Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Ar”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 199 records · Page 11

First Demonstration of a Liquid Argon Time Projection Chamber Based Search for Intranuclear Neutron-Antineutron Transitions and Annihilation in $^{40}$Ar using the MicroBooNE Detector

We present a novel methodology to search for intranuclear neutron-antineutron transition ($n\rightarrow\bar{n}$) followed by $\bar{n}$-nucleon annihilation within an $^{40}$Ar nucleus, using the MicroBooNE liquid argon time projection chamber (LArTPC) detector. A discovery of $n\rightarrow\bar{n}$ transition or a new best limit on the lifetime of this process would either constitute physics beyond the Standard Model or greatly constrain theories of baryogenesis, respectively. The approach presented in this paper makes use of deep learning methods to select $n\rightarrow\bar{n}$ events based on their unique features and differentiate them from cosmogenic backgrounds. The achieved signal and background efficiencies are (70.22$\pm$6.04)\% and (0.0020$\pm$0.0003)\%, respectively. A demonstration of a search is performed with a data set corresponding to an exposure of $3.32 \times10^{26}\,$neutron-years, and where the background rate is constrained through direct measurement, assuming the presence of a negligible signal. With this approach, no excess of events over the background prediction is observed, setting a demonstrative lower bound on the $n\rightarrow\bar{n}$ lifetime in $^{40}$Ar of $\tau_{\textrm{m}} \gtrsim 1.

43 PARTICLE ACCELERATORS↗

Basis for Dose and Reactor Safety Design Criteria for Army Regulation AR 50–7 and DA Pamphlet

This report describes the basis used to develop the radiological dose acceptance and design criteria contained in the draft updates to Army Regulation 50–7 (AR 50–7) Army Reactor Program and its accompanying draft Department of the Army (DA) Pamphlet (PAM), Army Reactor Program Procedures. These criteria will apply to Army nuclear reactors that fall under AR 50–7 and its accompanying DA PAM and ensure alignment with the overall objectives of the Army Reactor Program. The development basis for the radiological dose and design criteria supports a modern, technology-neutral, risk-informed, and performance-based approach to Army regulation of reactors and the demonstration of “adequate protection of the public.” To establish these criteria that support the Army’s unique operational requirements, multiple well-known and well-established standards and their supporting documentation were reviewed to ensure consistency with existing regulatory safety levels, including guidance from U.S. and international sources. These include the U.S. Nuclear Regulatory Commission’s (NRC’s) regulations and policy, the Canadian Nuclear Safety Commission’s (CNSC’s) regulatory documents, the International Atomic Energy Agency’s (IAEA’s) safety standards, as well as industry input that is tailored specifically to advanced microreactors. This report walks through the key definitions and associated references used for these criteria, which are outlined in Section 2.0. Based on these definitions, the dose acceptance criteria were established for various receptors for routine reactor operations (Section 3.2), design basis accidents (Section 3.3), and beyond design basis accidents (Section 3.4). Comparisons of multiple national and international dose limits are provided in these sections. Lastly, Section 4.0 outlines the reactor safety design criteria contained in the draft DA PAM and their associated bases.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Effects of SRPPF ARS Effluent Variations on Magnesium Oxysulfate Solidification

