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At least 199 records · Page 11

Miniature DC electromagnetic pumps of molten lead and sodium to support development of Gen-IV nuclear reactors

This work developed designs of submerged, dual-regions, miniature DC-EM pumps for circulating molten lead and liquid sodium at ≤500 °C without active cooling for use in ex-pile and in-pile test loops to support of materials and fuel developments for Gen-IV sodium and molten lead fast nuclear reactor. These pumps with two pumping regions are 57 mm, 66.8 mm, 95.4 mm, and 133.5 mm in diameter and have two Alnico 5 permanent magnets with Hiperco-50 pole pieces for focusing the magnetic field lines in the flow duct. The Equivalent Circuit Model (ECM) linked to the Finite Element Method Magnetics (FEMM) software in MATLAB platform calculated the pumps characteristics for a wide range of parameters. Also determined are the pumps dimensions for the highest cumulative pumping power and peak efficiency. These dimensions are the height, width, and length of the flow duct, the thickness of the Alnico magnets, the length of current electrodes, and the separation distance between the two pumping regions. For molten lead, the pumping power increases from 368 W to 728 W, and the peak efficiency from 14.7% to 31.6% with increased pump diameter from 57 mm to 133.5 mm. In conclusion, for liquid sodium, both the pumping power and peak efficiency are higher, increasing from 392 W to 767 W and from 44.3 to 51.2%, respectively, with increased pump diameter from 57 mm to 133.5 mm.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Nuclear thermal propulsion test facility requirements and development strategy

The Nuclear Thermal Propulsion (NTP) subpanel of the Space Nuclear Propulsion Test Facilities Panel evaluated facility requirements and strategies for nuclear thermal propulsion systems development. High pressure, solid core concepts were considered as the baseline for the evaluation, with low pressure concepts an alternative. The work of the NTP subpanel revealed that a wealth of facilities already exists to support NTP development, and that only a few new facilities must be constructed. Some modifications to existing facilities will be required. Present funding emphasis should be on long-lead-time items for the major new ground test facility complex and on facilities supporting nuclear fuel development, hot hydrogen flow test facilities, and low power critical facilities.

Allen, George C.↗

A Nuclear Cryogenic Propulsion Stage for Near-Term Space Missions

Development efforts in the United States have demonstrated the viability and performance potential of NTP systems. For example, Project Rover (1955 - 1973) completed 22 high power rocket reactor tests. Peak performances included operating at an average hydrogen exhaust temperature of 2550 K and a peak fuel power density of 5200 MW/m3 (Pewee test), operating at a thrust of 930 kN (Phoebus-2A test), and operating for 62.7 minutes on a single burn (NRXA6 test). Results from Project Rover indicated that an NTP system with a high thrust-toweight ratio and a specific impulse greater than 900 s would be feasible. Excellent results have also been obtained by Russia. Ternary carbide fuels developed in Russia may have the potential for providing even higher specific impulses.

Houts, Michael G.↗

NASA's Research in Aircraft Vulnerability Mitigation

Since its inception in 1958, the National Aeronautics and Space Administration s (NASA) role in civil aeronautics has been to develop high-risk, high-payoff technologies to meet critical national aviation challenges. Following the events of Sept. 11, 2001, NASA recognized that it now shared the responsibility for improving homeland security. The NASA Strategic Plan was modified to include requirements to enable a more secure air transportation system by investing in technologies and collaborating with other agencies, industry, and academia. NASA is conducting research to develop and advance innovative and commercially viable technologies that will reduce the vulnerability of aircraft to threats or hostile actions, and identify and inform users of potential vulnerabilities in a timely manner. Presented in this paper are research plans and preliminary status for mitigating the effects of damage due to direct attacks on civil transport aircraft. The NASA approach to mitigation includes: preventing loss of an aircraft due to a hit from man-portable air defense systems; developing fuel system technologies that prevent or minimize in-flight vulnerability to small arms or other projectiles; providing protection from electromagnetic energy attacks by detecting directed energy threats to aircraft and on/off-board systems; and minimizing the damage due to high-energy attacks (explosions and fire) by developing advanced lightweight, damage-resistant composites and structural concepts. An approach to preventing aircraft from being used as weapons of mass destruction will also be discussed.

