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At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Uranium and Nickel Partitioning in a Contaminated Riparian Wetland

Uranium (U) and nickel (Ni) released 50 years ago have been immobilized in the Tims Branch wetlands located on the Savannah River Site in the United States. Sediments were collected from seven locations to identify the factors responsible for this attenuation. Ni and U contents in the solids were significantly correlated, suggesting that depositional as opposed to chemical processes contributed to their spatial distribution. Based on sequential extractions, 63 ± 16% of the U was partitioned into the organic fraction, whereas Ni was distributed between several sediment fractions. An inverse pH-organic matter (OM) correlation and positive correlations of OM with total U and organic-bound U/Ni suggest that increased OM preservation and binding to the mineral surfaces were likely responsible for Ni- and especially U-sediment retention (Tims Branch pH = 4.84 ± 0.68). EXAFS analysis indicated the predominance of U(VI) coordinated with clay minerals (~65%), together with ~35% coordinated to either OM (in areas with elevated OM levels) or iron oxides. The desorption-Kd coefficients of U (3972 ± 1370 L/kg) and Ni (30 ± 8 L/kg) indicate that dissolved Ni poses a greater long-term risk than dissolved U for migrating downstream. This study suggests that a delicate balance of geochemical properties controls whether wetlands behave as sinks or sources of contaminants.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗
DOE OSTI2023

Chemical abrasion: the mechanics of zircon dissolution

Chemical abrasion is a technique that combines thermal annealing and partial dissolution in hydrofluoric acid (HF) to selectively remove radiation-damaged portions of zircon crystals prior to U–Pb isotopic analysis, and it is applied ubiquitously to zircon prior to U–Pb isotope dilution thermal ionization mass spectrometry (ID-TIMS). The mechanics of zircon dissolution in HF and the impact of different leaching conditions on the zircon structure, however, are poorly resolved. We present a microstructural investigation that integrates microscale X-ray computed tomography (µCT), scanning electron microscopy, and Raman spectroscopy to evaluate zircon dissolution in HF. We show that µCT is an effective tool for imaging metamictization and complex dissolution networks in three dimensions. Acid frequently reaches crystal interiors via fractures spatially associated with radiation damage zoning and inclusions to dissolve soluble high-U zones, some inclusions, and material around fractures, leaving behind a more crystalline zircon residue. Other acid paths to crystal cores include the dissolution of surface-reaching inclusions and the percolation of acid across zones with high defect densities. In highly crystalline samples dissolution is crystallographically controlled with dissolution proceeding almost exclusively along the c axis. Increasing the leaching temperature from 180 to 210 °C results in deeper etching textures, wider acid paths, more complex internal dissolution networks, and greater volume losses. How a grain dissolves strongly depends on its initial radiation damage content and defect distribution as well as the size and position of inclusions. As such, the effectiveness of any chemical abrasion protocol for ID-TIMS U–Pb geochronology is likely sample-dependent. We also briefly discuss the implications of our findings for deep-time (U-Th)/He thermochronology.

58 GEOSCIENCES↗
NASA NTRS1982

An instrument for measuring thermal inertia in the field

Features and test results of a thermal inertial meter (TIM) for cataloging the thermal inertial of surface material in situ as a basis for satellite remote sensing of geologic materials are described. The instrument is employed to determine the temperature rise of the materials in the field, with the assumptions that the sample and a standard are homogeneous in composition, the heat flux density is constant at the surface of each material, and the specimens are thick enough to be treated as semi-infinite bodies. A formula for calculating thermal inertia is presented, and the components of the TIM are detailed. A box with three compartments, two holding standards, is placed on the sample surface with the third compartment open to the specimen. Dolomite and quartz are used as references when all samples are measured after heating. Tests with rocks and sand in Nevada and California revealed that chert has a higher thermal inertia than barite.

Marsh, S. E.↗
NASA NTRS1984

Active airborne infrared laser system for identification of surface rock and minerals

Emissivity and reflectivity in the thermal infrared spectral region (8-13 microns) may be used to discriminate among rocks and minerals. Although considerable success has been achieved in remote sensing classification of rock types based on emissivity measurements made with NASA's Thermal Infreared Multispectral Scanner (TIMS), classification based on reflectivity offers several advantages: much narrower bandwidths are used, higher signal to noise ratios are possible, and measurements are little affected by surface temperature. As a demonstration, an airborne CO2 laser instrument was flown along the margin of Death Valley, California. Measurements of spectral reflectance collected with this device were compared with emissivity measurements made with the TIMS. Data from either instrument provided the means for recognizing boundaries between geologic units including different rock types and fan surfaces of different ages.

