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Induced activation study of LDEF

Analysis of the induced radioactivity of the Long Duration Exposure Facility (LDEF) is continuing with extraction of specific activities for various spacecraft materials. Data and results of activation measurements from eight facilities are being collected for interpretation at Eastern Kentucky University and NASA/Marshall Space Flight Center. The major activation mechanism in LDEF components is the proton flux in the South Atlantic Anomaly (SAA). This flux is highly anisotropic, and could be sampled by taking advantage of the gravity-gradient stabilization of the LDEF. The directionally-dependent activation due to these protons was clearly observed in the data from aluminum experiment tray clamps (reaction product Na-22), steel trunnions (reaction product Mn-54 and others) and is also indicated by the presence of a variety of nuclides in other materials. A secondary production mechanism, thermal neutron capture, was observed in cobalt, indium, and tantalum, which are known to have large capture cross sections. Experiments containing samples of these metals and significant amounts of thermalizing low atomic number (Z) material showed clear evidence of enhanced activation of Co-60, In-114m, and Ta-182. Other mechanisms which activate spacecraft material that are not as easily separable from SAA proton activation, such as galactic proton bombardment and secondary production by fast neutrons, are being investigated by comparison to radiation environmental calculations. Deviations from one-dimensional radiation models indicate that these mechanisms are more important at greater shielding depths. The current status of the induced radioactivity measurements as of mid-year 1992 are reviewed. Specific activities for a number of materials which show SAA effects and thermal neutron capture are presented. The results for consistency by combining data from the participating institutions is also examined.

Harmon, B. A.↗

Signature of a Massive Rotating Metal-poor Star Imprinted in the Phoenix Stellar Stream

The Phoenix stellar stream has a low intrinsic dispersion in velocity and metallicity that implies the progenitor was probably a low-mass globular cluster. In this work we use Magellan/Magellan Inamori Kyocera Echelle (MIKE) high-dispersion spectroscopy of eight Phoenix stream red giants to confirm this scenario. In particular, we find negligible intrinsic scatter in metallicity ($σ$([FE II/H]) = ${0.04}_{-0.03}^{+0.11}$) and a large peak-to-peak range in [Na/Fe] and [Al/Fe] abundance ratios, consistent with the light element abundance patterns seen in the most metal-poor globular clusters. However, unlike any other globular cluster, we also find an intrinsic spread in [Sr II/Fe] spanning ~1 dex, while [Ba II/Fe] shows nearly no intrinsic spread ($σ$([Ba II/H]) = ${0.03}_{-0.02}^{+0.10}$). This abundance signature is best interpreted as slow-neutron-capture element production from a massive fast-rotating metal-poor star (15–20 $M$ ⊙ , $v$ ini /$v$ crit = 0.4, [Fe/H] = -3.8). The low inferred cluster mass suggests the system would have been unable to retain supernovae ejecta, implying that any massive fast-rotating metal-poor star that enriched the interstellar medium must have formed and evolved before the globular cluster formed. Furthermore, neutron-capture element production from asymptotic giant branch stars or magneto-rotational instabilities in core-collapse supernovae provide poor fits to the observations. We also report one Phoenix stream star to be a lithium-rich giant ($A$(Li) = 3.1 ± 0.1). At [Fe/H ] = -2.93; it is among the most metal-poor lithium-rich giants known.

79 ASTRONOMY AND ASTROPHYSICS↗

Neutron tagging following atmospheric neutrino events in a water Cherenkov detector

We present the development of neutron-tagging techniques in Super-Kamiokande IV using a neural network analysis. The detection efficiency of neutron capture on hydrogen is estimated to be 26%, with a mis-tag rate of 0.016 per neutrino event. The uncertainty of the tagging efficiency is estimated to be 9.0%. Measurement of the tagging efficiency with data from an Americium-Beryllium calibration agrees with this value within 10%. The tagging procedure was performed on 3,244.4 days of SK-IV atmospheric neutrino data, identifying 18,091 neutrons in 26,473 neutrino events. The fitted neutron capture lifetime was measured as 218±9 μs.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Big-Bang Nucleosynthesis after Planck