Allen, Cheryl L.↗

Advanced Microscopy Report on UCO Fuel Kernels from Selected AGR-1 and AGR-2 Experiments

A variety of neutron irradiation experiments were completed at Idaho National Laboratory (INL) on tristructural isotropic (TRISO) coated particles contained in a graphitic matrix as part of the Advanced Gas Reactor (AGR) fuel development and qualification program. Although the initial advanced microscopy and microanalysis studies on AGR-1 particles focused predominantly on the SiC layer?s role as the main fission-product containment, studies were further expanded to evaluate UCO kernels of selected AGR-1 and AGR-2 coated particles. Fuel kernels tested in the AGR-1 and AGR-2 experiments is composed of a mixture of UO2 and UC, with a nominal as-fabricated stoichiometry of UO1.37 C0.35 and UO1.43 C0.39, respectively. These as-fabricated kernel-stoichiometry values are determined at the completion of kernel fabrication and do not account for any changes that will occur during the subsequent coating and compacting processes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-5/6/7 Irradiation As Run Predictions Using PARFUME

The PARticle FUel ModEl (PARFUME), a fuel performance modeling code used for high-temperature gas-cooled reactors, was used to model the Advanced Gas Reactor (AGR)-5/6/7 irradiation test using as-run physics and thermal data. The AGR-5/6/7 irradiation test consists of the combined fifth, sixth, and seventh planned irradiations of the AGR Fuel Development and Qualification Program. The AGR-5/6/7 test train is a multi-capsule, instrumented experiment that is designed for irradiation in the 133.4-mm diameter northeast flux trap position of the Advanced Test Reactor (ATR) at Idaho National Laboratory. Each capsule contains compacts filled with uranium oxycarbide unaltered fuel particles. This report documents the calculations performed to predict the failure probability of tristructural isotropic (TRISO)-coated fuel particles during the AGR-5/6/7 experiment. In addition, this report documents the calculated fission product release fraction from the fuel. The calculations include modeling of the AGR 5/6/7 irradiation that occurred from February 2018 to July 2020 over nine ATR cycles, including six normal cycles and three power axial locator mechanism cycles, for a total of approximately 376 effective full power days (EFPD). The irradiation conditions and material properties of the AGR-5/6/7 test predicted zero fuel particle failures in Capsules 1, 3, and 4. Fuel particle failures were predicted in two of the compacts in Capsule 2 and one particle failure is predicted in each one of the compacts in Capsule 5. All compacts that exhibited fuel particle failures predicted by PARFUME were caused by localized stress concentrations in the silicon carbide (SiC) layer caused by cracking in the inner pyrolytic (IPyC) layer. In addition, shrinkage of the buffer and IPyC layer during irradiation resulted in formation of a buffer-IPyC gap. Compacts with a lower irradiation temperature and fluence experienced the smallest buffer-IPyC gap formation. Conversely, higher irradiated temperature compacts with a high fluence experienced the largest buffer-IPyC gap formation. Compact 3-6-3 experienced the largest buffer IPyC gap formation of just under 21.7 µm. The release fraction of fission products silver (Ag), cesium (Cs), and strontium (Sr) vary depending on capsule location and irradiation temperature. The maximum release fraction of Ag occurs in Capsule 3, reaching up to 59.5% for the TRISO fuel particles (compact 3-6-3). The release fraction of the other two fission products, Cs and Sr, are much smaller. A maximum Cs release fraction of 1.1% occurred in compact 3-4-3 and 4.4% for Sr in compact 3-6-3.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Safety Testing of AGR-5/6/7 Compacts 2-2-2 and 2-2-4

