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At least 199 records · Page 11

N2 and H2 Broadened Isobutane Infrared Absorption Cross Sections and Butane Upper Limits on Titan

High resolution infrared absorption cross sections of isobutane, (CH3)3CH, were measured in the 1050-1900 cm-1spectral range by Fourier transform spectroscopy. Four sample temperatures (210, 234, 265 and 296 K) were used with three pressures (10, 30 and 100 Torr) of N2and H2broadening gas. Spectra of pure isobutane samples were also recorded. These cross sections are useful for the interpretation of infrared spectra of the Giant Planets and Titan. The isobutane cross sections give an upper limit of 3.91e-8for its fractional abundance on Titan based on CIRS/Cassini infrared spectra. Using n-butane, CH3(CH2)2CH3, cross sections from the literature, we obtain an upper limit of 5.13e-7for its abundance on Titan. The combined upper limit for both isomers of butane, C4H10, on Titan of 5.52e-7is consistent with the lower limit of recent model predictions

Dan Hewett↗

The radar cross section of dielectric disks

A solution is presented for the backscatter (monostatic) radar cross section of dielectric disks of arbitrary shape, thickness, and dielectric constant. The result is obtained by employing a Kirchhoff-type approximation to obtain the fields inside the disk. The internal fields induce polarization and conduction currents from which the scattered fields and the radar cross section can be computed. The solution for the radar cross section obtained in this manner will be shown to agree with known results in the special cases of normal incidence, thin disks, and perfect conductivity. It will also be shown that the solution can be written as a product of the reflection coefficient of an identically oriented slab times the physical optics solution for the backscatter cross section of a perfectly conducting disk of the same shape. This result follows directly from the Kirchhoff-type approximation without additional assumptions.

Radar cross section↗

Photoabsorption cross section of CH3CN - Photodissociation rates by solar flux and interstellar radiation

The photoabsorption cross section of CH2CN vapor was measured in the 106-180 nm region using synchrotron radiation as a light source. The cross section and the quantum yield for the production of CN (A, B-X) fluorescence were measured and were used to infer the photodissociation cross section of CH3CN. The cross sections were used to calculate the photodissociation rates of CH3CN by the solar flux and by the interstellar radiation. In both the stratosphere and the troposphere, the solar photodissociation of CH3CN is negligible in comparison with chemical degradation.

Suto, M.↗

Ultraviolet absorption cross sections of hydrogen peroxide

Absorption cross-sections of hydrogen peroxide vapor and of neutral aqueous solutions of hydrogen peroxide were measured in the wavelength range from 195 to 350 nm at 296 K. The spectrophotometric procedure is described, and the reported cross-sections are compared with values obtained by other researchers. Photodissociation coefficients of atmospheric H2O2 were calculated for direct absorption of unscattered solar radiation, and the vertical distributions of these coefficients are shown for various solar zenith angles.

Lin, C. L.↗

Database work for the new cross section standards evaluation

An effort is now underway to produce a new evaluation of the neutron standards. It is important to maintain experimental programs to increase the quality and extend the database for the neutron cross section standards in order to improve evaluations of them that will be used to convert cross section measurements made relative to those standards. Measurements have been made for most of the standard cross sections since the last evaluation of the standards. The improved database includes the cross sections for the H(n,n), 6Li(n,t), 10B(n,αγ), 10B(n,α), C(n,n), Au(n,γ), 235U(n,f) and 238U(n,f) standard reactions and ratios among them. The database also includes the 238U(n,γ) and 239Pu(n,f) cross sections in addition to the standard cross sections. Those data were included since there are many ratio measurements of those cross sections with the standards and absolute data are available for them.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

First Measurement of Differential Charged Current Quasielasticlike $\nu_{\mu}$ -Argon Scattering Cross Sections with the MicroBooNE Detector