We assess the status of big-bang nucleosynthesis (BBN) in light of the final Planck data release and other recent developments, and in anticipation of future measurements. Planck data from the recombination era fix the cosmic baryon density to 0.9% precision, and now damping tail measurements determine the helium abundance and effective number of neutrinos with precision approaching that of astronomical and BBN determinations respectively. All three parameters are related by BBN. In addition, new high-redshift measurements give D/H to better precision than theoretical predictions, and new Li/H data reconfirm the lithium problem. We present new 7 Be(n, p) 7 Li rates using new neutron capture measurements; we have also examined the effect of proposed changes in the d(p, γ) 3 He rates. Using these results we perform a series of likelihood analyses. We assess BBN/CMB consistency, with attention to how our results depend on the choice of Planck data, as well as how the results depend on the choice of non-BBN, non-Planck data sets. Most importantly the lithium problem remains, and indeed is more acute given the very tight D/H observational constraints; new neutron capture data reveals systematics that somewhat increases uncertainty and thus slightly reduces but does not essentially change the problem. We confirm that d(p, γ) 3 He theoretical rates brings D/H out of agreement and slightly increases 7 Li; new experimental data are needed at BBN energies. Setting the lithium problem aside, we find the effective number of neutrino species at BBN is Nν = 2.86±0.15. Future CMB Stage-4 measurements promise substantial improvements in BBN parameters: helium abundance determinations will be competitive with the best astronomical determinations, and Neff will approach sensitivities capable of detecting the effects of Standard Model neutrino heating of the primordial plasma.

79 ASTRONOMY AND ASTROPHYSICS↗

The R-Process Alliance: Hunting for gold in the near-UV spectrum of 2MASS J05383296–5904280

Over the past few years, the R-Process Alliance (RPA) has successfully carried out a search for stars that are highly enhanced in elements produced via the rapid neutron-capture (r-) process. In particular, the RPA has identified a number of relatively bright, highly r-process-enhanced (r-II) stars, suitable for observations with the Hubble Space Telescope (HST), facilitating abundance derivation of elements such as gold (Au) and cadmium (Cd). This paper presents the detailed abundances derived for the metal-poor ([Fe/H] = −2.55) highly r-process-enhanced ([Eu/Fe] = +1.29) r-II star 2MASS J05383296–5904280. One-dimensional local thermodynamic equilibrium (LTE) elemental abundances were derived via equivalent width and spectral synthesis using high-resolution high signal-to-noise near-UV HST/STIS and optical Magellan/MIKE spectra. Abundances were determined for 43 elements, including 26 neutron-capture elements. In particular, abundances of the rarely studied elements Nb, Mo, Cd, Lu, Os, Pt, and Au are derived from the HST spectrum. These results, combined with RPA near-UV observations of two additional r-II stars, increase the number of Cd abundances derived for r-process-enriched stars from seven to ten and Au abundances from four to seven. A large star-to-star scatter is detected for both of these elements, highlighting the need for more detections enabling further investigations, specifically into possible non-LTE effects.

chemically peculiar stars↗

An Updated Picture of Presolar History from Short-lived Radioactive Isotopes and Inferences on the Birth of the Sun

We examine the origin of the short-lived radionuclides (SLRs; defined as having half-lives between 0.1 and 100 Ma) present in the early solar system (ESS) by investigating how predictions of their abundances in the interstellar medium (ISM) from steady-state equilibrium relate to their ESS values. For this, we take into account the non-negligible time t iso elapsed between the isolation of the presolar molecular cloud and the formation of the ESS, during which the SLRs decayed freely. We also consider the alternative scenario in which the presolar molecular cloud remained partially mixed with the ISM, with a mixing timescale t mix . We find that the ESS abundances of 107 Pd and 182 Hf produced by slow neutron captures (s-process) and of 53 Mn and 60 Fe produced by explosive nucleosynthesis can be consistently explained within these scenarios. Their required tiso is 9–12 Ma and their required tmix is 11–14 Ma (with one potential exception of t mix = 38 Ma), depending on galactic uncertainties, such as the galactic star formation history and efficiency and the star-to-gas mass ratio. Another s -process SLR, 205 Pb, has a more uncertain ESS value and falls within only some of these time values. The same applies to the SLRs produced by the p -process ( 92 Nb and 146 Sm), depending on the latter’s half-life. In agreement with previous studies, we find that the ESS abundances of the rapid neutron-capture isotopes ( 129 I, 244 Pu, and 247 Cm) and of the most short-lived radionuclides ( 26 Al, 36 Cl, and 41 Ca) cannot be explained by assuming steady-state equilibrium in the ISM.

