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At least 199 records · Page 11

Recent progress in laser wire-based H- beam diagnostics at the SNS linac

Laser wire has been used for nonintrusive profile and emittance measurements of operational hydrogen ion (H-) beam at the SNS linac. In this talk, we will describe the following recent developments in the laser wire system. 1) An upgraded light source and laser transport line which enables novel measurement capabilities including longitudinal profile measurement and high-energy proton beam extraction over potentially an entire macropulse. 2) A dual-detector emittance measurement scheme that boosted the dynamic range by an order of magnitude. 3) Design and implementation laser-wire-based nonintrusive longitudinal phase space measurement system.

Liu, Yun↗

Designed metal-insulator transition in low-symmetry magnetic intermetallics

Compounds exhibiting half-metallic character and metal-insulator transitions draw considerable attention in condensed-matter and materials physics due to their potential use in spintronics. Here we show that specific electron doping plays a crucial role in tailoring thermodynamic, structural, electronic, and magnetic properties of materials derived from low-symmetry magnetic intermetallics, exemplified on triclinic Mn 4 Al 11 . Upon chemical doping of Al by Ge, we predict improved phase stability and adherence to a generalized “18-n rule” governing closed-shell configurations in intermetallic with narrow bandgaps. Validating experiments include measurements of phase stability and electronic transport properties of electron-doped Mn 4 Al 10 Ge that crystallizes in the Mn 4 Al 11 -type structure, confirming the bandgap opening as predicted by chemical analysis and density-functional theory. Here we also demonstrate theoretically that hydrostatic pressure enhances the predicted half-metallic gap in the up-spin channel, which leads to a ferrimagnetic-to-ferromagnetic transition driven by Mn-Mn charge ordering in the Mn 4 Al 11 parent. We have also discussed the generality of our approach in predicting the design of other classes of intermetallics including half and full Heusler compounds.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Image Processing Pipeline for Fluoroelastomer Crystallite Detection in Atomic Force Microscopy Images

Phase transformations in materials systems can be tracked using atomic force microscopy (AFM), enabling the examination of surface properties and macroscale morphologies. In situ measurements investigating phase transformations generate large datasets of time-lapse image sequences. The interpretation of the resulting image sequences, guided by domain-knowledge, requires manual image processing using handcrafted masks. Here this approach is time-consuming and restricts the number of images that can be processed. Her in this study, we developed an automated image processing pipeline which integrates image detection and segmentation methods. We examine five time-series AFM videos of various fluoroelastomer phase transformations. The number of image sequences per video ranges from a hundred to a thousand image sequences. The resulting image processing pipeline aims to automatically classify and analyze images to enable batch processing. Using this pipeline, the growth of each individual fluoroelastomer crystallite can be tracked through time. We incorporated statistical analysis into the pipeline to investigate trends in phase transformations between different fluoroelastomer batches. Understanding these phase transformations is crucial, as it can provide valuable insights into manufacturing processes, improve product quality, and possibly lead to the development of more advanced fluoroelastomer formulations.

36 MATERIALS SCIENCE↗

Improved measurement of the strong-phase difference $\delta _D^{K\pi }$ in quantum-correlated $D{\overline{D}}$ decays