Kahle, A. B.↗
NASA NTRS1984

Mapping alluvial fans in Death Valley, California, using multichannel thermal infrared images

Alluvial fans have been mapped in Death Valley, California using NASA's 8-12 micron six-channel airborne Thermal Infrared Multispectral Scanner (TIMS). Both composition and relative age differences were recognized. Age unit boundries are generally consistent with those obtained by conventional mapping. Composition was verified by field investigation and comparison with existing geologic maps. Bedrock and its young derived fan gravels have similar emissivities. The original composition of the fans is modified by differential erosion and weathering, permitting relative age mapping with TIMS.

Gillespie, A. R.↗
NASA NTRS1986

Investigation of forest canopy temperatures recorded by the thermal infrared multispectral scanner at H. J. Andrews Experimental Forest

Thermal Infrared Multispectral Scanner (TIMS) data were collected over the H. J. Andrews Experimental Forest in Western Oregon on July 29, 1983 at approximately 1:30 p.m., Pacific Standard Time. The relation of changes in canopy temperature to green leaf biomass levels in reforested clearcuts and old-growth forest was investigated. A digital data base was generated in order to isolate that portion of the thermal emission that could be attributed to surface properties other than the vegetation biomass component. The TIMS appears to be capable of detecting subtle differences in ERT as related to canopy closure and green lead biomass, however calibration techniques are needed to correct for emissivity and atmospheric effects.

Sader, Steven A.↗
NASA NTRS1986

The Red River Valley archeological project

The Red River Valley Archeology Project is a long-term effort involving numerous individuals and institutions engaged in archeological investigations in the Texas and Oklahoma portions of the Red River Valley. To date the focus of the project was on site location. The project acquired both Thermal Infrared Multispectral Scanner (TIMS), TMS, and color infrared photographs over a significant portion of the project area in an effort to define signatures for archeological sites and to assist in the detailed geomorphological mapping of the flood plain. Preliminary analysis of acquired data indicates that both the TIMS and TMS can make a substantial contribution to landform definition, the identification of cultural resources, and to the clarification of site-landform correlations in this riverine environment.

Bennett, Jack↗
NASA NTRS1987

Aircraft and satellite remote sensing of desert soils and landscapes

Remote sensing data on desert soils and landscapes, obtained by the Landsat TM, Heat Capacity Mapping Mission (HCMM), Simulated SPOT, and Thermal IR Multispectral Scanner (TIMS) aboard an aircraft, are discussed together with the analytical techniques used in the studies. The TM data for southwestern Nevada were used to discriminate among the alluvial fan deposits with different degrees of desert pavement and varnish, and different vegetation cover. Thermal-IR data acquired from the HCMM satellite were used to map the spatial distribution of diurnal surface temperatures and to estimate mean annual soil temperatures in central Utah. Simulated SPOT data for northwestern New Mexico identified geomorphic features, such as differences in eolian sand cover and fluvial incision, while the TIMS data depicted surface geologic features of the Saline Valley in California.

Petersen, G. W.↗
NASA NTRS1989

Modeling surface temperature distributions in forest landscapes

A model of the frequency distributions of the spatial variability in surface temperature is presented. Surface temperature data are obtained from two daytime and two nighttime flights of the Thermal IR Multispectral Scanner (TIMS) over forest land in western Oregon in August, 1985. The temperature values are corrected for atmospheric attenuation and thermal radiation emission with the LOWTRAN-6 algorithm. The temperature distributions were modeled with a two-parameter beta probability density distribution and the fit of the model was evaluated by comparison with the TIMS data set. Use of the model's parameters to identify and classify surface types shows good discrimination among various surfaces for the daytime images, with less distinct discrimination for the nighttime images.

Holbo, H. R.↗
NASA NTRS1989

Thermal characteristics of mountain desert terrain derived from thermal infrared multispectral scanner measurements

The spatial and temporal variability of mountain-desert territory thermal is examined with an airborne thermal infrared multispectral scanner (TIMS). The purpose of the study is to demonstrate that inhomogeneities of the surface temperatures in the area can be adequately large to influence mesoscale circulations and the turbulence characteristics of boundary-layer flow. Ground truth measurements are compared to the TIMS imagery, with focus placed on the thermal infrared sensitivity to wet and dry soils, terrain elevation, and soil type. The results indicate that variations in the thermal features are dependent on soil type and soil moisture, and that the dependence on surface radiative temperatures on terrain elevation is apparent in daytime measurements.