79 ASTRONOMY AND ASTROPHYSICS↗

Direct Mass Measurements to Inform the Behavior of 128m $\mathrm{Sb}$ in Nucleosynthetic Environments

Nuclear isomer effects are pivotal in understanding nuclear astrophysics, particularly in the rapid neutron-capture process where the population of metastable isomers can alter the radioactive decay paths of nuclei produced during astrophysical events. The β-decaying isomer 128m Sb was identified as potentially impactful since the β-decay pathway along the A = 128 isobar funnels into this state bypassing the ground state. Here we report the first direct mass measurements of the 128 Sb isomer and ground state using the Canadian Penning Trap mass spectrometer at Argonne National Laboratory. We find mass excesses of -84564.8(25) keV and -84608.8(21) keV, respectively, resulting in an excitation energy for the isomer of 43.9(33) keV. These results provide the first key nuclear data input for understanding the role of 128m Sb in nucleosynthesis, and we show that it will influence the flow of the rapid neutron-capture process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

StarHorse results for spectroscopic surveys and Gaia DR3: Chrono-chemical populations in the solar vicinity, the genuine thick disk, and young alpha-rich stars

The Gaia mission has provided an invaluable wealth of astrometric data for more than a billion stars in our Galaxy. The synergy between Gaia astrometry, photometry, and spectroscopic surveys gives us comprehensive information about the Milky Way. Using the Bayesian isochrone-fitting code StarHorse, we derive distances and extinctions for more than 10 million unique stars listed in both Gaia Data Release 3 and public spectroscopic surveys: 557 559 in GALAH+ DR3, 4 531 028 in LAMOST DR7 LRS, 347 535 in LAMOST DR7 MRS, 562 424 in APOGEE DR17, 471 490 in RAVE DR6, 249 991 in SDSS DR12 (optical spectra from BOSS and SEGUE), 67 562 in the Gaia-ESO DR5 survey, and 4 211 087 in the Gaia RVS part of the Gaia DR3 release. StarHorse can increase the precision of distance and extinction measurements where Gaia parallaxes alone would be uncertain. We used StarHorse for the first time to derive stellar ages for main-sequence turnoff and subgiant branch stars, around 2.5 million stars, with age uncertainties typically around 30%; the uncertainties drop to 15% for subgiant-branch-only stars, depending on the resolution of the survey. With the derived ages in hand, we investigated the chemical-age relations. In particular, the α and neutron-capture element ratios versus age in the solar neighbourhood show trends similar to previous works, validating our ages. We used the chemical abundances from local subgiant samples of GALAH DR3, APOGEE DR17, and LAMOST MRS DR7 to map groups with similar chemical compositions and StarHorse ages, using the dimensionality reduction technique t-SNE and the clustering algorithm HDBSCAN. We identify three distinct groups in all three samples, confirmed by their kinematic properties: the genuine chemical thick disk, the thin disk, and a considerable number of young alpha-rich stars (427) that are also a part of the delivered catalogues. We confirm that the genuine thick disk’s kinematics and age properties are radically different from those of the thin disk and compatible with high-redshift (z ≈ 2) star-forming disks with high dispersion velocities. We also find a few extra chemical populations in GALAH DR3 thanks to the availability of neutron-capture element information.

79 ASTRONOMY AND ASTROPHYSICS↗

The R -Process Alliance: Exploring the cosmic scatter among ten r -process sites with stellar abundances

Context. The astrophysical origin of the rapid neutron-capture process (r-process), responsible for producing roughly half of the elements heavier than iron, remains uncertain. Detailed chemical signatures from the oldest, most metal-poor stars, which act as fossil records of the earliest nucleosynthesis events, can be used to identify the dominant r-process sites. Aims. We present a homogeneous chemical abundance analysis of ten r-process element-enhanced stars. These old and metal-poor stars are strongly enriched in r-process elements with minimal contamination from other nucleosynthetic sources. By focusing on this chemically pure sample, we aim to investigate intrinsic variations in the r-process abundance patterns and explore their implications for the nature and potential diversity of r-process sites. Methods. We performed a detailed chemical abundance analysis of high-resolution, high-signal-to-noise spectra. For each star, we inspected over 1400 individual absorption lines using a combination of equivalent width measurements and spectral synthesis. The analysis was conducted under the assumption of 1D local thermodynamic equilibrium and employing the MOOG radiative transfer code. Results. We derived abundances for 54 chemical species, including 29 neutron-capture (n-capture) elements, covering the full mass range of the r-process abundance pattern. A kinematic analysis reveals that stars likely originated from ten kinematically distinct systems. Based on this assumption, we used the sample to probe the maximum variation expected from ten independent r-process nucleosynthesis events and computed the intrinsic dispersion of each element relative to Zr and Eu for the light and heavy r-process elements, respectively. This exercise resulted in a remarkably low cosmic scatter across the ten r-process sites enriching these stars; for the rare earth and third peak elements, for example, we find σ [La/Eu] = 0.08 and σ [Os/Eu] = 0.11 dex, while the scatter between light and heavy elements, σ [Zr/Eu] , is slightly higher at 0.18 dex. Conclusions. The elemental abundance patterns across the ten independent r-process sites show remarkably small cosmic dispersions. This minimal dispersion suggests a high degree of uniformity in r-process yields across diverse astrophysical environments.

