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At least 199 records · Page 11

Cautionary Notes on Cosmogenic W-182 and Other Nuclei in Lunar Samples

Leya et al. (2000) showed that neutron capture on Ta-181 results in a production rate of Ta-182 (decays with a half-life of 114 days to W-182) sufficiently high to cause significant shifts in W-182 abundances considering the neutron fluences due to the cosmic ray cascade that were known to occur near the lunar surface. Leya et al. concluded that this cosmogenic production of W-182 may explain the large positive epsilon(sub W-182) values that Lee et al. (1997) had reported in some lunar samples rather than being produced from decay of now extinct Hf-182 (bar tau = 13 x 10(exp 6) yr). If the large range in epsilon(sub W-182) of lunar samples (0 to +11 in whole rock samples) was due to decay of now extinct Hf-182, it would require a very early time of formation and differentiation of the lunar crust-mantle system (with high Hf/W ratios) during the earliest stages of Earth s accretion. This result was both surprising and difficult to understand. The ability to explain these results by a more plausible mechanism is therefore very attractive. In a recent report Lee et al. (2002) showed that there were excesses of W-182 and that epsilon(sub W-182) was correlated with the Ta/W ratios in the mineral phases of individual lunar rock samples. This is in accord with W-182 variations in lunar samples being produced by cosmic-ray induced neutron capture on Ta-182.

Yin, Qingzhu↗

Full-core high-burnup BWR LOCA fuel performance analysis and FFRD susceptibility

The susceptibility of the boiling water reactor (BWR) Limerick Unit 1 to fuel fragmentation, relocation, and dispersal during a postulated large-break loss-of-coolant accident (LBLOCA) was calculated using a multiphysics framework. The simulations include full-core, rod-resolved neutronic, thermal hydraulic, and fuel performance models using the VERA, TRACE, and BISON codes. This work focused on the transient BISON simulations, which include both the normal operation and LBLOCA periods in the same simulations. Cladding integrity was assessed using two correlations that are included with BISON. make page break Several new BWR-specific features were recently added to BISON. This work represents the first time these features have been included in a core-scale set of simulations. This study hence evaluates the performance of these new models for an operating reactor with realistic operating conditions. Simulation results showed that cladding integrity was maintained (i.e., no rods burst). Finally, future work to improve BWR and PWR predictions using this framework is suggested.

BISON↗

On the relation between X-ray burst properties and the persistent X-ray luminosity

Published data on X-ray bursts is analyzed, assuming that the peak luminosity of X-ray bursts with radius expansion is a standard candle and that the ratio of the anisotropy factors, xi(b) and xi(p) (Sztajno et al., 1987) is the same for all burst sources. It is shown that the effective burst duration, defined as the ratio of burst fluence to maximum burst flux, is strongly anticorrelated with the persistent luminosity. A positive correlation with the persistent luminosity of the ratio of the average persistent flux to the time-averaged burst flux is found. It is concluded that, independent of the accretion rate, after a given waiting time burst sources produce bursts with approximately the same (average) energy. This suggests that continuous stable burning of a sizeable fraction of the nuclear fuel is a general phenomenon on the surface of accreting neutron stars. It is suggested that this fraction is a gradually increasing function of the accretion rate.

Van Paradijs, J.↗

Causes of fuel–ablator mix inferred from modeling of monochromatic time-gated radiography of OMEGA cryogenic implosions

Here, we present evidence, in the context of OMEGA cryogenic target implosions, that laser imprint, known to be capable of degrading laser-direct-drive target performance, plays a major role in generating fuel–ablator mix. OMEGA cryogenic target implosions show a performance boundary correlated with acceleration-phase shell stability; for sufficiently low adiabats (where the adiabat is the ratio of the pressure to the Fermi pressure) and high in-flight aspect ratios (IFAR's), the neutron-weighted shell areal density and neutron yield relative to the clean simulated values sharply decline. Direct evidence of Rayleigh–Taylor fuel–ablator mixing was previously obtained using a Si Heα backlighter driven by an ~20-ps short pulse generated by OMEGA EP. The shadow cast by the shell shortly prior to stagnation, as diagnosed using backlit radiographs, shows a softening near the limb, which is evidence of an ablator–fuel mix region for a low-adiabat implosion (α ~ 1.9, IFAR = 14) but not for a moderate adiabat implosion (α ~ 2.5, IFAR = 10). We find good agreement between experimental and synthetic radiographs in simulations that model laser imprint and account for uncertainty in the initial ablator thickness. Furthermore, we further explore the role of other mechanisms such as classical instability growth at the fuel–ablator interface, species concentration diffusion, and long-wavelength drive and target asymmetries.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Statistical Properties of SGR 1806-20 Bursts

