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At least 199 records · Page 11

Minimizing Current and Voltage Losses to Reach 25% Efficient Monolithic Two-Terminal Perovskite–Silicon Tandem Solar Cells

The rapid rise in efficiency and tunable bandgap of metal-halide perovskites makes them highly attractive for use in tandems on silicon. Recently we demonstrated a perovskite–silicon monolithic two-terminal tandem with 23.6% power conversion efficiency. Here, we present work on optical optimization to improve light harvesting that includes thinning out the top transparent electrode to reduce front-surface reflection and parasitic absorption; introducing metal fingers to minimize series resistance losses; and further minimizing reflection loss with a polydimethylsiloxane (PDMS) stamp with random, pyramidal texture. Additionally, to reduce voltage loss while achieving current matching, we employ poly[bis(4-phenyl)(2,4,6-trimethylphenyl)amine] (PTAA) as a hole transport material instead of NiO x and a wider 1.68 eV bandgap perovskite composition. Furthermore, these optimizations boost the open-circuit voltage to 1.77 V and the short-circuit current density to 18.4 mA/cm 2 , culminating in a 25% efficient perovskite–silicon tandem with a 1 cm 2 active area.

14 SOLAR ENERGY↗

Carbon Outgassing in the Antarctic Circumpolar Current Is Supported by Ekman Transport From the Sea Ice Zone in an Observation‐Based Seasonal Mixed‐Layer Budget

Despite its importance for the global cycling of carbon, there are still large gaps in our understanding of the processes driving annual and seasonal carbon fluxes in the high-latitude Southern Ocean. This is due in part to a historical paucity of observations in this remote, turbulent, and seasonally ice-covered region. Here, we use autonomous biogeochemical float data spanning 6 full seasonal cycles and with circumpolar coverage of the Southern Ocean, complemented by atmospheric reanalysis, to construct a monthly climatology of the mixed layer budget of dissolved inorganic carbon (DIC). We investigate the processes that determine the annual mean and seasonal cycle of DIC fluxes in two different zones of the Southern Ocean—the Sea Ice Zone (SIZ) and Antarctic Southern Zone (ASZ). We find that, annually, mixing with carbon-rich waters at the base of the mixed layer supplies DIC which is, in the ASZ, either used for net biological production or outgassed to the atmosphere. In contrast, in the SIZ, where carbon outgassing and the biological pump are weaker, the surplus of DIC is instead advected northward to the ASZ. In other words, carbon outgassing in the southern Antarctic Circumpolar Current (ACC), which has been attributed to remineralized carbon from deep water upwelled in the ACC, is also due to the wind-driven transport of DIC from the SIZ. These results stem from the first observation-based carbon budget of the circumpolar Southern Ocean and thus provide a useful benchmark to evaluate climate models, which have significant biases in this region.

Sauvé, Jade↗

Automated setup for magnetic hysteresis characterization based on a voltage controlled current source with 500 kHz full power bandwidth and 10 A peak-to-peak current

This paper describes the design of a system for the characterization of magnetic hysteresis behavior in soft ferrite magnetic cores. The proposed setup can test magnetic materials exciting them with controlled arbitrary magnetic field waveforms, including the capability of providing a DC bias, in a frequency bandwidth up to 500 kHz, with voltages up to 32 V peak-to-peak, and currents up to 10 A peak-to-peak. In order to have an accurate control of the magnetic field waveform, the system is based on a voltage controlled current source. The electronic design is described focusing on closed loop feedback stabilization and passive components choice. The system has real-time hysteretic loop acquisition and visualization. The comparisons between measured hysteresis loops of sample magnetic materials and datasheet available ones are shown. Results showing frequency and thermal behavior of the hysteresis of a test sample prove the system capabilities. Moreover, the B-H loops obtained with a multiple waveforms excitation signal, including DC bias, are reported. The proposal is a low-cost and replicable solution for hysteresis characterization of magnetic materials used in power electronics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Simulation of injector dynamics during steady inductive helicity injection current drive in the HIT-SI experiment

We present simulations of inductive helicity injection in the Helicity Injected Torus with Steady Inductive helicity injection (HIT-SI) device that treats the entire plasma volume in a single dynamic MHD model. A new fully 3D numerical tool, the PSI-center TETrahedral mesh code, was developed that provides the geometric flexibility required for this investigation. Implementation of a zero-β Hall MHD model using PSI-TET will be presented including formulation of a new self-consistent magnetic boundary condition for the wall of the HIT-SI device. Results from simulations of HIT-SI are presented focusing on injector dynamics that are investigated numerically for the first time. Asymmetries in the plasma loading between the two helicity injectors and progression of field reversal in each injector are observed. Analysis indicates cross-coupling between injectors through confinement volume structures. Injector impedance is found to scale with toroidal current at fixed density, consistent with experimental observation. Comparison to experimental data with an injector drive frequency of 14.5 kHz shows good agreement with magnetic diagnostics. Global mode structures from Bi-Orthogonal decomposition agree well with experimental data for the first four modes.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Thermal generation of spin current in epitaxial CoFe 2 O 4 thin films

