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At least 199 records · Page 11

Model test of CCN-cloud albedo climate forcing

Cloud condensation nuclei (CCN) influence cloud albedo through their effect on the cloud droplet size distribution. A number of studies have evaluated the climatic impact of the CCN-cloud albedo feedback, but all have assumed that cloud distributions, cloud thicknesses, and cloud liquid water contents would remain constant as the climate adjusted. This assumption has been tested using the Livermore version of the National Center for Atmospheric Research Community Climate Model. The results indicate that there are no significant compensating changes in cloud properties that would counteract the 1.7 percent global albedo increase resulting from a fourfold increase in marine CCN concentration. Furthermore, when ocean surface temperatures are decreased 4 C in a manner broadly consistent with the enhanced cloud albedos, an increase in cloud fraction of 3.5 percent and a reduction in cloud altitude are predicted, leading to a positive feedback from clouds that would imply a climate impact roughly double that calculated from cloud droplet size distribution change alone.

Ghan, S. J.↗

Climatology of the Vertical Profiles of Polarimetric Radar Variables and Retrieved Microphysical Parameters in Continental/Tropical MCSs and Landfalling Hurricanes

Most existing cloud models tend to overestimate the size of cloud ice particles and underestimate their concentration. This emphasizes the need to provide a reliable observational reference to optimize cloud model performance, particularly in areas of high concentration of ice at high altitudes. The dual-polarization radars give the community a unique opportunity to quantify cloud ice with a good accuracy using polarimetric radar retrievals. Here, in this study, we utilize the network of operational WSR-88D radars to build a climatology of the vertical profiles of radar variables, such as radar reflectivity Z, differential reflectivity Z DR , and specific differential phase K DP as well as the radar-retrieved vertical profiles of ice water content (IWC) above the melting layer and liquid water content below it, mean volume diameter D m , and total number concentration N t of ice and liquid particles. Such climatology was created for continental/marine mesoscale convective systems (MCSs) and tropical cyclones including hurricanes. The dataset includes 13 continental MCSs, 10 marine MCSs, and 11 tropical cyclones. Separate statistics of the “background” vertical profiles and the ones associated with high IWC aloft have been obtained in the course of this study. It is shown that continental MCSs exhibit larger size of ice in lower concentration aloft compared to the marine MCSs and especially tropical cyclones/hurricanes. A combination of high KDP and low Z aloft signifies lower D m , higher N t , and often substantial IWC.

54 ENVIRONMENTAL SCIENCES↗

Comparison of Lidar Backscatter with Particle Distribution and GOES-7 Data in Hurricane Juliette

Measurements of calibrated backscatter, using two continuous wave Doppler lidars operating at wavelengths 9.1 and 10.6 micrometers were obtained along with cloud particle size distributions in Hurricane Juliette on 21 September 1995 at altitude approximately 11.7 km. Agreement between backscatter from the two lidars and with the cloud particle size distribution is excellent. Features in backscatter and particle number density compare well with concurrent GOES-7 infrared images.

Jarzembski, Maurice A.↗

The three-dimensional structure of cumulus clouds over the ocean. 1: Structural analysis

Thermal channel (channel 6, 10.4-12.5 micrometers) images of five Landsat thematic mapper cumulus scenes over the ocean are examined. These images are thresholded using the standard International Satellite Cloud Climatology Project (ISCCP) thermal threshold algorithm. The individual clouds in the cloud fields are segmented to obtain their structural statistics which include size distribution, orientation angle, horizontal aspect ratio, and perimeter-to-area (PtA) relationship. The cloud size distributions exhibit a double power law with the smaller clouds having a smaller absolute exponent. The cloud orientation angles, horizontal aspect ratios, and PtA exponents are found in good agreement with earlier studies. A technique also is developed to recognize individual cells within a cloud so that statistics of cloud cellular structure can be obtained. Cell structural statistics are computed for each cloud. Unicellular clouds are generally smaller (less than or equal to 1 km) and have smaller PtA exponents, while multicellular clouds are larger (greater than or equal to 1 km) and have larger PtA exponents. Cell structural statistics are similar to those of the smaller clouds. When each cell is approximated as a quadric surface using a linear least squares fit, most cells have the shape of a hyperboloid of one sheet, but about 15% of the cells are best modeled by a hyperboloid of two sheets. Less than 1% of the clouds are ellipsoidal. The number of cells in a cloud increases slightly faster than linearly with increasing cloud size. The mean nearest neighbor distance between cells in a cloud, however, appears to increase linearly with increasing cloud size and to reach a maximum when the cloud effective diameter is about 10 km; then it decreases with increasing cloud size. Sensitivity studies of threshold and lapse rate show that neither has a significant impact upon the results. A goodness-of-fit ratio is used to provide a quantitative measure of the individual cloud results. Significantly improved results are obtained after applying a smoothing operator, suggesting the eliminating subresolution scale variations with higher spatial resolution may yield even better shape analyses.