The decay D → K - π + is studied in a sample of quantum-correlated D$\overline{D}$ pairs, based on a data set corresponding to an integrated luminosity of 2.93 fb -1 collected at the ψ(3770) resonance by the BESIII experiment. The asymmetry between CP-odd and CP-even eigenstate decays into K - π + is determined to be A Kπ = 0.132 ± 0.011 ± 0.007, where the first uncertainty is statistical and the second is systematic. This measurement is an update of an earlier study exploiting additional tagging modes, including several decay modes involving a $K^{0}_{L}$ meson. The branching fractions of the $K^{0}_{L}$ modes are determined as input to the analysis in a manner that is independent of any strong phase uncertainty. Using the predominantly CP-even tag D → π + π - π 0 and the ensemble of CP-odd eigenstate tags, the observable $A^{πππ^0}_{Kπ}$ is measured to be 0.130 ± 0.012 ± 0.008. The two asymmetries are sensitive to $r^{Kπ}_{D}$ cos $δ^{Kπ}_{D}$ where $r^{Kπ}_{D}$ and $δ^{Kπ}_{D}$ are the ratio of amplitudes and phase difference, respectively, between the doubly Cabibbo-suppressed and Cabibbo-favoured decays. In addition, events containing D → K - π + tagged by D → $K^{0}_{S,L}$π + π - are studied in bins of phase space of the three-body decays. This analysis has sensitivity to both $r^{Kπ}_{D}$ cos $δ^{Kπ}_{D}$ and $r^{Kπ}_{D}$, sin $δ^{Kπ}_{D}$. A fit to A Kπ , $A^{πππ^0}_{Kπ}$ and the phase-space distribution of the D → $K^{0}_{S,L}$π + π - tags yields $δ^{Kπ}_{D}$ = ($187.6^{+8.9+5.4}_{-9.7-6.4}$)°, where external constraints are applied for $r^{Kπ}_{D}$ and other relevant parameters. This is the most precise measurement of $δ^{Kπ}_{D}$ in quantum-correlated D$\overline{D}$ decays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Visualization of phase-space orbit topological boundary using imaging neutral particle analyzer

A newly-developed imaging neutral particle analyzer (INPA) in the DIII-D tokamak interrogates phase space occupied by fast ions on multiple different orbit topologies, including passing, stagnation, trapped and potato orbits. Depending on plasma parameters and beam injection geometries, this new INPA system is capable of visualizing distributions of fast ions on the selected orbit topology and its associated orbit topology boundaries. More importantly, the system is able to directly visualize the pitch angle scattering process in phase space by measuring fast ions that are scattered across the trapped-passing orbit topology boundaries. It also enables visualization of fast ion confined-loss boundaries, which are determined by particle energy, plasma current and magnetic field.The key goal of this new INPA system is to directly measure pitch angle scattering across phase space induced by drift waves and its interaction with Alfv'en eigenmodes, i.e., a key issue towards \redit{a} future fusion power plant.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

AGR-1 UCO Kernel Phase Analysis Imaging Archive

UCO kernels in tri-structural isotropic (TRISO) particles consist of a heterogeneous mixture of uranium oxide and uranium carbide. During the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program, mean kernel composition was specified based on bulk measurements of uranium, oxygen, and carbon content, as well as the resulting O/U, C/U, and O+C/U ratios. Further development of quality control characterization methods has resulted in a method for more direct measurement of phase fractions on a per-kernel basis using optical microscopy of polished kernel cross sections. This report provides benchmark values for this analysis method when applied to kernels from the AGR-1 campaign and to the raw images used.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measurements of nematic susceptibility with phase sensitive nuclear magnetic resonance in pulsed strain fields

Here, we present nuclear magnetic resonance data in BaFe 2 As 2 in the presence of pulsed strain fields that are interleaved in time with the radio frequency excitation pulses. In this approach, the preceding nuclear magnetization acquires a phase shift that is proportional to the strain and pulse time. The sensitivity of this approach is limited by the homogeneous decoherence time, T 2 , rather than the inhomogeneous linewidth. We measure the nematic susceptibility as a function of temperature and demonstrate a three orders of magnitude improvement in sensitivity. This approach will enable studies of the strain response in a broad range of materials that previously were inaccessible due to inhomogeneous broadening.

36 MATERIALS SCIENCE↗

A Comparison of Three Ways to Measure Time-Dependent Densities With Quantum Simulators

Quantum algorithms are touted as a way around some classically intractable problems such as the simulation of quantum mechanics. At the end of all quantum algorithms is a quantum measurement whereby classical data is extracted and utilized. In fact, many of the modern hybrid-classical approaches are essentially quantum measurements of states with short quantum circuit descriptions. Here, we compare and examine three methods of extracting the time-dependent one-particle probability density from a quantum simulation: direct Z -measurement, Bayesian phase estimation, and harmonic inversion. We have tested these methods in the context of the potential inversion problem of time-dependent density functional theory. Our test results suggest that direct measurement is the preferable method. We also highlight areas where the other two methods may be useful and report on tests using Rigetti's quantum virtual device. This study provides a starting point for imminent applications of quantum computing.