Astronomy and AstroPhysics↗

Solid, structured composite neutron detectors with high dynamic range capability

Neutron detectors are essential across disciplines such as fundamental science, nuclear security, safeguards, and civilian applications. While 3 He-filled gas proportional counters have long been revered for their efficacy in detecting thermal neutrons and praised for their efficiency, neutron/gamma discrimination, and stability, the scarcity of 3He has spurred a search for alternatives. Here, we explore a solid structured scintillating particle composite (SPC) consisting of 6 Li-containing scintillating glass particles within an acrylic matrix as a neutron detector for high dynamic range applications. We show for the first time that an SPC neutron detector can boast an intrinsic detection efficiency of 0.261% for pure 252 Cf fission neutrons and an overall neutron detection efficiency of (0.546 ± 0.003)% at the Neutron Free-in-Air facility while being able to function in an intense gamma-ray environment. We also show that the SPC neutron detector supports fast neutron capture times and enables a dual-readout scheme that extends the detector dynamic range to high incident neutron fluxes. A scalable fabrication process allows for tailoring the SPC detector properties to the requirements of specific applications. Good agreement is found between the experimental results taken with a National Institute of Standards and Technology traceable 252 Cf source and the coupled MCNP6 and optical-ray-tracing simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Study of 149 Sm Capture and Total Cross Sections for Burnup Credit Applications [Slides]

This presentation highlights how capture and transmission measurements were performed with the DANCE (Detector for Advanced Neutron Capture Experiments) instrument with capture data from 8 eV – 1 keV, and DICER (Device for Indirect Capture Experiments on Radionuclides) instruments with transmission data from 1meV – 1 keV. There were additional measurements of 147 Sm which had contaminant in the samples, 3.4 eV strong resonance, interesting abnormalities. The data analysis is complete and the R-Matrix analysis almost (90%) complete.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Lunar neutron stratigraphy.

Study of the isotopic composition of gadolinium and samarium in four soil and seven drill stem samples returned by the Apollo 15 mission. The results show the possibility to date sedimentary processes on the lunar surface for time scales of around 100 million years because of the particular dependence of neutron capture reactions on depth. The neutron flux has a distinct peak as a function of depth. This peak appears to lie below the level of shallow cratering for time scales of less than one billion years and consequently forms a readily identified marker layer of both depth and time.

Russ, G. P., III↗

Production of Xenon-135 from isotopically enriched Xenon-134 and Xenon-136 Targets

Atmospheric radioxenon analyses conducted under the Comprehensive Test Ban Treaty Organization (CTBTO) necessitates the collection and analysis of air samples to quantify 135Xe, an indicator for nuclear explosions and reactor operations. Analytical instrument calibration for these analyses requires high quality, monoisotopic reference standards that are typically short lived, and therefore must be produced and shipped promptly to monitoring stations worldwide. This work describes the preparation of 135Xe by neutron capture (n, ?) on monoisotopic 134Xe, neutron irradiation (n,2n) on monoisotopic 136Xe, and high energy photon irradiation (?, n) on monoisotopic 136Xe. The targets are prepared by electromagnetic isotope separation of natural xenon. Results from each process are compared for 135Xe yield and purity.

07 ISOTOPE AND RADIATION SOURCES↗

Optimization of an Energy Tuning Assembly for High Explosives Detection

The Portable Isotopic Neutron Spectroscopy (PINS) system, employs neutron-induced gamma-ray spectroscopy and provides a nondestructive method for high explosives detection. In standard operation it uses Californium-252 as a neutron source. Operating PINS with a deuterium-tritium (DT) neutron generator has some advantages over Cf-252, including lifetime and ability to produce high-energy inelastic scattering gamma rays. However, current systems using DT neutron generators suffer from a high environmental background and reduced ability to induce neutron capture, reducing spectral quality and limiting nitrogen sensitivity. Here, this study presents the development of an energy-tuning assembly (ETA) designed to optimize the DT neutron energy spectrum to increase nitrogen reaction rates in a target, thereby improving high explosive detection capabilities. A metaheuristic optimization framework, MultiGNOWEE, coupled with MCNP, was employed to generate two ETA configurations: a single-objective ETA, which maximizes nitrogen capture reactions, and a multi-objective ETA, which balances neutron capture and inelastic scattering. Simulations demonstrated the optimized configurations achieved up to a 10-fold improvement in nitrogen capture rates compared to the bare configuration. Experimental validation was conducted using a DT neutron generator and a high-purity germanium (HPGe) detector. Two prototype ETAs were constructed and assessed on a melamine simulant. Measurements demonstrated improved nitrogen detection for both prototype ETA configurations when compared to the standard system.