We present statistics of SGR 1806-20 bursts, combining 290 events detected with the Rossi X-Ray Timing Explorer/Proportional Counter Array, 111 events detected with the Burst and Transient Source Experiment, and 134 events detected with the International Cometary, Explorer. We find that the fluence distribution of bursts observed with each instrument are well described by power laws with indices 1.43, 1.76, and 1.67, respectively. The distribution of time intervals between successive bursts from SGR 1806-20 is described by a lognormal function with a peak at 103 s. There is no correlation between the burst intensity and either the waiting times until the next burst or the time elapsed since the previous burst. In all these statistical properties, SGR 1806-20 bursts resemble a self-organized critical system, similar to earthquakes and solar flares. Our results thus support the hypothesis that the energy source for soft gamma repeater bursts is crustquakes due to the evolving, strong magnetic field of the neutron star, rather than any accretion or nuclear power.

Gogus, Ersin↗

Lunar Instrument Data Integration Into the Virtual Reality Mission Simulation System for Decision Communication and Situational Awareness

In situ resource utilization (ISRU) technologies are a key advancement required to make human habitation on the Moon and Mars viable. The upcoming Volatiles Investigating Polar Exploration Rover (VIPER) mission will provide crucial correlations between volatiles and lunar geology to understand the water content available for ISRU on the moon. The mission will require the coordination of multi-disciplinary teams across the country making real time decisions based on rover instrument data. The virtual reality Mission Simulation System (vMSS) is a virtual reality platform designed at MIT by the Resource Exploration and Science of our Cosmic Environment (RESOURCE) team to provide teams with a collaboration interface for planetary missions like VIPER. Herein we determine the integration pathway for analog based datasets that are examples of VIPER's two main instruments, the near-infrared volatile spectrometer subsystem (NIRVSS) and the neutron spectrometer subsystem (NSS), into vMSS to provide the most valuable visualization tools. Focusing on improving situational awareness, decision making, reducing task load and incorporating comments from scientists working previous analogs and on the current VIPER mission, we recommend critical elements to implement into vMSS and the best approaches for data visualization. We present a review of relevant analogs and state of the art mission software. We have developed a design concept and path to flight of analysed instrument data integrated with data maps that allow for virtual manipulation and annotation between non-co-located team members. We focus on pre-mission mapping of a priori data for improved situational awareness, layering of analysed instrument data, correlative mapping and interactive capabilities for in-mission decision making, as well as archiving and annotation tools for post-mission analysis. Finally, we lay out the roadmap for the future development of immersive sample site visualization capabilities and the use of integrated instrument data in vMSS with automated temporal and geospatial planning.

Cody Alison Paige↗

Producing Evaluation-quality 239 Pu Average Prompt Fission Neutron Multiplicities using a Correlated Fission Model

An evaluation of the average prompt fission neutron multiplicity, $\bar{ν}_p$, of 239 Pu(n,f) is shown. This evaluation includes (a) the correlated fission model CGMF, and (b) a detailed analysis of past and recently published experimental data. Using CGMF-calculated $\bar{ν}_p$ as prior enables to link, through the use of evaluated model input parameters, $\bar{ν}_p$ to other fission observables such as the prompt fission neutron spectrum (PFNS), preneutron emission fission yields as a function of mass, and the average total kinetic energy of the fragments. These evaluated parameters produce realistic predictions of many fission observables, while the evaluated $\bar{ν}_p$ agrees well (χ 2 ≈ 1) with data. Moreover, with the new evaluated $\bar{ν}_p$, the effective neutron multiplication factor of fast Pu ICSBEP critical assemblies are predicted with a mean bias of 58 pcm compared to 18 pcm with ENDF/B-VIII.0, when paired with a new 239 Pu PFNS and fission cross section. Due to these encouraging validation results, the evaluated $\bar{ν}_p$ is currently part of a release candidate for the 239 Pu ENDF/B-VIII.1 file. Hence, a correlated fission model was used for the first time for evaluating $\bar{ν}_p$ that is of evaluation quality. This is an important step towards consistent evaluations of prompt fission observables.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Statistical Properties of SGR 1900+14 Bursts