Yang, Jun↗

Multiscale Interaction of Turbulence, Temperature, and Soot Formation: Measurements for Critical Assessments of Chemical Kinetics and Mechanisms

This program targeted an improved understanding of how turbulence affects soot formation chemistry (directly and indirectly) with a particular focus on detailing the multiscale coupling between flow turbulence, mixing, thermal transport, and soot formation kinetics in gas-phase reacting systems. In this project, simultaneous, quantitative multi-dimensional velocity, soot volume fraction, and gas-phase temperature measurements in turbulent non-premixed sooting flames were developed. These new diagnostics tools can be used to elucidate the relative effects of fluid kinematics, mixing, thermal processes, and turbulence/scalar time/length scales on soot formation chemistry and topology. Simultaneous multi-parameter measurements were acquired within a series of flames with different Reynolds numbers and spatial locations to investigate the inter-dependence of soot, temperature, and turbulence within the soot inception, growth, and oxidation region. Preliminary assessment of the results has been completed at the project end and detailed analysis is planned following the completed program.

02 PETROLEUM↗

The discriminant power of bubble wall velocities: gravitational waves and electroweak baryogenesis

A precise determination of the bubble wall velocity v$_{w}$ is crucial for making accurate predictions of the baryon asymmetry and gravitational wave (GW) signals in models of electroweak baryogenesis (EWBG). Working in the local thermal equilibrium approximation, we exploit entropy conservation to present efficient algorithms for computing v$_{w}$, significantly streamlining the calculation. We then explore the parameter dependencies of v$_{w}$, focusing on two sample models capable of enabling a strong first-order electroweak phase transition: a ℤ$_{2}$-symmetric singlet extension of the SM, and a model for baryogenesis with CP violation in the dark sector. We study correlations among v$_{w}$ and the two common measures of phase transition strength, α$_{n}$ and v$_{n}$/T$_{n}$. Interestingly, we find a relatively model-insensitive relationship between v$_{n}$/T$_{n}$ and α$_{n}$. We also observe an upper bound on α$_{n}$ for the deflagration/hybrid wall profiles naturally compatible with EWBG, the exact value for which varies between models, significantly impacting the strength of the GW signals. In summary, our work provides a framework for exploring the feasibility of EWBG models in light of future GW signals.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Constraining the phase shift of relativistic species in DESI BAOs

In the early Universe, neutrinos decouple quickly from the primordial plasma and propagate without further interactions. The impact of free-streaming neutrinos is to create a temporal shift in the gravitational potential that impacts the acoustic waves known as baryon acoustic oscillations (BAOs), resulting in a non-linear spatial shift in the Fourier-space BAO signal. In this work, we make use of and extend upon an existing methodology to measure the phase shift amplitude $\beta _{\phi }$ and apply it to the Dark Energy Spectroscopic Instrument (DESI) Data Release 1 (DR1) BAOs with an anisotropic BAO fitting pipeline. We validate the fitting methodology by testing the pipeline with two publicly available fitting codes applied to highly precise cubic box simulations and realistic simulations representative of the DESI DR1 data. We find further study towards the methods used in fitting the BAO signal will be necessary to ensure accurate constraints on $\beta _{\phi }$ in future DESI data releases. Using DESI DR1, we present individual measurements of the anisotropic BAO distortion parameters and the $\beta _{\phi }$ for the different tracers, and additionally a combined fit to $\beta _{\phi }$ resulting in $\beta _{\phi } = 2.7 \pm 1.7$. After including a prior on the distortion parameters from constraints using Planck we find $\beta _{\phi } = 2.7^{+0.60}_{-0.67}$ suggesting $\beta _{\phi } > 0$ at 4.3$\sigma$ significance. This result may hint at a phase shift that is not purely sourced from the standard model expectation for $N_{\rm {eff}}$ or could be a upwards statistical fluctuation in the measured $\beta _{\phi }$; this result relaxes in models with additional freedom beyond Lambda-cold dark matter.

