Heating dynamics of CO{sub 2}-laser irradiated silica particles with evaporative shrinking: Measurements and modeling
The heating dynamics of CO{sub 2}-laser heated micron-sized particles were determined for temperatures <3500 K measured using infrared imaging. A coupled mass and energy conservation model is derived to predict single particle temperatures and sizes, which were compared with data from particles deposited on non-absorbing substrates to assess the relevant heat transfer processes. Analysis reveals substrate conduction dominates all other heat losses, while laser absorption determined from Mie theory is strongly modulated by particle evaporative shrinking. This study provides insights into the light coupling and heating of particle arrays where the material optical properties are temperature-dependent and particle size changes are significant.