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At least 199 records · Page 11

Kaluza-Klein graviton freeze-in and big bang nucleosynthesis

In models featuring extra spatial dimensions, particle collisions in the early Universe can produce Kaluza-Klein gravitons. Such particles will later decay, potentially impacting the process of big bang nucleosynthesis. In this paper, we consider scenarios in which gravity is free to propagate throughout n flat, compactified extra dimensions, while the fields of the Standard Model are confined to a ( 3 + 1 )-dimensional brane. We calculate the production and decay rates of the states that make up the Kaluza-Klein graviton tower and determine the evolution of their abundances in the early Universe. We then go on to evaluate the impact of these decays on the resulting light element abundances. We identify significant regions of previously unexplored parameter space that are inconsistent with measurements of the primordial helium and deuterium abundances. In particular, we find that for the case of one extra dimension (two extra dimensions), the fundamental scale of gravity must be M ⋆ ≳ 2 × 10 13 GeV ( M ⋆ ≳ 1 0 10 GeV ) unless the temperature of the early Universe was never greater than T ∼ 2 TeV ( T ∼ 1 GeV ). For larger values of n , these constraints are less stringent. For the case of n = 6 , for example, our analysis excludes all values of M ⋆ less than ∼ 10 6 GeV , unless the temperature of the Universe was never greater than T ∼ 3 TeV . The results presented here severely limit the possibility that black holes were efficiently produced through particle collisions in the early Universe’s thermal bath. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Metastability of Liquid Water Freezing into Ice VII under Dynamic Compression

The ubiquitous nature and unusual properties of water have motivated many studies on its metastability under temperature- or pressure-induced phase transformations. Here, nanosecond compression by a high-power laser is used to create the nonequilibrium conditions where liquid water persists well into the stable region of ice VII. Through our experiments, as well as a complementary theoretical/computational analysis based on classical nucleation theory, we report that the metastability limit of liquid water under nearly isentropic compression from ambient conditions is at least 8 GPa, higher than the 7 GPa previously reported for lower loading rates.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Composite Cathode Architectures Made By Freeze-Casting for All Solid State Lithium Batteries (CRADA Final Report)

As part of a Battery 500 seedling project, MBRDNA partnered with LBNL and Montana State University (MSU) to develop solid-state batteries based on an Al-substituted LLZO (Li 7 La 3 Zr 2 O 12 ) ceramic ion-conductor. All solid-state lithium batteries are attractive contenders for use as power sources for electric vehicles because of their potential for better safety and higher energy density than state-of-the-art lithium-ion batteries, although they are still at early stages of development. Al-substituted LLZO is one of the most promising solid electrolytes for battery applications based on high ionic conductivity, a wide operating voltage window, and apparent stability vs. reduction by lithium. However, difficulties with processing thin (< 20 $\textit{um}$ and dense LLZO membranes have hampered development of devices based on this material. It is non-compressible and must be sintered at high temperatures to densify components. It is also difficult to maintain contact between the active cathode material and LLZO in the composite cathodes, which is critical for successful operation. This research project aimed to use novel processing methods to overcome these issues. The end result was the first ever-reported truly all solid-state battery based on LLZO operating at room temperature without application of exogenous pressure. During the course of the project, we also identified a number of issues that need to be addressed to improve the technology readiness level of this battery.

25 ENERGY STORAGE↗

Freezing Processes in Southern Ocean Mixed Phase Clouds (Final Technical Report)

Southern Ocean (SO) low-level clouds remain a challenge for Earth system models to represent accurately. This project utilized DOE ARM observations and the Community Atmosphere Model (CAM) to improve process-level understanding of aerosol-cloud interactions and cloud microphysics for SO mixed-phase clouds. Specifically, our efforts include two main topics: 1) investigate the SO aerosol, cloud condensation nuclei (CCN), and ice nucleating particle (INP) population based on observations and determine predictive skill of simulating SO INPs, and 2) assess the ice formation pathways, including ice nucleation and secondary ice production, in SO mixed phase clouds utilizing a combination of observations and modeling tools. Studies focused on SO aerosol and INP resulted four manuscripts. Ice formation pathways in SO mixed phase clouds were investigated, revealing observed evidence of SIP active across all mixed phase temperatures. However, a key finding of this project is that despite significant progress in predicting SO INPs, the role of INP variability in SO cloud phase, precipitation, and radiative properties remain unknown due to challenges in microphysics parameterizations.

54 ENVIRONMENTAL SCIENCES↗