Kuo, Kwo-Sen↗

Cloud microstructure as determined by an optical cloud particle spectrometer.

Use of an improved single-particle light-scattering instrument for measurement of cloud microstructure in field studies. Cloud particle size and number information is measured over 12 sizing intervals, in the range from 4 to 85 microns in diameter. The microstructure can be observed in real time and with a spatial resolution not previously reported. The general features of water cloud droplet size and number distributions are consistent with previous direct capture and replication studies. The transition from water to ice phase regions in cumuliform clouds can be inferred from dramatic changes observed in the distribution features. Results are also presented for stratus and cirrus cloud penetrations.

Ryan, R. T.↗

Particle size distributions in Arctic polar stratospheric clouds, growth and freezing of sulfuric acid droplets, and implications for cloud formation

The paper uses particle size and volume measurements obtained with the forward scattering spectrometer probe model 300 during January and February 1989 in the Airborne Arctic Stratospheric Experiment to investigate processes important in the formation and growth of polar stratospheric cloud (PSC) particles. It is suggested on the basis of comparisons of the observations with expected sulfuric acid droplet deliquescence that in the Arctic a major fraction of the sulfuric acid droplets remain liquid until temperatures at least as low as 193 K. It is proposed that homogeneous freezing of the sulfuric acid droplets might occur near 190 K and might play a role in the formation of PSCs.

Dye, James E.↗

Evidence for Natural Variability in Marine Stratocumulus Cloud Properties Due to Cloud-Aerosol

In this study, aircraft observations from the Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter are used to characterize the variability in drizzle, cloud, and aerosol properties associated with cloud rifts and the surrounding solid clouds observed off the coast of California. A flight made on 16 July 1999 provided measurements directly across an interface between solid and rift cloud conditions. Aircraft instrumentation allowed for measurements of aerosol, cloud droplet, and drizzle spectra. CCN concentrations were measured in addition to standard thermodynamic variables and the winds. A Forward Scatter Spectrometer Probe (FSSP) measured size distribution of cloud-sized droplets. A Cloud Imaging Probe (CIP) was used to measure distributions of drizzle-sized droplets. Aerosol distributions were obtained from a Cloud Aerosol Scatterprobe (CAS). The CAS probe measured aerosols, cloud droplets and drizzle-sized drops; for this study. The CAS probe was used to measure aerosols in the size range of 0.5 micron - 1 micron. Smaller aerosols were characterized using an Ultrafine Condensation Particle Counter (CPC) sensor. The CPC was used to measure particles with diameters greater than 0.003 micron. By subtracting different count concentrations measured with the CPC, this probe was capable of identifying ultrafine particles those falling in the size range of 3 nanometers - 7 nanometers that are believed to be associated with new particle production.

Albrecht, Bruce↗

Are turbulence effects on droplet collision–coalescence a key to understanding observed rain formation in clouds?

Rain formation is a critical factor governing the lifecycle and radiative forcing of clouds and therefore it is a key element of weather and climate. Cloud microphysics–turbulence interactions occur across a wide range of scales and are challenging to represent in atmospheric models with limited resolution. Based on past experiments and idealized numerical simulations, it has been postulated that cloud turbulence accelerates rain formation by enhancing drop collision–coalescence. We provide substantial evidence for significant impacts of turbulence on the evolution of cloud droplet size distributions and rain formation by comparing high-resolution observations of cumulus congestus clouds with state-of-the-art large-eddy simulations coupled with a Lagrangian particle-based microphysics scheme. Turbulent coalescence must be included in the model to accurately represent the observed drop size distributions, especially for drizzle drop sizes at lower heights in the cloud. Turbulence causes earlier rain formation and greater rain accumulation compared to simulations with gravitational coalescence only. The observed rain size distribution tail just above cloud base follows a power law scaling that deviates from theoretical scalings considering either a purely gravitation collision kernel or a turbulent kernel neglecting droplet inertial effects, providing additional evidence for turbulent coalescence in clouds. In contrast, large aerosols acting as cloud condensation nuclei (“giant CCN”) do not significantly impact rain formation owing to their long timescale to reach equilibrium wet size relative to the lifetime of rising cumulus thermals. Overall, turbulent drop coalescence exerts a dominant influence on rain initiation in warm cumulus clouds, with limited impacts of giant CCN.