We report on the first measurement of flux-integrated single differential cross sections for charged-current (CC) muon neutrino ($\nu_{\mu}$) scattering on argon with a muon and a proton in the final state, 40 Ar $(\nu_{\mu},μp)X$. The measurement was carried out using the Booster Neutrino Beam at Fermi National Accelerator Laboratory and the MicroBooNE liquid argon time projection chamber detector with an exposure of 4.59 × 10 19 protons on target. Events are selected to enhance the contribution of CC quasielastic (CCQE) interactions. The data are reported in terms of a total cross section as well as single differential cross sections in final state muon and proton kinematics. We measure the integrated per-nucleus CCQE-like cross section (i.e., for interactions leading to a muon, one proton, and no pions above detection threshold) of (4.93 ± 0.76 stat ± 1.29 sys )×10 -38 cm 2 , in good agreement with theoretical calculations. The single differential cross sections are also in overall good agreement with theoretical predictions, except at very forward muon scattering angles that correspond to low-momentum-transfer events.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

The abundance of N-14 at the cosmic-ray source - A study using new fragmentation cross sections

The abundance of N-14 at the Galactic cosmic ray source was examined using new fragmentation cross sections measured by the University of New Hampshire group for 12 different source nuclei (ranging from C-12 to Ni-58) which cover about 70 percent of all cosmic-ray nuclei arriving at earth. A new cross-section program was used to estimate unmeasured cross sections. These cross sections were then incorporated into a Galactic propagation program to calculate the interstellar production of B and N. Results indicate that atomic selection effects alone cannot explain adequately the observed depletion of N-14 relative to O-16 in the cosmic-ray source with respect to the solar corona, indicating that some part of this depletion must have a nuclear/nucleosynthetic origin.

Gupta, M.↗

Cross Section Evaluation for Exclusive Channels of K+Λ and K+Σ0 Electroproduction off Protons Using CLAS Detector Data

In this work, a method for evaluating the cross sections of electroproduction of K+Λ0 and K+Σ0 off protons in the region of invariant masses of final hadrons MK + MY <W < 2.65 GeV (MK and MY being the masses of the kaon and hyperon, respectively) and squares of four-momentum transfers of virtual photons, i.e., photon virtualities 0 < Q2 < 5 GeV2, is developed based on experimental data of these exclusive channels’ cross sections measured by the CLAS detector in Hall B at Jefferson Lab. A set of algorithms has been implemented to evaluate the differential cross sections of these channels, along with their statistical and systematic uncertainties. A program was developed for the evaluation of differential cross sections and structure functions using C++ and Python libraries. An interactive website was created for working with the program, enabling the analysis of one-dimensional and two-dimensional dependences of structure functions and differential cross sections. The evaluation of differential cross sections for the K+Λ and K+Σ0 electroproduction channels is necessary for extracting the structure function σLT from the data on the polarization asymmetry of electroproduction reactions of these final states with longitudinally polarized electrons. The obtained results are also important for the development of realistic Monte Carlo event generators in planning future experiments and for evaluating the efficiency of detecting final particles when extracting reaction cross sections from experimental data.

Golda, A. V.↗

High-resolution Laboratory Measurements of K-shell X-ray Line Polarization and Excitation Cross Sections in Helium-like S XV Ions

We report measurements of electron-impact excitation cross sections for the strong K-shell n = 2 -> 1 transitions in S XV, using the LLNL EBIT-I electron beam ion trap, two crystal spectrometers, and the EBIT Calorimeter Spectrometer. The cross sections are determined by direct normalization to the well-known cross sections of radiative electron capture, measured simultaneously. Using contemporaneous polarization measurements with the two crystal spectrometers, whose dispersion planes are oriented parallel and perpendicular to the electron beam direction, the polarization of the direct excitation line emission is determined, and in turn the isotropic total cross sections are extracted. We further experimentally investigate various line-formation mechanisms, finding that radiative cascades and collisional inner-shell ionization dominate the degree of linear polarization and total line emission cross sections of the forbidden line, z.

atomic data↗

High-resolution Laboratory Measurements of K-shell X-Ray Line Polarization and Excitation Cross Sections in Helium-like S XV Ions