A magnesium oxysulfate (MOS) grout formulation has been identified to solidify the liquid effluent from the Savannah River Plutonium Processing Facility (SRPPF) Aqueous Recovery System (ARS). The formulation uses reactive, light burnt MgO (28 wt%), anhydrous MgSO 4 (10 wt%), and dead burnt MgO (62 wt%), resulting in a grout with good mixability, acceptable density, acceptable setting times, and a leachate pH around 9.4, within the assumed Waste Isolation Pilot Plant (WIPP) brine pH range. A series of tests were then designed to observe how this formula reacted to variations in the liquid effluent. Liquid effluent temperature, the caustic pH level, concentration of NaNO 3 , and the presence of neutralization products, trace metals, and/or sodium sulfate (all potential residuals found in the effluent from upstream processing), were evaluated to see how each impacts the grout mixing time, peak temperature, setting time, presence of bleed water, leachate pH, and density. The standard mix has an average mixing time of 18 minutes, peak temperature of 100.5 °C, and set time of 60 minutes. Increasing the temperature of the liquid effluent increased the reaction rate of the mix and reduced mixing and setting times. Between 30 and 40°C the change was relatively small, raising no more than 6 °C compared to the standard mix maximum temperature. Increasing the pH of the liquid effluent had no significant impact on the mix. The addition of neutralization products and trace metals had an overall impact of decreasing the reactivity of the mix. The addition of more ions in the liquid effluent, such as an increase in the concentration of NaNO 3 and the addition of Na 2 SO 4 , generally decreased the reactivity of the mix. None of the variations to the liquid effluent hindered solidification as indicated by the lack of bleed water found on all the samples. The leachate pH values for all mixes tested did not significantly vary from the expected pH of 9.4 and none of the density values fell below 1.8 g/cm 3 . Overall, changes to the liquid effluent were found to have a minimal impact on the formulation suggesting the grout's ability to properly form despite increased temperatures and the presence of residuals typically found in the liquid effluent from the ARS.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Peeking Between the Pulses: The Far-UV Spectrum of the Previously Unseen White Dwarf in AR Scorpii

The compact object in the interacting binary AR Sco has widely been presumed to be a rapidly rotating, magnetized white dwarf (WD), but it has never been detected directly. Isolating its spectrum has proven difficult because the spin-down of the WD generates pulsed synchrotron radiation that far outshines the WD's photosphere. As a result, a previous study of AR Sco was unable to detect the WD in the averaged far-ultraviolet spectrum from a Hubble Space Telescope (HST) observation. In an effort to unveil the WD's spectrum, we reanalyze these HST observations by calculating the average spectrum in the troughs between synchrotron pulses. We identify weak spectral features from the previously unseen WD and estimate its surface temperature to be 11,500 ± 500 K. Additionally, during the synchrotron pulses, we detect broad Lyα absorption consistent with hot WD spectral models. We infer the presence of a pair of hotspots, with temperatures between 23,000 and 28,000 K, near the magnetic poles of the WD. As the WD is not expected to be accreting from its companion, we describe two possible mechanisms for heating the magnetic poles. Here, the Lyα absorption of the hotspots appears relatively undistorted by Zeeman splitting, constraining the WD's field strength to be ≲100 MG, but the data are insufficient to search for the subtle Zeeman splits expected at lower field strengths.

79 ASTRONOMY AND ASTROPHYSICS↗

Vibrationally inelastic low-energy CO/+/ - Ar collisions.

Examination of relative differential cross sections for inelastic scattering of CO(+) by Ar with a high-resolution ion-beam apparatus in which a CO(+) beam interacts with a neutral-Ar beam, and the energy, mass, and angular distribution of scattered ions are measured. Maxima in the inelastic energy-loss spectra occur at energies corresponding to CO(+) spectroscopic vibrational spacings. Weakly inelastic processes are observed below the threshold for vibrational energy loss, corresponding to rotational excitation with the relative importance of rotational transitions increasing with decreasing energy and scattering angle.

Petty, F.↗

Thermal release characteristics of spallogenic He, Ne, and Ar from the Carbo iron meteorite.

Analysis of the thermal release patterns of He, Ne, and Ar from samples of the Carbo iron meteorite, showing that virtually no fractionation of He 3, He 4, Ne 21, and Ar 38 occurs. Thus conclusions about iron meteorites based on measured noble gas ratios will be unaffected by gas loss, and measurement of these ratios cannot yield information about possible loss. Further, noble gas loss cannot explain the abnormal elemental and isotopic patterns observed in some iron meteorites, notably hexahedrites. The release of He and Ne was continuously observed throughout the stepwise heating sequence, and ratios of diffusion coefficients at two consecutive temperatures have been determined from measurements of the relative degassing rates at these temperatures at the time of temperature increase. Effective activation energies of 100 plus or minus 20 kcal/mol for both He 3 and Ne 21 are calculated from the diffusion coefficient ratios at temperatures above 1050 C. A sharp maximum at 750 C in both the effective activation energy and the gas release is correlated with the alpha, gamma-phase transition.