Astling, E. G.↗
NASA NTRS1990

Estimation of tropical forest canopy temperatures, thermal response numbers, and evapotranspiration using an aircraft-based thermal sensor

Thermal infrared Multispectral Scanner (TIMS) data were collected at a resolution of 5 to 10 m from a tropical rain forest over an elevation gradient from 35 to 2700 m in the Braulio Carrillo National Park in Costa Rica. Flight lines were repeated with a 15 to 30 minute time difference for measurement of forest canopy thermal response over time. Concurrent radiosonde measurements of atmospheric profiles of air temperature and moisture provided inputs to LOWTRAN6 for atmospheric radiance corrections of the TIMS data. Techniques for using calibrated aircraft-based thermal scanner data to examine tropical forest canopy thermal properties are described. Forest canopy temperature changes over time assessed between repeated, duplicated flight lines were combined with estimates of surface radiative energy measurements from towers above the forest canopy to determine temperature spatial variability, calculate Thermal Response Numbers (TRN), and estimate evapotranspiration along the elevation gradient from selected one hectare forest inventory plots.

Luvall, Jeffrey C.↗
NASA NTRS1986

Utility of remotely sensed data for identification of soil conservation practices

Discussed are a variety of remotely sensed data sources that may have utility in the identification of conservation practices and related linear features. Test sites were evaluated in Alabama, Kansas, Mississippi, and Oklahoma using one or more of a variety of remotely sensed data sources, including color infrared photography (CIR), LANDSAT Thematic Mapper (TM) data, and aircraft-acquired Thermal Infrared Multispectral Scanner (TIMS) data. Both visual examination and computer-implemented enhancement procedures were used to identify conservation practices and other linear features. For the Kansas, Mississippi, and Oklahoma test sites, photo interpretations of CIR identified up to 24 of the 109 conservation practices from a matrix derived from the SCS National Handbook of Conservation Practices. The conservation practice matrix was modified to predict the possibility of identifying the 109 practices at various photographic scales based on the observed results as well as photo interpreter experience. Some practices were successfully identified in TM data through visual identification, but a number of existing practices were of such size and shape that the resolution of the TM could not detect them accurately. A series of computer-automated decorrelation and filtering procedures served to enhance the conservation practices in TM data with only fair success. However, features such as field boundaries, roads, water bodies, and the Urban/Ag interface were easily differentiated. Similar enhancement techniques applied to 5 and 10 meter TIMS data proved much more useful in delineating terraces, grass waterways, and drainage ditches as well as the features mentioned above, due partly to improved resolution and partly to thermally influenced moisture conditions. Spatially oriented data such as those derived from remotely sensed data offer some promise in the inventory and monitoring of conservation practices as well as in supplying parameter data for a variety of computer-implemented agricultural models.

Pelletier, R. E.↗
NASA NTRS1991

Mojave remote sensing field experiment

The Mojave Remote Sensing Field Experiment (MFE), conducted in June 1988, involved acquisition of Thermal Infrared Multispectral Scanner (TIMS); C, L, and P-band polarimetric radar (AIRSAR) data; and simultaneous field observations at the Pisgah and Cima volcanic fields, and Lavic and Silver Lake Playas, Mojave Desert, California. A LANDSAT Thematic Mapper (TM) scene is also included in the MFE archive. TM-based reflectance and TIMS-based emissivity surface spectra were extracted for selected surfaces. Radiative transfer procedures were used to model the atmosphere and surface simultaneously, with the constraint that the spectra must be consistent with field-based spectral observations. AIRSAR data were calibrated to backscatter cross sections using corner reflectors deployed at target sites. Analyses of MFE data focus on extraction of reflectance, emissivity, and cross section for lava flows of various ages and degradation states. Results have relevance for the evolution of volcanic plains on Venus and Mars.

Arvidson, Raymond E.↗
NASA NTRS1992

Determination of water surface temperature based on the use of Thermal Infrared Multispectral Scanner data

A straightforward method for compensating Thermal Infrared Multispectral Scanner (TIMS) digital data for the influence of atmospheric path radiance and the attenuation of target energy by the atmosphere is presented. A band ratioing model useful for estimating water surface temperatures, which requires no ground truth measurements, is included. A study conducted to test the potential of the model and the magnitudes of the corrections for atmosphere encountered is presented. Results of the study, which was based on data collected during an engineering evaluation flight of TIMS, indicate errors in the estimate of the surface temperature of the water fall from +/- 1.0 C for uncorrected data to +/- 0.4 C when data have been corrected according to the model presented. This value approaches the noise-limited thermal resolution of the sensor at the time of the flight.