We report measurements of electron-impact excitation cross sections for the strong K-shell n = 2 → 1 transitions in S xv, using the LLNL EBIT-I electron beam ion trap, two crystal spectrometers, and the EBIT Calorimeter Spectrometer. The cross sections are determined by direct normalization to the well-known cross sections of radiative electron capture, measured simultaneously. Using contemporaneous polarization measurements with the two crystal spectrometers, whose dispersion planes are oriented parallel and perpendicular to the electron beam direction, the polarization of the direct excitation line emission is determined, and in turn the isotropic total cross sections are extracted. We further experimentally investigate various line-formation mechanisms, finding that radiative cascades and collisional inner-shell ionization dominate the degree of linear polarization and total line-emission cross sections of the forbidden line, z.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Derivation and verification of the direct-sampling method for simulating Monte Carlo flight paths in tetrahedral meshes with linear finite-element cross sections

This paper provides a derivation of a direct-sampling approach for modeling continuously varying cross sections in tetrahedral-mesh-based Monte Carlo codes. Specifically, cross sections are spatially approximated using linear nodal finite elements. A linearization strategy is provided for non-linearly varying cross sections. The method is verified against seven analytical pure-absorber test problems. These test problems also highlight the benefit of using linear finite elements over element-wise-constant cross sections.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections σ tot of 16,18 O, 58 64 Ni, 103 Rh, and 112,124 Sn have been measured at the Los Alamos Neutron Science Center from low to intermediate energies (3 ≤ E lab ≤ 450 MeV) by leveraging wave-form-digitizer technology. The σ tot relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled σ tot -measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ( 16,18 O) and systems with open neutron shells ( 58,64 Ni and 112,124 Sn). Here, the valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Improved Cross Section Generation Capability of Griffin in FY22

The Griffin code is a Multiphysics Object-Oriented Simulation Environment (MOOSE) based reactor multiphysics analysis application jointly developed by Idaho National Laboratory and Argonne National Laboratory. The code includes a variety of deterministic steady-state transport solvers for fixed source, k-eigenvalue, adjoint, and subcritical multiplication as well as transient solvers for spatial dynamics with the improved quasi-static method. Griffin uses cross section data in the ISOXML format generated from external deterministic or Monte Carlo cross section generation codes. In recent years, the MC 2 -3 modules have been added to Griffin for fast reactor cross section generation, and the self-shielding application programming interface (SSAPI) was implemented in the ISOXML module for thermal reactor cross section generation. The on-the-fly slowing down method and double-heterogeneity treatment have been implemented to SSAPI and verified against particulate fuel-bearing graphite-moderated thermal reactor problems with high accuracy. This year, work has been focused on improving the cross section generation capability of ISOXML and streamlining the cross section generation procedures. In addition, the form function data were added to ISOXML in order to support the pin power reconstruction capability that was newly implemented in Griffin in this fiscal year. To facilitate the cross section generation using MC 2 -3 and SSAPI in Griffin, the cross section generation workflows have been set up for both fast and thermal spectrum reactors. The MOOSE action system tool was devised for fast spectrum problems, and the MOOSE stochastic tool was adopted to the branch calculation procedure for thermal spectrum problems. Meanwhile, to ensure the accuracy of group-constants, the thermal up-scattering kernel calculator accounting for resonance scattering was implemented in ISOXML, demonstrating the accurate computation of a Doppler-broadened scattering kernel of any Legendre order within a reasonable timescale. Other aspects of ISOXML, such as deletion solver and data, documentation, ISOXML file management, and the interface for Mixture, were improved as well.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Applying a Template of Expected Uncertainties to Updating 239 Pu(n,f) Cross-section Covariances in the Neutron Data Standards Database