97 MATHEMATICS AND COMPUTING↗

Innovative approaches to neutron beam optimization: A case study of FP14 at LANSCE

This paper describes an experimental method to acquire high resolution energy- and spatially- resolved neutron beam spots using the time-gated neutron imaging system with Teledyne Pi-MAX4 camera. These experimental data offer a unique opportunity for benchmarking beam spot simulations. High-quality simulations depend significantly on a high-fidelity geometry model, which can be challenging for legacy facilities. We informed our MCNPX geometry model by latest metrology survey employing Leica laser tracker ATS600. It gave us a high fidelity description of our facility geometry. Such a robust integration of novel tools and methods yields a previously unattainable level of accuracy in both predicting and capturing neutron beam spots, marking a notable advancement over traditional methods reliant on static image plates. Here, to demonstrate the practical application of these tools, we are showing a non-uniform beam spot challenge at our Flight Path 14 (FP14) at the Los Alamos Neutron Science Center (LANSCE). Our precise MCNPX prediction of beam spot shifting as function of neutron energy was confirmed by experimental beam spot measured with extremely high level of detail. Results of this research demonstrate a significant leap in neutron beam optimization at LANSCE and set a new benchmark in beam spot characterization. The advanced methods presented here have potential for adoption at similar research facilities worldwide, aiming at substantial improvement in neutron beam delivery for experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutron-induced capture-to-fission cross section ratio measured at LANSCE

Capture-to-fission cross section ratios are used as an alternative to absolute cross section measurements. This is due to the simplification on the calculations and the reduction of the uncertainties with respect to an absolute measurement of the cross section by eliminating experimental complications like self-absorption, beam/target overlap and non-uniformities. Different capture-to-fission reactions have been measured through the years at the Los Alamos Neutron Science Center (LANSCE) at Los Alamos National Laboratory (LANL) using the Detector for Advanced Neutron Capture Experiments (DANCE) combined with different fission detectors. Some of these are a Parallel Plate Avalanche Counter (PPAC) to detect fission fragments (FF), and the NEUtron detector array at DANCE (NEUANCE) to detect fission neutrons. As DANCE detects the γ-rays produced in capture and fission reactions, the fission instrument placed inside the DANCE cavity is used to tag the fission γ-rays for background identification and subtraction. Some examples of capture-to-fission ratio measurements performed with DANCE in the last years are the 233 U, 235 U and 239 Pu. The measurement technique, the different setups, and other potential applications of the instruments will be explained.

Nuclear Criticality Safety Program (NCSP)↗

High deuteron and neutron yields from the interaction of a petawatt laser with a cryogenic deuterium jet

A compact high-flux, short-pulse neutron source would have applications from nuclear astrophysics to cancer therapy. Laser-driven neutron sources can achieve fluxes much higher than spallation and reactor neutron sources by reducing the volume and time in which the neutron-producing reactions occur by orders of magnitude. We report progress towards an efficient laser-driven neutron source in experiments with a cryogenic deuterium jet on the Texas Petawatt laser. Neutrons were produced both by laser-accelerated multi-MeV deuterons colliding with Be and mixed metallic catchers and by d (d,n) 3 He fusion reactions within the jet. We observed deuteron yields of 10 13 /shot in quasi-Maxwellian distributions carrying ~8-10% of the input laser energy. We obtained neutron yields greater than 10 10 /shot and found indications of a deuteron-deuteron fusion neutron source with high peak flux (>10 22 cm -2 s -1 ). The estimated fusion neutron yield in our experiment is one order of magnitude higher than any previous laser-induced dd fusion reaction. Though many technical challenges will have to be overcome to convert this proof-of-principle experiment into a consistent ultra-high flux neutron source, the neutron fluxes achieved here suggest laser-driven neutron sources can support laboratory study of the rapid neutron-capture process, which is otherwise thought to occur only in astrophysical sites such as core-collapse supernova, and binary neutron star mergers.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