.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Xyce TM XDM Netlist Translator User Guide (V 2.0)

This manual describes the installation and use of the XyCe TM XDM Net list Translator. XDM simplifies the translation of netlists generated by commercial circuit simulator tools into Xyce-compatible netlists. XDM currently supports translation from PSpice and HSPICE netlists into Xyce TM netlists.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2022

Potential safety impacts associated with production of gaseous PuF 6 due to reactions between 3013-compliant PuO 2 with Novec TM 1230 at temperature

A part of the NNSA/SRNS Surplus Plutonium Disposition (SPD) project is a planned expansion of an existing facility with capabilities to handle, process, package, and characterize large amounts of plutonium oxide materials for permanent disposition at WIPP. The facility design for this future processing capability will include glovebox operations, HEPA filters, and exhaust/ventilation systems. An NNSA review of the facility support systems included comments on the potential residual reactivity of previously-stabilized PuO 2 , and on the possibility of chemical interactions between stabilized PuO 2 and a new fire suppressant (Novec TM 1230), a replacement for chlorinated/brominated compounds such as HALON TM , to be employed in the event of a room/glovebox fire where PuO 2 will be processed.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2024

Advancements in Multiphysics Microdepletion Analysis of an eVinci TM -like Microreactor Leveraging OpenMC-CRAB Workflow

Nuclear microreactors (MRs) are a class of nuclear reactor technology, characterized by reduced dimensions, modular design, and reduced power output in contrast to conventional Light Water Reactors (LWRs). MRs are proposed for supplying electricity and eventual process heat to remote locations, such as military installations and disaster-affected areas. Current research work sponsored by the US Department of Energy Microreactor Program (MRP) is devoted to the development of novel modeling and simulation tools to better support MR vendors and regulatory bodies. Notably, the NRC is projected to utilize the CRAB multiphysics software driver for executing both design and beyond-design-basis accident analyses. Furthermore, the NRC has been utilizing the MELCOR code to calculate mechanistic source terms during accidents. Since MELCOR relies on isotopic inventory and reactor temperature/power profiles under accident conditions, which theoretically can be derived from CRAB, the goal is to establish a comprehensive CRAB-MELCOR computational framework. Past work was focused on testing and demonstrating CRAB's capability to generate results that can be used to inform mechanistic source term calculations in MELCOR. In particular, a computational workflow leveraging OpenMC-generated microscopic cross sections and CRAB was first applied to perform multiphysics microscopic depletion calculation followed by an accident scenario for a stylized microreactor problem. In fiscal year 2024, the research work has been focused on applying the OpenMC-CRAB workflow, which was first tested in fiscal year 2023, to a realistic 3D heat-pipe cooled MR problem representative of the eVinci TM design. The latter computational problem was developed with inputs from WEC to conserve selected neutronic and thermal characteristics of the eVinci TM design without releasing proprietary data. The results of this simulation, encompassing isotopic inventory, power density distribution, and kinetic parameters, will inform both MELCOR and the WEC-developed FATE code for mechanistic source terms calculations. The results from the two codes will then be compared for code verification purposes. This report contains the design characteristics of the realist heat pipe cooled microreactor developed as a use-case for the verification exercise, and the current results for the multiphysics microscopic depletion performed with the OpenMC-CRAB workflow. The results include eigenvalue as a function of time, power distribution at EOL, in addition to nuclides inventory's time evolution and spatial distribution. Finally, we report improvements to the workflow efficiency achieved through a collaboration with the NEAMS programs. Through this collaborative effort, we were able to strongly decrease the computational time for the multiphysics microdepletion calculation (i.e., from 17.4 hours to 5.7 hours on 280 processors) in addition to simplifying the interface to generate isotopics spatial distribution utilizable by FATE and MELCOR. Future work, including the improvement of the current microscopic cross-sections' library and the simulation of an accident scenario at EOL, is also discussed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2020

Low-Energy Electron Elastic Total Cross Sections for Ho, Er, Tm, Yb, Lu, and Hf Atoms