The longitudinal spin Seebeck effect (LSSE) has been investigated in high-quality epitaxial CoFe 2 O 4 (CFO) thin films. The thermally excited spin currents in the CFO films are electrically detected in adjacent Pt layers due to the inverse spin Hall effect (ISHE). The LSSE signal exhibits a linear increase with increasing temperature gradient, yielding a LSSE coefficient of –100 nV/K at room temperature. The temperature dependence of the LSSE is investigated from room temperature down to 30 K, showing a significant reduction at low temperatures, revealing that the total amount of thermally generated magnons decreases. Moreover, we demonstrate that the spin Seebeck effect is an effective tool to study the magnetic anisotropy induced by epitaxial strain, especially in ultrathin films with low magnetic moments.

36 MATERIALS SCIENCE↗

A two-fluid study of oblique tearing modes in a force-free current sheet

Kinetic simulations have demonstrated that three-dimensional reconnection in collisionless regimes proceeds through the formation and interaction of magnetic flux ropes, which are generated due to the growth of tearing instabilities at multiple resonance surfaces. Since kinetic simulations are intrinsically expensive, it is desirable to explore the feasibility of reduced two-fluid models to capture this complex evolution, particularly, in the strong guide field regime, where two-fluid models are better justified. With this goal in mind, this paper compares the evolution of the collisionless tearing instability in a force-free current sheet with a two-fluid model and fully kinetic simulations. Our results indicate that the most unstable modes are oblique for guide fields larger than the reconnecting field, in agreement with the kinetic results. The standard two-fluid tearing theory is extended to address the tearing instability at oblique angles. The resulting theory yields a flat oblique spectrum and underestimates the growth of oblique modes in a similar manner to kinetic theory relative to kinetic simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A hybrid Rayleigh-Taylor-current-driven coupled instability in a magnetohydrodynamically collimated cylindrical plasma with lateral gravity

We present an MHD theory of Rayleigh-Taylor instability on the surface of a magnetically confined cylindrical plasma flux rope in a lateral external gravity field. The Rayleigh-Taylor instability is found to couple to the classic current-driven instability, resulting in a new type of hybrid instability that cannot be described by either of the two instabilities alone. The lateral gravity breaks the axisymmetry of the system and couples all azimuthal modes together. The coupled instability, produced by combination of helical magnetic field, curvature of the cylindrical geometry, and lateral gravity, is fundamentally different from the classic magnetic Rayleigh-Taylor instability occurring at a two-dimensional planar interface. The theory successfully explains the lateral Rayleigh-Taylor instability observed in the Caltech plasma jet experiment [Moser and Bellan, Nature 482, 379 (2012)]. Potential applications of the theory include magnetic controlled fusion, solar emerging flux, solar prominences, coronal mass ejections, and other space and astrophysical plasma processes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A simple approximation for the current-voltage characteristics of high-power, relativistic diodes

A simple approximation for the current-voltage characteristics of a relativistic electron diode is presented. The approximation is accurate from non-relativistic through relativistic electron energies. Although it is empirically developed, it has many of the fundamental properties of the exact diode solutions. The approximation is simple enough to be remembered and worked on almost any pocket calculator, so it has proven to be quite useful on the laboratory floor.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Radial direct bandgap p-i-n GaNP microwire solar cells with enhanced short circuit current

We report the demonstration of dilute nitride heterostructure core/shell microwire solar cells utilizing the combination of top-down reactive-ion etching to create the cores (GaP) and molecular beam epitaxy to create the shells (GaNP). Systematic studies of cell performance over a series of microwire lengths, array periods, and microwire sidewall morphologies examined by transmission electron microscopy were conducted to shed light on performance-limiting factors and to optimize the cell efficiency. We show by microscopy and correlated external quantum efficiency characterization that the open circuit voltage is degraded primarily due to the presence of defects at the GaP/GaNP interface and in the GaNP shells, and is not limited by surface recombination. Compared to thin film solar cells in the same growth run, the microwire solar cells exhibit greater short circuit current but poorer open circuit voltage due to greater light absorption and number of defects in the microwire structure, respectively. The comprehensive understanding presented in this work suggests that performance benefits of dilute nitride microwire solar cells can be achieved by further tuning of the epitaxial quality of the underlying materials.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Surface-enhanced spin current to charge current conversion efficiency in CH3NH3PbBr3-based devices