Compacts 2-2-2 and 2-2-4 from the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program’s final irradiation campaign (AGR-5/6/7) were each separately subjected to a thermal soak at 1600°C for 300 h under flowing helium to simulated conditions experienced during a postulated high-temperature gas-cooled reactor (HTGR) depressurization conduction cooldown event. The safety testing of the fuel compacts’ performance under accident conditions was conducted in the Oak Ridge National Laboratory (ORNL) Core Conduction Cooldown Test Facility (CCCTF), which utilizes a stand-alone hot cell at the Irradiated Fuels Examination Laboratory (IFEL). The CCCTF heats fuel to temperatures up to 1900°C in a non-oxidizing environment while continuously monitoring the sweep gas for radioactive 85 Kr to detect release levels associated with hermetic failure of the tristructural-isotropic (TRISO) coating surrounding each fuel kernel. In addition, certain metallic radionuclides that escape the fuel compact are collected on deposition cups that are periodically exchanged with a new cup to obtain information on the overall retention behavior of the TRISO coating layers. Because cesium can diffuse through intact pyrocarbon layers, abnormal degradation of the silicon carbide (SiC) layer in the absence of holistic TRISO coating failure is indicated by release of 134 Cs at levels equivalent to an individual particle inventory in the absence of significant 85 Kr release (Hunn et al. 2014). Additional description of the CCCTF system is provided in Appendix A.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessment of buffer-IPyC thermomechanical debonding behavior using new experimental strength data in BISON

TRIstructural ISOtropic (TRISO) fuel is a nuclear fuel commonly used in High Temperature Gas-cooled Reactors (HTGRs). A single sub-millimeter-diameter TRISO fuel particle consists of a spherical fuel kernel surrounded by four coating layers: a low-density pyrocarbon buffer layer, an inner pyrolytic carbon (IPyC) layer, a silicon carbide (SiC) layer, and an outer pyrolytic carbon (OPyC) layer. The kernel is commonly made of UO2 or a mixture of uranium carbide and uranium oxide (UCO). During reactor operation, the TRISO coating layers are subjected to irradiation-induced dimensional changes and the associated thermomechanical behavior of each layer. One of the observed behaviors is gap formation between the buffer and IPyC layer due to the porous buffer’s irradiation-induced shrinkage exceeding that of the IPyC layer. Not all irradiated particles will experience buffer-IPyC gap formation. The debonding may be partial, or it may be nearly total. However, from post-irradiation examination of UCO TRISO fuels irradiated as part of the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program, it was concluded that partial buffer-IPyC debonding was the most common type of buffer-IPyC interaction. To predict TRISO thermomechanical performance, multi-physics models have been built that are being continually updated and refined. The BISON code is a finite element-based nuclear fuel performance code that may be used for 1D, 2D, and 3D TRISO particle simulations. This code is used to calculate fuel temperature, kernel swelling, buffer densification, thermal and irradiation creep, fracture, and fission gas production and release. One of the recent additions to the BISON code is the ability to model the process of layer debonding. This paper will focus on the simulation results of the improved BISON debonding model that will utilize updated strengths measured from irradiated AGR TRISO fuel particles. The new experimental strength data from micromechanical tests of irradiated TRISO fuel samples were exercised in the BISON simulations and compared to baseline strength data to assess their applicability in the models. This also includes updated buffer-IPyC bond strengths to simulate layer delamination. Based on current experimental observations it is noted that the buffer-IPyC separation occurs not exactly at the junction of these two layers, but more on the side of the buffer layer. That observation is also implemented in the TRISO interface debonding model. This improved modeling approach using experimental strength data to characterize buffer-IPyC debonding and its potential subsequent cracking will be presented in the paper along with comparisons to available experimental observations.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Buffer-IPyC separation process in TRISO fuel particles simulated with Bison code