We study the statistics of soft gamma repeater (SGR) bursts, using a data base of 187 events detected with BATSE and 837 events detected with RXTE PCA, all from SGR 1900+14 during its 1998-1999 active phase. we find that the fluence or energy distribution of bursts is consistent with a power law of index 1.66, over 4 orders of magnitude. This scale-free distribution resembles the Gutenberg-Richter Law for earthquakes, and gives evidence for self-organized criticality in SGRS. The distribution of time intervals between successive bursts from SGR 1900+14 is consistent with a log-normal distribution. There is no correlation between burst intensity and the waiting times till the next burst, but there is some evidence for a correlation between burst intensity and the time elapsed since the previous burst. We also find a correlation between the duration and the energy of the bursts, but with significant scatter. In all these statistical properties, SGR bursts resemble earthquakes and solar flares more closely than they resemble any known accretion-powered or nuclear-powered phenomena. Thus our analysis lends support to the hypothesis that the energy source for SGR bursts is internal to the neutron star, and plausibly magnetic.

Gogus, Ersin↗

Statistical Properties of SGR 1900+14 Bursts

We study the statistics of soft gamma repeater (SGR) bursts using a database of 187 events detected with BATSE and 837 events detected with the Rossi X-Ray Timing Explorer Proportional Counter Array: all events are from SGR 1900+14 during its 1998-1999 active phase. We find that the fluence or energy distribution of bursts is consistent with a power law of index 1.66, over 4 orders of magnitude. This scale-free distribution resembles the Gutenberg-Richter law for earthquakes and gives evidence for self-organized criticality in SGRS. The distribution of time intervals between successive bursts from SGR 1900+14 is consistent with a lognormal distribution. There is no correlation between burst intensity and the waiting times till the next burst, but there is some evidence for a correlation between burst intensity and the time elapsed since the previous burst. We also find a correlation between the duration and the energy of the bursts, but with significant scatter. In all these statistical properties, SGR bursts resemble earthquakes and solar flares more closely than they resemble any known accretion-powered or nuclear-powered phenomena. Thus, our analysis lends support to the hypothesis that the energy source for SGR bursts is internal to the neutron star and plausibly magnetic.

Gogus, Ersin↗

High-precision Measurement of the 16 O($n, n'γ$) Cross Section using $γ$-ray Detection in Liquid Scintillators with H 2 O and BeO Targets

The 16 O($n, n'γ$) reaction was measured at the Los Alamos Neutron Science Center white neutron source using γ-ray detection in liquid scintillators present in the upper hemisphere of the Correlated Gamma-Neutron Array for sCattering (CoGNAC). Separate measurements of this reaction were performed using H 2 O and BeO targets in successive years. The unique high energies of γ rays emitted from the 16 O($n, n'γ$) reaction facilitated a clean selection of this reaction from threshold to 9.8 MeV incident neutron energy without the need for precise measurements of the γ-ray energy or the scattered neutrons. The precise time resolution of the liquid scintillator detectors was then exploited to obtain high-resolution incident neutron energy measurements, and good agreement was obtained between the H 2 O and BeO results reported here. The dominant literature data sets for this reaction have systematic differences between them, but the present results improve upon the neutron energy resolution of earlier measurements and show important discrepancies in recent data. Finally, tentative data are also shown up to 20 MeV incident neutron energy but are potentially subject to improved understanding of the relative γ-ray and α decay branches from 16 O excited states.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Correlating Broadband Photoluminescence with Structural Dynamics in Layered Hybrid Halide Perovskites