54 ENVIRONMENTAL SCIENCES↗

Modeling the Impact of Drizzle and 3D Cloud Structure on Remote Sensing of Effective Radius

Remote sensing of cloud particle size with passive sensors like MODIS is an important tool for cloud microphysical studies. As a measure of the radiatively relevant droplet size, effective radius can be retrieved with different combinations of visible through shortwave infrared channels. MODIS observations sometimes show significantly larger effective radii in marine boundary layer cloud fields derived from the 1.6 and 2.1 pm channel observations than for 3.7 pm retrievals. Possible explanations range from 3D radiative transport effects and sub-pixel cloud inhomogeneity to the impact of drizzle formation on the droplet distribution. To investigate the potential influence of these factors, we use LES boundary layer cloud simulations in combination with 3D Monte Carlo simulations of MODIS observations. LES simulations of warm cloud spectral microphysics for cases of marine stratus and broken stratocumulus, each for two different values of cloud condensation nuclei density, produce cloud structures comprising droplet size distributions with and without drizzle size drops. In this study, synthetic MODIS observations generated from 3D radiative transport simulations that consider the full droplet size distribution will be generated for each scene. The operational MODIS effective radius retrievals will then be applied to the simulated reflectances and the results compared with the LES microphysics.

Platnick, Steven↗

What does reflection from cloud sides tell us about vertical distribution of cloud droplets?

In order to accurately measure the interaction of clouds with aerosols, we have to resolve the vertical distribution of cloud droplet sizes and determine the temperature of glaciation for clean and polluted clouds. Knowledge of the droplet vertical profile is also essential for understanding precipitation. So far, all existing satellites either measure cloud microphysics only at cloud top (e.g., MODIS) or give a vertical profile of precipitation sized droplets (e.g., Cloudsat). What if one measures cloud microphysical properties in the vertical by retrieving them from the solar and infrared radiation reflected or emitted from cloud sides? This was the idea behind CLAIM-3D (A 3D - cloud aerosol interaction mission) recently proposed by NASA GSFC. This presentation will focus on the interpretation of the radiation reflected from cloud sides. In contrast to plane-parallel approximation, a conventional approach to all current operational retrievals, 3D radiative transfer will be used for interpreting the observed reflectances. As a proof of concept, we will show a few examples of radiation reflected from cloud fields generated by a simple stochastic cloud model with prescribed microphysics. Instead of fixed values of the retrieved effective radii, the probability density functions of droplet size distributions will serve as possible retrievals.

Marshak, A.↗

Physical and Optical/Radiative Characteristics of Small Particles in Tropical Cirrus

Whether cirrus clouds heat or cool the Earth-atmosphere system depends on the relative importance of the cloud shortwave albedo effect and the cloud thermal greenhouse effect. Both an determined by the distribution of ice condensate with cloud particle size. The microphysics instrument package flown aboard the DC-8 In TOGA/COARE included an ice crystal replicator, a 2D Greyscale Cloud Particle Probe and a Forward Scattering Spectrometer Aerosol Probe. In combination. these instruments permitted particle size measurements between 0.5 micrometers and 2.6 mm diameter. Ice crystal replicas were used to validate signals from the electro-optical instruments. Typical results show a prevalence in tropical cirrus clouds of micron-sized particles, in addition to cloud particles that exceed 100 micrometer radius. The mechanism of their formation is growth of (hygroscopic, possibly ocean-derived) aerosol particles along the Kohler curves. The concentration of small particles is higher and less variable in space and time, and their tropospheric residence time is longer, than those of large cloud particles because of lower sedimentation velocities. Small particles shift effective cloud particle radii to sizes much smaller than the mean diameter of the cloud particles. This causes an increase in shortwave reflectivity and IR emissivity. and a decrease in transmissivity. In the cirrus outflow of tropical cyclone Oliver on 8 February, 1993, the reflectivity increases with altitude (decreasing temperature) stronger than does cloud emissivity, yielding enhanced radiative cooling at higher altitudes.