During High Temperature Gas-cooled Reactor (HTGR) operation, tristructural isotropic (TRISO) coated-particle fuel undergoes irradiation-induced changes in morphology and thermomechanical properties. Experimental results from the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program show, among other things, the mechanism of gap formation between the buffer and inner pyrolytic carbon (IPyC) layers, which could be explored further via computational simulations using the Bison code. Two simulation models were developed, the debonding restricted model, where no gap formation between buffer and IPyC layers is permitted, and the debonding enabled model, where the gap between those layers is created. The inputs of the simulated models are based on the irradiation conditions from the AGR-1 experiment. The research included simulations on spherical and aspherical fuel types. Under the specific temperatures and fluences of the AGR-1 irradiation experiment, and the Bison simulations, it was concluded that the most common scenario is a gap formation along the buffer-IPyC interface, while the least possible scenario is the situation where there is no gap formation at the buffer-IPyC junction. The computational results confirmed that the sphericity of the fuel influences the thickness of the gap that occurs at the buffer-IPyC junction, in a way that with increasing aspect ratio the gap thickness increases. The results obtained for spherical and aspherical fuel are nearly identical. Finally, performed simulations match conclusions observed from the AGR-1 experiment, which as such shows that the Bison code is a good computational method for simulating the TRISO fuel. Future simulations will include the validation of performed research and comparison of the results between Bison and PARFUME codes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-2 TRISO Shadow Imaging Archive

As a part of fuel quality control characterization, backlit shadow images of particles produced by the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program’s AGR-2 irradiation campaign were acquired at Oak Ridge National Laboratory (ORNL). These images may be of use for the development of image processing algorithms with the benchmark values measured at ORNL. This report provides those benchmark values, along with the raw images and data generated by the ORNL shadow imaging process.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Quantitative Insight to Fission Gas Bubble Distribution in Irradiated Annular U-10Zr Metallic Fuel Using Deep Learning

U-10Zr Metal fuel is a promising nuclear fuel candidate for next-generation sodium-cooled fast spectrum reactors. Porosity is one of the key facts to impact the performance of metallic fuel. Additionally, a mechanical understanding of fission gas bubbles evolution behavior is a prerequisite for fuel development and qualification. Previous study of fission gas bubbles relied on a simple threshold method working on low resolution optical microscopy images, which has challenges in recognizing bubble boundaries, and caused inaccurate statistics of bubble properties. In this paper, a pre-trained deep learning model on Scanning Electron Microscopy (SEM) images from an annular U-10Zr fuel (AF1), was applied to another U-10Zr annular fuel (AF2). More accurate fission gas bubble segmentation results were generated, which leads to more precise qualitative analysis on the morphology, size, density, and orientation of bubbles. Furthermore, we investigated the lanthanide movement along the radial temperature gradient and obtained conclusive findings.

36 MATERIALS SCIENCE↗

AGR-2 TRISO Layer Thickness Imaging Archive

As a part of fuel quality control characterization, optical microscopy images of particle cross sections near midplane were acquired at Oak Ridge National Laboratory (ORNL). These particles were produced by the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program’s AGR-2 irradiation campaign. These images may be of use for the development of image processing algorithms with the benchmark values measured at ORNL. This report provides those benchmark values, along with the raw images and data generated by the ORNL particle layer thickness analysis process.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Unitized Regenerative Fuel Cell System Model Development

A Unitized Regenerative Fuel Cell (URFC) Energy Storage System is being developed at the NASA Glenn Research Center. This URFC system is unique in that it uses the surface area of the hydrogen and oxygen storage tanks as radiating heat surfaces for overall thermal control of the system. The tank surfaces also play an important role in the temperature control of regenerative gas dryers/humidifiers used to dry the hydrogen and oxygen gases produced by electrolysis during the charging and also used to humidify the hydrogen and oxygen gases used by fuel cell during the discharging of the URFCS. A bi- directional pressure controller is used to control the pressure of the oxygen and hydrogen gas inside the URFC stack during both charging and discharging of the URFC system. A water storage accumulator is used to store water reactant and control water pressure inside the URFC stack.