Anderson, James E.↗
NASA NTRS1992

Multispectral thermal infrared mapping of the 1 October 1988 Kupaianaha flow field, Kilauea volcano, Hawaii

Multispectral thermal infrared radiance measurements of the Kupaianaha flow field were acquired with the NASA airborne Thermal Infrared Multispectral Scanner (TIMS) on the morning of 1 October 1988. The TIMS data were used to map both the temperature and emissivity of the surface of the flow field. The temperature map depicted the underground storage and transport of lava. The presence of molten lava in a tube or tumulus resulted in surface temperatures that were at least 10 C above ambient. The temperature map also clearly defined the boundaries of hydrothermal plumes which resulted from the entry of lava into the ocean. The emissivity map revealed the boundaries between individual flow units within the Kupaianaha field. Distinct spectral anomalies, indicative of silica-rich surface materials, were mapped near fumaroles and ocean entry sites. This apparent enrichment in silica may have resulted from an acid-induced leaching of cations from the surfaces of glassy flows.

Realmuto, Vincent J.↗
NASA NTRS1992

Geologic remote sensing - New technology, new information

Results of geologic studies using data collected by the NASA/JPL Thermal Infrared Imaging Spectrometer (TIMS), Airborne Visible/Infrared Imaging Spectrometer (AVIRIS), and the Airborne Synthetic Aperture Radar (AIRSAR) are discussed. These instruments represent prototypes for the Earth Observing System (EOS) satellite instruments ASTER, High Resolution Imaging Spectrometer (HIRIS), and EOS SAR. Integrated analysis of this data type is one of the keys to successful geologic research using EOS. TIMS links the physical properties of surface materials in the 8-12-*mm region to their composition. Calibrated aircraft data make direct lithological mapping possible. AVIRIS, an analog for HIRIS, provides quantitative information about the surface composition of materials based on their detailed visible and infrared spectral signatures (0.4-2.45 mm). Calibrated AVIRIS data make direct identification of minerals possible. The AIRSAR provides additional complementary information about the surface morphology of rocks and soils.

Kruse, F. A.↗
NASA NTRS1992

Lithological and textural controls on radar and diurnal thermal signatures of weathered volcanic deposits, Lunar Crater region, Nevada

Radar backscatter intensity as measured by calibrated synthetic aperture radar (SAR) systems is primarily controlled by three factors: local incidence angle, wavelength-scale roughness, and dielectric permittivity of surface materials. Radar observations may be of limited use for geological investigations of surface composition, unless the relationships between lithology and the above characteristics can be adequately understood. In arid terrains, such as the Southwest U.S., weathering signatures (e.g. soil development, fracturing, debris grain size and shape, and hill slope characteristics) are controlled to some extent by lithologic characteristics of the parent bedrock. These textural features of outcrops and their associated debris will affect radar backscatter to varying degrees, and the multiple-wavelength capability of the JPL Airborne SAR (AIRSAR) system allows sampling of textures at three distinct scales. Diurnal temperature excursions of geologic surfaces are controlled primarily by the thermal inertia of surface materials, which is a measure of the resistance of a material to a change in temperature. Other influences include albedo, surface slopes affecting insolation, local meteorological conditions and surface emissivity at the relevant thermal wavelengths. To first order, thermal inertia variations on arid terrain surfaces result from grain size distribution and porosity differences, at scales ranging from micrometers to tens of meters. Diurnal thermal emission observations, such as those made by the JPL Thermal Infrared Multispectral Scanner (TIMS) airborne instrument, are thus influenced by geometric surface characteristics at scales comparable to those controlling radar backscatter. A preliminary report on a project involving a combination of field, laboratory and remote sensing observations of weathered felsic-to basaltic volcanic rock units exposed in the southern part of the Lunar Crater Volcanic Field, in the Pancake Range of central Nevada is presented. Focus is on the relationship of radar backscatter cross sections at multiple wavelengths, apparent diurnal temperature excursions identified in multi-temporal TIMS images, surface geometries related to weathering style, and parent bedrock lithology.

Plaut, Jeffrey J.↗
NASA NTRS1993

The difference between laboratory and in-situ pixel-averaged emissivity: The effects on temperature-emissivity separation

Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) is a Japanese future imaging sensor which has five channels in thermal infrared (TIR) region. To extract spectral emissivity information from ASTER and/or TIMS data, various temperature-emissivity (T-E) separation methods have been developed to date. Most of them require assumptions on surface emissivity, in which emissivity measured in a laboratory is often used instead of in-situ pixel-averaged emissivity. But if these two emissivities are different, accuracies of separated emissivity and surface temperature are reduced. In this study, the difference between laboratory and in-situ pixel-averaged emissivity and its effect on T-E separation are discussed. TIMS data of an area containing both rocks and vegetation were also processed to retrieve emissivity spectra using two T-E separation methods.

Matsunaga, Tsuneo↗