Pueschel, R. F.↗

Using the Bootstrap Method for a Statistical Significance Test of Differences between Summary Histograms

A new method is proposed to compare statistical differences between summary histograms, which are the histograms summed over a large ensemble of individual histograms. It consists of choosing a distance statistic for measuring the difference between summary histograms and using a bootstrap procedure to calculate the statistical significance level. Bootstrapping is an approach to statistical inference that makes few assumptions about the underlying probability distribution that describes the data. Three distance statistics are compared in this study. They are the Euclidean distance, the Jeffries-Matusita distance and the Kuiper distance. The data used in testing the bootstrap method are satellite measurements of cloud systems called cloud objects. Each cloud object is defined as a contiguous region/patch composed of individual footprints or fields of view. A histogram of measured values over footprints is generated for each parameter of each cloud object and then summary histograms are accumulated over all individual histograms in a given cloud-object size category. The results of statistical hypothesis tests using all three distances as test statistics are generally similar, indicating the validity of the proposed method. The Euclidean distance is determined to be most suitable after comparing the statistical tests of several parameters with distinct probability distributions among three cloud-object size categories. Impacts on the statistical significance levels resulting from differences in the total lengths of satellite footprint data between two size categories are also discussed.

Xu, Kuan-Man↗

Small-Scale Variability of Large Cloud Drops

Cloud droplet size distribution is one of the most fundamental subjects in cloud physics. Understanding of spatial distribution and small-scale fluctuations of cloud droplets is essential for both cloud physics and atmospheric radiation. For cloud physics, it relates to the coalescence growth of raindrops while for radiation, it has a strong impact on a cloud's radiative properties. Most of the existing cloud radiation and precipitation formation models assume that the mean number of drops with a given radius varies proportionally to volume. The analysis of microphysical data on liquid water drop sizes shows that, for sufficiently small volumes, the number is proportional to the drop size dependent power of the volume. For abundant small drops present, the exponent is 1 as assumed in the conventional approach. However, for rarer large drops, the exponents fall below unity. At small scales, therefore, the mean number of large drops decreases with volume at a slower rate than the conventional approach assumes, suggesting more large drops at these scales than conventional models account for; their impact is consequently underestimated. Size dependent models of spatial distribution of cloud drops that simulate the observed power laws show strong drop clustering, the more so the larger the drops. The degree of clustering is determined by the observed exponents. The strong clustering of large drops arises naturally from the observed power-law statistics. Current theories of photon-cloud interaction and warm rain formation will need radical revision in order to produce these statistics; their underlying equations are unable to yield the observed power law.

Marshak, Alexander↗

Cloud microstructure studies

Over two thousand individual cloud droplet size distributions were measured with an optical cloud particle spectrometer flown on the NASA Convair 990 aircraft. Representative droplet spectra and liquid water content, L (gm/cu m) were obtained for oceanic stratiform and cumuliform clouds. For non-precipitating clouds, values of L range from 0.1 gm/cu m to 0.5 gm/cu m; with precipitation, L is often greater than 1 gm/cu m. Measurements were also made in a newly formed contrail and in cirrus clouds.

Blau, H. H., Jr.↗

The Shortwave Spectral Radiometer for Atmospheric Science: Capabilities and Applications from the ARM User Facility

Industry advances have greatly reduced the cost and size of ground-based shortwave (SW) sensors for the ultraviolet, visible, and near-infrared spectral ranges that make up the solar spectrum, while simultaneously increasing their ruggedness, reliability, and calibration accuracy needed for outdoor operation. These sensors and collocated meteorological equipment are an important part of the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) User Facility, which has supported parallel integrated measurements of atmospheric and surface properties for more than two decades at fixed and mobile sites around the world. The versatile capability of these ground-based measurements includes 1) rich spectral information required for retrieving cloud and aerosol microphysical properties, such as cloud phase, cloud particle size, and aerosol size distributions, and 2) high temporal resolution needed for capturing fast evolution of cloud microphysical properties in response to rapid changes in meteorological conditions. Here we describe examples of how ARM's spectral radiation measurements are being used to improve understanding of the complex processes governing microphysical, optical, and radiative properties of clouds and aerosol.