The robust Regge-pole methodology wherein is fully embedded the essential electron-electron correlation effects and the vital core polarization interaction has been used to explore negative ion formation in the large lanthanide Ho, Er, Tm, Yb, Lu, and Hf atoms through the electron elastic total cross sections (TCSs) calculations. These TCSs are characterized generally by dramatically sharp resonances manifesting ground, metastable, and excited negative ion formation during the collisions, Ramsauer-Townsend minima, and shape resonances. The novelty and generality of the Regge-pole approach is in the extraction of the negative ion binding energies (BEs) of complex heavy systems from the calculated electron TCSs. The extracted anionic BEs from the ground state TCSs for Ho, Er, Tm, Yb, Lu, and Hf atoms are 3.51 eV, 3.53 eV, 3.36 eV, 3.49 eV, 4.09 eV and 1.68 eV, respectively. The TCSs are presented and the extracted from the ground; metastable and excited anionic states BEs are compared with the available measured and/or calculated electron affinities. We conclude with a remark on the existing inconsistencies in the meaning of the electron affinity among the various measurements and/or calculations in the investigated atoms and make a recommendation to resolve the ambiguity.

Felfli, Zineb↗
NASA NTRS1984

CCRS proposal for evaluating LANDSAT-4 MSS and TM data

The measurement of registration errors in LANDSAT MSS data is discussed as well as the development of a revised algorithm for the radiometric calibration of TM data and the production of a geocoded TM image.

Strome, W. M.↗
NASA NTRS1984

TM Digital Image Products for Applications

LANDSAT-4 Thematic Mapper (TM) digital image products recorded onto computer compatible tapes (CCTs), which were available for internal research purposes prior to August, 1983, are reviewed. The SCROUNGE image processing system at Goddard Space Flight Centr generated in tape formats: (1) raw band-sequential data (CCT-BT), generally used for internal transportation of digital data from one ground processing system to another; (2) calibrated data (CCT-AT), useful for reseachers doing radiometric characterization; and (3) geometrically resampled data (CCT-PT), the final product. The formats represent different steps in the process of producing fully-corrected TM data. The CCT-BT images are re-sequenced from telemetry format to image format, but are uncorrected radiometrically and geometrically. The CCT-AT images had data from two faulty data channels replaced and all data radiometrically calibrated. The CCT-PT images were resampled by cubic convolution procedures to provide a geometrically corrected image using satellite ephemeris and altitude data and scan-mirror correction data. The final product, the CCT-PT, is the one to which all of the radiometric and geometric corrections were applied.

Barker, J. L.↗
NASA NTRS1984

Calibration of TM data from ground-based measurements

Methods of calibrating Thematic Mapper (TM) data by the use of ground based measurements are presented. Applications of the TM remote sensing data are discussed in addition to the ground truth measurement equipment and techniques.

Rasool, S. I.↗
NASA NTRS1984

Investigation of TM Band-to-band Registration Using the JSC Registration Processor

The JSC registration processor performs scene-to-scene (or band-to-band) correlation based on edge images. The edge images are derived from a percentage of the edge pixels calculated from the raw scene data, excluding clouds and other extraneous data in the scene. Correlations are performed on patches (blocks) of the edge images, and the correlation peak location in each patch is estimated iteratively to fractional pixel location accuracy. Peak offset locations from all patches over the scene are then considered together, and a variety of tests are made to weed out outliers and other inconsistencies before a distortion model is assumed. Thus, the correlation peak offset locations in each patch indicate quantitatively how well the two TM bands register to each other over that patch of scene data. The average of these offsets indicate the overall accuracies of the band-to-band registration. The registration processor was also used to register one acquisition to another acquisition of multitemporal TM data acquired over the same ground track. Band 4 images from both acquisitions were correlated and an rms error of a fraction of a pixel was routinely obtained.