79 ASTRONOMY AND ASTROPHYSICS↗

Reconstructing neutrinoless double beta decay event kinematics in a xenon gas detector with vertex tagging

If neutrinoless double beta decay is discovered, the next natural step would be understanding the lepton number violating physics responsible for it. Several alternatives exist beyond the exchange of light neutrinos. Some of these mechanisms can be distinguished by measuring phase-space observables, namely the opening angle cos θ among the two decay electrons, and the electron energy spectra, T 1 and T 2 . In this work, we study the statistical accuracy and precision in measuring these kinematic observables in a future xenon gas detector with the added capability to precisely locate the decay vertex. For realistic detector conditions (a gas pressure of 10 bar and spatial resolution of 4 mm), we find that the average $\overline{cos θ}$ and $\overline{T_1}$ values can be reconstructed with a precision of 0.19 and 110 keV, respectively, assuming that only 10 neutrinoless double beta decay events are detected.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Sodium Void Worth and Control Rod Worth Measurements in ZPPR 15

Sodium void worth and control rod worth were measured in Phases A, B, C and D of the ZPPR15 experimental program. Sodium voiding was simulated by replacing stainless steel cans containing sodium by empty stainless steel cans of the same sizes. The control rod worth measurements were measurements of simulated control rods (CRs) and simulated empty control rod positions (CRPs). A CRP consisted of a 2 x 2 array of drawers filled with sodium plates. A CR consisted of a 2 x 2 array of drawers containing alternating columns of boron carbide plates and sodium plates in the front 18 inches and just sodium plates in the back 18 inches. The ZPPR staff published the measured sodium void worths and control rod worths and the statistical uncertainties in the measured values. In reality, the published uncertainty for each of these measurements is only one component of the total uncertainty. There are additional contributions from uncertainties related to measurement technique, plate compositions and reproducibility. However, the dominant uncertainty for the sodium void worth and control rod worth measurements is the uncertainty in βeff which is required to convert from the natural measurement units, cents, to the calculation units, pcm or Δ/k 1 k 2 . A full uncertainty analysis was performed for the sodium void worth and control rod worth measurements. The significant uncertainties were quantified, and a total uncertainty was derived for each sodium void worth or control rod worth measurement. The ZPPR-15 experimental records were used to create detailed as-built Monte Carlo models of the sodium void worth and control rod worth configurations. These models were used to compute the sodium void worths and control rod worths. (C/E – 1) and the related uncertainty in (C/E – 1) were derived for the measured worths.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Unconventional supercurrent phase in Ising superconductor Josephson junction with atomically thin magnetic insulator

Abstract In two-dimensional (2D) NbSe 2 crystal, which lacks inversion symmetry, strong spin-orbit coupling aligns the spins of Cooper pairs to the orbital valleys, forming Ising Cooper pairs (ICPs). The unusual spin texture of ICPs can be further modulated by introducing magnetic exchange. Here, we report unconventional supercurrent phase in van der Waals heterostructure Josephson junctions (JJs) that couples NbSe 2 ICPs across an atomically thin magnetic insulator (MI) Cr 2 Ge 2 Te 6 . By constructing a superconducting quantum interference device (SQUID), we measure the phase of the transferred Cooper pairs in the MI JJ. We demonstrate a doubly degenerate nontrivial JJ phase ( ϕ ), formed by momentum-conserving tunneling of ICPs across magnetic domains in the barrier. The doubly degenerate ground states in MI JJs provide a two-level quantum system that can be utilized as a new dissipationless component for superconducting quantum devices. Our work boosts the study of various superconducting states with spin-orbit coupling, opening up an avenue to designing new superconducting phase-controlled quantum electronic devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Multiphase tin equation of state using density functional theory