Burke, Kenneth A.↗

AGR TRISO Fuel Performance Modeling in FY-25

This report summarizes the activities performed in FY-25 to support fuel performance modeling for the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program. This includes implementation of a new uranium oxycarbide (UCO) kernel swelling rate model, inner pyrolytic carbon (IPyC) cracking behavior and failure predictions, development of new UCO and silicon carbide (SiC) cesium diffusion parameters, and the thermomechanical behavior of particle layers using experimental data from micro-tensile strength testing.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Develop and test fuel cell powered on-site integrated total energy system. Phase 3: Full-scale power plant development

An integrated 5 kW power system based upon methanol fuel and a phosphoric acid fuel cell operating at about 473 K is described. Description includes test results of advanced fuel cell catalysts, a semiautomatic acid replenishment system and a completed 5 kW methanol/system reformer. The results of a preliminary system test on a reformer/stack/inverter combination are reported. An initial design for a 25 kW stack is presented. Experimental plans are outlined for data acquisition necessary for design of a 50 kW methanol/steam reformer. Activities related to complete mathematical modelling of the integrated power system, including wasteheat utilization, are described.

Kaufman, A.↗

EDM Hole Drilling Template

The Fuels Development Team's goal is to try to learn drilling speeds and electrode dimensions to achieve desired diameters on a ZrC disk. We desire to send both the drawing and material to Sodick for drilling.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Multiscale, mechanistic modeling of irradiation-enhanced silver diffusion in TRISO particles

Tristructural isotropic (TRISO) particles are under consideration for use in several proposed advanced nuclear reactor concepts. The silicon carbide (SiC) layer in TRISO acts as a barrier to prevent the release of the fission products. However, despite remarkable retention, silver (Ag) release has been observed from intact particles, which requires investigation since the Ag isotope ( 110m Ag) has a long half-life. Previous work focused on developing a multiscale, mechanistic model for Ag diffusion accounting for temperature and microstructure effect and has been successfully validated. In this work, we expand the previous model to account for irradiation-enhanced Ag diffusivity in SiC and improve its accuracy over a wider grain size and temperature ranges relevant for advanced reactor conditions. A temperature, grain size, and flux dependent diffusivity is therefore derived using the mesoscale code MARMOT and implemented in the fuel performance code BISON. The irradiation-enhanced Ag diffusivity in SiC is compared against experimental data and validated using BISON against Ag release measurements from the Advanced Gas Reactor Fuel Development and Qualification Program (AGR-1 and AGR-2). Herein, we quantify the impact of SiC grain size, irradiation, and temperature on Ag release. In agreement with previous studies, we find accounting for SiC grain size improves agreement between BISON predictions and experimental observations for most cases. In conclusion, we also find that accounting for irradiation improves agreement for cases where Ag release was underestimated, but the impact was less significant than accounting for microstructure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Refining Absorber Shroud Geometry to Maximize Power Output and Reduce Power Peaking in ATF Test Train

In the wake of the Fukushima Daiichi nuclear power plant accident in 2011, the accident tolerant fuels (ATF) program was initiated to enhance the safety of light-water reactor fuels, placing significant emphasis on cladding. A crucial step for the broad implementation of ATF in commercial reactors involves irradiation testing of the fuel designs. ATF-2D, the latest experiment in the ATF series, is slated to undergo irradiation in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). ATF-2D is a joint effort of the INL with industry partners General Electric Global Research; Framatome; General Atomics; the Japan Atomic Energy Agency; Hitachi-GE Nuclear Energy, Ltd; Global Nuclear Fuel-Japan Co., Ltd; Nippon Nuclear Fuel Development Co., Ltd; and Mitsubishi Heavy Industries, Ltd. The ATF-2D test train design consists of four tiers, each housing six rodlets. The device will be inserted in Loop 2A within the central flux trap of the ATR, and is anticipated to undergo irradiation throughout three 60-day cycles. Typical pressurized water reactor conditions will be emulated during the irradiation. The objective of the work presented here is to dimension neutron-absorbing hafnium (Hf) components surrounding the fuel rodlets, such that the axial power profile is flattened, while simultaneously ensuring that the total fission power output of the entire test train remains below 200 kW.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