Yao, S. S.↗
NASA NTRS1984

Relative Accuracy Assessment of LANDSAT-4 MSS and TM Data for Level 1 Land Cover Inventory

Digital data for the Washington, D.C. scene from the LANDSAT-4 Multispectral Scanner (MSS) and the LANDSAT-4 Thematic Mapper (TM) are compared. Classification success for the TM and MSS data sets was determined by a per pixel comparison with digitized ground verification data (GVD). These GVD were comprised of Level I land cover (developed, agriculture, forest, water, wetlands, and barren) for four USGS 7.5-minute topographic quadrangle maps. Classification accuracy was computed as an average value and for each cover type. Accuracy was expressed two ways: (1) as the percent correspondence with GVD (% correct) and (2) as the percent correspondence relative to both the GVD and LANDSAT classification schemes. Errors of omission and commission associated with the LANDSAT classifications were also computed. Specific results are discussed.

Middleton, E. M.↗
NASA NTRS1984

TM digital image products for applications

Computer compatible tapes (CCTs) of LANDSAT 4 thematic mapper (TM) digital image products are compared and reviewed. The following tape formats are discussed: (1) raw band-sequential data (CCT-BT); (2) calibrated data (CCT-AT); and (3) geometrically resampled data (CCT-PT). Each format represents different steps in the process of producing fully corrected TM data. The CCT-BT images are uncorrected radiometrically or geometrically, CCT-AT data are radiometrically calibrated, and CCT-PT images are both radiometrically and geometrically corrected.

Barker, J. L.↗
NASA NTRS1984

Relative radiometric calibration of LANDSAT TM reflective bands

A common scientific methodology and terminology is outlined for characterizing the radiometry of both TM sensors. The magnitude of the most significant sources of radiometric variability are discussed and methods are recommended for achieving the exceptional potential inherent in the radiometric precision and accuracy of the TM sensors.

Barker, J. L.↗
NASA NTRS1984

Characterization of Landsat-4 MSS and TM digital image data

The launch of Landsat-4 in July 1982 represents a continuation in the remote sensing of earth resources. The 80-m spatial resolution provided by the Multispectral Scanner (MSS) on board the satellite is fine enough to resolve many natural features and land-use details in both rural and urban settings. The second sensor of the spacecraft, the Thematic Mapper (TM), introduces a new era of sensing with refined spatial resolution (30 m) and expanded spectral coverage (7 bands). This paper describes results from engineering studies of the characteristics of digital image data from the two Landsat-4 sensors. These studies form a part of the Landsat-4 Image Data Quality Analysis program (LIDQA). The image data were generally found to be of high quality and the TM provided several improvements over the MSS, in its spatial and spectral characteristics.

Malila, W. A.↗
NASA NTRS1985

TM Geometric Performance: Line to Line Displacement Analysis (LLDA)

An early acquired TM data frame (track 23, frame 35 of 22 August 1982) was used to assess the geometric performance of the LANDSAT-4 thematic mapper instrument. The developed method consists in determining the displacements of adjacent lines by locating the maximum of the correlation profile between the two lines. Then the line to line displacement is used to characterize the TM instrument in respect to: scan to scan jitter and image skew, scan profile non-linearity, along scan jitter, detector to detector displacement, and band to band displacement. To verify the quality of the reported performance parameters, some extracted geometric parameters were used to correct the original raw data. Comparison between P-tape data and results of reprocessed data shows no significant differences in an area of 1024 x 1024 pixels.

Fusco, L.↗
NASA NTRS1985

Analysis and Evaluation of the LANDSAT-4 MSS and TM Sensors and Ground Data Processing Systems: Early Results

The MSS and TM sensor performances were evaluated by studying both the sensors and the characteristics of the data. Information content analysis, image statistics, band-to-band registration, the presence of failed or failing detectors, and sensor resolution are discussed. The TM data were explored from the point of view of adequacy of the ground processing and improvements that could be made to compensate for sensor problems and deficiencies. Radiometric correction processing, compensation for a failed detector, and geometric correction processing are also considered.

Bernstein, R.↗