The emission of white light from a single material is atypical and is of interest for solid-state lighting applications. Broadband light emission has been observed in some layered perovskite derivatives, A 2 PbBr 4 (A = R-NH 3 + ), and correlates with static structural distortions corresponding to out-of-plane tilting of the lead bromide octahedra. While materials with different organic cations can yield distinct out-of-plane tilts, the underlying origin of the octahedral tilting remains poorly understood. Using high energy resolution (e.g., quasi-elastic) neutron scattering, this contribution details the rotational dynamics of the organic cations in A 2 PbBr 4 materials where A = n-butylammonium (nBA), 1,8-diaminooctammonium (ODA), and 4-aminobutyric acid (GABA). The organic cation dynamics differentiate (nBA) 2 PbBr 4 from (ODA)PbBr 4 or (GABA) 2 PbBr 4 in that the larger spatial extent of dynamics of nBA yields a larger effective cation radius. The larger effective volume of the nBA cation in (nBA) 2 PbBr 4 yields a closer to ideal A-site geometry, preventing the out-of-plane tilt and broadband luminescence. In all three compounds, we observe hydrogen dynamics attributed to rotation of the ammonium headgroup and at a time scale faster than the white light photoluminescence studied by time-correlated single photon counting spectroscopy. This supports a previous assignment of the broadband emission as resulting from a single ensemble, such that the emissive excited state experiences many local structures faster than the emissive decay. Furthermore, the findings presented here highlight the role of the organic cation and its dynamics in hybrid organic–inorganic perovskites and white light emission.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Microscopic theory of angular momentum distributions across the full range of fission fragments

Modern nuclear theory provides qualitative insights into the fundamental mechanisms of nuclear fission and is increasingly capable of making reliable quantitative predictions. Most quantities of interest pertain to the primary fission fragments, whose subsequent decay is typically modeled using statistical reaction models. Consequently, a key objective of fission theory is to inform these models by predicting the initial conditions of the primary fragments. Here, in this work, we employ a framework that combines joint angular momentum and particle number projection with time-dependent configuration mixing to calculate the angular momentum distributions of primary fragments. Focusing on the benchmark cases of neutron-induced fission of 235 U and 239 Pu , we predict—for the first time—microscopic angular momentum distributions for all fragments observed in experiments. Our results reveal a pronounced sawtooth pattern in the average angular momentum as a function of fragment mass, consistent with recent measurements. Additionally, we observe substantial variations in angular momentum distributions along isobaric chains, indicating that commonly used empirical formulas lack sufficient accuracy. We also quantify a strong correlation between the angular momentum and the deformation of the fragments at scission, and a weak correlation in the magnitude of the angular momentum between fragment partners. The generated data will enable estimation of the impact of microscopic distributions on fission spectra, paving the way toward fission modeling based on microscopic inputs.

Physics - Nuclear physics and radiation physics↗

A Pulsar-Inspired Timing Framework for Power System: Optimization and Performance Evaluation

Due to their excellent stability, neutron pulsar stars are considered promising candidate timing sources for power system applications. However, the complexity of pulsar signals necessitates advanced processing algorithms to provide accurate timing references. This paper presents the foundational framework for pulsar signal processing, serving as the basis for further optimization. To enhance the timing accuracy and computation efficiency in pulsar period searches, three algorithms are proposed as the initial optimization step: wavelet de-noising, fast folding, and cross-correlation for profile evaluation. Wavelet de-noising improves signal-to-noise ratio (SNR) by 36%–70%. Fast folding reduces computation time from hundreds of seconds to mere milliseconds. Cross-correlation works better than traditional SNR-based methods by effectively identifying the optimal period. The performance of the proposed algorithms is evaluated using observation data from telescopes. Together, these algorithms significantly improve pulsar timing performance, reducing the error of the Pulse Per Second (PPS) signal from hundreds to tens of microseconds.

Wu, Ori [ORNL] (ORCID:0000000326723410)↗

Feynman-α analysis using BGO gamma-ray detector in UTR-KINKI reactor

In conventional reactor noise measurement based on neutron detection, a neutron detector must be placed as close to a core as possible, to observe a largest possible correlation amplitude. For most of reactors other than critical assemblies, however, the placement is hardly possible. We focused on an alternative reactor noise measurement using prompt gamma-rays having a long flight range, to overcome the above constraint. A Feynman-α analysis using a NaI(Tl) scintillation detector was previously performed in UTR-KINKI, however, white noise originating from radioactivation of the scintillator significantly degraded the correlation amplitude. In this study, another Feynman-α analysis using a BGO gamma-ray detector, which never suffers from any radioactivation, is performed. A series of Feynman-α analyses for a critical state and several subcritical states of UTR-KINKI reactor has been carried out using two BGO detectors and a BF{sub 3} neutron detector to determine prompt-neutron decay constant. In the present analysis, the dead-time effect of these detectors and the delayed-neutron effect are considered. The prompt-neutron decay constant determined from Feynman-α analysis based on gamma-ray detection agrees with that from the analysis based on neutron detection. The Feynman-α analysis based on detecting gamma rays appears to be able to determine prompt-neutron decay constant at least as efficiently as the conventional analysis detecting neutrons.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Preliminary benchmarks and analysis of boundary conditions in a trenched microstructured silicon radiation detector