Hybrid organic-inorganic perovskites have shown great promise for spintronic applications due to their large spin-orbit coupling induced by the Pb and halogen atoms. Particularly, the large observed surface-induced Rashba splitting in CH3NH3PbBr3 indicates efficient spin-current-to-charge-current (StC) conversion, which, however, has not been demonstrated yet. In this work, the StC conversion efficiency in ferromagnet/CH3NH3PbBr3-based devices is studied using the pulsed spin-pumping technique measured by the inverse spin Hall effect. We found that the StC conversion efficiency is anomalous in that it increases at small perovskite layer thickness. This indicates the existence of a surface-dominated StC mechanism such as the inverse Rashba-Edelstein effect. By inserting a thin LiF layer between the ferromagnet and the perovskite film, the StC conversion efficiency is greatly suppressed, validating the existence of a Rashba surface in the CH3NH3PbBr3 film.

Sun, Dali (ORCID:0000000346623265)↗

Coil current and vacuum magnetic flux calculation for axisymmetric equilibria

In fixed-boundary axisymmetric equilibrium calculations the plasma shape is assigned from input. In several circumstances, the plasma shape may not be known a priori, or one may desire to also compute the magnetic field in the volume surrounding the plasma through the calculation of a free-boundary equilibrium. This requires either the coil currents or the magnetic poloidal flux on a curve in the vacuum region to be assigned as input for the free-boundary equilibrium calculation. The FREE-FIX code presented in this article is a general tool for calculating coil currents being given a fixed-boundary calculation. Finally, a new formulation is presented, which considerably reduces the computational cost of the calculation. FREE-FIX performs well for different geometries and experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Improved understanding of the hot cathode current modes and mode transitions [Mechanism of the hot cathode current mode transitions]

Hot cathodes are crucial components in a variety of plasma sources and applications, but they induce mode transitions and oscillations that are not fully understood. It is often assumed that negatively biased hot cathodes have a space-charge limited (SCL) sheath whenever the current is limited. Here, we show on theoretical grounds that a SCL sheath cannot persist. First, charge-exchange ions born within the virtual cathode (VC) region get trapped and build up. After the ion density reaches the electron density at a point in the VC, a new neutral region is formed and begins growing in space. In planar geometry, this 'new plasma' containing cold trapped ions and cold thermoelectrons grows towards the anode and fills the gap, leaving behind an inverse cathode sheath. This explains how transitions from temperature-limited mode to anode glow mode occur in thermionic discharge experiments with magnetic fields. If the hot cathode is a small filament in an unmagnetized plasma, the trapped ion region is predicted to grow radially in both directions, get expelled if it reaches the cathode, and reform periodically. Filament-induced current oscillations consistent with this prediction have been reported in experiments. Here, we set up planar geometry simulations of thermionic discharges and demonstrate several mode transition phenomena for the first time. Lastly, our continuum kinetic code lacks the noise of particle simulations, enabling a closer study of the temporal dynamics.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Lattice calculation of nucleon isovector axial charge with improved currents

We employ dimension-4 operators to improve the local vector and axial-vector currents and calculate the nucleon isovector axial coupling $g$ ${^3}_{A}$ with overlap valence on 2 + 1-flavor domain wall fermion (DWF) sea. Using the equality of $g$ ${^3}_{A}$ from the spatial and temporal components of the axial-vector current as a normalization condition, we find that $g$ ${^3}_{A}$ is increased by a few percent towards the experimental value. Here, the excited-state contamination has been taken into account with three time separations between the source and sink. The improved axial charges $g$ ${^3}_{A}$ (24I) = 1.22 (4) (3) and $g$ ${^3}_{A}$ (32I) = 1.21 (3)(3) are obtained on a 24 3 × 64 lattice at pion mass of 330 MeV and a 32 3 × 64 lattice at pion mass 300 MeV and are increased by 3.4% and 1.7% from their unimproved values, respectively. We have also used clover fermions on the same DWF configurations and find the same behavior for the local axial charge as that with overlap fermions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for active-sterile neutrino mixing using neutral-current interactions in NOvA

Here, we report results from the first search for sterile neutrinos mixing with active neutrinos through a reduction in the rate of neutral-current interactions over a baseline of 810 km between the NOvA detectors. Analyzing a 14-kton detector equivalent exposure of 6.05 × 10 20 protons-on-target in the NuMI beam at Fermilab, we observe 95 neutral-current candidates at the Far Detector compared with 83.5 ± 9.7(stat) ± 9.4(syst) events predicted assuming mixing only occurs between active neutrino species. No evidence for νμ→νs transitions is found. Interpreting these results within a 3+1 model, we place constraints on the mixing angles θ 24 < 20.8° and θ 34 < 31.2° at the 90% C.L. for 0.05 eV 2 ≤ Δm 41 2 ≤ 0.5 eV 2 , the range of mass splittings that produce no significant oscillations over the Near Detector baseline.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