Nyquist, L. E.↗

K-Ar dating of lunar fines - Apollo 12, Apollo 14, and Luna 16.

K-Ar ages were determined on a 6-in. double-focus mass spectrometer in fines of less than 1 mm from Apollo 14 and 16, and Luna 16 lunar soil samples. Age estimates of about 2.8 AE and about 4.0 AE are suggested for the two low-K components whose presence in the samples must be assumed to accommodate the age data. An average value of 0.1849 plus or minus 0.0008 was obtained for the Ar-18/Ar-36 ratio in the solar wind from ordinate intercept correlations for the Apollo 14 and Luna 16 samples. Cosmic ray exposure ages were close to 440 m.y. for both Apollo 14 samples and close to 840 m.y. for both Luna 16 samples.

Pepin, R. O.↗

He, Ne and Ar in chondritic Ni-Fe as irradiation hardness sensors.

Noble gas analyses of the Ni-Fe of 9 L, 5 H, and 2 LL chondrites quantitatively support previous suggestions of radiogenic He-4 recoil and He-3 deficits. Furthermore, noble gases in the Ni-Fe show evidence for in situ produced radiogenic He-4 and in some cases for recoil loss of Ar-38 and gain of Ne-21. The ratio of spallogenic Ar-38 and Ne-21 in the metal phase is found to correlate strongly with He-3/Ne-21 and Ne-22/Ne-21 in bulk samples of these chondrites. This is proof of the dependence of these ratios on the irradiation hardness experienced by the meteoroid in space. 'Hardness indices' n equals 1.9-2.2 are found, indicating that on the average the stone meteoroids from which the samples came were smaller in mass than iron meteoroids. The spallogenic Ne-21/Ar-38 ratio in metallic Ni-Fe can be used with the semi-empirical production model deduced from the Grant iron meteorite to calibrate spallogenic He-3/Ne-21 and Ne-21/Ar-38 in bulk samples of L, LL and H chondrites for meteoroid size and sample location allowing the estimation of minimal meteoroid masses.

Nyquist, L.↗

Multiplet effects on the L/sub 2,3/ fluorescence yield of multiply ionized Ar

The 2p fluorescence yield of Ar in the presence of zero to six 3p holes has been calculated by statistically averaging the fluorescence yields of initial states that consist of individual multiplet configurations, formed by coupling the 2p vacancy to the partially filled 3p shell. The L(sub 2,3) fluorescence yields for the (2p)-1 (3p)-n configurations of Ar are found to be 1.48, 17.97, 24.83, 37.84, 79.61, 112.16, and 121.48 x .0001 for n = 0, 1, 2, 3, 4, 5, and 6, respectively. Results agree reasonably well with experimental fluorescence yields deduced from ion-atom collision measurements.

Chen, M. H.↗

K-Ar analysis of Apollo 11 fines 10084

Regolithic history of Mare Tranquillitatus is studied with rare gas and mass spectrometric techniques. Grain size-ordinate intercept analysis is applied to bulk soil, ilmenite, and plagioclase separates obtained from 1 mm or smaller fines sample 10084,48. K-Ar ages for ilmenite, plagioclase, and total soil separates are determined to be 2.80, 3.38 and 4.00 AE, respectively. It appears that 10084,48 may consist primarily of two components. In this view, the first is locally derived, forms 65-75% of the present day regolith and may show that a local degassing event(s) occurred between 2.8 and 3.5 AE ago. The second component is similar to material from the lunar highlands. It may be local or foreign in origin and contributes the remaining 25-35% of the soil. This component exhibits an age of 4.00 AE and is either slightly older than, or contemporaneous with, the oldest of the returned Apollo 11 basalts. Within the limits of experimental error, the trapped Ar-38/Ar-36 ratio is constant at 0.1890 for all the soil components examined.

Basford, J. R.↗

Episodic release of Ar-40 from the interior of the moon

Measurements of lunar atmosphere made by the mass spectrometer at the Apollo 17 landing site during the first 9 lunations of 1973 show an apparently cyclical variation of radiogenic Ar-40, with maximum to minimum abundance ratio of about 2. There seems to be a 6-7 month periodicity in the oscillation, but the limited data base makes a fixed oscillatory pattern uncertain. The significance of the variation of atmospheric argon lies in the implication that its source is episodic in nature, ranging in strength from about 1% of the total rate of production of Ar-40 in the moon to near zero. This requires a presently active mechanism for transient venting of gas from deep within the moon.