Templates of uncertainties expected in specific measurement types were recently developed. One aim of these templates is to help evaluators in identifying (1) missing or suspiciously low uncertainties and (2) missing correlations between uncertainties of the same and different experiments, when estimating covariances for experimental data employed in their evaluations. These templates also provide realistic estimates of standard deviations and correlations for a particular uncertainty source and measurement type that can be used by evaluators in situations where they are not supplied by the experimenters. This information allows for a more comprehensive uncertainty analysis across all measurements considered in an evaluation and, thus, more realistic evaluated covariances. Here, in this work, we extend a template that is applicable to uncertainties expected in neutron-induced fission, (n,f), cross-section measurements. It is applied to improving covariances of 239 Pu(n,f) cross-section measurements in the database underlying the Neutron Data Standards evaluations. This particular example was chosen since this evaluation is primarily based on experimental information. Also, some uncertainties of individual 239 Pu(n,f) cross-section experiments in this database were suspected to be underestimated. The evaluated uncertainties obtained after updating the covariances in the database by means of the template indeed do increase compared to their original values. Even more importantly, the evaluated mean values change noticeably. These modified cross sections impact application calculations significantly, as is demonstrated by employing them in simulations of the effective neutron multiplication factor for a few selected critical assemblies. However, this updated evaluated 239 Pu(n,f) cross section should not be interpreted as the final one that should replace values of the current Neutron Data Standards project. Evaluations for the Neutron Data Standards of the 239 Pu(n,f) cross section must be linked to many other observables included in the associated database, most notably to cross sections for 235 U(n,f), but also to those for 10 B(n, α ), 6 Li(n,t), 238 U(n,f), and 238 U(n, γ ), because of included measurements of the 239 Pu(n,f) cross section that appear as ratios to these reactions. Some of these other reactions are correlated to further observables in the database. Hence, updating uncertainties of data sets of any of these observables can potentially impact the 239 Pu(n,f) cross section. Uncertainties for all measurements of these linked physical observables have to be updated before a comprehensive evaluation of the 239 Pu(n,f) cross section and its corresponding uncertainties can be provided.

239Pu Neutron-induced fission cross-section↗

Analytic error analysis of cross section interpolation methods in nodal diffusion codes - I : Theory

This paper discusses two cross section interpolation methods commonly found in popular nodal codes; the partial derivatives and multiple tables models. The motivation for choosing a model, and thus a case matrix structure, is a trade off between accuracy and computational cost. Due to decades of experience, there are default structures that are sufficient for current light water reactor analysis. However, this is not necessarily the case for advanced reactor designs. Therefore, it is advantageous to understand the sources of error in cross section interpolation models so that the quality of a case matrix may be improved. A mathematical framework for these models is presented in this work that provides a more rigorous connection between the nuclear engineering field's cross section interpolation methods and the broader mathematical field of function approximation. The two cross section models examined in this paper were found to utilize Lagrange interpolation and are a subset of Lagrange tensor products. Classical results of Lagrange polynomial error analysis were then applied to the partial derivative and multiple tables models to derive expressions for the total point-wise error. The analytical results classify the total error into two parts: the model form error and interpolation error. Finally, based on our observations, a better foundation for improving the quality of a case matrix is proposed. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Measurement of the J/ψ photoproduction cross section over the full near-threshold kinematic region

Here, we report the total and differential cross sections for $J/\psi$ photoproduction with the large acceptance GlueX spectrometer for photon beam energies from the threshold at 8.2 GeV up to 11.44 GeV and over the full kinematic range of momentum transfer squared, $t$. Such coverage facilitates the extrapolation of the differential cross sections to the forward ($t = 0$) point beyond the physical region. The forward cross section is used by many theoretical models and plays an important role in understanding $J/\psi$ photoproduction and its relation to the $J/\psi$-proton interaction. These measurements of $J/\psi$ photoproduction near threshold are also crucial inputs to theoretical models that are used to study important aspects of the gluon structure of the proton, such as the gluon Generalized Parton Distribution (GPD) of the proton, the mass radius of the proton, and the trace anomaly contribution to the proton mass. We observe possible structures in the total cross section energy dependence and find evidence for contributions beyond gluon exchange in the differential cross section close to threshold, both of which are consistent with contributions from open-charm intermediate states.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