Microstructured neutron detectors have the benefit of enhanced neutron detection efficiency as compared to planar devices, achieved by etching 6 LiF-filled trenches on the top surface of a silicon PIN diode. This sensor geometry results in a complex electric field distribution and depletion characteristics within the diode under reverse bias. For the first time on record, the effects of a fixed oxide charge on the microstructured device depletion characteristics and mobile carrier transport is investigated. Prototype detectors were fabricated with non-conformal surface doping. Capacitance voltage and current voltage measurements were performed for these prototypes and compared with COMSOL Multiphysics simulations. A spectral response from an 241Am alpha particle source was acquired and analyzed. It was found that monoenergetic alpha particles produce three prominent peaks in the pulse height spectrum output by the device. The peaks were confirmed by simulations to correlate with dead layers and incident trajectories into the microstructure. It was also found that significant differences in pulse rise time result, corresponding with events arriving in a low-field region in the fins and a high-field region in the bulk. Geant4 was utilized for radiation transport, interaction modeling, and benchmarking the spectral data. The results of this simulation work provide confidence in the ability to attain and benchmark electrical characteristics and spectral data for semiconductor radiation detectors employing complex microstructures.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Air pollution source identification

The techniques available for source identification are reviewed: remote sensing, injected tracers, and pollutants themselves as tracers. The use of the large number of trace elements in the ambient airborne particulate matter as a practical means of identifying sources is discussed. Trace constituents are determined by sensitive, inexpensive, nondestructive, multielement analytical methods such as instrumental neutron activation and charged particle X-ray fluorescence. The application to a large data set of pairwise correlation, the more advanced pattern recognition-cluster analysis approach with and without training sets, enrichment factors, and pollutant concentration rose displays for each element is described. It is shown that elemental constituents are related to specific source types: earth crustal, automotive, metallurgical, and more specific industries. A field-ready source identification system based on time and wind direction resolved sampling is described.

Fordyce, J. S.↗

Neutrinos from SN 1987A - Implications for cooling of the nascent neutron star and the mass of the electron antineutrino

Data on neutrinos from SN 1987A are compared here with parameterized models of the neutrino emission using a consistent and straightforward statistical methodology. The empirically measured detector background spectra are included in the analysis, and the data are compared with a much wider variety of neutrino emission models than was explored previously. It is shown that the inferred neutrino emission model parameters are strongly correlated. The analysis confirms that simple models of the neutrino cooling of the nascent neutron star formed by the SN adequately explain the data. The inferred radius and binding energy of the neutron star are in excellent agreement with model calculations based on a wide range of equations of state. The results also raise the upper limit of the electron antineutrino rest mass to roughly 25 eV at the 95 percent confidence level, roughly 1.5-5 times higher than found previously.

Loredo, Thomas J.↗

Search For Electron-Antineutrinos Associated With 2 Gravitational-Wave Events GW150914, GW151012, GW151226, 3 GW170104, GW170608, GW170814, and GW170817 at Daya Bay

Providing a possible connection between neutrino emission and gravitational-wave (GW) bursts is important to our understanding of the physical processes that occur when black holes or neutron stars merge. In the Daya Bay experiment, using the data collected from December 2011 to August 2017, a search has been performed for electron-antineutrino signals coinciding with detected GW events, including GW150914, GW151012, GW151226, GW170104, GW170608, GW170814, and GW170817. We used three time windows of ±10 s, ±500 s, and ±1000 s relative to the occurrence of the GW events, and a neutrino energy range of 1.8 to 100 MeV to search for correlated neutrino candidates. The detected electron-antineutrino candidates are consistent with the expected background rates for all the three time windows. Assuming monochromatic spectra, we found upper limits (90% confidence level) on electron-antineutrino fluence of (1.13 - 2.44)×1011 cm-2 at 5 MeV to 8.0×107cm-2at 100 MeV for the three timewindows. Under the assumption of a Fermi-Dirac spectrum, the upper limits were found to be (5.4 - 7.0)×109 cm-2 for the three time windows.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