Hodges, R. R., Jr.↗

Adsorption of Ar on a nonuniform MgO surface

Data are presented for the adsorption of Ar and N2 on a strongly heterogeneous MgO surface at 84 K and for Ar at a range of temperatures between 130 and 250 K. The high-temperature data are analyzed according to a model which separates the contributions to the potential into bulk and surface terms, providing a method for the determination of the surface area from parameters characteristic of the bulk material. A solid-gas energy parameter and parameters indicating the strength of the impurity sites are also evaluated.

Hinman, D. C.↗

Ar-40/Ar-39 dating of collisional events in chondrite parent bodies

Ar-40/Ar-39 age dating of a number of shocked ordinary chondrites is interpreted in terms of collisional degassing events of meteorite parent bodies, probably in the asteroid belt. Examples of L, H, and at least one LL chondrite show episodic degassing. Degassing ages suggest several distinct events ranging from about 0.03 aeon to 0.7 aeon and probably higher. All specimens of either the H or L chondrites are not consistent with a single age event. A direct correlation exists between the degree of shock heating and the fraction of argon lost during degassing. However, no chondrite yet analyzed shows complete degassing of its high-temperature phase. Consequently, whole rock K-Ar ages are not accurate monitors of the time of the shock event.

Bogard, D. D.↗

Studies of Ar and N2 using threshold photoelectron spectroscopy by electron attachment /TPSA/

Threshold photoelectron spectra of Ar and N2 are studied by a technique called threshold photoelectron spectroscopy by electron attachment, which involves the attachment of the threshold electron to SF6 followed by the detection of SF6(-). Studies on Ar provide a measure of the rejection ratio for nonthreshold electrons of this technique. A rotational propensity rule is given which states that an autoionizing N2 state prefers to decay to N2(+) states with a minimum change in rotational angular momentum.

Chutjian, A.↗

AR-39Ar-40 dating of basalts and rock breccias from Apollo 17 and the malvern achondrite

The principles and the potential of the Ar-39/Ar-40 dating technique are illustrated by means of results obtained for 12 Apollo 17 rocks. Emphasis is given to methodical problems and the geological interpretation of lunar rock ages. Often it is ambigious to associate a given lunar breccia with a certain formation, or a formation with a basin. In addition, large-scale events on the Moon have not necessarily reset radiometric clocks completely. One rock fragment has a well-defined plateau age of 4.28 b.y., but the ages of two Apollo 17 breccias define an upper limit for the formation age of the Serenitatis basin at 4.05 b.y. Ages derived from five mare basalts indicate cessation of mare volcanism at Taurus-Littrow approximately 3.78 b.y. ago. Ca/Ar-37 exposure ages show that Camelot Crater was formed by an impact approximately 95 m.y. ago. After a short summary of the lunar timetable as it stands at the end of the Apollo program, we report about Ar-39/Ar-40 and rare gas studies on the Malvern meteorite. This achondrite resembles lunar highland breccias in texture as well as in rare-gas patterns. It was strongly annealed at some time between 3.4 and 3.8 b.y. ago. The results indicate that very similar processes have occurred on the Moon and on achondritic parent bodies at comparable times, leading to impact breccias with strikingly similar features, including the retention of rare-gas isotopes from various sources.

Kirsten, T.↗

Large volume multiple path nuclear lasing of /He-3/-Ar

Output power of 550 W has been achieved from a nuclear-pumped multiple path laser system containing (He-3)-Ar by using the (He-3)(n, p)3(H) nuclear reaction for power deposition. Lasing was achieved in Ar at 1790 nm. The complex beam profile was resolved by an InAs array detector. Laser output was directly proportional to thermal neutron flux, and also increased proportionally with increasing (He-3) pressure up to 292.6 kPa. The variation of the laser output power with the number of passes through the excited medium was found to peak at 5-7 passes.

De Young, R. J.↗