In this work, we perform density functional theory (DFT) calculations of five solid phases and the liquid phase of tin. The calculations include cold curves of the five solid phases, phonon calculations in the quasiharmonic approximation over a range of volumes for each solid phase, and DFT-based molecular dynamics (DFT-MD) simulations of the liquid phase, including those of the melt curve using the Z method. Using the DFT results, we construct a tabular multiphase sesame equation of state for tin, referred to as sesame 2162. Comparisons to experimental data are made and show a high level of agreement in isobaric data, isothermal data, shock data, and phase boundary measurements, including measurements of the melt curve. The 2162 EOS will be useful for hydrodynamics simulations and has been designed with an eye toward hydrodynamics simulations that incorporate materials strength models and allow for modeling of the kinetics of phase transitions.

3-dimensional systems↗

Measurements at peak operational beam current in the SNS beam test facility

Work at the SNS beam test facility has focused on high dimensional and high dynamic range measurements of the medium energy (2.5 Mev) beam distribution. This is motivated by the need to understand and predict beam losses down to one-part-per-million. The initial demonstration of full-and-direct 6D phase space measurement was done at a current of 40 mA transported through the RFQ. Since that demonstration, more detailed studies have been performed at lower transported currents (in the range 30 mA and below). This is due to a hardware change - recent runs utilize the original SNS RFQ, which after a decade of service in the SNS achieves transmission significantly below design (50-60%, vs >80%). A short run in 2023 with a newly-commissioned RFQ enables maximum transmission. Preliminary results from beam distribution measurements during this run are discussed.

Ruisard, Kiersten↗

Turn-key constrained parameter space exploration for particle accelerators using Bayesian active learning

Abstract Particle accelerators are invaluable discovery engines in the chemical, biological and physical sciences. Characterization of the accelerated beam response to accelerator input parameters is often the first step when conducting accelerator-based experiments. Currently used techniques for characterization, such as grid-like parameter sampling scans, become impractical when extended to higher dimensional input spaces, when complicated measurement constraints are present, or prior information known about the beam response is scarce. Here in this work, we describe an adaptation of the popular Bayesian optimization algorithm, which enables a turn-key exploration of input parameter spaces. Our algorithm replaces the need for parameter scans while minimizing prior information needed about the measurement’s behavior and associated measurement constraints. We experimentally demonstrate that our algorithm autonomously conducts an adaptive, multi-parameter exploration of input parameter space, potentially orders of magnitude faster than conventional grid-like parameter scans, while making highly constrained, single-shot beam phase-space measurements and accounts for costs associated with changing input parameters. In addition to applications in accelerator-based scientific experiments, this algorithm addresses challenges shared by many scientific disciplines, and is thus applicable to autonomously conducting experiments over a broad range of research topics.

43 PARTICLE ACCELERATORS↗

Exchange field enhanced upper critical field of the superconductivity in compressed antiferromagnetic EuTe2

Abstract Understanding the interplay between superconductivity and magnetism has been a longstanding challenge in condensed matter physics. Here we report high pressure studies on the C -type antiferromagnetic semiconductor EuTe 2 up to 36.0 GPa. A structural transition from the I4/mcm to the C2/m space group is identified at ~16 GPa. Superconductivity is observed above ~5 GPa in both structures. In the low-pressure phase, magnetoresistance measurements reveal strong couplings between the local moments of Eu 2+ and the conduction electrons of Te 5 p orbits. The upper critical field of superconductivity is well above the Pauli limit. While EuTe 2 becomes nonmagnetic in the high-pressure phase and the upper critical field drops below the Pauli limit. Our results demonstrate that the high upper critical field of EuTe 2 in the low-pressure phase is due to the exchange field compensation effect of Eu 2+ and the superconductivity in both structures may arise in the framework of the Bardeen-Cooper-Schrieffer theory.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