54 ENVIRONMENTAL SCIENCES↗

Rainbow Fourier Transform

We present a novel technique for remote sensing of cloud droplet size distributions. Polarized reflectances in the scattering angle range between 135deg and 165deg exhibit a sharply defined rainbow structure, the shape of which is determined mostly by single scattering properties of cloud particles, and therefore, can be modeled using the Mie theory. Fitting the observed rainbow with such a model (computed for a parameterized family of particle size distributions) has been used for cloud droplet size retrievals. We discovered that the relationship between the rainbow structures and the corresponding particle size distributions is deeper than it had been commonly understood. In fact, the Mie theory-derived polarized reflectance as a function of reduced scattering angle (in the rainbow angular range) and the (monodisperse) particle radius appears to be a proxy to a kernel of an integral transform (similar to the sine Fourier transform on the positive semi-axis). This approach, called the rainbow Fourier transform (RFT), allows us to accurately retrieve the shape of the droplet size distribution by the application of the corresponding inverse transform to the observed polarized rainbow. While the basis functions of the proxy-transform are not exactly orthogonal in the finite angular range, this procedure needs to be complemented by a simple regression technique, which removes the retrieval artifacts. This non-parametric approach does not require any a priori knowledge of the droplet size distribution functional shape and is computationally fast (no look-up tables, no fitting, computations are the same as for the forward modeling).

Alexandrov, Mikhail D.↗

The effect of cloud sides on reflected solar radiation as deduced from satellite observations

The observation of a feature that is characteristic of the reflection of solar radiation from absorbing finite clouds is reported. When absorption takes place, more radiation can be reflected by broken cloud fields than by extensive unbroken cloud fields. This feature is observed in solar radiation at 3.7 microns reflected by low-level, single-layered systems of water clouds over the Pacific Ocean. Interpreting the effect as due to geometrical factors, it is noted that absorption causes the reflected radiances to be highly anisotropic, so that they are generally greater from the sun-facing cloud sides than from the cloud tops. Diffusive leakage of radiation through the cloud sides is also reduced, and as a result maximum reflectivities occur in situations that maximize the contributions to the reflected radiation from the sides relative to that from the tops. Interpreting the effect as due to changes in liquid water content and cloud droplet sizes, it is noted that the observations at 0.63, 3.7, and 11 microns are consistent with a cloud model in which the liquid water content and droplet sizes are greater in the cloud centers and smaller at their edges. Theoretical calculations that qualitatively support both interpretations are presented.

Coakley, J. A., Jr.↗

Comparison of aircraft measurements during GoAmazon2014/5 and ACRIDICON-CHUVA

The indirect effect of atmospheric aerosol particles on the Earth's radiation balance remains one of the most uncertain components affecting climate change throughout the industrial period. The large uncertainty is partly due to the incomplete understanding of aerosol–cloud interactions. One objective of the GoAmazon2014/5 and the ACRIDICON (Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems)-CHUVA (Cloud Processes of the Main Precipitation Systems in Brazil) projects was to understand the influence of emissions from the tropical megacity of Manaus (Brazil) on the surrounding atmospheric environment of the rainforest and to investigate its role in the life cycle of convective clouds. During one of the intensive observation periods (IOPs) in the dry season from 1 September to 10 October 2014, comprehensive measurements of trace gases and aerosol properties were carried out at several ground sites. In a coordinated way, the advanced suites of sophisticated in situ instruments were deployed aboard both the US Department of Energy Gulfstream-1 (G1) aircraft and the German High Altitude and Long-Range Research Aircraft (HALO) during three coordinated flights on 9 and 21 September and 1 October. Here, we report on the comparison of measurements collected by the two aircraft during these three flights. Such comparisons are challenging but essential for assessing the data quality from the individual platforms and quantifying their uncertainty sources. Similar instruments mounted on the G1 and HALO collected vertical profile measurements of aerosol particle number concentrations and size distribution, cloud condensation nuclei concentrations, ozone and carbon monoxide mixing ratios, cloud droplet size distributions, and downward solar irradiance. We find that the above measurements from the two aircraft agreed within the measurement uncertainties. The relative fraction of the aerosol chemical composition measured by instruments on HALO agreed with the corresponding G1 data, although the total mass loadings only have a good agreement at high altitudes. Furthermore, possible causes of the discrepancies between measurements on the G1 and HALO are examined in this paper. Based on these results, criteria for meaningful aircraft measurement comparisons are discussed.

47 OTHER INSTRUMENTATION↗